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RESEARCH PAPER · Chemical Communications · 2019

The first lithium difluorophosphate LiPO 2 F 2 with a neutral polytetrahedral microporous architecture

Guopeng Han, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

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The first lithium difluorophosphate LiPO 2 F 2 with a neutral polytetrahedral microporous architectureOriginalBa 3 B 10 O 17 F 2 ·0.1KF: the first mixed alkali/alkaline-earth metal fluorooxoborate with unprecedented double-layered B–O/F anionic arrangement17A new iodate-phosphate Pb 2 (IO 3 )(PO 4 ) achieving great improvement in birefringence activated by (IO 3 ) − groups53Influence of structure-directing polyhedra and heterocyclic ligands on the chain structures and O/F ordering in a series of zinc vanadium oxyfluorides1K 4 (PO 2 F 2 ) 2 (S 2 O 7 ): first fluorooxophosphorsulfate with mixed-anion [S 2 O 7 ] 2− and [PO 2 F 2 ] − groups14Two new ammonium/alkali-rare earth metal difluorophosphates ALa(PO 2 F 2 ) 4 (A = NH 4 and K) with moderate birefringence and short cutoff edges26Armoring LiNi 1/3 Co 1/3 Mn 1/3 O 2 Cathode with Reliable Fluorinated Organic–Inorganic Hybrid Interphase Layer toward Durable High Rate Battery133K2Na(IO3)2(I3O8) with Strong Second Harmonic Generation Response Activated by Two Types of Isolated Iodate Anions46BaB 4 O 5 F 4 with reversible phase transition featuring unprecedented fundamental building blocks of [B 16 O 21 F 16 ] in the α -phase and [B 4 O 6 F 4 ] in the β -phase19From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)9RbMo 2 P 3 O 14 with large birefringence mainly induced by highly distorted [MoO 6 ] in uncommon [Mo 2 P 3 O 14 ] ∞ layers9Sodium difluorophosphate: facile synthesis, structure, and electrochemical behavior as an additive for sodium-ion batteries49Nickel-rich NMC materials for lithium-ion batteries : surface reactivity and gas production0Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence0Lithium dendritic growth inhibitor enabling high capacity, dendrite-free, and high current operation for rechargeable lithium batteries39Novel layered heterobimetallic fluorides with large optical band gaps3Chemical reactivity of lithium difluorophosphate as electrolyte additive in LiNi0.6Co0.2Mn0.2O2/graphite cells22A bicomponent electrolyte additive towards stabilized interface for high-performance lithium-ion batteries3BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge4In Situ Diffuse Reflectance Infrared Fourier-Transform Spectroscopy Investigation of Fluoroethylene Carbonate and Lithium Difluorophosphate Dual Additives in SEI Formation over Cu Anode21From Monofluorophosphates A2PO3F to Difluorophosphates APO2F2 (A = alkali metal): Design of a Potential Deep-Ultraviolet Nonlinear Optical Materials System with a Shortened Phase-Matching Wavelength41Fluorination strategy toward chemical and functional modification65Fluorine-driven materials design of novel deep-ultraviolet nonlinear optical crystal materials: Research progress and challenges6Engineering Stable Decomposition Products on Cathode Surfaces to Enable High Voltage All‐Solid‐State Batteries8Engineering Stable Decomposition Products on Cathode Surfaces to Enable High Voltage All‐Solid‐State Batteries25Discrepant lithium transference numbers due to heterogeneous speciation4Highly Polarizable Phosphorus‐Centered Tetrahedra and π‐Conjugated Carbon‐Centered Triangular Moieties Inducing Large Anisotropy and Short‐Wavelength Phase‐Matching23A review for high-value utilization of retired spent electrolyte for lithium-ion battery: how to reduce the waste of resources?6Primary exothermic reaction pathways between solid electrolyte interphases and electrolytes during the onset of thermal runaway in lithium-ion batteries9One‐Step Biphasic Interfacial Engineering Stabilizes Single‐Crystal Ultrahigh‐Nickel Cathodes13Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes11Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes2Optimized synthesis of novel LiPOF4 electrolyte additives and their application in lithium-sulfur batteries0Machine-Learning-Guided Insights into Solid-Electrolyte Interphase Conductivity: Are Amorphous Lithium Fluorophosphates the Key?4Rational Lithium Salt Selection Principle for Designing High-Entropy Electrolytes toward High-Performance Lithium Metal Batteries36Pretreatment-derived LiF/LiPO2F2 species enable robust high-voltage NCM811 cathode interphases0

