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RESEARCH PAPER · Advanced Energy Materials · 2020

Challenges and Recent Progress on Key Materials for Rechargeable Magnesium Batteries

Fanfan Liu, Tiantian Wang, Xiaobin Liu, Li‐Zhen Fan

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Challenges and Recent Progress on Key Materials for Rechargeable Magnesium BatteriesOriginalAdvances in rechargeable Mg batteries148Recent advances in developing organic electrode materials for multivalent rechargeable batteries256Ultrahigh rate capability and long cycling stability of dual-ion batteries enabled by TiO 2 microspheres with abundant oxygen vacancies16A Synergistic Approach to Unraveling the Thermodynamic Stability of Binary and Ternary Chevrel Phase Sulfides22Stable Hydrogel Electrolytes for Flexible and Submarine-Use Zn-Ion Batteries1512D Ti3C2 MXene embedded with Co(II)(OH)n nanoparticles as the cathode material for hybrid magnesium–lithium-ion batteries21Hydrated MgxV5O12 Cathode with Improved Mg2+ Storage Performance58Advanced energy materials for flexible batteries in energy storage: A review316Recent Advances and Perspectives on Calcium‐Ion Storage: Key Materials and Devices191Effect of Interaction among Magnesium Ions, Anion, and Solvent on Kinetics of the Magnesium Deposition Process29The potential application of VS2 as an electrode material for Mg ion battery: A DFT study991T-VSe 2 Nanoparticles Cooperated with Reduced Graphene Oxide as a Superior Cathode Material For Rechargeable Mg-Ion Batteries0Boosting magnesium storage in MoS 2 via a 1T phase introduction and interlayer expansion strategy: theoretical prediction and experimental verification10Facilitated magnesium atom adsorption and surface diffusion kinetics via artificial bismuth-based interphases27MgCo 2 O 4 -based electrode materials for electrochemical energy storage and conversion: a comprehensive review164Organic cation (DMPI) intercalated graphite anode for high voltage next generation dual-ion batteries8Rechargeable Mg–Na and Mg–K hybrid batteries based on a low-defect Co 3 [Co(CN) 6 ] 2 nanocube cathode6Recent Advances in Non‐nucleophilic Mg Electrolytes16In Situ/Operando (Soft) X‐ray Spectroscopy Study of Beyond Lithium‐ion Batteries60Binder-free MnO2 as a high rate capability cathode for aqueous magnesium ion battery31Magnesium-ion batteries for electric vehicles: Current trends and future perspectives76Solid Electrolyte Interphase Growth on Mg Metal Anode: Case Study of Glyme‐Based Electrolytes30Ultralong-Lifespan Magnesium Batteries Enabled by the Synergetic Manipulation of Oxygen Vacancies and Electronic Conduction25Interlayer Engineering of Preintercalated Layered Oxides as Cathode for Emerging Multivalent Metal-ion Batteries: Zinc and Beyond182An Overview on Anodes for Magnesium Batteries: Challenges towards a Promising Storage Solution for Renewables130Nb-based compounds for rapid lithium-ion storage and diffusion20Computational investigation of 2D 3d/4d hexagonal transition metal borides for metal-ion batteries29Revisiting the degradation of solid/electrolyte interfaces of magnesium metal anodes: Decisive role of interfacial composition93Progress on graphitic carbon materials for potassium- based energy storage27Designs and applications of multi-functional covalent organic frameworks in rechargeable batteries83High-performance heterojunction Ti3C2/CoSe2 with both intercalation and conversion storage mechanisms for magnesium batteries71Energy storage mechanism of monocrystalline layered FePS3 and FePSe3 as active materials for Mg batteries and pseudocapacitors26High-rate performance magnesium batteries achieved by direct growth of honeycomb-like V2O5 electrodes with rich oxygen vacancies41A Chlorine-Free Electrolyte Based on Non-nucleophilic Magnesium Bis(diisopropyl)amide and Ionic Liquid for Rechargeable Magnesium Batteries293D Carbon Networks: Design and Applications in Sodium Ion Batteries17Ab initio investigations on metal ion pre-intercalation strategy of layered V2O5 cathode for magnesium-ion batteries23A Pyrite