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RESEARCH PAPER · Journal of the American Chemical Society · 2020

Precise Molecular Design Toward Organic–Inorganic Zinc Chloride ABX3 Ferroelectrics

Li-Zhuang Chen, Wei‐Qiang Liao, Yong Ai, Jun‐Yi Li, Siyu Deng, Yun‐Long Hou, Yuan‐Yuan Tang

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Precise Molecular Design Toward Organic–Inorganic Zinc Chloride ABX3 FerroelectricsOriginalAbove room-temperature dielectric switching and semiconducting properties of a layered organic–inorganic hybrid compound: (C 6 H 12 N) 2 Pb(NO 3 ) 418Properties and mechanism of strain and piezoelectricity of hybrid molecular ferroelectrics1Confinement-Driven Ferroelectricity in a Two-Dimensional Hybrid Lead Iodide Perovskite167The synthesis, structure, thermal stability and optical properties of organic-inorganic hybrid [(4-ethoxyanilinum)(18-crown-6)][BF4] crystals8The Soft Molecular Polycrystalline Ferroelectric Realized by the Fluorination Effect142Dynamics of Chiral Cations in Two-Dimensional CuX4 and PbX4 Perovskites (X = Cl and Br)24Record Enhancement of Phase Transition Temperature Realized by H/F Substitution114Molecular Design Principles for Ferroelectrics: Ferroelectrochemistry597Recent progress in the piezoelectricity of molecular ferroelectrics84Neutral 1D Perovskite-Type ABX3 Ferroelectrics with High Mechanical Energy Harvesting Performance46Organometallic-Based Hybrid Perovskite Piezoelectrics with a Narrow Band Gap110Two-Dimensional Hybrid Perovskite Ferroelectric Induced by Perfluorinated Substitution166A multiaxial molecular ferroelectric with record high T C designed by intermolecular interaction modulation34(C 2 H 5 NH 3 ) 3 [InBr 6 ]: an indium( iii ) organic–inorganic hybrid phase transition compound exhibiting a switchable dielectric response9A multifunctional molecular ferroelectric with chiral features, a high Curie temperature, large spontaneous polarization and photoluminescence: (C 9 H 14 N) 2 CdBr 450Modulating the ferroelectric performance by altering halogen anions in the crystals of tetranuclear copper-clusters3Monofluorine substitution achieved high- T c dielectric transition in a one-dimensional lead bromide hybrid photoluminescent perovskite semiconductor21PFM (piezoresponse force microscopy)-aided design for molecular ferroelectrics143Temperature‐Induced Reversible Phase Transition with Switchable Dielectric Response in a A2BX4‐Type Hybrid Compound: [TEAMA]2[CdBr4] (TEAMA=(CH3CH2)3NCH3)3General Synthesis of Ultrafine Monodispersed Hybrid Nanoparticles from Highly Stable Monomicelles67Structural phase transition and dielectric switching in an organic-inorganic hybrid rare-earth double perovskite-type compound: (DMP)2LaRb(NO3)6 (DMP = N,N-dimethylpyrrolidinium cation)37Synthesis, structural, spectral and antibacterial activity of organic-inorganic compound (C7H9N4O2).[ZnCl3(H2O)] with theophyllinium as Counter Cation2Organic Enantiomeric Ferroelectrics with High Piezoelectric Performance: Imidazolium l - and d -Camphorsulfonate37Ferroelastic Hybrid Bismuth Bromides with Dual Dielectric Switches69H/F substitution for advanced molecular ferroelectrics104A novel organic–inorganic hybrid phase transition compound based on 4-ethylmorpholine with switchable dielectric and luminescent properties11Dicyanamide-perovskites at the edge of dense hybrid organic–inorganic materials21Band gap modulation of organic–inorganic Sb( iii ) halide by molecular design17Ferroelectric properties in metal-coordinated complex tris(2-hydroxyethyl) ammonium trichloro cadmium( ii )5Multi-functional hybrid perovskites with triple-channel switches and optical properties39Reversible thermochromism to tune the bandgap of organic–inorganic hybrid materials24Symmetry breaking of A 3 M 2 X 9 -type perovskite derivatives induced by polar quaternary ammonium cations: achieving efficient nonlinear optical properties28Unusual symmetry breaking in high-temperature enantiomeric ferroelectrics with large spontaneous polarization20Ferroelectric Lithography in Single‐Component Organic Enantiomorphic Ferroelectrics35Ferroelectric Lithography in Single‐Component Organic Enantiomorphic Ferroelectrics5Study on the Luminescence and Coordination Behavior of Semi‐rigid Dual‐Benzimidazole Ligands and Complexes0Two‐Step Dielectric Responsive Organic‐Inorganic Hybrid Material with Mid‐Band Light Emission11Insights into the Molecular Dynamics of Quasi-Spherical (Chloromethyl)triethylammonium Confined in a Weakly Bound Ionic Cocrystal9Dielectric Response Behavior and Displacement‐Type Metal‐Free Organic‐Inorganic Hybrid Phase Transition Material: