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RESEARCH PAPER · Chemical Society Reviews · 2020

Energy-efficient separation alternatives: metal–organic frameworks and membranes for hydrocarbon separation

Lifeng Yang, Siheng Qian, Xiaobing Wang, Xili Cui, Banglin Chen, Huabin Xing

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Energy-efficient separation alternatives: metal–organic frameworks and membranes for hydrocarbon separationOriginalMetal–organic frameworks for C 2 H 2 /CO 2 separation86Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene184Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene40Fine-Tuning and Selective-Binding within an Anion-Functionalized Ultramicroporous Metal–Organic Framework for Efficient Olefin/Paraffin Separation72Selective capture of carbon dioxide from humid gases over a wide temperature range using a robust metal–organic framework72Separation of propylene and propane with a microporous metal–organic framework via equilibrium‐kinetic synergetic effect57Luminescence response mode and chemical sensing mechanism for lanthanide-functionalized metal–organic framework hybrids278Microregulation of Pore Channels in Covalent-Organic Frameworks Used for the Selective and Efficient Separation of Ethane63Host-guest interaction-mediated nanointerface engineering for radioiodine capture97A hydrolytically stable cage-based metal–organic framework containing two types of building blocks for the adsorption of iodine and dyes932D framework materials for energy applications121Tailoring the Pore Size and Chemistry of Ionic Ultramicroporous Polymers for Trace Sulfur Dioxide Capture with High Capacity and Selectivity90A novel mechanism of controlling ultramicropore size in carbons at sub-angstrom level for molecular sieving of propylene/propane mixtures58Advanced microporous membranes for H2/CH4 separation: Challenges and perspectives61Engineering metal–organic frameworks for adsorption-based gas separations: from process to atomic scale64Nanoconfinement and mass transport in metal–organic frameworks188Rational strategies for proton-conductive metal–organic frameworks334A Series of Metal–Organic Framework Isomers Based on Pyridinedicarboxylate Ligands: Diversified Selective Gas Adsorption and the Positional Effect of Methyl Functionality41Supramolecular control of MOF pore properties for the tailored guest adsorption/separation applications271In Situ Porphyrin Substitution in a Zr(IV)‐MOF for Stability Enhancement and Photocatalytic CO2 Reduction161Cage‐Like Porous Materials with Simultaneous High C2H2Storage and Excellent C2H2/CO2Separation Performance171Selective Gas Uptake and Rotational Dynamics in a (3,24)-Connected Metal–Organic Framework Material57Construction of an Anion-Pillared MOF Database and the Screening of MOFs Suitable for Xe/Kr Separation99Asymmetric catalysis using metal-organic frameworks142Cyclotetrabenzoin Acetate: A Macrocyclic Porous Molecular Crystal for CO 2 Separations by Pressure Swing Adsorption**46Efficient adsorption separation of methane from CO2 and C2–C3 hydrocarbons in a microporous closo-dodecaborate [B12H12]2- pillared metal–organic framework44Zeolitic imidazolate framework membranes for gas separations: Current state-of-the-art, challenges, and opportunities59Nanoporous Water-Stable Zr-Based Metal–Organic Frameworks for Water Adsorption46Solvatomorphism Influence of Porous Organic Cage on C2H2/CO2Separation55Isoreticular chemistry within metal–organic frameworks for gas storage and separation584C2s/C1 hydrocarbon separation: The major step towards natural gas purification by metal-organic frameworks (MOFs)145Ligand‐Conformer‐Induced Formation of Zirconium–Organic Framework for Methane Storage and MTO Product Separation120Insights into the Enhancement of MOF/Polymer Adhesion in Mixed-Matrix Membranes via Polymer Functionalization78MOF‐Nanocomposite Mixed‐Matrix Membrane for Dual‐Luminescence Ratiometric Temperature Sensing104Formation of a N/O/F-Rich and Rooflike Cluster-Based Highly Stable Cu(I/II)-MOF for Promising Pipeline Natural Gas Upgrading by the Recovery of Individual C3H8 and C2H6 Gases46A metal-organic framework for C2H2/CO2 separation under highly humid conditions: Balanced hydrophilicity/hydrophobicity88Covalent‐Organic Frameworks (COFs) as Proton Conductors287A 3D ultramicroporous porous organic frameworks for SO2 and aromatic sulfides capture with high capacity and selectivity41Room-temperature synthesis of hydrophobic/oleophilic ZIF-90-CF3/melamine foam