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RESEARCH PAPER · Nature Reviews Materials · 2020

Chiral-perovskite optoelectronics

Guankui Long, Randy Pat Sabatini, Makhsud I. Saidaminov, Girish Lakhwani, Abdullah Rasmita, Xiaogang Liu, Edward Hartley Sargent, Weibo Gao

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Chiral-perovskite optoelectronicsOriginalAll-inorganic copper( i )-based ternary metal halides: promising materials toward optoelectronics99Circularly polarized luminescence of nanoassemblies via multi-dimensional chiral architecture control87Band Gap-Tunable, Chiral Hybrid Metal Halides Displaying Second-Harmonic Generation110Metal Halide Perovskites in Quantum Dot Solar Cells: Progress and Prospects307Photoredox Organic Synthesis Employing Heterogeneous Photocatalysts with Emphasis on Halide Perovskite72Strategies to Achieve High Circularly Polarized Luminescence from Colloidal Organic–Inorganic Hybrid Perovskite Nanocrystals200Emergent Nonreciprocal Circularly Polarized Emission from an Organic Thin Film111Chiral Transition Metal Oxides: Synthesis, Chiral Origins, and Perspectives74Ligand-Induced Chirality in Asymmetric CdSe/CdS Nanostructures: A Close Look at Chiral Tadpoles94Two-Dimensional Perovskite Chiral Ferromagnets140Optically Active Perovskite CsPbBr3 Nanocrystals Helically Arranged on Inorganic Silica Nanohelices136Organic-to-inorganic structural chirality transfer in a 2D hybrid perovskite and impact on Rashba-Dresselhaus spin-orbit coupling456High‐Performance Circularly Polarized Light‐Sensing Near‐Infrared Organic Phototransistors for Optoelectronic Cryptographic Primitives125Solid-State NMR and NQR Spectroscopy of Lead-Halide Perovskite Materials140Chirality-Induced Spin–Orbit Coupling, Spin Transport, and Natural Optical Activity in Hybrid Organic–Inorganic Perovskites105The Emergence of Halide Layered Double Perovskites161Direct detection of circular polarized light in helical 1D perovskite-based photodiode340Spin-Dependent Photovoltaic and Photogalvanic Responses of Optoelectronic Devices Based on Chiral Two-Dimensional Hybrid Organic–Inorganic Perovskites173Reversible Crystal–Glass Transition in a Metal Halide Perovskite131Chiral Lead‐Free Hybrid Perovskites for Self‐Powered Circularly Polarized Light Detection239Pathways to increase the dissymmetry in the interaction of chiral light and chiral molecules314Recent Progress on Two-Dimensional Materials472Room-temperature ferroelectric and ferroelastic orders coexisting in a new tetrafluoroborate-based perovskite73Tailoring of a visible-light-absorbing biaxial ferroelectric towards broadband self-driven photodetection142Chiral halide perovskite crystals for optoelectronic applications238Giant Optical Activity and Second Harmonic Generation in 2D Hybrid Copper Halides93Chirality communications between inorganic and organic compounds82Unprecedented 2D Homochiral Hybrid Lead‐Iodide Perovskite Thermochromic Ferroelectrics with Ferroelastic Switching157Perspectives of Organic and Perovskite‐Based Spintronics103Chirality‐Dependent Circular Photogalvanic Effect in Enantiomorphic 2D Organic–Inorganic Hybrid Perovskites125Direct Detection of Circularly Polarized Light Using Chiral Copper Chloride–Carbon Nanotube Heterostructures147Circularly polarized luminescence from organic micro-/nano-structures419Chiral Perovskites for Next‐Generation Photonics: From Chirality Transfer to Chiroptical Activity263Circularly polarized luminescence of agglomerate emitters174Chiral 2D-Perovskite Nanowires for Stokes Photodetectors205Recent Progress of Chiral Perovskites: Materials, Synthesis, and Properties314Memory Seeds Enable High Structural Phase Purity in 2D