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RESEARCH PAPER · Journal of the American Chemical Society · 2020

Molecular Design Principles for Ferroelectrics: Ferroelectrochemistry

Huiyu Liu, Han‐Yue Zhang, Xiao-Gang Chen, Ren‐Gen Xiong

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Molecular Design Principles for Ferroelectrics: FerroelectrochemistryOriginalTwo-Dimensional Hybrid Perovskite Ferroelectric Induced by Perfluorinated Substitution166A multiaxial molecular ferroelectric with record high T C designed by intermolecular interaction modulation34Coupling Narrow Band Gap and Switchable SHG Responses in a New Molecule Ferroelectric: Imidazolyl Propylamine Pentabromo Stibium(III)31(( R )-(−)-3-Hydroxyquinuclidium)[FeCl 4 ]; a plastic hybrid compound with chirality, ferroelectricity and long range magnetic ordering28A multifunctional molecular ferroelectric with chiral features, a high Curie temperature, large spontaneous polarization and photoluminescence: (C 9 H 14 N) 2 CdBr 450An unprecedented hexagonal double perovskite organic–inorganic hybrid ferroelastic material: (piperidinium) 2 [KBiCl 6 ]43Coexistence of magnetic and electric orderings in a divalent Cr 2+ -based multiaxial molecular ferroelectric58Halogen regulation triggers NLO and dielectric dual switches in hybrid compounds with green fluorescence44Homochiral one-dimensional ABX 3 lead halide perovskites with high- T c quadratic nonlinear optical and dielectric switchings61PFM (piezoresponse force microscopy)-aided design for molecular ferroelectrics143Large Electrostrictive Coefficient in a Two-Dimensional Hybrid Perovskite Ferroelectric174Chiral halide perovskite crystals for optoelectronic applications238Observation of Transition from Ferroelasticity to Ferroelectricity by Solvent Selective Effect in Anilinium Bromide68Improper molecular ferroelectrics with simultaneous ultrahigh pyroelectricity and figures of merit66Plastic/ferroelectric molecular crystals: Ferroelectric performance in bulk polycrystalline forms57X-site doping in ABX3 triggers phase transition and higher Tc of the dielectric switch in perovskite34Two enantiomeric perovskite ferroelectrics with a high Tc raised by inserting intermolecular hydrogen bonds25Unprecedented 2D Homochiral Hybrid Lead‐Iodide Perovskite Thermochromic Ferroelectrics with Ferroelastic Switching157Engineering Elastic Properties of Isostructural Molecular Perovskite Ferroelectrics via B‐Site Substitution32Record Enhancement of Curie Temperature in Host–Guest Inclusion Ferroelectrics104Hybrid organic–inorganic perovskite ferroelectrics bring light to semiconducting applications: Bandgap engineering as a starting point42A New Anhydrous Polar Rare-Earth Iodate Fluoride, Ce(IO3)2F2, Exhibiting a Large Second-Harmonic-Generation Effect and Improved Overall Performance35Ferroelectrochemistry49The First High‐Temperature Supramolecular Radical Ferroics58Bromine-Substitution-Induced High-Tc Two-Dimensional Bilayered Perovskite Photoferroelectric93A Photoluminescent Lead Bromide Hybrid Perovskite Molecular Ferroelastic Semiconductor with Sequential High-Tc Phase Transitions33Hybrid Optical-Electrical Perovskite Can Be a Ferroelastic Semiconductor64Structural phase transition and dielectric switching in an organic-inorganic hybrid rare-earth double perovskite-type compound: (DMP)2LaRb(NO3)6 (DMP = N,N-dimethylpyrrolidinium cation)37Ferroelectricity and Rashba effect in 2D organic–inorganic hybrid perovskites85Eco‐Friendly and Highly Efficient Light‐Emission Ferroelectric Scintillators by Precise Molecular Design110100 years of ferroelectricity—A celebration69Organic Enantiomeric Ferroelectrics with High Piezoelectric Performance: Imidazolium l - and d -Camphorsulfonate37Ferroelastic Hybrid Bismuth Bromides with Dual Dielectric Switches69Optical Control of Polarization