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  1. Ba 3 B 10 O 17 F 2 ·0.1KF: the first mixed alkali/alkaline-earth metal fluorooxoborate with unprecedented double-layered B–O/F anionic arrangement

    Chemical Communications · 2019-01-01

    Yahui Li, Hongwei Yu, Guopeng Han, Hao Li, Zhihua Yang, Shilie Pan

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  2. A new iodate-phosphate Pb 2 (IO 3 )(PO 4 ) achieving great improvement in birefringence activated by (IO 3 ) − groups

    Chemical Communications · 2019-12-04

    Xiaohan Zhang, Bing‐Ping Yang, Jin Chen, Chun‐Li Hu, Zhi Gang Fang, Zujian Wang, Jiang‐Gao Mao

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  3. Influence of structure-directing polyhedra and heterocyclic ligands on the chain structures and O/F ordering in a series of zinc vanadium oxyfluorides

    CrystEngComm · 2020-01-01

    Belal Ahmed, Hongil Jo, Suheon Lee, Kwang‐Yong Choi, Kang Min Ok

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  4. K 4 (PO 2 F 2 ) 2 (S 2 O 7 ): first fluorooxophosphorsulfate with mixed-anion [S 2 O 7 ] 2− and [PO 2 F 2 ] − groups

    Dalton Transactions · 2020-01-01

    Wenyao Zhang, Wenqi Jin, Zhihua Yang, Shilie Pan

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  5. Two new ammonium/alkali-rare earth metal difluorophosphates ALa(PO 2 F 2 ) 4 (A = NH 4 and K) with moderate birefringence and short cutoff edges

    Dalton Transactions · 2020-01-01

    Wenyao Zhang, Zhonglei Wei, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  6. Armoring LiNi 1/3 Co 1/3 Mn 1/3 O 2 Cathode with Reliable Fluorinated Organic–Inorganic Hybrid Interphase Layer toward Durable High Rate Battery

    Advanced Functional Materials · 2020-03-13

    Yu Chen, Weimin Zhao, Quanhai Zhang, Guangzhi Yang, Jianming Zheng, Wei Tang, Qunjie Xu, Chunyan Lai, Junhe Yang, Chengxin Peng

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  7. K2Na(IO3)2(I3O8) with Strong Second Harmonic Generation Response Activated by Two Types of Isolated Iodate Anions

    Chemistry of Materials · 2020-04-02

    Tushagu Abudouwufu, Min Zhang, Shichao Cheng, Hao Zeng, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  8. BaB 4 O 5 F 4 with reversible phase transition featuring unprecedented fundamental building blocks of [B 16 O 21 F 16 ] in the α -phase and [B 4 O 6 F 4 ] in the β -phase

    Chemical Communications · 2021-01-01

    Wenbin Zhang, Siru Guo, Shujuan Han, Liying Wang, Xin Hua Zhou, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  9. From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)

    Dalton Transactions · 2021-01-01

    Wenyao Zhang, Wenqi Jin, Meng Cheng, Ruonan Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  10. RbMo 2 P 3 O 14 with large birefringence mainly induced by highly distorted [MoO 6 ] in uncommon [Mo 2 P 3 O 14 ] ∞ layers

