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RESEARCH PAPER · ACS Energy Letters · 2020

The Emergence of Halide Layered Double Perovskites

Brenda Cabral Vargas, Germán Rodrı́guez-López, Diego Solís-Ibarra

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The Emergence of Halide Layered Double PerovskitesOriginalEfficient Emission in Halide Layered Double Perovskites: The Role of Sb 3+ Substitution in Cs 4 Cd 1– x Mn x Bi 2 Cl 12 Phosphors48Phase Transitions in Low-Dimensional Layered Double Perovskites: The Role of the Organic Moieties42An unprecedented hexagonal double perovskite organic–inorganic hybrid ferroelastic material: (piperidinium) 2 [KBiCl 6 ]43Monofluorine substitution achieved high- T c dielectric transition in a one-dimensional lead bromide hybrid photoluminescent perovskite semiconductor21Strong Self‐Trapped Exciton Emissions in Two‐Dimensional Na‐In Halide Perovskites Triggered by Antimony Doping139Strong Self‐Trapped Exciton Emissions in Two‐Dimensional Na‐In Halide Perovskites Triggered by Antimony Doping13Doubling the Stakes: The Promise of Halide Double Perovskites159Doubling the Stakes: The Promise of Halide Double Perovskites55Dark Self-Healing-Mediated Negative Photoconductivity of a Lead-Free Cs 3 Bi 2 Cl 9 Perovskite Single Crystal94Lead-free halide perovskites, beyond solar cells and LEDs28Non-toxic near-infrared light-emitting diodes40Bismuth/Silver-Based Two-Dimensional Iodide Double and One-Dimensional Bi Perovskites: Interplay between Structural and Electronic Dimensions66Colloidal synthesis and charge carrier dynamics of Cs4Cd1−Cu Sb2Cl12 (0 ≤ x ≤ 1) layered double perovskite nanocrystals32Electronic structure and stability of the (0 0 1) surface of halide double perovskite Cs2AgBiBr64Halide Perovskites for Memristive Data Storage and Artificial Synapses91Structure and Optical Properties of Hybrid-Layered-Double Perovskites (C 8 H 20 N 2 ) 2 AgMBr 8 (M = In, Sb, and Bi)24Cyan Emission in Two-Dimensional Colloidal Cs2CdCl4:Sb3+ Ruddlesden–Popper Phase Nanoplatelets67Metal Halide Semiconductors beyond Lead-Based Perovskites for Promising Optoelectronic Applications54Red-emissive nanocrystals of Cs 4 Mn x Cd 1− x Sb 2 Cl 12 layered perovskites11Temperature-induced orbital polarizations and tunable charge dynamics in layered double perovskite thin films10Exciton Self-Trapping for White Emission in 100-Oriented Two-Dimensional Perovskites via Halogen Substitution131(BA) 10 AgBi 2 Br 19 : a one-dimensional halide double perovskite with a unique Br trimer7Dehydration-activated structural phase transition in a two-dimensional hybrid double perovskite14The construction of a two-dimensional organic–inorganic hybrid double perovskite ferroelastic with a high T c and narrow band gap82The effect of halogenated spacer cations on structural symmetry-breaking in 2D halide double perovskites10Stabilization of Metastable Halide Perovskite Lattices in the 2D Limit64Theoretical Prediction of Mixed-Valence Layered Halide Perovskites Cs4M(IV)M(II)2X12 (M = Ge, Sn; X = Cl, Br)14Two-Step Crystallization for Low-Oxidation Tin-Based Perovskite Light-Emitting Diodes36Strain-Induced Band-Edge Modulation in Lead-Free Antimony-Based Double Perovskite for Visible-Light Absorption22Chemical Control of Magnetic Ordering in Hybrid Fe–Cl Layered Double Perovskites58Physically Detachable and Operationally Stable Cs2SnI6 Photodetector Arrays Integrated with µ‐LEDs for Broadband Flexible Optical Systems58Polyoxomolybdate Layered Crystals Constructed from a Heterocyclic Surfactant: Syntheses, Pseudopolymorphism and Introduction of Metal Cations4Tailoring Photoluminescence by Strain-Engineering in Layered Perovskite Flakes25Construction, photoelectric response and phase transition for new hybrid double perovskites showing narrow band gaps41Structural properties of defective (CH 3 NH 3 ) 2 Cu(Cl 1– x Br x ) 4 compounds5Strategies for high‐performance perovskite solar cells from materials, film engineering to carrier dynamics and photon management56Progress on Emerging Ferroelectric Materials for Energy Harvesting, Storage and Conversion187Chiral Methylbenzylammonium Bismuth Iodide with Zero-Dimensional Perovskite Derivative Structure37Pb-free halide perovskites for solar