Iron Disulfide Cathode with a Copper Current Collector for High‐Energy Reversible Magnesium‐Ion Storage103First-principles prediction of layered MoO 2 and MoOSe as promising cathode materials for magnesium ion batteries7Design Principles for Multinary Metal Chalcogenides: Toward Programmable Reactivity in Energy Conversion31Progress and innovation of nanostructured sulfur cathodes and metal-free anodes for room-temperature Na–S batteries6Enhancing Mg2+ and Mg2+/Li+ Storage by Introducing Active Defect Sites and Edge Surfaces in MoSe210A thermodynamic assessment of the Mg–Sn–Sb ternary system15Ti3C2 MXene with pillared structure for hybrid magnesium-lithium batteries cathode material with long cycle life and high rate capability29Synergy Strategy of Electrical Conductivity Enhancement and Vacancy Introduction for Improving the Performance of VS4 Magnesium-Ion Battery Cathode37Development of Magnesium Borate Electrolytes: Explaining the Success of Mg[B(hfip)4]2 Salt91A Se-Doped S@CMK3 Composite as a High-Performance Cathode for Magnesium–Sulfur Batteries with Mg2+/Li+ Hybrid Electrolytes17Insight into the coordinating mechanism of multi-electron reaction and structural stability induced by K+ pre-intercalation for magnesium ions batteries41Is proton a charge carrier for δ-MnO2 cathode in aqueous rechargeable magnesium-ion batteries?37Engineering kinetics-favorable 2D graphene@CuS with long-term cycling stability for rechargeable magnesium batteries30Bimetallic sulfide NiCo 2 S 4 yolk–shell nanospheres as high-performance cathode materials for rechargeable magnesium batteries34Development of chloride-free electrolyte for rechargeable magnesium battery0Lattice Expanding by Te-Substitution to Boost Electrochemical Mg Storage of Cu7.2s4 Nanotube Cathode30Nonaqueous rechargeable aluminum batteries168Anionic Te-Substitution Boosting the Reversible Redox in CuS Nanosheet Cathodes for Magnesium Storage113A Moisture‐Assisted Rechargeable Mg−CO2 Battery37A Moisture‐Assisted Rechargeable Mg−CO2 Battery12In Operando Closed-cell Transmission Electron Microscopy for Rechargeable Battery Characterization: Scientific Breakthroughs and Practical Limitations33Comparative Study of Conventional Electrolytes for Rechargeable Magnesium Batteries33A stable covalent organic framework cathode enables ultra-long cycle life for alkali and multivalent metal rechargeable batteries1121 T-VSe2 Nanoparticles cooperated with reduced graphene oxide as a superior cathode material for rechargeable Mg-ion batteries33Understanding rechargeable magnesium ion batteries via first-principles computations: A comprehensive review64Highly reversible Mg metal anodes enabled by interfacial liquid metal engineering for high-energy Mg-S batteries101Recent progress of flexible aqueous multivalent ion batteries75Vanadium-based cathodes for aqueous zinc-ion batteries: Mechanism, design strategies and challenges329Pyrrolidinium-Based Organic Cation (BMP)-Intercalated Organic (Coronene) Anode for High-Voltage Dual-Ion Batteries: A Comparative Study with Graphite10RETRACTED: Evaluating the potential of graphene-like boron nitride as a promising cathode for Mg-ion batteries50Review of room-temperature liquid metals for advanced metal anodes in rechargeable batteries84Off-Planar, Two-Dimensional Polymer Cathode for High-Rate, Durable Rechargeable Magnesium Batteries24Beyond Li-ion Batteries for Grid-Scale Energy Storage16Electrochemical Proton Storage: From Fundamental Understanding to Materials to Devices96Negative sulfur-based electrodes and their application in battery cells: Dual-ion batteries as an example1TFSI Anion Grafted Polymer as an Ion-Conducting Protective Layer on Magnesium Metal for Rechargeable Magnesium Batteries53Modification of a Cu Mesh with Nanowires and Magnesiophilic Ag Sites to Induce Uniform Magnesium Deposition30Robust Self‐Standing Single‐Ion Polymer Electrolytes Enabling High‐Safety Magnesium Batteries at Elevated Temperature55Electrolytes for Multivalent Metal‐Ion Batteries: Current Status and Future Prospect33Octylamine‐Supporting