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RESEARCH PAPER · Chemical Society Reviews · 2021

PFM (piezoresponse force microscopy)-aided design for molecular ferroelectrics

Han‐Yue Zhang, Xiao-Gang Chen, Yuan‐Yuan Tang, Wei‐Qiang Liao, Fang‐Fang Di, Xin Mu, Hang Peng, Ren‐Gen Xiong

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PFM (piezoresponse force microscopy)-aided design for molecular ferroelectricsOriginalA hybrid hydrochromic molecular crystal applicable to invisible ink with high reversibility5Halogen regulation triggers NLO and dielectric dual switches in hybrid compounds with green fluorescence44High-temperature enantiomeric azobenzene-based photoisomerized piezoelectrics: 4-(phenyldiazenyl)anilinium) d - and l -tartrate8Unique cation-template three-dimensional hybrid material demonstrates dielectric switchable response11Optical Control of Polarization Switching in a Single-Component Organic Ferroelectric Crystal96“May the Force Be with You!” Force–Volume Mapping with Atomic Force Microscopy44High Curie temperature bismuth-based piezo-/ferroelectric single crystals of complex perovskite structure: recent progress and perspectives29Highest- T c single-component homochiral organic ferroelectrics23Crown Ether Host‐Guest Molecular Ferroelectrics54Post-synthetic modification within MOFs: a valuable strategy for modulating their ferroelectric performance14An organic plastic ferroelectric with high Curie point36Achieving circularly polarized luminescence and large piezoelectric response in hybrid rare-earth double perovskite by a chirality induction strategy76An unprecedented azobenzene-based organic single-component ferroelectric23Chemical design of homochiral heterocyclic organic ferroelectric crystals8Dual-channel control of ferroelastic domains in a host–guest inclusion compound17Ferroelectricity in organic materials: from materials characteristics to de novo design39The first salicylaldehyde Schiff base organic–inorganic hybrid lead iodide perovskite ferroelectric14Unusual high-temperature host–guest inclusion compound-based ferroelectrics with nonlinear optical switching and large spontaneous polarization behaviours25Recent Advances in Organic and Organic–Inorganic Hybrid Materials for Piezoelectric Mechanical Energy Harvesting335High-Sensitivity Organic–Inorganic Hybrid Materials with Reversible Thermochromic Property and Dielectric Switching31Study on the Luminescence and Coordination Behavior of Semi‐rigid Dual‐Benzimidazole Ligands and Complexes0Multiaxial Ferroelectricity and Ferroelasticity in a Chiral Perovskite51Two-Dimensional Organic–Inorganic Hybrid Materials with Dielectric Switching and Photoluminescence Properties29Two‐Step Dielectric Responsive Organic‐Inorganic Hybrid Material with Mid‐Band Light Emission11Ammonium Sulfate Structure-Type Hybrid Metal Halide Ferroelectric with Giant Uniaxial Spontaneous Strain21Lead-free bilayer heterometallic halide perovskite with reversible phase transition and photoluminescence properties36An Effective Strategy of Introducing Chirality to Achieve Multifunctionality in Rare‐Earth Double Perovskite Ferroelectrics34Rational Design of Molecular Ferroelectrics with Negatively Charged Domain Walls21Discovery of a 2D Hybrid Silver/Antimony‐Based Iodide Double Perovskite Photoferroelectric with Photostrictive Effect and Efficient X‐Ray Response77Enantiomeric Hydrogen-bonded Chains Driving Ferroelectric and Nonlinear Optical Behavior22Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets32Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets0High-Tc Quadratic Nonlinear Optical and Dielectric Switchings in Fe-Based Plastic Crystalline Ferroelectric20Design strategies and effect comparisons toward efficient piezocatalytic system1573D-printed polymer composite devices based on a ferroelectric chiral ammonium salt for high-performance piezoelectric energy harvesting21High-Tc Fe-based