cells, light-emitting diodes, and photocatalysts34Low‐Frequency Phonon Modes in Layered Silver‐Bismuth Double Perovskites: Symmetry, Polarity, and Relation to Phase Transitions10Improving Charge Carrier Mobility Estimations When Using Space-Charge-Limited Current Measurements49Raman spectroscopy in layered hybrid organic-inorganic metal halide perovskites38Lead‐Free Halide Double Perovskites: Fundamentals, Challenges, and Photovoltaics Applications124Discovery of a 2D Hybrid Silver/Antimony‐Based Iodide Double Perovskite Photoferroelectric with Photostrictive Effect and Efficient X‐Ray Response77NH4+/K+-substitution-induced C–F–K coordination bonds for designing the highest-temperature hybrid halide double perovskite ferroelastic11Two-Dimensional Lead-Free Double Perovskite with Superior Stability and Optoelectronic Properties for Solar Cell Application10Design, synthesis, optical studies, and application of all-inorganic layered double perovskites as stabilizers in ambient air processed perovskite solar cells16Progress in all-inorganic heterometallic halide layered double perovskites26Recent Advances on Mn2+‐Doping in Diverse Metal Halide Perovskites662D nanosheets of layered double perovskites: synthesis, photostable bright orange emission and photoluminescence blinking9All-green Cs 4 CuSb 2 Cl 12 perovskite films deposited in situ by AACVD and their doping with F − ions for photodetectors and memdiodes10Challenges and future prospects2Discovering layered lead-free perovskite solar absorbers via cation transmutation12Effect of Mn 2+ doping on exciton recombination and carrier trapping in the Cs 2 CdCl 4 metal halide24Influence of Mn2+ doping on the optical properties of Cs2AgBiCl6 double perovskite luminescent phosphors16Modulating the Schottky barriers of metal–2D perovskite junctions through molecular engineering of spacer ligands4Molybdenum chloride double perovskites: dimensionality control of optical and magnetic properties25An Inorganic–Organic Hybrid Framework Composed of Polyoxotungstate and Long-Chained Bolaamphiphile4Elucidating the Mn2+ Dopant Sites in Two-Dimensional Na–In Halide Perovskite15Doping Mn2+ in a New Layered Halide Double Perovskite PPA4NaInCl8 (PPA+ = C6H5(CH2)3NH3+): Dimensional Reduction Accelerating Mn2+ Dissolution and Separation for Efficient Light Emission10Regulation of excitation energy transfer in Sb-alloyed Cs4MnBi2Cl12 perovskites for efficient CO2 photoreduction to CO and water oxidation toward H2O222Lanthanide Double Perovskite Nanocrystals with Emissions Covering the UV‐C to NIR Spectral Range73Lead‐Free Double Perovskite Semiconductor with Rigid Spacer‐Induced High‐Tc Dielectric Switch Features10Photoluminescence Emission Studies on a Lanthanum-Doped Lead Free Double Halide Perovskite, La:Cs2SnCl652Structural, Electronic, Optical, and Mechanical Properties of Cu(I)Au(III)‐Based Double Perovskites: A First‐Principles Study4Thickness optimization of SnO2 electron transporting layer in perovskite solar cells assembled under ambient atmosphere10Methylammonium Tetrel Halide Perovskite Ion Pairs and Their Dimers: The Interplay between the Hydrogen-, Pnictogen- and Tetrel-Bonding Interactions7Magnetic hybrid transition metal halides17Wide‐Bandgap Perovskite‐Inspired Materials: Defect‐Driven Challenges for High‐Performance Optoelectronics65Enhanced stability and optoelectronic properties of double perovskite Cs2AgSbI6 by Br doping for solar cells22In/Bi-based Direct- and Indirect-Gap Hybrid Double-Perovskite-Derived 1D Halides with Near-Unity Quantum Yield via Sb 3+ Doping34Ab-initio modeling of photo-active materials beyond conventional lead halide perovskites0Lead‐Free Cs 3 Bi 2 I 9 Perovskite‐Like Material as Efficient Photocatalyst for Improved Hydrogen Evolution in Presence of Platinum Co‐Catalyst70D Pyramid‐intercalated 2D Bimetallic Halides with Tunable Electronic Structures and Enhanced Emission under Pressure180D Pyramid‐intercalated 2D Bimetallic Halides with Tunable Electronic Structures and Enhanced Emission under Pressure1Bromination of organic spacer impacts on the structural arrangement, phase transitions, and optical and electrical properties of a hybrid halide compound:[(CH 3 ) 3 N(CH 2 ) 3 Br] 2 PdBr 45Molecular Design of Layered Hybrid Silver