    Dalton Transactions · 2021-01-01

    Rui Zhang, Xin Su, Jie Zhang, Mingyao Xiong, Yineng Huang

    Read original paper ↗ ·

  11. Sodium difluorophosphate: facile synthesis, structure, and electrochemical behavior as an additive for sodium-ion batteries

    Journal of Materials Chemistry A · 2021-01-01

    Huan Yang, Jinkwang Hwang, Yuto Tonouchi, Kazuhiko Matsumoto, Rika Hagiwara

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  12. Nickel-rich NMC materials for lithium-ion batteries : surface reactivity and gas production

    Unknown journal · 2021-02-02

    Ana Cristina Martinez

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  13. Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence

    SSRN Electronic Journal · 2022-01-01

    Xuqi Zhang, Yanyan Xue, Lei Yang, Chao Wu, Zhipeng Huang, Jun Xu, Mark Graeme Humphrey, Chi Zhang

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  14. Lithium dendritic growth inhibitor enabling high capacity, dendrite-free, and high current operation for rechargeable lithium batteries

    Energy storage materials · 2022-01-06

    Hee Jae Kim, Nurzhan Umirov, Jae-Sang Park, Jae‐Hong Lim, Jiefang Zhu, Sung‐Soo Kim, Seung‐Taek Myung

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  15. Novel layered heterobimetallic fluorides with large optical band gaps

    Journal of Solid State Chemistry · 2022-02-02

    Belal Ahmed, Kang Min Ok

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  16. Chemical reactivity of lithium difluorophosphate as electrolyte additive in LiNi0.6Co0.2Mn0.2O2/graphite cells

    Electrochimica Acta · 2022-06-23

    Ana Cristina Martinez, Sébastien Rigaud, Sylvie Grugeon, Pierre Tran‐Van, Michel B. Armand, Dominique Cailleu, Serge Pilard, Stéphane Laruelle

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  17. A bicomponent electrolyte additive towards stabilized interface for high-performance lithium-ion batteries

    Ionics · 2022-06-24

    Ziyang Yu, Maohui Bai, Bo Hong, Yanqing Lai, Yexiang Liu

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  18. BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge

    Inorganic Chemistry · 2023-01-04

    Jinbin Fan, Mengfan Wu, Bingliang Cheng, Jian Wei Han

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  19. In Situ Diffuse Reflectance Infrared Fourier-Transform Spectroscopy Investigation of Fluoroethylene Carbonate and Lithium Difluorophosphate Dual Additives in SEI Formation over Cu Anode

    ACS Applied Energy Materials · 2023-04-17

    Bikila Nagasa Olana, Leyela Hassen Adem, Shawn D. Lin, Bing‐Joe Hwang, Yi‐Chen Hsieh, Gunther Brunklaus, Martin Winter

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  20. From Monofluorophosphates A2PO3F to Difluorophosphates APO2F2 (A = alkali metal): Design of a Potential Deep-Ultraviolet Nonlinear Optical Materials System with a Shortened Phase-Matching Wavelength

    Chemistry of Materials · 2023-07-06

    Wenqi Jin, Congwei Xie, Xueling Hou, Meng Cheng, Evgenii Tikhonov, Mengfan Wu, Shilie Pan, Zhihua Yang

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  21. Fluorination strategy toward chemical and functional modification

    Fundamental Research · 2023-12-19

    Haotian Qiu, Shilie Pan, Miriding Mutailipu

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  22. Fluorine-driven materials design of novel deep-ultraviolet nonlinear optical crystal materials: Research progress and challenges

    Chinese Science Bulletin (Chinese Version) · 2024-07-01

    Zhihua Yang, Shilie Pan

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  23. Engineering Stable Decomposition Products on Cathode Surfaces to Enable High Voltage All‐Solid‐State Batteries

    Angewandte Chemie · 2024-11-12

    Lanting Qian, Yangyang Huang, Cameron Dean, Ivan R. Kochetkov, Baltej Singh, Linda F. Nazar