Switching in a Single-Component Organic Ferroelectric Crystal96Salicylideneaniline is a Photoswitchable Ferroelectric Crystal30Recent advances in molecular ferroelectrics25High-Curie Temperature Multilayered Hybrid Double Perovskite Photoferroelectrics Induced by Aromatic Cation Alloying77Roadmap on organic–inorganic hybrid perovskite semiconductors and devices201H/F substitution for advanced molecular ferroelectrics104Optically Induced Ferroelectric Polarization Switching in a Molecular Ferroelectric with Reversible Photoisomerization71Unusual ferroelectric-dependent birefringence in 2D trilayered perovskite-type ferroelectric exploited by dimensional tailoring63Crown Ether Host‐Guest Molecular Ferroelectrics54Multichannel Control of Multiferroicity in Single-Component Homochiral Organic Crystals95An organic plastic ferroelectric with high Curie point36A room-temperature antiferroelectric in hybrid perovskite enables highly efficient energy storage at low electric fields32Design of above-room-temperature ferroelectric two-dimensional layered halide perovskites54Ferroelectricity in organic materials: from materials characteristics to de novo design39Ferroic phase transition molecular crystals45Multi-functional hybrid perovskites with triple-channel switches and optical properties39Origin of Ferroelectricity in Two Prototypical Hybrid Organic–Inorganic Perovskites87Advances in single crystals and thin films of chiral hybrid metal halides38Recent Advances in Organic and Organic–Inorganic Hybrid Materials for Piezoelectric Mechanical Energy Harvesting335A Photochromic Organic–Inorganic Hybrid Schiff Base Metal Halide Ferroelectric28Realization of In‐Plane Polarized Light Detection Based on Bulk Photovoltaic Effect in A Polar Van Der Waals Crystal31Giant electromechanical effects in polymers48Multiaxial Ferroelectricity and Ferroelasticity in a Chiral Perovskite51Ferroelectric Polymer Drives Performance Enhancement of Non‐fullerene Organic Solar Cells68Metal‐Free Perovskite Piezoelectric Nanogenerators for Human–Machine Interfaces and Self‐Powered Electrical Stimulation Applications74Anisotropy in a 2D Perovskite Ferroelectric Drives Self‐Powered Polarization‐Sensitive Photoresponse for Ultraviolet Solar‐Blind Polarized‐Light Detection73Spin-Electric Coupling with Anisotropy-Induced Vanishment and Enhancement in Molecular Ferroelectrics39Lead-free bilayer heterometallic halide perovskite with reversible phase transition and photoluminescence properties36Unprecedented Ferroelectricity and Ferromagnetism in a Cr 2+ ‐Based Two‐Dimensional Hybrid Perovskite83Intercalation-driven ferroelectric-to-ferroelastic conversion in a layered hybrid perovskite crystal64Homochiral Multiferroic Cyanido‐Bridged Dimetallic Complexes Assembled by C−F⋅⋅⋅K Interactions40Ferroelasticity in Organic–Inorganic Hybrid Perovskites63Zero-Dimensional Molecular Ferroelectrics with Significant Nonlinear Effect and Giant Entropy33Robust Spin-Dependent Anisotropy of Circularly Polarized Light Detection from Achiral Layered Hybrid Perovskite Ferroelectric Crystals85Hybrid Germanium Bromide Perovskites with Tunable Second Harmonic Generation123Reversible Phase Transition and Second-Harmonic Response Based on a Zero-Dimensional Organic–Inorganic Hybrid Compound26Recent progress of bulk photovoltaic effect in acentric single crystals and optoelectronic devices62Record high-Tc and large practical utilization level of electric polarization in metal-free molecular antiferroelectric solid solutions29The First Chiro‐Inositol Organosilicon Ferroelectric Crystal34Switchable Dielectric Two-Dimensional Lead-Free Perovskite with Reversible Thermochromic Response26Polymorphs with Remarkably Distinct Physical and/or Chemical Properties50Giant Near-Room-Temperature Pyroelectric Figures-of-Merit Originating from Unusual Dielectric