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RESEARCH PAPER · Angewandte Chemie International Edition · 2018

An Asymmetric Anion‐Pillared Metal–Organic Framework as a Multisite Adsorbent Enables Simultaneous Removal of Propyne and Propadiene from Propylene

Lifeng Yang, Xili Cui, Zhaoqiang Zhang, Qiwei Yang, Zongbi Bao, Qilong Ren, Huabin Xing

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An Asymmetric Anion‐Pillared Metal–Organic Framework as a Multisite Adsorbent Enables Simultaneous Removal of Propyne and Propadiene from PropyleneOriginalA Metal–Organic Framework with Suitable Pore Size and Specific Functional Sites for the Removal of Trace Propyne from Propylene178A Metal–Organic Framework with Suitable Pore Size and Specific Functional Sites for the Removal of Trace Propyne from Propylene108Simultaneous Trapping of C2H2 and C2H6 from a Ternary Mixture of C2H2/C2H4/C2H6 in a Robust Metal–Organic Framework for the Purification of C2H4337Simultaneous Trapping of C2H2 and C2H6 from a Ternary Mixture of C2H2/C2H4/C2H6 in a Robust Metal–Organic Framework for the Purification of C2H485Low-Cost and High-Performance Microporous Metal–Organic Framework for Separation of Acetylene from Carbon Dioxide58A novel interpenetrated anion-pillared porous material with high water tolerance afforded efficient C 2 H 2 /C 2 H 4 separation47A temperature-responsive smart molecular gate in a metal–organic framework for task-specific gas separation48Reaction duration-dependent formation of two Cu( ii )-MOFs with selective adsorption properties of C 3 H 4 over C 3 H 618Recent Progress Towards Light Hydrocarbon Separations Using Metal–Organic Frameworks180A Microporous Metal‐Organic Framework Supramolecularly Assembled from a CuII Dodecaborate Cluster Complex for Selective Gas Separation284A Microporous Metal‐Organic Framework Supramolecularly Assembled from a CuII Dodecaborate Cluster Complex for Selective Gas Separation60A water-stable fcu-MOF material with exposed amino groups for the multi-functional separation of small molecules53Robust Microporous Metal–Organic Frameworks for Highly Efficient and Simultaneous Removal of Propyne and Propadiene from Propylene91Robust Microporous Metal–Organic Frameworks for Highly Efficient and Simultaneous Removal of Propyne and Propadiene from Propylene20Porous metal-organic frameworks for gas storage and separation: Status and challenges891Efficient Separation of n‐Butene and iso‐Butene by Flexible Ultramicroporous Metal‐Organic Frameworks with Pocket‐like Cavities32Engineering the Pore Size of Pillared-Layer Coordination Polymers Enables Highly Efficient Adsorption Separation of Acetylene from Ethylene88Current Status of Microporous Metal–Organic Frameworks for Hydrocarbon Separations41Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving137Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving59Polycatenated Molecular Cage-Based Propane Trap for Propylene Purification with Recorded Selectivity73Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons184Energy-efficient separation alternatives: metal–organic frameworks and membranes for hydrocarbon separation746Opportunities and critical factors of porous metal–organic frameworks for industrial light olefins separation62Solvent-dependent supramolecular self-assembly of boron cage pillared metal–organic frameworks for selective gas separation53Halogen–C2H2 Binding in Ultramicroporous Metal–Organic Frameworks (MOFs) for Benchmark C2H2/CO2 Separation Selectivity89Metal-organic frameworks chelated by zinc fluorides for ultra-high affinity to acetylene during C2/C1 separations11Efficient Separation of Propene and Propane Using Anion-Pillared Metal–Organic Frameworks58Fluorinated Biphenyldicarboxylate-Based Metal–Organic Framework Exhibiting Efficient Propyne/Propylene Separation41Calcium-Based Metal–Organic Framework for Simultaneous Capture of Trace Propyne and Propadiene from Propylene43A periodic table of metal-organic frameworks121Crystal Engineering of Hybrid Coordination