Interlayer Expanded Molybdenum Diselenide as a High‐Power Cathode for Rechargeable Mg Batteries18Towards better Mg metal anodes in rechargeable Mg batteries: Challenges, strategies, and perspectives126Cathodes for Mg batteries: A condensed review13Amorphous germanium-crystalline bismuth films as a promising anode for magnesium-ion batteries44Cu7S4 superionic with liquid-like mobility of copper ions for high-performance room-temperature rechargeable magnesium batteries7A coupled experimental and thermodynamic assessment of the Mg-Bi-Sb and Zn-Bi-Sb ternary system and extrapolate to the Mg-Bi-Zn-Sb system6In-situ synthesis of Bi nanospheres anchored in 3D interconnected cellulose nanocrystal derived carbon aerogel as anode for high-performance Mg-ion batteries41Zinc‐ion hybrid supercapacitors: Design strategies, challenges, and perspectives62An efficient Hauser-base electrolyte for rechargeable magnesium batteries25Co-substitution of Mg2+ and Ti4+ in Na3V2(PO4)3 nanoparticles coated with highly conductive carbon nanotubes for superior sodium storage25Eye Tear Activated Mg‐Air Battery Driven by Natural Eye Blinking for Smart Contact Lenses20From Cathodes to Conductive Pastes: A New Perspective into the Recycle of Silver Element0Borohydride Ammoniate Solid Electrolyte Design for All‐Solid‐State Mg Batteries27Rechargeable Batteries for Grid Scale Energy Storage1765Advances and challenges in multiscale characterizations and analyses for battery materials10Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium95Organic Electrolyte Design for Rechargeable Batteries: From Lithium to Magnesium3Tailoring a Hybrid Functional Layer for Mg Metal Anodes in Conventional Electrolytes with a Low Overpotential25Stacked Si2BN monolayers as ultra-high-capacity anode material for divalent Mg-ion batteries12Development of a Mg/O ReaxFF Potential to describe the Passivation Processes in Magnesium‐Ion Batteries**19In Situ Formed Magnesiophilic Sites Guiding Uniform Deposition for Stable Magnesium Metal Anodes63Recent Progress in Bi-Based Anodes for Magnesium Ion Batteries8Regulated electrochemical performance of manganese oxide cathode for potassium-ion batteries: A combined experimental and first-principles density functional theory (DFT) investigation56A Molybdenum Polysulfide In-Situ Generated from Ammonium Tetrathiomolybdate for High-Capacity and High-Power Rechargeable Magnesium Battery Cathodes41Progress and perspective on rechargeable magnesium-ion batteries38A Rising 2D Star: Novel MBenes with Excellent Performance in Energy Conversion and Storage177High-Performance NiS 2 Hollow Nanosphere Cathodes in Magnesium-Ion Batteries Enabled by Tunable Redox Chemistry56Study the application of nitrogenated holey graphene (C2N) nanosheets as a high-performance anode material for magnesium ion battery (MIB): DFT study25Vanadium-based cathode materials for rechargeable magnesium batteries28Solvent Molecule Design Enables Excellent Charge Transfer Kinetics for a Magnesium Metal Anode112A practical perspective on the potential of rechargeable Mg batteries138A two-dimensional VO 2 /VS 2 heterostructure as a promising cathode material for rechargeable Mg batteries: a first principles study11An interfacial covalent bonding coupled ultrafine CuS-nanocrystals/MXene heterostructure for efficient and durable magnesium storage27Current material design strategies on the copper chalcogenide cathodes for rechargeable magnesium batteries: a review17High-density cathode structure of independently acting Prussian-blue-analog nanoparticles: a high-power Zn–Na-ion battery discharging ∼200 mA cm −2 at 1000C3Magnesium: properties and rich chemistry for new material synthesis and energy applications118Progress and Perspective of Metal-Organic Frameworks as Sei Instability Mitigator in Magnesium Batteries0Synthesis and catalytic applications of metal boride ceramics1Ca2+ Solvation and Electrochemical Solid/Electrolyte Interphase Formation Toward the Multivalent-Ion Batteries8A Single Mg Ion-conductive Polymer-coated MgCo2O4 for Mg Rechargeable Batteries3Deeping