Bistability of Two-Dimensional Perovskite Ferroelectric Crystals32Structural Optimization and Property Tunability by Halogen Regulation in Zero-Dimensional Zinc Halide Organic–Inorganic Hybrid Materials36Axial-Chiral BINOL Multiferroic Crystals with Coexistence of Ferroelectricity and Ferroelasticity67Design principles based on intramolecular interactions for hydroxyl-functionalized covalent organic frameworks31Ferroelectric hybrid organic–inorganic perovskites and their structural and functional diversity195A chiral lead-free tin(IV)-based halide organic-inorganic semiconductor with dielectric switching and phase transition44Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets32Inch-Size Molecular Ferroelectric Crystal with a Large Electromechanical Coupling Factor on Par with Barium Titanate64Discrete Molecular Copper(II) Complex for Efficient Piezoelectric Energy Harvesting Above Room‐Temperature26An organic-inorganic hybrid thermochromic ferroelastic with multi-channel switches40Multifunctional lanthanide-based single-molecule magnets exhibiting luminescence thermometry and photochromic and ferroelectric properties34Perspectives on recent advancements in energy harvesting, sensing and bio-medical applications of piezoelectric gels161Recent progress in metal halide perovskite photocatalysts for hydrogen evolution31Zero-dimensional organic–inorganic hybrid manganese bromide with coexistence of dielectric–thermal double switches and efficient photoluminescence27Strong Anisotropic Two-Dimensional In2Se3 for Light Intensity and Polarization Dual-Mode High-Performance Detection58Remarkable Enhancement of Piezoelectric Performance by Heavy Halogen Substitution in Hybrid Perovskite Ferroelectrics84Inversion of Molecular Chirality Associated with Ferroelectric Switching in a High-Temperature Two-Dimensional Perovskite Ferroelectric88Photoexcited Ultraviolet‐to‐Infrared (II) Pyroelectricity in a 2D Ferroelectric Perovskite Driving Broadband Self‐Powered Photoactivities63Two-dimensional (n = 1) ferroelectric film solar cells27Bilayered Dion–Jacobson Hybrid Perovskite Bulk Single Crystals Constructed with Aromatic Diammonium for Ultraviolet–Visible–Near-Infrared Photodetection28Large piezoelectric response in a Jahn-Teller distorted molecular metal halide45Facile Control of Ferroelectricity Driven by Ingenious Interaction Engineering36Sonopiezoelectric Nanomedicine and Materdicine58A high-temperature double perovskite molecule-based antiferroelectric with excellent anti-breakdown capacity for energy storage38Photochromic Single-Component Organic Fulgide Ferroelectric with Photo-Triggered Polarization Response26Mono‐ and Bi‐Dentate Chiral Ligands Lead to Efficient Circularly Polarized Luminescence in 0D and 3D Semiconducting Copper(I) Iodides37Superior ferroelectricity and nonlinear optical response in a hybrid germanium iodide hexagonal perovskite133Chirality Inducing Polar Photovoltage in a 2D Lead-Free Double Perovskite toward Self-Powered X-ray Detection116The First Enantiomeric Stereogenic Sulfur‐Chiral Organic Ferroelectric Crystals41Molecular Design of a Metal-Nitrosyl Ferroelectric with Reversible Photoisomerization51Centimeter‐Size Single Crystals of Halide Perovskite Photoferroelectric Solid Solution with Ultrahigh Pyroelectricity Boosted Photodetection29Ferroelectric polymers take a step toward bioelectronics38Organic radical ferroelectric crystals with martensitic phase transition40Building Block‐Inspired Hybrid Perovskite Derivatives for Ferroelectric Channel Layers with Gate‐Tunable Memory Behavior26Ferroelectric Materials for High Energy Density Batteries: Progress and Outlook52Ferroics in Hybrid Organic–Inorganic Perovskites: Fundamentals, Design Strategies, and Implementation42Discovery of Ferroelectricity in the Fullerene Adduct C60S834A review: Polyacrylonitrile as