composite for the efficient removal of organic compounds from wastewater51High Degradation of Methylene Blue Using a New Nanocomposite Based on Zeolitic Imidazolate Framework-8111Shining Light on Porous Liquids: From Fundamentals to Syntheses, Applications and Future Challenges110Multivariate Polycrystalline Metal–Organic Framework Membranes for CO 2 /CH 4 Separation192Rapid Screening of Metal–Organic Frameworks for Propane/Propylene Separation by Synergizing Molecular Simulation and Machine Learning103High performance of PES-GNs MMMs for gas separation and selectivity42Covalent‐Linking‐Enabled Superior Compatibility of ZIF‐8 Hybrid Membrane for Efficient Propylene Separation111A humidity sensor based on ionic liquid modified metal organic frameworks for low humidity detection70Halogen bonding in cadmium( ii ) MOFs: its influence on the structure and on the nitroaldol reaction in aqueous medium40A new yttrium‐based metal–organic framework for molecular sieving of propane from propylene with high propylene capacity39Recent progress on porous MOFs for process-efficient hydrocarbon separation, luminescent sensing, and information encryption136Fluorinated metal–organic frameworks for gas separation271Hierarchical porous metal–organic gels and derived materials: from fundamentals to potential applications151MOF or COF membranes for olefin/paraffin separation: Current status and future research directions46Tailoring a robust Al-MOF for trapping C 2 H 6 and C 2 H 2 towards efficient C 2 H 4 purification from quaternary mixtures59Host-guest nanofiltration membranes having amino-complexed cucurbituril supramolecular channel for monovalent/divalent salts separation40Facile and controllable preparation of nanocrystalline ZSM-5 and Ag/ZSM-5 zeolite with enhanced performance of adsorptive desulfurization from fuel55Comprehensive Pore Tuning in an Ultrastable Fluorinated Anion Cross‐Linked Cage‐Like MOF for Simultaneous Benchmark Propyne Recovery and Propylene Purification110Mitigated Aging in a Defective Metal–Organic Framework Pillared Polymer of an Intrinsic Porosity Hybrid Membrane for Efficient Gas Separation57Room-temperature synthesis of defect-engineered Zirconium-MOF membrane enabling superior CO2/N2 selectivity with zirconium-oxo cluster source83Chiral Metal–Organic Frameworks579Recent advances of functional heterometallic-organic framework (HMOF) materials: Design strategies and applications93Adsorption in Reversed Order of C 2 Hydrocarbons on an Ultramicroporous Fluorinated Metal‐Organic Framework57Hydrogen-bonded metal-nucleobase frameworks for highly selective capture of ethane/propane from methane and methane/nitrogen separation41A versatile route to fabricate Metal/UiO-66 (Metal = Pt, Pd, Ru) with high activity and stability for the catalytic oxidation of various volatile organic compounds103Enhancing CH4 Capture from Coalbed Methane through Tuning van der Waals Affinity within Isoreticular Al-Based Metal–Organic Frameworks71Reverse-selective metal–organic framework materials for the efficient separation and purification of light hydrocarbons140Electrostatic‐Induced Crystal‐Rearrangement of Porous Organic Cage Membrane for CO2 Capture55Synergistic binding sites in a hybrid ultramicroporous material for one-step ethylene purification from ternary C 2 hydrocarbon mixtures136Recent Advances in the Development of Metal–Organic Frameworks for Propylene and Propane Separation49Progress and potential of metal-organic frameworks (MOFs) for gas storage and separation: A review356A gating ultramicroporous metal-organic framework showing high adsorption selectivity, capacity and rate for xylene separation44A review on anion-pillared metal–organic frameworks (APMOFs) and their composites with the balance of adsorption capacity and separation selectivity for efficient gas separation102A Metal‐Organic Framework with Nonpolar Pore Surfaces for the One‐Step Acquisition of C 2 H 4 from a C 2 H 4 and C 2 H 6 Mixture129Progress in Hybridization of Covalent Organic Frameworks and Metal–Organic Frameworks106Metal–Organic Frameworks for CO 2 Separation from Flue and Biogas Mixtures132Ultramicroporous material based parallel and extended paraffin nano-trap for benchmark olefin purification112Uniform stain pattern of robust MOF-mediated probe for flexible paper-based colorimetric sensing toward environmental pesticide exposure89On the Role of Flexibility for Adsorptive Separation155Robust Metal–Organic Frameworks with High Industrial Applicability in Efficient