trans‐(NH3C6H10NH3)[NO3]24Structure, optical and magnetic properties of the pyridinium cobaltate (C6H9N2)2[CoCl4]16Water‐Resistant Lead‐Free Perovskitoid Single Crystal for Efficient X‐Ray Detection64Multiaxial Molecular Ferroelectrics with a Large Viable Temperature Range23Lead-free bilayer heterometallic halide perovskite with reversible phase transition and photoluminescence properties36Metal-dependent structural phase transition and dielectric response in two organic–inorganic hybrids of [C4H10N]2[SbCl5] and [C4H10N]3[BiCl6]13Anions Distorting Triggering Ferroelectricity in a Molecular Crystal†4Ferroelasticity in Organic–Inorganic Hybrid Perovskites63Organic–Inorganic Hybrid Compound [H2-1,5-Diazabicyclo[3.3.0]octane]ZnBr4 with Reverse Symmetry Breaking Shows a Switchable Dielectric Anomaly and Robust Second Harmonic Generation Effect19Organic Cation Modulation Triggered Second Harmonic Response in Manganese Halides with Bright Fluorescence46Synthesis and Characterization of a Displacement-Type Ferroelectric–Ferroelectric Phase Transition Compound [(NH3)(CH2)3(NH3)]2[InBr6]Br·H2O10H/F-Substitution-Induced Confinement Effect for Designing High-Phase-Transition-Temperature Organic–Inorganic Hybrid Materials16Switchable Dielectric Two-Dimensional Lead-Free Perovskite with Reversible Thermochromic Response26Two 3D Rubidium Halide Organic–Inorganic Hybrid Perovskite Ferroelectrics Templated by Quasi‐Spherical Organic Amine 1,4‐Diazabicyclo[3.2.2]nonane15Ferroelectric hybrid organic–inorganic perovskites and their structural and functional diversity195Selective synthesis and structural study of amino amide trichlorozincates2Metal Halides Based Flexible X‐Ray Detectors9Solid-state molecular dynamics of a torsion-variable ammonium embedded in a deformable supramolecular framework4A multifunctional molecular ferroelectric with a high Curie temperature and electrical–thermal double-switch coexistence: (C 8 H 14 NO)[FeCl 4 ]8Amplification of polarization ratio is observed in monolayer Dion–Jacobson hybrid perovskites6High temperature switchable dielectric properties in molecular crystal material 1,4,7-triazacyclononane trihydrochloride7Lead-Free Hybrid Organic–Inorganic Ferroelectric: (3,3-Difluoropyrrolidinium)2ZnCl4·H2O12Switchable Dielectric Materials Based on a Diprotonated Organic Cation Containing Two Different Anions: (C5H16N2)BF4X (X = Cl, Br, NO3)0A pyrazole-functional 3D cobalt-organic framework for fluorescence detection of Cu2+ and Hg2+13A high-temperature double perovskite molecule-based antiferroelectric with excellent anti-breakdown capacity for energy storage38Allantoin eutectics with choline chloride and zinc chloride: interactions and wound healing applications6Crystal structures and phase transition in a new organic-inorganic hybrid material TEACCl·FeCl45An amide groups functionalized Cd-MOF as multi-responsive luminescent sensor for detecting Fe3+, Cr2O72− and OTC in water media19H/Br substitution in ethylamine improves the phase transition temperature of in-based material (BrC2H4NH3)3[InBr6]0Crown‐Ether‐Ring Size Dependent Crystal Structures, Phase Transition and Dielectric Properties of [M(crown)]BF4⋅xH2O (M+=Na+, K+; crown=15‐crown‐5, 18‐crown‐6; x=0 or 1)31D Chiral Enantiomer Lead-Free Perovskites Induced Chiralopical Activity and Photoelectric Response20Tuning and Enhancing Nonlinear Optical Behavior in Hybrid Arylammonium Perrhenate Salts through Halogen Substitution20A multifunctional fluorescence probe based on a new Cd-MOF for HSO4−, acidic amino acids, and continuous basic amino acids detection74Alkali Metal Organic–Inorganic Hybrid Compounds with Different Crystal Dimensions Show Phase-Transition, Dielectric, and SHG Properties Based on a Quasi-Spherical Amine (1S,4S)-2,5-Diazabicyclo[2.2.1]heptane12Comprehensively understanding the distinct properties of crystal structure, phase transition and dielectrics in [M(crown) n ]ReO 4 (M + = Na + , K + , NH 4 + ; crown = 15-crown-5, 18-crown-6; n = 1 or 2)4The past 10 years of molecular ferroelectrics: structures, design, and properties173Halogen Bonding versus Nucleophilic Substitution in the Co-Crystallization of Halomethanes and Amines6Synthesis of a crystalline functional material based on an aminopyridine-type cobalt thiocyanate complex and characterization of its dielectric-ferroelectric properties0Structural Investigation, Spectroscopic Properties, DFT Calculations and Electrical Properties of [C6H9N2]2 Sb2Cl8 Hybrid Compound4Site-specific molecular design of low-dielectric benzocyclobutene (BCB)-sub-nanometer inorganic nanocomposites0Alkali Metal–Substitution–Induced Confinement Effect for Designing High