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RESEARCH PAPER · Angewandte Chemie International Edition · 2021

The First High‐Temperature Supramolecular Radical Ferroics

Chaoran Huang, Yibao Li, Yongfa Xie, Ye Du, Hang Peng, Yu‐Ling Zeng, Jun‐Chao Liu, Ren‐Gen Xiong

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The First High‐Temperature Supramolecular Radical FerroicsOriginalHigh-temperature enantiomeric azobenzene-based photoisomerized piezoelectrics: 4-(phenyldiazenyl)anilinium) d - and l -tartrate8Room-temperature dielectric switching in a host–guest crown ether inclusion complex27Crown Ether Host‐Guest Molecular Ferroelectrics542D lead-free organic–inorganic hybrid exhibiting dielectric and structural phase transition at higher temperatures12A Cd-based perovskite with optical-electrical multifunctional response9A ferroelastic molecular rotator [(Me 2 N(CH 2 ) 2 NH 3 )(18-crown-6)]triflate with dual dielectric switches20A new crown-ether clathrate [15-crown-5][Y(NO 3 ) 2 (H 2 O) 5 ][NO 3 ] with switchable dielectric constant behaviour2Achieving circularly polarized luminescence and large piezoelectric response in hybrid rare-earth double perovskite by a chirality induction strategy76Ferroelectricity in organic materials: from materials characteristics to de novo design39High- T p -triggered phase transition exhibiting switchable dielectric–thermal responses and long photoluminescence lifetime in a novel inclusion luminophor6Solvent-induced reversible high-temperature phase transition in crown ether clathrates8Thermally stimuli-responsive materials with transformable double channels of nonlinear optical and dielectric properties5Two host–guest grown ether supramolecules show switchable phase transition, dielectric and second-harmonic generation effect11Recent Advances in Organic and Organic–Inorganic Hybrid Materials for Piezoelectric Mechanical Energy Harvesting335Supramolecular semiquinone radicals confined with DNAzymes for dissipative ROS generation and therapy25Dielectric and Magnetic Relaxations Exhibited in a 2D Parallel Interpenetrating Frustrated Star Net3Chaotropic Effect Stabilized Radical‐Containing Supramolecular Organic Frameworks for Photothermal Therapy33Insights into the Molecular Dynamics of Quasi-Spherical (Chloromethyl)triethylammonium Confined in a Weakly Bound Ionic Cocrystal9Homochiral Multiferroic Cyanido‐Bridged Dimetallic Complexes Assembled by C−F⋅⋅⋅K Interactions1Homochiral Multiferroic Cyanido‐Bridged Dimetallic Complexes Assembled by C−F⋅⋅⋅K Interactions40Ferroelasticity in Organic–Inorganic Hybrid Perovskites63Selenoviologen‐Appendant Metallacycles with Highly Stable Radical Cations and Long‐Lived Charge Separation States for Electrochromism and Photocatalysis10Selenoviologen‐Appendant Metallacycles with Highly Stable Radical Cations and Long‐Lived Charge Separation States for Electrochromism and Photocatalysis60Reversible Phase Transition and Second-Harmonic Response Based on a Zero-Dimensional Organic–Inorganic Hybrid Compound26Piezo-Responsive Hydrogen-Bonded Frameworks Based on Vanillin-Barbiturate Conjugates5An organic-inorganic hybrid thermochromic ferroelastic with multi-channel switches40Halogen-regulating induced reversible high-temperature dielectric and thermal transitions in novel layered organic–inorganic hybrid semiconducting crystals7Piezoelectric Self-Powered Power Supply Driven by Ferroelastic Host-Guest Supramolecule with Considerable Electromechanical Conversion Capability0Remarkable enhancement of optical and electric properties by temperature-controlled solid-phase molecular motion23A Poling-Free Supramolecular Crown Ether Compound with Large Piezoelectricity68Bistable Optoelectronic Properties Originated from the Scissoring Motion of the TEMPO Skeleton in Supramolecular Radical Ferroelectrics4Design and Piezoelectric Energy Harvesting Properties of a Ferroelectric Cyclophosphazene Salt15Zero‐Dimensional Sn‐Based Enantiomeric Phase‐Transition Materials with High‐Tc and Dielectric Switching6Complexation of AAPH (2,2′-azobis(2-methylpropionamidine) dihydrochloride) with cucurbit[7]uril enhances the yield of AAPH-derived radicals5Piezoelectric self-power supply driven by ferroelastic host–guest supramolecule with considerable electromechanical conversion capability29Organic radical ferroelectric crystals with martensitic phase transition40Applications of macrocycle-based solid-state host–guest chemistry179Multifunctional single-component organic molecular materials: ferroelectricity, negative thermal expansion, and polymorphism9The past 10 years of molecular ferroelectrics: structures, design, and properties173Biodegradable ferroelectric molecular crystal with large piezoelectric response267Electrostrictive Effect0Inducing Polar Phase in Poly(Vinylidene Fluoride) with a Molecular Ferroelectric Copper(II) Complex for Piezoelectric Energy Harvesting29Organic Ferroelectrics for Regulation of Electronic and Ionic Transport Toward Neuromorphic Applications15Esterified phenylalanine supramolecular motion: Anion order–disorder rotation induced reversible phase transition and dielectric-ferroelectric properties2Ferroelectric crystals with naphthenic hydrocarbon-modified carborane vertices2Thermal-responsive luminescence/dielectric responses with reversibly shifted light emissions12The First Kleinman‐type Second‐Harmonic Generation Circular Dichroism On/Off Switchable Ferroelectrics28The First Kleinman‐type Second‐Harmonic Generation Circular Dichroism On/Off Switchable Ferroelectrics4Synthesis and properties of L-arginine crown ether type supramolecular phase change materials0Two nonlinear optically responsive crown ether inclusion compounds based on a sulfonimide anion assembly2Halogen-substitution-induced magnetic-phase transition photoelectric synergy in l-valine crown ether inclusion complexes3A Chiral Organic Radical Ferroelectric with Magnetic Circular Dichroism6A Chiral Organic Radical Ferroelectric with Magnetic Circular Dichroism1Asymmetric Coordination Designed Heterocrown Ether Host–Guest Ferroelectrics with Ultrahigh Tc10Hybrid rare-earth double perovskite based on K(I)/pr(III) exhibiting two isostructural phase transitions, switchable dielectric properties, and long fluorescence lifetime4An organic–inorganic hybrid indium molecular ferroelectric originating from a “butterfly-flapping” model of 1,5-diazabicyclo[3.3.0]octane2Multifunctional Lanthanide Molecular Ferroelectrics [ R / S -H 2 MPPA][Ln(btfa) 4 ] 2 Constructed by Hydrogen Bond Linking Functional Blocks3Recent advances in supramolecular ferroelectrics based on macrocycles and cages0

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  15. Supramolecular semiquinone radicals confined with DNAzymes for dissipative ROS generation and therapy

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  16. Dielectric and Magnetic Relaxations Exhibited in a 2D Parallel Interpenetrating Frustrated Star Net

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  17. Chaotropic Effect Stabilized Radical‐Containing Supramolecular Organic Frameworks for Photothermal Therapy

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  18. Insights into the Molecular Dynamics of Quasi-Spherical (Chloromethyl)triethylammonium Confined in a Weakly Bound Ionic Cocrystal

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