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RESEARCH PAPER · Advanced Energy Materials · 2020

Alloy Anode Materials for Rechargeable Mg Ion Batteries

Jiazheng Niu, Zhonghua Zhang, Doron Aurbach

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Alloy Anode Materials for Rechargeable Mg Ion BatteriesOriginalPrimary Sjogren's syndrome: rarity in India.203Mg/Mg 2 Sn anodes with unprecedented electrochemical performance towards viable magnesium-ion batteries38Advances in rechargeable Mg batteries148Fundamentals and perspectives in developing zinc-ion battery electrolytes: a comprehensive review918Metallurgical approach to enhance the electrochemical activity of magnesium anodes for magnesium rechargeable batteries43Revealing the Magnesium‐Storage Mechanism in Mesoporous Bismuth via Spectroscopy and Ab‐Initio Simulations54Revealing the Magnesium‐Storage Mechanism in Mesoporous Bismuth via Spectroscopy and Ab‐Initio Simulations5Magnesium batteries: Current picture and missing pieces of the puzzle114A review on current anode materials for rechargeable Mg batteries123A Novel Regulation Strategy of Solid Electrolyte Interphase Based on Anion‐Solvent Coordination for Magnesium Metal Anode61Transformations de phases et comportement électrochimique d’électrodes négatives à base d’InSb et d’In-Pb pour les batteries Mg-ion0Computational Design of Ductile Magnesium Alloy Anodes for Magnesium Batteries10Effect of Interaction among Magnesium Ions, Anion, and Solvent on Kinetics of the Magnesium Deposition Process29Recent Advances and Perspectives of Zn‐Metal Free “Rocking‐Chair”‐Type Zn‐Ion Batteries227Recent Progress and Challenges in the Optimization of Electrode Materials for Rechargeable Magnesium Batteries90Advanced electrode materials for nonaqueous calcium rechargeable batteries55Application of expanded graphite-based materials for rechargeable batteries beyond lithium-ions60Self-healing liquid Ga-based anodes with regulated wetting and working temperatures for advanced Mg ion batteries36Experimental visualization of reversible magnesium storage and surface chemistry of magnesium silicide anode3Recent Progress and Challenges in Multivalent Metal‐Ion Hybrid Capacitors31An Overview on Protecting Metal Anodes with Alloy‐Type Coating28Interlayer Engineering of Preintercalated Layered Oxides as Cathode for Emerging Multivalent Metal-ion Batteries: Zinc and Beyond182Progress and perspectives on alloying-type anode materials for advanced potassium-ion batteries103An Overview on Anodes for Magnesium Batteries: Challenges towards a Promising Storage Solution for Renewables130Few-Layer Siloxene as an Electrode for Superior High-Rate Zinc Ion Hybrid Capacitors94Designing Nanostructured Metal Chalcogenides as Cathode Materials for Rechargeable Magnesium Batteries94Research advances in magnesium and magnesium alloys worldwide in 2020970Multidimensional Nonstoichiometric Electrode Materials for Electrochemical Energy Conversion and Storage46Recent Advances in Rechargeable Li–CO2 Batteries85Advancing Electrolyte Solution Chemistry and Interfacial Electrochemistry of Divalent Metal Batteries32Metal Chalcogenides with Heterostructures for High‐Performance Rechargeable Batteries76Exploration of amorphous hollow FeOOH@C nanosphere on energy storage for sodium ion batteries13Dealloying induced nanoporosity evolution of less noble metals in Mg ion batteries14Realizing reversible storage of trivalent aluminum ions using VOPO4·2H2O nanosheets as cathode material in aqueous aluminum metal batteries48A Machine Learning Shortcut for Screening the Spinel Structures of Mg/Zn Ion Battery Cathodes with a High Conductivity and Rapid Ion Kinetics66Opportunities and Limitations of Ionic Liquid‐ and Organic Carbonate Solvent‐Based Electrolytes for Mg‐Ion‐Based Dual‐Ion