Networks: From Form to Function77Molecular Sieving of C2‐C3 Alkene from Alkyne with Tuned Threshold Pressure in Robust Layered Metal–Organic Frameworks128Molecular Sieving of C2‐C3 Alkene from Alkyne with Tuned Threshold Pressure in Robust Layered Metal–Organic Frameworks15Remarkable separation of C5 olefins in anion-pillared hybrid porous materials25Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene184Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene40Gallate-Based Metal–Organic Frameworks for Highly Efficient Removal of Trace Propyne from Propylene26Rational design and synthesis of ultramicroporous metal-organic frameworks for gas separation218Understanding how pore surface fluorination influences light hydrocarbon separation in metal–organic frameworks57Fine‐Tuning Pore Dimension in Hybrid Ultramicroporous Materials Boosting Simultaneous Trapping of Trace Alkynes from Alkenes39Supramolecular Cu( ii )–dipyridyl frameworks featuring weakly coordinating dodecaborate dianions for selective gas separation28Simultaneous interlayer and intralayer space control in two-dimensional metal−organic frameworks for acetylene/ethylene separation163Crystal engineering of porous coordination networks for C3 hydrocarbon separation66Cd-MOF: specific adsorption selectivity for linear alkyne (propyne, 2-butyne and phenylacetylene) molecules5Separation of Xylene Isomers in the Anion‐Pillared Square Grid Material SIFSIX‐1‐Cu20Ultrafine tuning of the pore size in zeolite A for efficient propyne removal from propylene8Structural Evolution from Noninterpenetrated to Interpenetrated Thorium–Organic Frameworks Exhibiting High Propyne Storage19Isoreticular chemistry within metal–organic frameworks for gas storage and separation584Geometry control of adsorption sites in sulfonate-pillared hybrid ultramicroporous materials for efficient C4 olefin separations34Interpenetration Symmetry Control Within Ultramicroporous Robust Boron Cluster Hybrid MOFs for Benchmark Purification of Acetylene from Carbon Dioxide213Interpenetration Symmetry Control Within Ultramicroporous Robust Boron Cluster Hybrid MOFs for Benchmark Purification of Acetylene from Carbon Dioxide25A Solid Transformation into Carboxyl Dimers Based on a Robust Hydrogen‐Bonded Organic Framework for Propyne/Propylene Separation139A Solid Transformation into Carboxyl Dimers Based on a Robust Hydrogen‐Bonded Organic Framework for Propyne/Propylene Separation22Efficient separation of C4 olefins using tantalum pentafluor oxide anion-pillared hybrid microporous material19Contribution of hydrogen bonding to liquid-phase adsorptive removal of hazardous organics with metal-organic framework-based materials162Confined Ionic Liquid-Built Gas Transfer Pathways for Efficient Propylene/Propane Separation26A new boron cluster anion pillared metal organic framework with ligand inclusion and its selective acetylene capture properties33A Review on Anion-Pillared Metal Organic Framework (Apmof) and its Composites with the Balance of Adsorption Capacity and Separation Selectivity for Efficient Gas Separation1Fluorinated metal–organic frameworks for gas separation271Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation83Strong Hydrogen Bond in the Crystal Structure Design of CuNbOF 5·4H 2O0An anion-functionalized zinc-organic framework for efficient C2H2/C2H4 separation12Comprehensive Pore Tuning in an Ultrastable Fluorinated Anion Cross‐Linked Cage‐Like MOF for Simultaneous Benchmark Propyne Recovery and Propylene Purification17Comprehensive Pore Tuning in an Ultrastable Fluorinated Anion Cross‐Linked Cage‐Like MOF for Simultaneous Benchmark Propyne Recovery and Propylene Purification110Stable Fluorinated Hybrid Microporous Material for the Efficient Separation of C2–C3 Alkyne/Alkene Mixtures22Double-Accessible Open Metal Sites in Metal–Organic Frameworks with Suitable Pore Size for Efficient Xe/Kr Separation29One-step removal of alkynes and propadiene from cracking gases using a multi-functional molecular separator42Progress and potential of