Bismuth Bromine Single Crystal for Ultra‐Stable X‐Ray Detection With Record Sensitivity58Halide Double Perovskites8Rational design of enantiomeric lead-free double perovskites by achiral-chiral cation intercalation28A polar two-dimensional lead-free hybrid perovskite for self-powered polarization-sensitive photodetection23A two-dimensional lead-free double perovskite for self-powered and high performance X-ray detection7Vacancy Ordered Lead Free Double Perovskite Based Flexible Supercapacitor for Sustainable Energy Applications23Electronic Structure, Optical Transitions, and Transport Properties of Thiocyanate-Substituted α-FAPbI 3 Perovskite Analogues4Efficient Deep‐Blue Light‐Emitting 2D (100)‐Oriented Perovskites and Spectral Broadening by Exciton Self‐Trapping for White‐light Emissions5B(I)‐Site Alkali Metal Engineering of Lead‐Free Perovskite Nanocrystals for Efficient X‐Ray Detection and Imaging23Structure Directing Forces in Hybrid Layered Double Perovskites Containing Aromatic Organic Cations5Fine Tuning Ag(I)–Sb(III) Hybrid Iodides for Light Detection5Lanthanide Doping into All-Inorganic Heterometallic Halide Layered Double Perovskite Nanocrystals for Multimodal Visible and Near-Infrared Emission66Lead-free magnetic double perovskites for photovoltaic and photocatalysis applications21Advancements in Photovoltaic Cell Materials: Silicon, Organic, and Perovskite Solar Cells248Stereochemically Active Lone Pair Leads to Birefringence in the Vacancy Ordered Cs3Sb2Cl9 Perovskite Single Crystals13Beyond lead halide perovskites: Crystal structure, bandgaps, photovoltaic properties and future stance of lead-free halide double perovskites88Two-Dimensional Double Perovskites in the Dion–Jacobson Phase Alleviate Parity Forbidden Transitions for Photovoltaic Applications1A Double Perovskite Single Crystal CsCuAgI38One-Dimensional Organic–Inorganic Hybrid Double Perovskites with Near-Unity Photoluminescence Quantum Yield and Advanced Multifunctional Applications37DFT study of optoelectronics and transport properties of double perovskites Cs2YCuX6 (X = Cl, Br, I) for energy conversion devices3Investigating structural, phonons, optoelectronics, and thermodynamic properties of lead-free double perovskites of A-site cation ordering in LiXTl2Cl6 (X= Sc and Y) compounds for green energy applications2New Lead‐free Hybrid Layered Double Perovskite Halides: Synthesis, Structural Transition and Ultralow Thermal Conductivity5New Lead‐free Hybrid Layered Double Perovskite Halides: Synthesis, Structural Transition and Ultralow Thermal Conductivity20Machine‐Learning‐Assisted Discovery of Mechanosynthesized Lead‐Free Metal Halide Perovskites for the Oxidative Photocatalytic Cleavage of Alkenes22Strain in Hybrid Organic‐Inorganic Metal Halide Perovskites Microstructures by Numerical Simulations1Tailorable Magnetic Exchange and Optical Absorption in 1-D Double Perovskite-like Halides (CH3NH3)2NaMoCl(6–x)Brx62D Metal Enabled Weak Fermi Level Pinning Effect and Tunable Charge Injection in Contacts with Inorganic 2D Perovskites4Modeling of a Single‐Band‐Ratiometric Sensor Based on Lattice Positive Thermal Expansion in Eu 3+ ‐Activated Halide Perovskite Cs 2 NaEuCl 622Highly stable and self-powered ultraviolet photodetector based on Dion-Jacobson phase lead-free double perovskite9Ambient processed highly stable self-powered lead-free Cs2AgBiBr6 double perovskite photodetector in HTM-free architecture with Carbon as electrode10Layered and Low-Dimensional Lead, Silver, and Bismuth Halide Perovskites Directed by Halogen-Substituted Spacer Cations12Polyurethane-coated double perovskite (Cs4Mn1-xCdxBi2Cl12) significantly improves stability and flexible anticounterfeiting1Iodide Double Perovskites and the Limits of their Structural Stability8Nanoscale scintillating materials for X-ray imaging: fundamentals and applications18First-principles investigation of electronic, magnetic and optical properties of double perovskite oxides Ba2NiYO6 (Y = Pd, Pt)3Lead-free metal halide double perovskites – from crystal design to optoelectronic applications13The impact of antimony on all-inorganic lead-free perovskites: progress in optical advancement and applications11Unity photoluminescence quantum yield and superior stability achieved