Batteries37High-Specific-Capacity and High-Performing Post-Lithium-Ion Battery Anode over 2D Black Arsenic Phosphorus38A Pyrite Iron Disulfide Cathode with a Copper Current Collector for High‐Energy Reversible Magnesium‐Ion Storage103Influence of Electrolyte on the Electrode/Electrolyte Interface Formation on InSb Electrode in Mg-Ion Batteries9Electrode materials for aqueous multivalent metal-ion batteries: Current status and future prospect73Sn Alloying to Inhibit Hydrogen Evolution of Zn Metal Anode in Rechargeable Aqueous Batteries312The Evaluation of Mg–Ga Compounds as Electrode Materials for Mg-Ion Batteries via Ab Initio Simulation15Surface modification and in situ carbon intercalation of two-dimensional niobium carbide as promising electrode materials for potassium-ion batteries48Advancing towards a Practical Magnesium Ion Battery47Mechanisms of electrochemical magnesium (de)alloying of Mg-Sn and Mg-Pb polymorphs7Unveiling the Magnesium Storage Mechanisms of Co-Sputtered Indium-Tin Alloy Films Using Operando X-ray Diffraction4Synchrotron X‐ray Spectroscopic Investigations of In‐Situ‐Formed Alloy Anodes for Magnesium Batteries26A two-dimensional metallic SnB monolayer as an anode material for non-lithium-ion batteries37Alloying electrode coatings towards better magnesium batteries40Exploring the Insertion Properties of Mg2+ in H2v3o8 as a Function of the Water Content in the Organic Electrolyte12Low‐strain TiP2O7 with three‐dimensional ion channels as long‐life and high‐rate anode material for Mg‐ion batteries117MgMoO 4 as an anode material for lithium ion batteries and its multi-electron reaction mechanism9Room Temperature Operation of Magnesium Rechargeable Batteries with a Hydrothermally Treated ZnMnO3 Defect Spinel Cathode101T-MoS2 monolayer as a promising anode material for (Li/Na/Mg)-ion batteries156A self-healing room-temperature liquid eutectic GaSn anode with improved wettability for advanced Mg ion batteries25K2.13V1.52Ti0.48(PO4)3 as an anode material with a long cycle life for potassium-ion batteries13Size‐Controllable Nickel Sulfide Nanoparticles Embedded in Carbon Nanofibers as High‐Rate Conversion Cathodes for Hybrid Mg‐Based Battery52A facile in situ Mg surface chemistry strategy for conditioning-free Mg[AlCl4]2 electrolytes11Rational Design Strategy of Novel Energy Storage Systems: Toward High‐Performance Rechargeable Magnesium Batteries100Understanding rechargeable magnesium ion batteries via first-principles computations: A comprehensive review64Highly reversible Mg metal anodes enabled by interfacial liquid metal engineering for high-energy Mg-S batteries101Mg2+ ion-powered hybrid supercapacitor with β-MnO2 as a cathode and α-Fe2O3 as an anode22An in-depth understanding of improvement strategies and corresponding characterizations towards Zn anode in aqueous Zn-ions batteries80Charging/discharging mechanism in Mg3Bi2 anode for Mg-ion batteries; The role of the spin-orbit coupling11Few‐Layered ReS2@CNTs as a High‐Performance Cathode for Aluminum‐Ion Batteries9Pseudocapacitive Zinc Cation Intercalation with Superior Kinetics Enabled by Atomically Thin V2O5 Nanobelts for Quasi-Solid-State Microbatteries60A long-cycle life recharge magnesium ion battery using the Na2Li2Ti6O14 nanoparticles as an anode material5Beyond Li-ion Batteries for Grid-Scale Energy Storage16Phase-boundary regulation boosting electrochemical reactivity of tin-based anodes for magnesium-ion batteries10A Novel and Highly Efficient Indolyl‐Based Electrolyte for Mg Batteries7Advanced protective layer design on the surface of Mg-based metal and application in batteries: Challenges and progress51Advances in rechargeable magnesium batteries employing graphene-based materials7Thermodynamic investigation of phase transformation in Sn anode for magnesium batteries3A DFT Study