metal-organic frameworks (MOFs) for gas storage and separation: A review356Efficient Separation of Trace SO2 from SO2/CO2/N2 Mixtures in a Th-Based MOF23A review on anion-pillared metal–organic frameworks (APMOFs) and their composites with the balance of adsorption capacity and separation selectivity for efficient gas separation102Machine-learning-assisted exploration of anion-pillared metal organic frameworks for gas separation31Enhancement of Propadiene/Propylene Separation Performance of Metal–Organic Frameworks by an Amine-Functionalized Strategy6Insights into the thermodynamic–kinetic synergistic separation of propyne/propylene in anion pillared cage MOFs with entropy–enthalpy balanced adsorption sites51Strong hydrogen bond in the crystal structure design of CuNbOF5·4H2O3Rationally Fabricating Three-Dimensional Covalent Organic Frameworks for Propyne/Propylene Separation82Dicopper( ii ) paddle-wheel metal–organic frameworks for high propyne storage under ambient conditions9Recent progress in metal–organic frameworks for the separation of gaseous hydrocarbons29Ultrastable 3D cage-like metal–organic frameworks constructed using polydentate cyanurate ligands and their gas adsorption properties6Designed metal-organic frameworks with potential for multi-component hydrocarbon separation118Anion‐pillared microporous material incorporated mixed‐matrix fiber adsorbents for removal of trace propyne from propylene7Highly Productive C3H4/C3H6 Trace Separation by a Packing Polymorph of a Layered Hybrid Ultramicroporous Material46Metal-organic frameworks for multicomponent gas separation35Mixed matrix membranes based on NbOF52− anion-pillared porous MOFs for efficient CO2 separation8Specific Propyne Trapping Sites within a Robust MOF for Efficient Propyne/Propadiene Separation with Record Propadiene Productivity36Metal–organic frameworks for petroleum-based platform compound separations15Recent advances on metal–organic frameworks for deep purification of olefins54Flexible–robust MOFs/HOFs for challenging gas separations137Immobilization of Amino‐site into a Pore‐Partitioned Metal–Organic Framework for Highly Efficient Separation of Propyne/Propylene5Immobilization of Amino‐site into a Pore‐Partitioned Metal–Organic Framework for Highly Efficient Separation of Propyne/Propylene29Modulating pore microenvironment in a robust ionic porous polymer for efficient propyne/propylene separation5A Flexible Dihydrogen-Bonded Organic Framework with Selective Gas Adsorption Properties4The Reinforced Separation of Intractable Gas Mixtures by Using Porous Adsorbents61A coordination polymer based on ionic-type ligand for efficient separation of C2H2/C2H4 and C3H4/C3H6 mixtures0Stepwise customizing pore environments of C2H2-selective frameworks for one-step C2H4 acquisition from ternary mixtures10Rapid Synthesis of Ultramicroporous Potassium-Pyrenetetracarboxylate Framework with Confined-Space-Charge-Driving CO2 Capture11Customizing Quasi-Discrete Pores with Gating Flexibility in 2D Supramolecular Isomers for Kinetic Propyne/Propylene Separation2Pillar-cage fluorinated hybrid porous frameworks featuring quasi-Johnson solid J283An Ambient Aqueous Route to Scalable ZIF-8 Fabrics for Harmful Gas Capture0An Ambient Aqueous Route to Scalable ZIF-8 Fabrics for Harmful Gas Capture0Covalent organic frameworks for gas storage and separation24Crystallographic visualization of C3-hydrocarbon-induced structural transformation and guest encapsulation within a flexible coordination network0Phosphonium Ionic Imine Cage with an Uncommon Tri 2 4 Di 6 Topology for Selective Capture of Propyne in Propyne/Propylene Separation4An ambient aqueous route to scalable ZIF-8 fabrics for harmful gas capture1Hierarchical Microporous Anion Pillared Metal–Organic Frameworks (APMOFs) for Gas Separation2Cage-based metal-organic framework with two-fold interpenetration for Propyne/propylene adsorptive separation0Aromaticity Regulation in Isostructural Metal‐Organic Frameworks for Propyne Storage and Propylene Purification0