in lanthanide-doped lead-free Cs 2 NaInCl 6 double perovskites for highly efficient light emitting diodes0Design of a novel eco-friendly bismuth-based solar cell by first-principles calculation and device simulation4Density functional theory based computation of the optoelectronic properties of double perovskites A2InAgBr6 (A= Na, Cs, Rb, and K) and their performance assessment as absorber for photovoltaic applications9Theoretical design of 2D hybrid lead-free halide perovskites for photovoltaic applications2Alkaline Earth Metal Ions Dynamics in Mixed Ionic-Electronic Conductors of Graphite Intercalation Compounds16Underlying Dynamics of Double-Halide Perovskites: Unraveling Structural Complexity, Bandgap Modulation, Optical, and Carrier Dynamics for Next-Generation Optoelectronics24Perovskite quantum dots Revolutionize Lithium-Sulfur battery Performance: Cathode catalytic Breakthrough with CsPbBr314Zero Phonon Line and Near-Infrared Luminescence in Cs4CdSb2–xCrxCl12 Quadruple-Layered Halide Double Perovskite1Tailoring Substitutional Sites for Efficient Lanthanide Doping in Lead-Free Perovskite Nanocrystals with Enhanced Near-Infrared Photoluminescence44Mixed-valence halide perovskites13Environmental‐Friendly Self‐Powered Polarization Photodetector Based on Lead‐Free Halide Double Perovskite Single Crystals with Asymmetric Contacts7A Copper-Rich Multinary Iodido Bismuthate with Cationic Ligands and Broad Red Emission3Dimensional reduction in Cs2AgBiBr6 enables long-term stable Perovskite-based gas sensing24Discovering novel halide perovskites using generative adversarial networks and random forest regression4M(III) Site‐Driven Structural Engineering on Lead‐Free Layered Double Perovskite Nanocrystals with Enhanced Photoelectrochemical Activity4Direction and Temperature-Dependent Properties of an Antimony-Based Two-Dimensional Halide Double Perovskite1Molecular Engineering of Layered Halide Double Perovskites: Challenges and Opportunities in Optoelectronics and Beyond22Lifting Triplet Degeneracy Through Organic‐Cation Driven Structural Perturbation to Modulate Luminescence of Sb 3+ ‐Doped Double Perovskite15Hybrid Simulation and Machine Learning Framework for Optimizing Cs₂InAgBr₆-Based Lead-Free Perovskite Solar Cells1Record Second‐Harmonic Generation in a Lead‐Free 2D Hybrid Halide Perovskite13A comprehensive study of the structural and optical properties of cesium-antimony based layered double perovskite for possible optoelectronic applications4A machine-learned interatomic potential for defects investigation in lead-free double perovskite Cs 2 NaYbCl 62Hydration-mediated morphological and electronic tuning in layered double perovskites for p-type transparent conductors3A 2D Double Perovskite Based on the Chiral Cystaminium Cation Exhibiting Multiple Switches in Quadratic Nonlinear Optical Response7Temperature-Dependent Exciton Dynamics of Cs 4 CuSb 2 Cl 12 Layered Double Perovskite Nanocrystal Thin Films2Thermally Stable Binary Two-Dimensional Hybrid Organic–Inorganic Perovskite Glasses5Boosting luminescence in Cs3Sb2Cl9-derived Cs4MnSb2Cl12 through Cd2+ dopant incorporation1Resolving 209Bi sites in mixed-halide double perovskites at 28 T2Wide energy bandgap Tyraminium–Hexafluorostannate (IV) hybrid: Synthesis, supramolecular assembly, Hirshfeld surface analysis, energy framework topology, DFT calculations, and perspectives for optoelectronic applications1Recent breakthroughs in lead-free perovskite nanocrystals7Studies of Electronic Defects in Cs 2 NaInCl 6 Double Perovskite by GFN1-xTB Calculations1Achieving record birefringence in metal-free semiorganic sulfate crystals via tetrahedral anionic group substitution0Exciton localization and trap-assisted recombination govern wavelength-selective photodetection in lead-free Cs 4 CuSb 2 Cl 12 double perovskite nanocrystals0High-entropy perovskite halides: design principles, properties, and emerging applications0Nanocrystal Synthesis Derived Approach to Silver Bismuth Iodide Layered Double Perovskites with Aliphatic Amines: (C n H (2 n +1) NH 3 ) 4 AgBiI 82A-Site Cation Functional Engineering Enables Lead-free Perovskite Photosynapse for Neuromorphic Visual Computing1Exploring Hybrid Metal Halide Materials beyond Halide Perovskites7