Phase–Transition–Temperature Molecular–Based Compounds Exhibiting Strong Photoluminescence1Gas adsorption and fluorescence studies of Cd2+ and Zn2+ metal organic frameworks based on the same fluorinated ligand11Negative Thermal Quenching and Self-Trapped Exciton Emission in (R/S-C3H10ON)MnCl323A novel naphthalene diimide-based compound:synthesis, photochromism, ammonia vapor and triethylamine detection10Lead-Free Bismuth-Based Perovskite X-ray Detector with High Sensitivity and Low Detection Limit16The Halogenation Effect Induces a Variety of Switchable Phase Transition and Second-Harmonic-Generation Materials13Ramifications of X-Site Ion Modification in a Zero-Dimensional Piezoelectric Tetrahalozincate1“Butterfly Effect” of Halogen Substitution on Phase Transition Features in One-Dimensional Spin-Peierls-type van der Waals Crystals1Study the electronic, optical, and thermoelectric characteristics of cubic perovskite BXO3 (X = P, As, Sb, Bi): DFT calculations2Halogen Substitution Strategy for Exploiting High‐Performance Molecular Ferroelectrics1Anion‐substituted Hybrid Zinc Halides with Remarkable Dielectric Switches2Versatile synthesis of uniform mesoporous superparticles from stable monomicelle units12Characterization of a New Hybrid Compound (C3H8N6)2ZnCl4·2Cl: X-ray Structure, Hirshfeld Surface, Vibrational, Thermal Stability, Dielectric Relaxation, and Electrical Conductivity17Unusual Thermo‐Enhanced Second Harmonic Generation in Organic Configurationally‐Locked Polyene Crystals8Synthesis and fluorescence recognition properties of two Cd-MOFs based on different mixed ligands7Reconstructive Phase Transition Enables Abnormal Negative Thermal Quenching of Photoluminescence in a 1D Hybrid Perovskite6A high phase transition temperature organic–inorganic Sn( iv )-based metal halide designed by applying amino positional isomerism to the cation11Dynamic control of halide perovskite structures for tailored ferroelectric and second-order nonlinear optical functionalities39Ferroelectricity in perovskites realized by a switchable skewed conformation2Synthesis, structural characterization, Hirshfeld surface analysis, and electrical properties of a zinc (II)-based organic–inorganic hybrid compound15Zero-Dimensional Plastic Phase Transition Iron-Based Compounds with High T c and Switchable SHG Responses5Decarboxylative synthesis of α-iodoalkylammonium salts via ammonio oxime esters2Isopropylammonium halidometallates. I. [Co X 4 ] 2− · X − ( X = Cl, Br), ZnCl 4 2− , and [ZnCl 3 − ] n salts0Cooperative Ligand Engineering Enabling Stepwise Optimization of Metal–Organic Frameworks for Improved C2H2 Separation from CO2 and CH49H/F Substitution‐Engineered Argentophilic Interactions for Enhanced Photoluminescence in 1D Hybrid Silver Halides3Highly Luminescent Hybrid Europium(II) Bromide for Electrically Driven Light‐Emitting Diodes1A Highly Electrostrictive A 2 BX 4 -Type Hybrid 2D Perovskite Ferroelectric and the Utility of Its Piezoelectric Nanogenerator in Wireless Mat-Sensor Technology6Two naphthalene diimide cadmium coordination polymers: Synthesis, photocontrolled luminescence, photo/electrochromism, inkless erasable printing and triethylamine detection3A high-performance photodetector enabled by melamine cation-based lead-free perovskitoid single crystals0Crystal structure, phase transitions, and Hirshfeld surface analysis of the organic–inorganic hybrid [N(CH 3 ) 2 (C 2 H 5 )(i-Pr)] 2 ZnBr 4 compound0A zero-dimensional zinc-based hybrid showing switchable dielectric constant, inverse symmetry breaking and fluorescence property0Emerging halide perovskite ferroelectric semiconductors: Structural diversity, chemical design and optoelectronic applications3Halogen Substitution Dual Regulation of Structure and Symmetry in an Edge-Shared ABX 3 Hybrid Ferroelectric3Organic-inorganic zinc halide multiferroic designed by tetrahedral halogen engineering0Hydrogen Bonding Engineering Achieved Hybrid Antiperovskite Ferroelastic in ( C 3 H 8 ON ) 3 ( SnCl 6 )Cl0Piezoelectric Elastomer with High Voltage Output Enhanced by Molecular Ferroelectric2Harnessing supramolecular confinement for the semihydrogenation of aromatic alkynes0H/F substitution strategy for molecular ferroelectrics: From design principles to emerging materials0Halogen Substitution-Controlled Phase Transition, Dielectric Anomaly, and SHG Switching in Ga-Based Hybrid Molecular Ferroelectrics0

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  50. H/F-Substitution-Induced Confinement Effect for Designing High-Phase-Transition-Temperature Organic–Inorganic Hybrid Materials

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