ferroelectric compound with large spontaneous polarization and narrow bandgap3Tuning the luminescent properties of a three-dimensional perovskite ferroelectric (Me-Hdabco)CsI 3 via Sn( ii ) doping6A Poling-Free Supramolecular Crown Ether Compound with Large Piezoelectricity68Light-Driven Domain Switching on a Photochromic Ferroelectric7Large Spontaneous Polarization Ferroelectric Property, Switchable Second-Harmonic Generation Responses, and Magnetism in an Fe-Based Compound18Superior ferroelectricity and nonlinear optical response in a hybrid germanium iodide hexagonal perovskite133The First Enantiomeric Stereogenic Sulfur‐Chiral Organic Ferroelectric Crystals41The First Enantiomeric Stereogenic Sulfur‐Chiral Organic Ferroelectric Crystals0Near-90° Switch in the Polar Axis of Dion–Jacobson Perovskites by Halide Substitution46Molecular Design of a Metal-Nitrosyl Ferroelectric with Reversible Photoisomerization51Nano-ferroelectric oxidase mimics for colorimetric detection of glutathione31Photochromic ferroelasticity observed in hybrid lead halide through effective structural regulation18Bidirectional Synaptic Phototransistor Based on Two-Dimensional Ferroelectric Semiconductor for Mixed Color Pattern Recognition66Discovery of ferroelectricity in natural product androstane1Precise Design of Molecular Ferroelectrics with High T C and Tunable Band Gap by Molecular Modification28Design and Piezoelectric Energy Harvesting Properties of a Ferroelectric Cyclophosphazene Salt15Revealing the Polarizations of Molecular Ferroelectrics via SHG Polarimetry at the Nanoscale13Molecular Ferroelectric with Directional Polarization Field for Efficient Tin‐Based Perovskite Solar Cells25Organic radical ferroelectric crystals with martensitic phase transition40Ferroics in Hybrid Organic–Inorganic Perovskites: Fundamentals, Design Strategies, and Implementation42Functional dielectric materials for high-performance solid-state batteries28A Metal‐Free Molecular Ferroelectric [4‐Me‐cyclohexylamine]ClO4 Introduced by Boat and Chair Conformations of Cyclohexylamine5Design of piezoelectric organic cage salts for energy harvesting27Organic‐Inorganic Hybrid Ferroelectric and Antiferroelectric with Afterglow Emission49Organic‐Inorganic Hybrid Ferroelectric and Antiferroelectric with Afterglow Emission10Optical Second Harmonic Generation on Ferroelectric Polarization Reversal for Ferroelectric Hf0.5Zr0.5O2 Capacitors3Crystalline water induced nonpolar‐to‐polar transition and high piezoelectric response in lamivudine hydrate crystal3Perovskite solar cells with ferroelectricity21Piezoelectricity in Molecular Ferroelectrics1Molecular orbital breaking in photo-mediated organosilicon Schiff base ferroelectric crystals23SHG Assisted Mixed‐Phases Anatomizing in a Molecular Ferroelectric7Room Temperature Giant Magnetoelectric Coupling for Magnetic Energy Harvesting in Single Phase {CoIII3DyIII} Molecular Nanogenerator0Perovskite ferroelectric nanostructures for photo(electro)catalysis0Relaxor ferroelectrics for neuromorphic computing0Ferroelectric Texture of Individual Barium Titanate Nanocrystals11Biodegradable Ferroelectric Molecular Plastic Crystal HOCH 2 (CF 2 ) 7 CH 2 OH Structurally Inspired by Polyvinylidene Fluoride21Wearable Photoferroelectric Perovskite X‐Ray Detectors38Solid Solutions of Plastic/Ferroelectric Crystals: Toward Tailor-Made Functional Materials20Experimental Observation of the Fully Ferroelectric–Fully Ferroelastic Effect in Multiferroic Hybrid Perovskites90Metal-Free Perovskite Ferroelectrics with the Most Equivalent Polarization Axes40Exploring Aqueous Solution‐Processed Pseudohalide Rare‐Earth Double Perovskite Ferroelectrics toward X‐Ray Detection with High Sensitivity6Exploring Aqueous Solution‐Processed Pseudohalide Rare‐Earth Double Perovskite Ferroelectrics toward X‐Ray Detection with High Sensitivity25A molecular ferroelectric thin film of imidazolium perchlorate