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  1. Efficient Emission in Halide Layered Double Perovskites: The Role of Sb 3+ Substitution in Cs 4 Cd 1– x Mn x Bi 2 Cl 12 Phosphors

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  2. Phase Transitions in Low-Dimensional Layered Double Perovskites: The Role of the Organic Moieties

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  3. An unprecedented hexagonal double perovskite organic–inorganic hybrid ferroelastic material: (piperidinium) 2 [KBiCl 6 ]

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  4. Monofluorine substitution achieved high- T c dielectric transition in a one-dimensional lead bromide hybrid photoluminescent perovskite semiconductor

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  7. Doubling the Stakes: The Promise of Halide Double Perovskites

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  9. Dark Self-Healing-Mediated Negative Photoconductivity of a Lead-Free Cs 3 Bi 2 Cl 9 Perovskite Single Crystal

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  10. Lead-free halide perovskites, beyond solar cells and LEDs

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  13. Colloidal synthesis and charge carrier dynamics of Cs4Cd1−Cu Sb2Cl12 (0 ≤ x ≤ 1) layered double perovskite nanocrystals

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  14. Electronic structure and stability of the (0 0 1) surface of halide double perovskite Cs2AgBiBr6

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  15. Halide Perovskites for Memristive Data Storage and Artificial Synapses

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  16. Structure and Optical Properties of Hybrid-Layered-Double Perovskites (C 8 H 20 N 2 ) 2 AgMBr 8 (M = In, Sb, and Bi)

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  21. Exciton Self-Trapping for White Emission in 100-Oriented Two-Dimensional Perovskites via Halogen Substitution

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  23. Dehydration-activated structural phase transition in a two-dimensional hybrid double perovskite

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  27. Theoretical Prediction of Mixed-Valence Layered Halide Perovskites Cs4M(IV)M(II)2X12 (M = Ge, Sn; X = Cl, Br)

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  29. Strain-Induced Band-Edge Modulation in Lead-Free Antimony-Based Double Perovskite for Visible-Light Absorption

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  30. Chemical Control of Magnetic Ordering in Hybrid Fe–Cl Layered Double Perovskites

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  31. Physically Detachable and Operationally Stable Cs2SnI6 Photodetector Arrays Integrated with µ‐LEDs for Broadband Flexible Optical Systems

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  32. Polyoxomolybdate Layered Crystals Constructed from a Heterocyclic Surfactant: Syntheses, Pseudopolymorphism and Introduction of Metal Cations

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  33. Tailoring Photoluminescence by Strain-Engineering in Layered Perovskite Flakes