Perovskite Films for High‐Efficiency Devices100Ferroelectricity and Rashba effect in 2D organic–inorganic hybrid perovskites85Emerging perovskite monolayers291Advances of Nonlinear Photonics in Low‐Dimensional Halide Perovskites67State of the Art and Prospects for Halide Perovskite Nanocrystals1478Chirality‐Dependent Second‐Order Nonlinear Optical Effect in 1D Organic–Inorganic Hybrid Perovskite Bulk Single Crystal245A new strategy to achieve enhanced upconverted circularly polarized luminescence in chiral perovskite nanocrystals70Great Amplification of Circular Polarization Sensitivity via Heterostructure Engineering of a Chiral Two-Dimensional Hybrid Perovskite Crystal with a Three-Dimensional MAPbI3 Crystal73Tuning the Circular Dichroism and Circular Polarized Luminescence Intensities of Chiral 2D Hybrid Organic–Inorganic Perovskites through Halogenation of the Organic Ions178Stimuli-responsive switchable halide perovskites: Taking advantage of instability98Spin‐Dependent Charge Transport in 1D Chiral Hybrid Lead‐Bromide Perovskite with High Stability97Structural descriptor for enhanced spin-splitting in 2D hybrid perovskites225Heterogeneous Integration of Chiral Lead–Chloride Perovskite Crystals with Si Wafer for Boosted Circularly Polarized Light Detection in Solar‐Blind Ultraviolet Region68Chiral Hybrid Perovskite Single‐Crystal Nanowire Arrays for High‐Performance Circularly Polarized Light Detection85Strong Second- and Third-Harmonic Generation in 1D Chiral Hybrid Bismuth Halides159Chiral Self‐Assembled Film from Semiconductor Nanorods with Ultra‐Strong Circularly Polarized Luminescence66Full‐Stokes Polarimeter Based on Chiral Perovskites with Chirality and Large Optical Anisotropy671D Chiral Lead Halide Perovskites with Superior Second‐Order Optical Nonlinearity100Alkyl–Aryl Cation Mixing in Chiral 2D Perovskites137Emerging materials for circularly polarized light detection97To nano or not to nano for bright halide perovskite emitters68Hierarchical self-assembly into chiral nanostructures202Frontiers in circularly polarized luminescence: molecular design, self-assembly, nanomaterials, and applications608Multidimensional nanoscopic chiroptics212The evolution and future of metal halide perovskite-based optoelectronic devices83Photonic and Plasmonic Metasensors129Ligand Exchange Strategy to Achieve Chiral Perovskite Nanocrystals with a High Photoluminescence Quantum Yield and Regulation of the Chiroptical Property65Achieving circularly polarized luminescence and large piezoelectric response in hybrid rare-earth double perovskite by a chirality induction strategy76Ultrasensitive Near‐Infrared Circularly Polarized Light Detection Using 3D Perovskite Embedded with Chiral Plasmonic Nanoparticles73Chiral Hybrid Copper(I) Halides for High Efficiency Second Harmonic Generation with a Broadband Transparency Window112Regulating Optical Activity and Anisotropic Second-Harmonic Generation in Zero-Dimensional Hybrid Copper Halides114High Responsivity Circular Polarized Light Detectors based on Quasi Two-Dimensional Chiral Perovskite Films148Circularly polarized luminescence in chiral materials443Multifunctional Chiral 2D Lead Halide Perovskites with Circularly Polarized Photoluminescence and Piezoelectric Energy Harvesting Properties112Circularly polarized luminescence of coordination aggregates114Rationalizing the design and implementation of chiral hybrid perovskites129Perovskite metasurfaces with large superstructural chirality153Chiral carbon dots: synthesis, optical properties, and emerging applications286Self‐Powered Visible‐Infrared Polarization Photodetection Driven by Ferroelectric Photovoltaic Effect in a Dion–Jacobson Hybrid