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  1. A Metal–Organic Framework with Suitable Pore Size and Specific Functional Sites for the Removal of Trace Propyne from Propylene

    Angewandte Chemie International Edition · 2018-09-22

    Libo Li, Hui‐Min Wen, Chaohui He, Rui‐Biao Lin, Rajamani Krishna, Hui Wu, Wei Zhou, Jinping Li, Bin Li, Banglin Chen

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  2. A Metal–Organic Framework with Suitable Pore Size and Specific Functional Sites for the Removal of Trace Propyne from Propylene

    Angewandte Chemie · 2018-09-22

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  3. Simultaneous Trapping of C2H2 and C2H6 from a Ternary Mixture of C2H2/C2H4/C2H6 in a Robust Metal–Organic Framework for the Purification of C2H4

    Angewandte Chemie International Edition · 2018-10-19

    Hongguo Hao, Yunfeng Zhao, Di‐Ming Chen, Jiamei Yu, Kui Tan, Shengqian Ma, Yves Jean Chabal, Zhiming Zhang, Jianmin Dou, Zihui Xiao, Gregory S. Day, Hong-Cai “Joe” Zhou, Tong‐Bu Lu

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  4. Simultaneous Trapping of C2H2 and C2H6 from a Ternary Mixture of C2H2/C2H4/C2H6 in a Robust Metal–Organic Framework for the Purification of C2H4

    Angewandte Chemie · 2018-10-19

    Hongguo Hao, Yunfeng Zhao, Di‐Ming Chen, Jiamei Yu, Kui Tan, Shengqian Ma, Yves Jean Chabal, Zhiming Zhang, Jianmin Dou, Zihui Xiao, Gregory S. Day, Hong-Cai “Joe” Zhou, Tong‐Bu Lu

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  5. Low-Cost and High-Performance Microporous Metal–Organic Framework for Separation of Acetylene from Carbon Dioxide

    ACS Sustainable Chemistry & Engineering · 2018-12-05

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  6. A novel interpenetrated anion-pillared porous material with high water tolerance afforded efficient C 2 H 2 /C 2 H 4 separation

    Chemical Communications · 2019-01-01

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  7. A temperature-responsive smart molecular gate in a metal–organic framework for task-specific gas separation

    Journal of Materials Chemistry A · 2019-01-01

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  8. Reaction duration-dependent formation of two Cu( ii )-MOFs with selective adsorption properties of C 3 H 4 over C 3 H 6

    Dalton Transactions · 2019-01-01

    Mingming Xu, Xiang‐Jing Kong, Tao He, Xue‐Qian Wu, Lin‐Hua Xie, Jian‐Rong Li

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  9. Recent Progress Towards Light Hydrocarbon Separations Using Metal–Organic Frameworks

    Trends in Chemistry · 2019-03-29

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  10. A Microporous Metal‐Organic Framework Supramolecularly Assembled from a CuII Dodecaborate Cluster Complex for Selective Gas Separation

    Angewandte Chemie International Edition · 2019-04-12

    Yuanbin Zhang, Lifeng Yang, Lingyao Wang, Simon Duttwyler, Huabin Xing

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  11. A Microporous Metal‐Organic Framework Supramolecularly Assembled from a CuII Dodecaborate Cluster Complex for Selective Gas Separation

    Angewandte Chemie · 2019-04-12

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  12. A water-stable fcu-MOF material with exposed amino groups for the multi-functional separation of small molecules

    Science China Materials · 2019-04-28

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  13. Robust Microporous Metal–Organic Frameworks for Highly Efficient and Simultaneous Removal of Propyne and Propadiene from Propylene

    Angewandte Chemie International Edition · 2019-05-06

    Yun‐Lei Peng, Chaohui He, Tony Pham, Ting Wang, Pengfei Li, Rajamani Krishna, Katherine A. Forrest, Adam Hogan, Shanelle Suepaul, Brian Space, Ming Fang, Yao Chen, Michael John Zaworotko, Jinping Li, Libo Li, Zhenjie Zhang, Peng Cheng, Banglin Chen

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  14. Robust Microporous Metal–Organic Frameworks for Highly Efficient and Simultaneous Removal of Propyne and Propadiene from Propylene

    Angewandte Chemie · 2019-05-06

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  15. Porous metal-organic frameworks for gas storage and separation: Status and challenges

    EnergyChem · 2019-06-27

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  16. Efficient Separation of n‐Butene and iso‐Butene by Flexible Ultramicroporous Metal‐Organic Frameworks with Pocket‐like Cavities

    Chemistry - An Asian Journal · 2019-07-06

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  17. Engineering the Pore Size of Pillared-Layer Coordination Polymers Enables Highly Efficient Adsorption Separation of Acetylene from Ethylene

    ACS Applied Materials & Interfaces · 2019-07-16

    Fang Zheng, Lidong Guo, Bixuan Gao, Liangying Li, Zhiguo Zhang, Qiwei Yang, Yiwen Yang, Baogen Su, Qilong Ren, Zongbi Bao

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  18. Current Status of Microporous Metal–Organic Frameworks for Hydrocarbon Separations

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  19. Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving

    Angewandte Chemie International Edition · 2019-11-20

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  20. Separation of Xe from Kr with Record Selectivity and Productivity in Anion‐Pillared Ultramicroporous Materials by Inverse Size‐Sieving

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  21. Polycatenated Molecular Cage-Based Propane Trap for Propylene Purification with Recorded Selectivity

    ACS Applied Materials & Interfaces · 2019-12-09

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  22. Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons

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  23. Energy-efficient separation alternatives: metal–organic frameworks and membranes for hydrocarbon separation