of Halogen (F−, Cl−, and Br−) Encapsulated Ga12X12 (X = N, P, and As) Nanocages for Sodium-Ion Batteries10Synthesis of novel 1–dimensional structure from Mo6S8 Chevrel phase of electrode for Mg batteries4A high-performance room-temperature magnesium ion battery with self-healing liquid alloy anode mediated with a bifunctional intermetallic compound18Phase Separation Induced Binary Core–Shell Alloy Nanoparticles Embedded in Carbon Sheets for Magnesium Storage14Amorphous germanium-crystalline bismuth films as a promising anode for magnesium-ion batteries44From Cathodes to Conductive Pastes: A New Perspective into the Recycle of Silver Element0Deformable Triphase Tin-Aluminium-Bismuth Anodes for Rechargeable Magnesium Ion Batteries4Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium95Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium3Enhanced Elastic Migration of Magnesium Cations in alpha‐Manganese Dioxide Tunnels Locally Tuned by Aluminium Substitution38The Key Role of Magnesium Polysulfides in the Development of Mg-S Batteries27Recent Progress in Bi-Based Anodes for Magnesium Ion Batteries8Multi-walled carbon nanotubes interlinked vanadium selenite nanocomposites as a positive electrode for high-performance aqueous zinc-ion batteries19Grain‐Boundary‐Rich Triphasic Artificial Hybrid Interphase Toward Practical Magnesium Metal Anodes57Surface Amalgam on Magnesium Electrode: Protective Coating or Not?4Progress and perspective on rechargeable magnesium-ion batteries38Monolayer of B3O3 as a promising material in anode of magnesium-ion batteries: A theoretical study6Toward High-Performance Mg-S Batteries via a Copper Phosphide Modified Separator57A practical perspective on the potential of rechargeable Mg batteries138Advancing next-generation nonaqueous Mg–CO 2 batteries: insights into reaction mechanisms and catalyst design16Chevrel phases: synthesis, structure, and electrocatalytic applications11Hierarchical BiOCl flowerlike microspheres via a room-temperature solid-state chemical reaction as a new anode for rechargeable magnesium-ion batteries22Magnesium: properties and rich chemistry for new material synthesis and energy applications118Monolayer α-beryllene as an anode material for magnesium ion batteries with high capacity and low diffusion energy barrier24Recent progress in block copo lymer s oft-template-assisted synthesis of versatile mesoporous materials for energy storage systems67The progress of cathode materials in aqueous zinc-ion batteries12Unveiling the electronic properties of native solid electrolyte interphase layers on Mg metal electrodes using local electrochemistry10Mn2+ doped BaSnF4-based solid state electrolyte for room-temperature fluoride ion batteries18The challenges and perspectives of developing solid-state electrolytes for rechargeable multivalent battery38Solid-state polymer magnesium supercapacitor8Anion‐Incorporated Mg‐Ion Solvation Modulation Enables Fast Magnesium Storage Kinetics of Conversion‐Type Cathode Materials70Phase engineering of layered anode materials during ion-intercalation in Van der Waal heterostructures9Application of purified kish flake graphite as a potential cathode material for high-performance aluminum ion batteries25Self‐Assembled Protein Nanofilm Regulating Uniform Zn Nucleation and Deposition Enabling Long‐Life Zn Anodes24Approaching Microsized Alloy Anodes via Solid Electrolyte Interphase Design for Advanced Rechargeable Batteries73Doping FePSe3 with Mg and Ca ions: A Density Functional Theory Study1Bismuth Nanoparticle-Embedded Carbon Microrod for High-Rate Electrochemical Magnesium Storage20Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities120A review on advanced optimization strategies of separators for aqueous zinc-ion batteries15Engineering hierarchical honeycomb-wall-like