Perovskite85Tunable Circularly Polarized Luminescence from Inorganic Chiral Photonic Crystals Doped with Quantum Dots93Structural Origin of Enhanced Circularly Polarized Luminescence in Hybrid Manganese Bromides113Enantiomorphic Single Crystals of Linear Lead(II) Bromide Perovskitoids with White Circularly Polarized Emission64Control of light, spin and charge with chiral metal halide semiconductors203Tailoring the Distinctive Chiral‐Polar Perovskites with Alternating Cations in the Interlayer Space for Self‐Driven Circularly Polarized Light Detection65Liquid crystal-templated chiral nanomaterials: from chiral plasmonics to circularly polarized luminescence266Robust Spin-Dependent Anisotropy of Circularly Polarized Light Detection from Achiral Layered Hybrid Perovskite Ferroelectric Crystals85Induction of Chiral Hybrid Metal Halides from Achiral Building Blocks103Configurable Organic Charge Carriers toward Stable Perovskite Photovoltaics84Recent Progress of Polarization‐Sensitive Perovskite Photodetectors134Chiral Rashba Ferroelectrics for Circularly Polarized Light Detection174Stereochemically Active Lone Pairs and Nonlinear Optical Properties of Two-Dimensional Multilayered Tin and Germanium Iodide Perovskites116Chiral Mesostructured Inorganic Materials with Optical Chiral Response110Achiral-Core-Metal Change in Isomorphic Enantiomeric Ag12Ag32 and Au12Ag32 Clusters Triggers Circularly Polarized Phosphorescence90Ferroelectric hybrid organic–inorganic perovskites and their structural and functional diversity195Revealing the Intrinsic Chiroptical Activity in Chiral Metal-Halide Semiconductors132Maximally Chiral Emission via Chiral Quasibound States in the Continuum74Terahertz Circular Dichroism Spectroscopy of Molecular Assemblies and Nanostructures65Multifunctionality of luminescent molecular nanomagnets based on lanthanide complexes67Metal Halide Perovskite for next-generation optoelectronics: progresses and prospects498Pyro-phototronic effect: An effective route toward self-powered photodetection116Highly Anisotropic Second-Order Nonlinear Optical Effects in the Chiral Lead-Free Perovskite Spiral Microplates93The rise of halide perovskite semiconductors137Nanoimprinted 2D‐Chiral Perovskite Nanocrystal Metasurfaces for Circularly Polarized Photoluminescence91Toward Efficient Two‐Photon Circularly Polarized Light Detection through Cooperative Strategies in Chiral Quasi‐2D Perovskites65Ligand Chemistry of Inorganic Lead Halide Perovskite Nanocrystals388Highly Efficient and Stable FA‐Based Quasi‐2D Ruddlesden–Popper Perovskite Solar Cells by the Incorporation of β‐Fluorophenylethanamine Cations96Current Understanding of Band-Edge Properties of Halide Perovskites: Urbach Tail, Rashba Splitting, and Exciton Binding Energy86Symmetry-Broken 2D Lead–Tin Mixed Chiral Perovskite for High Asymmetry Factor Circularly Polarized Light Detection93Inversion of Molecular Chirality Associated with Ferroelectric Switching in a High-Temperature Two-Dimensional Perovskite Ferroelectric88Metal‐Halide Perovskite Lasers: Cavity Formation and Emission Characteristics92Carbon Dots for Electroluminescent Light‐Emitting Diodes: Recent Progress and Future Prospects121Chirality-Dependent Structural Transformation in Chiral 2D Perovskites under High Pressure75Emerging Opportunities in Lead-Free and Lead–Tin Perovskites for Environmentally Viable Photodetector Applications72Spin Polarization of Chiral Amorphous Fe‐Ni Electrocatalysts Enabling Efficient Electrochemical Oxygen Evolution67Phase-pure two-dimensional layered perovskite thin films199Macroscopic Assembly of Chiral Hydrogen‐bonded Metal‐free Supramolecular Glasses for Enhanced Color‐tunable Ultralong Room Temperature