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  24. Opportunities and critical factors of porous metal–organic frameworks for industrial light olefins separation

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  25. Solvent-dependent supramolecular self-assembly of boron cage pillared metal–organic frameworks for selective gas separation

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  26. Halogen–C2H2 Binding in Ultramicroporous Metal–Organic Frameworks (MOFs) for Benchmark C2H2/CO2 Separation Selectivity

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  27. Metal-organic frameworks chelated by zinc fluorides for ultra-high affinity to acetylene during C2/C1 separations

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  28. Efficient Separation of Propene and Propane Using Anion-Pillared Metal–Organic Frameworks

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  29. Fluorinated Biphenyldicarboxylate-Based Metal–Organic Framework Exhibiting Efficient Propyne/Propylene Separation

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  30. Calcium-Based Metal–Organic Framework for Simultaneous Capture of Trace Propyne and Propadiene from Propylene

    ACS Applied Materials & Interfaces · 2020-03-18

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  31. A periodic table of metal-organic frameworks

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  32. Crystal Engineering of Hybrid Coordination Networks: From Form to Function

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  33. Molecular Sieving of C2‐C3 Alkene from Alkyne with Tuned Threshold Pressure in Robust Layered Metal–Organic Frameworks

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  34. Molecular Sieving of C2‐C3 Alkene from Alkyne with Tuned Threshold Pressure in Robust Layered Metal–Organic Frameworks

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  35. Remarkable separation of C5 olefins in anion-pillared hybrid porous materials

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  36. Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene

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  37. Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene

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  38. Gallate-Based Metal–Organic Frameworks for Highly Efficient Removal of Trace Propyne from Propylene

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  39. Rational design and synthesis of ultramicroporous metal-organic frameworks for gas separation

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  40. Understanding how pore surface fluorination influences light hydrocarbon separation in metal–organic frameworks

    Chemical Engineering Journal · 2020-09-30

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  41. Fine‐Tuning Pore Dimension in Hybrid Ultramicroporous Materials Boosting Simultaneous Trapping of Trace Alkynes from Alkenes

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  42. Supramolecular Cu( ii )–dipyridyl frameworks featuring weakly coordinating dodecaborate dianions for selective gas separation

    CrystEngComm · 2020-11-25

    Lingyao Wang, Tao Jiang, Simon Duttwyler, Yuanbin Zhang

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  43. Simultaneous interlayer and intralayer space control in two-dimensional metal−organic frameworks for acetylene/ethylene separation

    Nature Communications · 2020-12-07

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  44. Crystal engineering of porous coordination networks for C3 hydrocarbon separation

    SmartMat · 2020-12-29

    Mei‐Yan Gao, Bai‐Qiao Song, Debobroto Sensharma, Michael John Zaworotko

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  45. Cd-MOF: specific adsorption selectivity for linear alkyne (propyne, 2-butyne and phenylacetylene) molecules

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  46. Separation of Xylene Isomers in the Anion‐Pillared Square Grid Material SIFSIX‐1‐Cu

    Chemistry - A European Journal · 2021-01-20

    Liping Yang, Hanbang Liu, Jiacheng Xing, Danhua Yuan, Yunpeng Xu, Zhongmin Liu

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  47. Ultrafine tuning of the pore size in zeolite A for efficient propyne removal from propylene

    Chinese Journal of Chemical Engineering · 2021-01-22

    Chaohui He, Rajamani Krishna, Yang Chen, Jiangfeng Yang, Jinping Li, Libo Li

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  48. Structural Evolution from Noninterpenetrated to Interpenetrated Thorium–Organic Frameworks Exhibiting High Propyne Storage

    Inorganic Chemistry · 2021-04-12

    Yuan-Bo Wu, Cheng Xiong, Qing‐Yan Liu, Jianguo Ma, Feng Luo, Yu‐Ling Wang

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  49. Isoreticular chemistry within metal–organic frameworks for gas storage and separation

    Coordination Chemistry Reviews · 2021-05-13

    Weidong Fan, Xiurong Zhang, Zixi Kang, Xiuping Liu, Daofeng Sun

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  50. Geometry control of adsorption sites in sulfonate-pillared hybrid ultramicroporous materials for efficient C4 olefin separations

    Chemical Engineering Journal · 2021-05-31

    Jiyu Cui, Zhaoqiang Zhang, Jianbo Hu, Lifeng Yang, Yijian Li, Liyuan Chen, Xili Cui, Huabin Xing

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