on silicon8Construction of CuO/BiVO4 S-scheme heterojunction with improved carrier separation for efficient piezo-photocatalytic degradation of tetracycline4Strain‐Induced Tunable Enhancement of Piezoelectricity in a Novel Molecular Multiferroic Material29Observation of Ferroelectricity in Carbapenem Intermediates Enables Reactive Oxygen Species Generation by Ultrasound15Ferroelectric Perovskite/MoS 2 Channel Heterojunctions for Wide‐Window Nonvolatile Memory and Neuromorphic Computing40Harnessing thermal waste with a poling-free molecular pyroelectric zinc( ii ) complex3Transition metal doped MoS2 for piezoelectric Fenton-catalyzed degradation of norfloxacin: Rapid innergenerated-H2O2 conversion and dual pathways of non-radicals and radicals29A low-dimensional ferrocenium lead-iodide perovskite ferroelastic with a narrow band gap7Design, Synthesis, and Properties of 1,3-Di-tert-butylazulene Derivatives0Dynamic control of halide perovskite structures for tailored ferroelectric and second-order nonlinear optical functionalities39Piezoelectricity in a mixture of chiral 1D hybrid lead bromide and iodide systems3Organic Photo‐Responsive Piezoelectric Materials Based on Pyrene Molecules for Flexible Sensors6Cholesterol Cocrystal Ferroelectrics Modulated by Solvent Effect6Piezoelectric behavior of a two-dimensional violet phosphorus for controllable neurophysical regeneration1A Homochiral Neutral Organic Molecule as Active Ferroelectric for Memtransistor7Customizing Room‐Temperature Perovskite Ferroelectrics toward the Multichannel Domain Manipulation11Customizing Room‐Temperature Perovskite Ferroelectrics toward the Multichannel Domain Manipulation1Spiro‐Driven Ferroelectric Coordination Polymer Exhibiting Distinct Phase Transitions Under Thermal and Pressure Stimuli0Spiro‐Driven Ferroelectric Coordination Polymer Exhibiting Distinct Phase Transitions Under Thermal and Pressure Stimuli5Polarization Rearrangement Induced High-Efficiency Piezocatalytic Overall Pure Water Splitting in Ultrathin (001)-Confined PbTiO 344Persulfate-assisted photocatalytic pollutant degradation on ferroelectric BaTiO3/CuFe2O4 material: Ferroelectric polarization enhanced electron transfer and persulfate activation29Optimizing the ferroelectric and piezoelectric performance of polyvinylidene fluoride (PVDF) /glass films using spin coating6Polarization direction dependent single-atom catalysis on transition metal-doped In₂Se₃ for OER and ORR7Atomic Off-Centering Driven Phonon-Glass Electron-Crystal-like Thermoelectric Transport in Entropy-Stabilized Quinary Telluride18A Chiral Organic Radical Ferroelectric with Magnetic Circular Dichroism6A Chiral Organic Radical Ferroelectric with Magnetic Circular Dichroism1Jahn–Teller Distortion Enables Enhanced Piezoelectric Energy Harvesting Properties of a Metal-Pyrazolylborate Complex2Next‐Generation Piezoelectric Materials in Wearable and Implantable Devices for Continuous Physiological Monitoring42Self-healing and flexible piezoelectric nanogenerators from sustainable sources: Natural rubber composites empowered by embedded machine learning protocol for real-time remote alert system3High‐Performance Second‐Harmonic Generation in Hybrid Ge Perovskite Ferroelectrics Enabled by Confinement Engineering8Piezoelectric Film-Based Bacterial Disinfection by Mechanical Agitation3Zero‐Dimensional Indium‐Based Multiaxial Ferroelectric for X‐Ray Detection1Tailored d-π Conjugation Boosts Piezocatalytic CO₂ Reduction in a Platinum(II)-Acetylide Framework0Eco‐Friendly Preparation of High‐Quality Lead‐Free Halide Ferroelectric Solid‐Solution Toward High‐Performance X‐ray Detection5Eco‐Friendly Preparation of High‐Quality Lead‐Free Halide Ferroelectric Solid‐Solution Toward High‐Performance X‐ray Detection0Zero‐Electrical‐Energy‐Consumption All‐Optical Synaptic Device Based on Ferroelectric Zero‐Dimensional Perovskite0Ferroelectricity through Reversible