insight of Mg(CF3SO3)2 and comprehensive modified electrolyte with ionic liquid enabling high-performance magnesium batteries74Organosulfur Materials for Rechargeable Batteries: Structure, Mechanism, and Application228Towards the understanding of (dis)charging mechanism of VS4 cathode for magnesium batteries12Self-Healing Polymer Electrolytes for Next-Generation Lithium Batteries73The challenges and perspectives of developing solid-state electrolytes for rechargeable multivalent battery38Bimetallic Bi–Sn micro-/nanospheres@cellulose nanocrystal derived carbon aerogel composite anode for high-performance Mg-ion batteries22Anion‐Incorporated Mg‐Ion Solvation Modulation Enables Fast Magnesium Storage Kinetics of Conversion‐Type Cathode Materials70Cationic Co-doping in copper sulfide nanosheet cathodes for efficient magnesium storage41Reactive Metals as Energy Storage and Carrier Media1Electrochemical performance of copper phosphosulfide (Cu3PS4) towards magnesium ion storage3Strategy for Ultrafast Cathode Reaction in Magnesium-Ion Batteries Using BF4 Anion Based Dual-Salt Electrolyte Systems: A Case Study of FePO413Preparation of pectin biopolymer electrolyte for zinc-ion battery application22Combining functionalized CNT film with CuS microflowers through hyperbranched polymers for a flexible and appliable rechargeable Mg battery14Cu+ redox activation and polyselenide stabilization via strong Se-C interaction for superior magnesium storage33Research development on electrolytes for magnesium-ion batteries157Research advances of the electrolytes for rechargeable magnesium ion batteries26Stable Anion-Rectifying Poly(alkoxide magnesium) Electrolytes for Reversible Magnesium Metal Batteries28Unusual Hybrid Magnesium Storage Mechanism in a New Type of Bi2O2CO3 Anode29To Be or Not to Be – Is MgSc 2 Se 4 a Mg‐Ion Solid Electrolyte?31Insights into the Energy Storage Differences of Zinc and Calcium Ions with Layered Vanadium Oxide as a Model Material17Li, Na, K, Mg, Zn, Al, and Ca Anode Interface Chemistries Developed by Solid‐State Electrolytes115A material perspective on advanced magnesium-ion batteries for electric vehicles0High‐Rate Nonaqueous Mg–CO2 Batteries Enabled by Mo2C‐Nanodot‐Embedded Carbon Nanofibers17Revealing the Structural Evolution of Electrode/Electrolyte Interphase Formation during Magnesium Plating and Stripping with operando EQCM‐D8Re-envisioning the Key Factors of Magnesium Metal Anodes for Rechargeable Magnesium Batteries69Toward High‐Performance Mg/S Batteries with M4‐Assisted Mg(AlCl4)2/PYR14TFSI/DME Electrolyte and MoS2@CMK/S Cathode10Bottom‐Up Magnesium Deposition Induced by Paper‐Based Triple‐Gradient Scaffolds toward Flexible Magnesium Metal Batteries62Multilevel gradient framework of Ce/Mo co-substituted Na3V2(PO4)3/C–CeO2@CNTs system with ultralong cyclic stability for half and full sodium ion cells10In-situ generated elemental selenium nanograins cooperated with NiSe2 microspheres for significantly enhanced magnesium-storage performance13Ultrafast cathode characteristics of a nano-V 2 (PO 4 ) 3 carbon composite for rechargeable magnesium batteries6Novel covalent organic framework/carbon nanotube composites with multiple redox-active sites for high-performance Na storage62Optimizing interfacial process of Mg metal anode by porphyrin adsorption layer in Cl-free conventional electrolyte13A Temperature‐Tolerant Magnesium‐Ion Battery Using Ball Cactus‐like MgV2O4 as High‐Performance Cathode8A review of metal sulfide cathode materials for non-aqueous multivalent ion (Mg2+, Ca2+, Al3+) batteries19Mg2+ ion-conducting ceramic solid electrolytes based on Moringa oleifera seed and magnesium nitrate for secondary magnesium battery applications20

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  50. Bimetallic sulfide NiCo 2 S 4 yolk–shell nanospheres as high-performance cathode materials for rechargeable magnesium batteries

    Nanoscale · 2022-01-01

    Yiming Ma, Yujie Zhang, Fan Wang, Haijiao Xie, Jin Wang

    Read original paper ↗ ·
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