MgP4O11/CoP nanosheets as advanced binder-less electrode for supercapacitors8Dissolution Mechanism of Eutectic and Hypereutectic Mg–Sn Alloy Anodes for Magnesium Rechargeable Batteries6Transferable and robust machine learning model for predicting stability of Si anodes for multivalent cation batteries16Visualizing the Interfacial Chemistry in Multivalent Metal Anodes by Transmission Electron Microscopy18Layered Materials in the Magnesium Ion Batteries: Development History, Materials Structure, and Energy Storage Mechanism24A novel rechargeable Magnesium–Air battery using “All in one” Mg anode with high reversibility15Self-healing Ga-based liquid metal/alloy anodes for rechargeable batteries26First-principles study of electronic structure and metallization of Mg2Pb under high pressure1Research advances in magnesium and magnesium alloys worldwide in 20200Research advances in magnesium and magnesium alloys worldwide in 20205Mg2Sn alloy anode materials with high interfacial activity for chloride ion batteries4Optimization and Mechanistic Investigation of Electrochemical Performance and Diffusion Behavior of MgFeP 2 O 7 Prepared via Sol-Gel Method in Magnesium Batteries0Unveiling the X‐Ray Absorption Chemistry of H3.78V6O13 Cathode for Aqueous Zinc‐Ion Batteries109Enabling Effective Thiocyanogen/Thiocyanate Couple for the Zinc─Pseudohalogen Battery12Multiphase MoS2 monolayer: A promising anode material for Mg-Ion batteries16Recent Advances in Aqueous Non‐Metallic Ion Batteries with Organic Electrodes19A material perspective on advanced magnesium-ion batteries for electric vehicles0Rational design of Two-Dimensional Buckled-Hexagonal Nb2S2 monolayer as an efficient anode material for Ca-ion Batteries: A First-Principles study47Re-envisioning the Key Factors of Magnesium Metal Anodes for Rechargeable Magnesium Batteries69Development and prospects of degradable magnesium alloys for structural and functional applications in the fields of environment and energy74Bottom‐Up Magnesium Deposition Induced by Paper‐Based Triple‐Gradient Scaffolds toward Flexible Magnesium Metal Batteries62Designing Chemically Replaced Interfacial Layer via Unveiling the Influence of Zn Crystal Facets for Practical Zn‐Metal Anodes43Potential Application of MgCu2 Alloy as a High-Performance Electrode Material for Mg-Ion Batteries: A Computational Study7Mg storage properties and reaction mechanism of PbSn alloy films in Mg ion batteries9Unraveling the effect of single atom catalysts on the charging behavior of nonaqueous Mg–CO 2 batteries: a combined density functional theory and machine learning approach20Magnesium dendrite growth during electrodeposition in conditioned Mg(TFSI)2/AlCl3/MgCl2/DME electrolyte21A Temperature‐Tolerant Magnesium‐Ion Battery Using Ball Cactus‐like MgV2O4 as High‐Performance Cathode8Elastic Restraint Induced by Carbon Coating Enhances Potassium-Ion Batteries' Performance via Phase Transition7Enhanced Oxygen Reduction Reaction Activity of Manganese Oxide via p−d Hybridization with Aluminum Group Element Dopants33Binary Mg‐1 at%Gd alloy anode for high‐performance rechargeable magnesium batteries6Roadmap for rechargeable batteries: present and beyond224Toward high-energy magnesium battery anode: recent progress and future perspectives34A metallic two-dimensional b-BS 2 monolayer as a superior Na/K-ion battery anode5Closed Battery Systems1Data-driven search for promising intercalating ions and layered materials for metal-ion batteries7Emerging application of 2D materials for dendrite-free metal batteries11Emerging Battery Technologies to Boost the Clean Energy Transition48Insights into Ti 3 N 2 T 2 /VS 2 (T = F, O, OH) heterostructures as innovative anode materials for lithium/sodium/magnesium-ion batteries9

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