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  34. Construction, photoelectric response and phase transition for new hybrid double perovskites showing narrow band gaps

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  35. Structural properties of defective (CH 3 NH 3 ) 2 Cu(Cl 1– x Br x ) 4 compounds

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  36. Strategies for high‐performance perovskite solar cells from materials, film engineering to carrier dynamics and photon management

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  37. Progress on Emerging Ferroelectric Materials for Energy Harvesting, Storage and Conversion

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  38. Chiral Methylbenzylammonium Bismuth Iodide with Zero-Dimensional Perovskite Derivative Structure

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    Parikshit Kumar Rajput, Ajay K. Poonia, Suman Mukherjee, Tariq Sheikh, Megha Shrivastava, K. V. Adarsh, Angshuman Nag

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  39. Pb-free halide perovskites for solar cells, light-emitting diodes, and photocatalysts

    APL Materials · 2022-06-01

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  40. Low‐Frequency Phonon Modes in Layered Silver‐Bismuth Double Perovskites: Symmetry, Polarity, and Relation to Phase Transitions

    Advanced Optical Materials · 2022-06-09

    Beatriz Martín‐García, Davide Spirito, Miao‐Ling Lin, Yu‐Chen Leng, Sergey Artyukhin, Ping‐Heng Tan, Roman Krahne

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  41. Improving Charge Carrier Mobility Estimations When Using Space-Charge-Limited Current Measurements

    ACS Energy Letters · 2022-06-10

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  42. Raman spectroscopy in layered hybrid organic-inorganic metal halide perovskites

    Journal of Physics Materials · 2022-06-16

    Davide Spirito, Yaiza Asensio, Luis E. Hueso, Beatriz Martín‐García

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  43. Lead‐Free Halide Double Perovskites: Fundamentals, Challenges, and Photovoltaics Applications

    Advanced Materials Technologies · 2022-07-06

    Naveen Kumar Tailor, Andrea Listorti, Silvia Colella, Soumitra Satapathi

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  44. Discovery of a 2D Hybrid Silver/Antimony‐Based Iodide Double Perovskite Photoferroelectric with Photostrictive Effect and Efficient X‐Ray Response

    Advanced Functional Materials · 2022-08-03

    Changfeng Wang, Haojin Li, Qun Ji, Chuang Ma, Lang Liu, Heng‐Yun Ye, Bo Cao, Guoliang Yuan, Hai‐Feng Lu, Da‐Wei Fu, Ming‐Gang Ju, Jinlan Wang, Kui Zhao, Yi Zhang

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  45. NH4+/K+-substitution-induced C–F–K coordination bonds for designing the highest-temperature hybrid halide double perovskite ferroelastic

    Chinese Chemical Letters · 2022-08-28

    Changfeng Wang, Na Wang, Chao Yi Shi, Heng‐Yun Ye, Yi Zhang, Le‐Ping Miao

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  46. Two-Dimensional Lead-Free Double Perovskite with Superior Stability and Optoelectronic Properties for Solar Cell Application

    The Journal of Physical Chemistry C · 2022-08-30

    Ming Chen, Xiaofeng Dong, Zhicheng Shan, Zhuo Xu, Shengzhong Frank Liu

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  47. Design, synthesis, optical studies, and application of all-inorganic layered double perovskites as stabilizers in ambient air processed perovskite solar cells

    Materials Research Bulletin · 2022-11-07

    Vahid Hoseinpour, Zahra Shariatinia‬, Luis A. Echegoyen

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  48. Progress in all-inorganic heterometallic halide layered double perovskites

    Trends in Chemistry · 2022-11-18

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  49. Recent Advances on Mn2+‐Doping in Diverse Metal Halide Perovskites

    Laser & Photonics Review · 2022-12-01

    Rui Yun, Huanxin Yang, Wenda Sun, Libing Zhang, Xiaowang Liu, Xiaodan Zhang, Xiyan Li

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  50. 2D nanosheets of layered double perovskites: synthesis, photostable bright orange emission and photoluminescence blinking

    Chemical Science · 2023-01-01

    Aditya Bhardwaj, Kaushik Kundu, Ranjan Sasmal, Paribesh Acharyya, Jayita Pradhan, Simanta Kalita, Sarit S. Agasti, Kanishka Biswas

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