Phosphorescence140Emerging Spintronic Materials and Functionalities106Synergy of 3D and 2D Perovskites for Durable, Efficient Solar Cells and Beyond249Multiple Stimuli‐Responsive Luminescent Chiral Hybrid Antimony Chlorides for Anti‐Counterfeiting and Encryption Applications114Manipulating Peierls Distortion in van der Waals NbOX 2 Maximizes Second-Harmonic Generation90Toward Chiral Lasing from All‐Solution‐Processed Flexible Perovskite‐Nanocrystal–Liquid‐Crystal Membranes68Integrating Achiral and Chiral Organic Ligands in Zero‐Dimensional Hybrid Metal Halides to Boost Circularly Polarized Luminescence81Spin selection in atomic-level chiral metal oxide for photocatalysis169Multifunctional Perovskite Photodetectors: From Molecular-Scale Crystal Structure Design to Micro/Nano-scale Morphology Manipulation116Chiral Inorganic Nanomaterials for Photo(electro)catalytic Conversion71Nucleation-mediated growth of chiral 3D organic–inorganic perovskite single crystals92Chiral Hybrid Germanium(II) Halide with Strong Nonlinear Chiroptical Properties114Bright circularly polarized photoluminescence in chiral layered hybrid lead-halide perovskites137Low‐Dimensional‐Materials‐Based Photodetectors for Next‐Generation Polarized Detection and Imaging155Recyclable soft photonic crystal film with overall improved circularly polarized luminescence76Spin Quantum Dot Light‐Emitting Diodes Enabled by 2D Chiral Perovskite with Spin‐Dependent Carrier Transport83Ligand Engineering Enables Efficient Pure Red Tin‐Based Perovskite Light‐Emitting Diodes71Circular polarization-resolved ultraviolet photonic artificial synapse based on chiral perovskite107Circularly Polarized Light-Dependent Pyro-Phototronic Effect from 2D Chiral–Polar Double Perovskites74Free Halogen Substitution of Chiral Hybrid Metal Halides for Activating the Linear and Nonlinear Chiroptical Properties140In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation68Chirality Engineering of Colloidal Copper Oxide Nanostructures for Tailored Spin-Polarized Catalysis95The first chiral cerium halide towards circularly-polarized luminescence in the UV region65Chiral Induced Spin Selectivity603Phase Transitions and Dynamics in Mixed Three- and Low-Dimensional Lead Halide Perovskites134Precise Modulation of Circularly Polarized Luminescence via Polymer Chiral Co‐assembly and Contactless Dynamic Chiral Communication92Chiral materials and mechanisms for circularly polarized light-emitting diodes289Mechanically Tunable Circularly Polarized Luminescence of Liquid Crystal‐Templated Chiral Perovskite Quantum Dots137Optical Phenomena in Molecule-Based Magnetic Materials154Chiral-structured heterointerfaces enable durable perovskite solar cells215Room-temperature spin injection across a chiral perovskite/III–V interface100Zero-dimensional halide hybrid bulk glass exhibiting reversible photochromic ultralong phosphorescence150Emerging chiral two-dimensional materials70Advanced Organic–Inorganic Hybrid Materials for Optoelectronic Applications222Materials and methods for cost-effective fabrication of perovskite photovoltaic devices70Metasurface-enabled broadband multidimensional photodetectors85Remote chirality transfer in low-dimensional hybrid metal halide semiconductors67Biomimetic optoelectronics with nanomaterials for artificial vision85Optimizing photocatalysis via electron spin control139

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  44. Chiral halide perovskite crystals for optoelectronic applications

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  46. Giant Optical Activity and Second Harmonic Generation in 2D Hybrid Copper Halides

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