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  24. Engineering Stable Decomposition Products on Cathode Surfaces to Enable High Voltage All‐Solid‐State Batteries

    Angewandte Chemie International Edition · 2024-11-12

    Lanting Qian, Yangyang Huang, Cameron Dean, Ivan R. Kochetkov, Baltej Singh, Linda F. Nazar

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  25. Discrepant lithium transference numbers due to heterogeneous speciation

    Physical Chemistry Chemical Physics · 2025-01-01

    Frederik Philippi, Yuna Matsuyama, Simon Buyting, Taku Sudoh, Keisuke Shigenobu, Wataru Shinoda, Monika Schönhoff, Masayoshi Watanabe, Kazuhide Ueno

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  26. Highly Polarizable Phosphorus‐Centered Tetrahedra and π‐Conjugated Carbon‐Centered Triangular Moieties Inducing Large Anisotropy and Short‐Wavelength Phase‐Matching

    Advanced Optical Materials · 2025-01-28

    Wen-Bin Zhang, Muhammad Arif, Huan Zhou, Ran An, Zhihua Yang, Xueling Hou, Shilie Pan, Shujuan Han

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  27. A review for high-value utilization of retired spent electrolyte for lithium-ion battery: how to reduce the waste of resources?

    Ionics · 2025-05-09

    Jie Wang, Hong Dong, Dongni Zhao, Xiaoling Cui, Linhu Song, Junlong Zhu, Yinong Wang, Feifei Zong, Ningshuang Zhang, Shiyou Li

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  28. Primary exothermic reaction pathways between solid electrolyte interphases and electrolytes during the onset of thermal runaway in lithium-ion batteries

    Energy storage materials · 2025-08-15

    Minuk Kim, Ahmed F. Ghoniem, Jongsup Hong

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  29. One‐Step Biphasic Interfacial Engineering Stabilizes Single‐Crystal Ultrahigh‐Nickel Cathodes

    Advanced Functional Materials · 2025-09-02

    Yiyang Xia, Guihong Mao, Tengyu Yao, Jieyu Yang, Yangjie Zhou, Ken Lin, Zhenming Xu, Duo Chen, Huaiyu Shao, Laifa Shen

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  30. Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes

    Angewandte Chemie International Edition · 2025-11-03

    Zhong‐Sheng Wang, Zhongming Wang, Zhiyuan He, Antai Zhu, Canglong Li, Tianbao Li, Lin Mei, Libao Chen

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  31. Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes

    Angewandte Chemie · 2025-11-03

    Zhongsheng Wang, Zhongming Wang, Zhiyuan He, Antai Zhu, Canglong Li, Tianbao Li, Lin Mei, Libao Chen

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  32. Optimized synthesis of novel LiPOF4 electrolyte additives and their application in lithium-sulfur batteries

    Journal of Solid State Electrochemistry · 2025-12-02

    Tao Liu, Shiyun Tang, Anjiang Tang, Junjiang Guo, Deju Wei, Cejun Hu

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  33. Machine-Learning-Guided Insights into Solid-Electrolyte Interphase Conductivity: Are Amorphous Lithium Fluorophosphates the Key?

    ACS Energy Letters · 2025-12-18

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  34. Rational Lithium Salt Selection Principle for Designing High-Entropy Electrolytes toward High-Performance Lithium Metal Batteries

    Journal of the American Chemical Society · 2026-01-13

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  35. Pretreatment-derived LiF/LiPO2F2 species enable robust high-voltage NCM811 cathode interphases

    Energy storage materials · 2026-08-01

    Yiyao Xiao, Xiaosong Zhang, Jiapei Li, Xia Zhao, Longhao Cao, Said Amzil, Tianle Zheng, Ya‐Jun Cheng, Peter Müller‐Buschbaum, Moses M. Solomon, Philip Hall, Yonggao Xia

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