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RESEARCH PAPER · ChemSusChem · 2019

MgSc2Se4—A Magnesium Solid Ionic Conductor for All‐Solid‐State Mg Batteries?

Liping Wang, Zhirong Zhao‐Karger, Franziska Klein, Johann Chable, Tobias Braun, Annika Regitta Schür, Chunru Wang, Yu‐Guo Guo, Maximilian Fichtner

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MgSc2Se4—A Magnesium Solid Ionic Conductor for All‐Solid‐State Mg Batteries?OriginalProgress in development of electrolytes for magnesium batteries247Ionic Transport in Potential Coating Materials for Mg Batteries120Dual Cation Exchanged Poly(ionic liquid)s as Magnesium Conducting Electrolytes11A materials perspective on magnesium-ion-based solid-state electrolytes106Advances in rechargeable Mg batteries148Recent Development of Mg Ion Solid Electrolyte68Analytical Measurements to Elucidate Structural Behavior of 2,5‐Dimethoxy‐1,4‐benzoquinone During Charge and Discharge10Alloy Anode Materials for Rechargeable Mg Ion Batteries252Challenges and Recent Progress on Key Materials for Rechargeable Magnesium Batteries295Water‐Pillared Sodium Vanadium Bronze Nanowires for Enhanced Rechargeable Magnesium Ion Storage58Mg3(BH4)4(NH2)2 as Inorganic Solid Electrolyte with High Mg2+ Ionic Conductivity40Analysis of optoelectronic and trasnport properties of magnesium based MgSc2X4 (X=S, Se) spinels for solar cell and energy storage device applications69Study of optoelectronic and transport properties of MgLu2Z4 (Z=S, Se) spinels for optoelectronic and energy harvesting applications54Ab initio study of the structural, electronic, optical and elastic properties of promising optoelectronic and thermoelectric compounds MgSc2X4 (X = S; Se)13Screening of Charge Carrier Migration in the MgSc2Se4 Spinel Structure21The metamorphosis of rechargeable magnesium batteries271Water scavenger as effective electrolyte additive and hybrid binder‐free organic/inorganic cathode for Mg battery applications13Recent progress of ceramic electrolytes for post Li and Na batteries19Insights into the structural, electronic and optical properties of MgA2B4(A = Sc, Y; B = S, Se) spinel compounds: Direct energy band gap materials14Rechargeable metal (Li, Na, Mg, Al)-sulfur batteries: Materials and advances137Revealing and excluding the root cause of the electronic conductivity in Mg-ion MgSc2Se4 solid electrolyte21Mechanism of Magnesium Transport in Spinel Chalcogenides22A low-cost and high-performance rechargeable magnesium battery based on povidone iodine cathode29Thermal annealing impact on structural, optical and dispersion parameters of zinc tetrapyridylporphyrin as a potential absorber thin film for energy conversion and storage devices2Multivalent Ion Conduction in Inorganic Solids38Solid‐State Electrolytes for Rechargeable Magnesium‐Ion Batteries: From Structure to Mechanism61Fast Room-Temperature Mg2+ Conductivity in Mg(BH4)2·1.6NH3–Al2O3 Nanocomposites40Ion Hopping: Design Principles for Strategies to Improve Ionic Conductivity for Inorganic Solid Electrolytes72Design and Characterization of Host Frameworks for Facile Magnesium Transport14Unravelling Charge Carrier Mobility in d 0 ‐Metal‐based Spinels7Nanoscale interface engineering of inorganic Solid-State electrolytes for High-Performance alkali metal batteries18Organic Crystalline Solid Electrolytes with High Mg-Ion Conductivity Composed of Nonflammable Ionic Liquid Analogs and Mg(TFSA)29Recent advances in kinetic optimizations of cathode materials for rechargeable magnesium batteries56Advantageous Al-ion intercalation in Mo15S19 nanosheets for aqueous symmetric supercapacitors13Mixed Metal‐Organic Frameworks as Efficient Semi‐Solid Electrolytes for Magnesium‐Ion Batteries15MgSc2Se4 Solid Electrolyte for Rechargeable Mg Batteries: An Electric Field‐Assisted All‐Solid‐State Synthesis10Ionic Liquid‐Incorporated Metal‐Organic Framework with High Magnesium Ion Conductivity for Quasi‐Solid‐State Magnesium Batteries27Progress and perspective on rechargeable magnesium-ion batteries38A practical perspective on the potential of rechargeable Mg batteries138Divalent closo -monocarborane solvates for solid-state ionic conductors14On the bramble way to Mg metal anodes in secondary Mg ion batteries22The challenges and perspectives of developing solid-state electrolytes for rechargeable multivalent battery38Advances in solid Mg-ion electrolytes for solid-state Mg batteries32To Be or Not to Be – Is MgSc 2 Se 4 a Mg‐Ion Solid Electrolyte?31Li, Na, K, Mg, Zn, Al, and Ca Anode Interface Chemistries