Anion-Relay Polarization Switching in a Two-Dimensional Metal–Organic Framework4Room Temperature Giant Magnetoelectric Coupling in {Co III 3 Dy III } Molecular Single Crystal Derived Nanogenerator5Chiral Nonlinear Optical Response in Achiral Quasi‐2D Perovskite Ferroelectric Featuring Unusually Large A‐Site Cation9Chiral Nonlinear Optical Response in Achiral Quasi‐2D Perovskite Ferroelectric Featuring Unusually Large A‐Site Cation2Strain‐Engineered Lattice‐Driven Chirality in CsPbBr 3 Nanorods0Pb(Mg 1/3 Nb 2/3 )O 3 -induced oxygen octahedral distortions and domain growth for concurrent enhancement of multiple parameters in PNN–PZT0Mixed-valence engineered SnSe with anisotropic reconstruction for enhanced piezoelectric ROS generation and MB degradation0Organosilicon cluster goes ferroelectric0Minimalistic metabolite piezoelectric self-assembly for the development of implantable bioelectronics for in vivo monitoring0An Ultrasound‐Triggered Antibacterial Hydrogel With Integrated Antioxidant and Angiogenic Functions for Infected Wound Care0Dual Ferro‐/Piezo‐Electric Coupling in Two‐Dimensional [Bi 2 O 2 ]‐Based Layered Structures for Synergistic Harvesting of Mechanical and Solar Energy2Polarization‐Enabled Piezoelectric Tellurium–Selenium (Te x Se 1– x ) Thin Films for Memory Switching and Artificial Synaptic Functions0Tailored D‐π Conjugation Boosts Piezocatalytic CO 2 Reduction in a Platinum(II)‐Acetylide Framework2Perspective on Ferroelectric and Nonferroelectric Low‐Dimensional Metal Halide Perovskites for Memristor Technology1Chiral Ni2+/Yb3+ molecular complex with room-temperature magnetic-field driven 180° polarization reversal0Piezoelectric Separation Membranes via Dual‐Side Polarization for Micro‐Powered and Fluid‐Responsive Functions0Stretchable, Tough, and Luminescent Perovskite Molecular Ferroelectric Composite: Empowering Reliable Self‐Powered Motion Sensing in High Humidity and Subzero Temperatures0A Novel Non‐centrosymmetric Biocrystal With Hydration‐Enabled Symmetry Breaking and High Piezoelectricity1Stretchable Piezoelectric Membrane of Ferroelectric Charge‐Transfer Cocrystals for Efficient Energy Harvesting and Self‐Powered Wearable Sensors0Ferroelectric Instability Driven Local Atomic Off-Centering and Low Thermal Conductivity in a Topological Crystalline Insulator Sn3Bi0.7Te40Acoustically Assisted Heterojunction Hydrogel Promotes Angiogenesis and Tissue Regeneration by Modulating the Inflammatory Microenvironment0Multistage Fluorination in a Metal‐Free Perovskite Ferroelectric Enables Multidirectional Self‐Powered X‐Ray Detection0Multistage Fluorination in a Metal‐Free Perovskite Ferroelectric Enables Multidirectional Self‐Powered X‐Ray Detection0High Saturation Polarization Ferroelectricity in a Pair of α‐Phase Enantiomorphic Crystals Based on Calabash‐Shaped Molecules0High Saturation Polarization Ferroelectricity in a Pair of α‐Phase Enantiomorphic Crystals Based on Calabash‐Shaped Molecules0Molecular Ferroelectric Catalysis: From Material Design Strategies to Catalytic Applications0Photoactive Biaxial Ferroelectric Polarizations in Flexible Hybrid Metal‐Halide Single‐Crystal Thin Films Driving Multidirectional Self‐Powered Optical Communications0A Polar Magnetic Tetrachloroferrate Hybrid Crystal Enabling Piezoelectric Energy Harvesting and Nonlinear Optical Functionality0Site-Selective Fe Incorporation in Layered Polar α-In2Se3: Crystal-Chemical Control of Localized Spin States and Ferroic Responses0Structure‐Polarization‐Function Relationship in Oxide Perovskite for Solar‐To‐Fuel Conversion Challenge0

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  43. The First Enantiomeric Stereogenic Sulfur‐Chiral Organic Ferroelectric Crystals

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  44. Near-90° Switch in the Polar Axis of Dion–Jacobson Perovskites by Halide Substitution

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