high-performance piezoelectric materials88Chiral‐Achiral Cations Intercalation Induced Lead‐Free Chiral‐Polar Hybrid Perovskites Enable Self‐Powered X‐Ray and Ultraviolet–Visible–Near‐Infrared Photo Detection33Advancements and challenges in molecular/hybrid perovskites for piezoelectric nanogenerator application: A comprehensive review50Strain Engineering in Perovskites: Mutual Insight on Oxides and Halides73Na 2 CeF 6 : A Highly Laser Damage‐Tolerant Double Perovskite Type Ce(IV) Fluoride Exhibiting Strong Second‐Harmonic Generation Effect30Homochirality in Ferroelectrochemistry32X-ray-Induced Pyroelectric Effect in a Perovskite Ferroelectric Drives Low Detection Limit Self-Powered Responses47Chiral three-dimensional organic–inorganic lead iodide hybrid semiconductors26The past 10 years of molecular ferroelectrics: structures, design, and properties173Tuning ferroelectric phase transition temperature by enantiomer fraction34A Chiral B−N Adduct as a New Frontier in Ferroelectrics and Piezoelectric Energy Harvesting32Chirality Triggered Biferroicity in a 3D Rubidium Based Perovskite27Carrier Transport Switching of Ferroelectric BTBT Derivative31Structure-Guided Approaches for Enhanced Spin-Splitting in Chiral Perovskite42A more biofriendly piezoelectric material50Biodegradable ferroelectric molecular crystal with large piezoelectric response267High‐performance Pyroelectric Property Accompanied by Spin Crossover in a Single Crystal of Fe(II) Complex30Efficient Charge Transport in Inverted Perovskite Solar Cells via 2D/3D Ferroelectric Heterojunction25Optical Phenomena in Molecule-Based Magnetic Materials154Ferroelectric Organic–Inorganic Hybrid Ammonium Halogenobismuthate(III) for Piezoelectric Energy Harvesting25Enhancement of phase transition temperature through hydrogen bond modification in molecular ferroelectrics29Intrinsic Elastomer with Remarkable Dielectric Constant via Elastification of Relaxor Ferroelectric Polymer38Inducing Polar Phase in Poly(Vinylidene Fluoride) with a Molecular Ferroelectric Copper(II) Complex for Piezoelectric Energy Harvesting29The First Discovery of Spherical Carborane Molecular Ferroelectric Crystals25X‐ray‐ultraviolet–visible‐near‐infrared photoresponses realized in a lead‐free hybrid perovskite ferroelectric through light‐induced ferro‐pyro‐phototronic effect26Molecular Engineering Regulation Achieving Out‐of‐Plane Polarization in Rare‐Earth Hybrid Double Perovskites for Ferroelectrics and Circularly Polarized Luminescence31Experimental Observation of the Fully Ferroelectric–Fully Ferroelastic Effect in Multiferroic Hybrid Perovskites90Chiral 3D Perovskite Formation Induced by Chiral Templates29A Multiferroic Spin‐Crossover Molecular Crystal32Metal-Free Perovskite Ferroelectrics with the Most Equivalent Polarization Axes40A Z/E isomeric cation designed organic-inorganic cadmium chloride ferroelectric with broadband white-light emission29Advanced Materials for Energy Harvesting and Soft Robotics: Emerging Frontiers to Enhance Piezoelectric Performance and Functionality108Porous flexible molecular-based piezoelectric composite achieves milliwatt output power density74Strain‐Induced Tunable Enhancement of Piezoelectricity in a Novel Molecular Multiferroic Material29Dion–Jacobson Perovskites with a Ferroelectrically Switchable Chiral Nonlinear Optical Response57Dynamic control of halide perovskite structures for tailored ferroelectric and second-order nonlinear optical functionalities39The First Kleinman‐type Second‐Harmonic Generation Circular Dichroism On/Off Switchable Ferroelectrics28Efficient Circularly Polarized Luminescence from Mn–Br Hybrid Perovskite Assembled by Achiral Architectures40Design and Manufacturing of Piezoelectric Biomaterials for Bioelectronics and Biomedical Applications80

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