Developed by Solid‐State Electrolytes115Recent Research Progress on All-Solid-State Mg Batteries14Prospects for magnesium ion batteries: A compreshensive materials review92Inorganic lithium-ion conductors for fast-charging lithium batteries: a review9Fast Room‐Temperature Mg‐Ion Conduction in Clay‐Like Halide Glassy Electrolytes19Effect of functional on structural, elastic stability, optoelectronic and thermoelectric characteristics of semiconducting MgX2Se4 (X = Lu, Y) spinels7Insights on solid electrolytes for solid-state magnesium batteries: Progress and prospects27Challenges and Progress in Anode‐Electrolyte Interfaces for Rechargeable Divalent Metal Batteries29MgB 2 Se 4 Spinels (B = Sc, Y, Er, Tm) as Potential Mg‐Ion Solid Electrolytes – Partial Ionic Conductivity and the Ion Migration Barrier16Nanoconfinement of an ammine magnesium borohydride composite electrolyte in a mesoporous silica scaffold9Exploring Rb2YCuCl6 and Cs2YCuCl6 double perovskites: Structural, electronic, optical, elastic, and thermoelectric properties via density functional theory18Electrolyte challenges and strategies toward better rechargeable magnesium-metal batteries11Magnesium borohydride pyridine derivatives as electrolytes for all-solid-state batteries3Simultaneous Exploration of Candidates for Electrode and Electrolyte Materials for All-Solid-State Batteries Using Predicted Rating from a Recommender System2Mg-Ion Conduction in Antiperovskite Solid Electrolytes Revealed by 25Mg Ultrahigh Field NMR and First-Principles Calculations2High-performance mg-ion battery materials: Recent progress and future perspectives10Roadmap for Next-Generation Electrochemical Energy Storage Technologies: Secondary Batteries and Supercapacitors149Investigation of Elastic and Thermodynamic Properties of XA2B4 (X = Mg, Zn, Cd; A = Sc, Y; B = S, Se) Spinel Compounds2Concomitant Enhancement of the Reorientational Dynamics of the BH 4 – Anions and Mg 2+ Ionic Conductivity in Mg(BH 4 ) 2 ·NH 3 upon Ligand Incorporation1Structural, Elastic, and Thermodynamic Properties of MgSc 2 X 4 (X = S, Se) Under High Pressure From First Principles0Interface Issues of Inorganic Solid‐State Electrolytes in Secondary Magnesium Batteries2Leveraging transfer learning for accurate estimation of ionic migration barriers in solids3Photovoltaic, photocatalytic and thermoelectric properties of X2LaAuBr6 (X = K, Rb, Cs) double perovskites1Electrolytes for rechargeable magnesium batteries12Emerging Developments of Inorganic Magnesium Solid-State Electrolytes1A combined DFT and machine learning study of Mg-site substitutional doping modulated electronic, optical and transport properties of MgSc2S4 spinels0Tackling the bottleneck in Mg anode/electrolyte interface1The structural, elastic, electronic, optical, thermodynamic, and phonon properties of MgX2Se4 (X=Er, Ho, Tm, Y) spinel compounds0Pressure induced bandgap variation for the optical and photo-catalytic properties of MgA2X4 (A = Sc, Y; X = S, Se) spinel compounds0

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  3. Dual Cation Exchanged Poly(ionic liquid)s as Magnesium Conducting Electrolytes

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  9. Challenges and Recent Progress on Key Materials for Rechargeable Magnesium Batteries

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  12. Analysis of optoelectronic and trasnport properties of magnesium based MgSc2X4 (X=S, Se) spinels for solar cell and energy storage device applications

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  14. Ab initio study of the structural, electronic, optical and elastic properties of promising optoelectronic and thermoelectric compounds MgSc2X4 (X = S; Se)

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  15. Screening of Charge Carrier Migration in the MgSc2Se4 Spinel Structure

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  16. The metamorphosis of rechargeable magnesium batteries

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  17. Water scavenger as effective electrolyte additive and hybrid binder‐free organic/inorganic cathode for Mg battery applications

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  18. Recent progress of ceramic electrolytes for post Li and Na batteries

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  19. Insights into the structural, electronic and optical properties of MgA2B4(A = Sc, Y; B = S, Se) spinel compounds: Direct energy band gap materials

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