Recovery of C3H8 and C2H6 from Natural Gas Upgrading76Efficient capture of C2H2 from CO2 and CnH4 by a novel fluorinated anion pillared MOF with flexible molecular sieving effect65Optimization of Pore-Space-Partitioned Metal–Organic Frameworks Using the Bioisosteric Concept89Insights into the thermodynamic–kinetic synergistic separation of propyne/propylene in anion pillared cage MOFs with entropy–enthalpy balanced adsorption sites51A new perchlorate-based hybrid ultramicroporous material with rich bare oxygen atoms for high C2H2/CO2 separation39A new honeycomb MOF for C 2 H 4 purification and C 3 H 6 enrichment by separating methanol to olefin products79Porous crystalline materials for memories and neuromorphic computing systems166Potential of nonporous adaptive crystals for hydrocarbon separation125Zeolites and metal–organic frameworks for gas separation: the possibility of translating adsorbents into membranes269Porous framework materials for energy & environment relevant applications: A systematic review137Stepwise Engineering the Pore Aperture of a Cage‐like MOF for the Efficient Separation of Isomeric C4 Paraffins under Humid Conditions66Programmed Polarizability Engineering in a Cyclen-Based Cubic Zr(IV) Metal–Organic Framework to Boost Xe/Kr Separation98Benchmark single-step ethylene purification from ternary mixtures by a customized fluorinated anion-embedded MOF195In Situ Fabrication of Metal–Organic Framework Thin Films with Enhanced Pervaporation Performance43A novel clover-like COFs membrane fabricated via one-step interfacial polymerization for dye/salt separation79Monitoring the Activation of Open Metal Sites in [FexM3–x(μ3-O)] Cluster-Based Metal–Organic Frameworks by Single-Crystal X-ray Diffraction62Pore Aperture Control Toward Size‐Exclusion‐Based Hydrocarbon Separations61A Robust Metal‐Organic Framework with Scalable Synthesis and Optimal Adsorption and Desorption for Energy‐Efficient Ethylene Purification78Challenges in Developing MOF-Based Membranes for Gas Separation129Engineering the Pore Structure and Functionality of Ionic Porous Polymers for Separating Acetylene over Carbon Dioxide39Metal-organic frameworks for C2H2/CO2 separation: Recent development142Covalent organic framework membrane with sub-nano pores for efficient desalination47Engineering Metal–Organic Frameworks for Selective Separation of Hexane Isomers Using 3-Dimensional Linkers80A path forward: Understanding and mitigating defects in polycrystalline membranes50Vertex Strategy in Layered 2D MOFs: Simultaneous Improvement of Thermodynamics and Kinetics for Record C 2 H 2 /CO 2 Separation Performance109Dynamic Bond-Directed Synthesis of Stable Mesoporous Metal–Organic Frameworks under Room Temperature65Linker Vacancy Engineering of a Robust ftw‐type Zr‐MOF for Hexane Isomers Separation45pH-stable MOFs: Design principles and applications196Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation103Metal–Organic Frameworks for Water Desalination127Multiscale CO 2 Electrocatalysis to C 2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication328Industrial Separation Challenges: How Does Supramolecular Chemistry Help?86A review from material functionalization to process feasibility on advanced mixed matrix membranes for gas separations65Tuning the Stacking Modes of Ultrathin Two‐Dimensional Metal–Organic Framework Nanosheet Membranes for Highly Efficient Hydrogen Separation66Kilogram-Scale Fabrication of a Robust Olefin-Linked Covalent Organic Framework for Separating Ethylene from a Ternary C 2 Hydrocarbon Mixture166Adaptive Pore Opening to Form Tailored Adsorption Sites in a Cooperatively Flexible Framework Enables Record Inverse Propane/Propylene Separation58Advanced strategies in MOF-based mixed matrix membranes for propylene/propane separation: A critical review66Simultaneous extraction of C3H8 and C2H6 from ternary C3H8/C2H6/CH4 mixtures in an ultra-microporous metal–organic framework51Robust Carborane-Based Metal–Organic Frameworks for Hexane Separation86A molecular sieve with ultrafast adsorption kinetics for propylene separation308Uniformly Distributed Mixed Matrix Membranes via a Solution Processable Strategy for Propylene/Propane Separation50A novel hydrophobic carborane-hybrid microporous material for reversed C 2 H 6 adsorption and efficient C 2 H 4 /C 2 H 6 separation under humid conditions44Non-CO 2 greenhouse gas separation using advanced porous materials177Recent advances on metal–organic frameworks for deep purification of olefins54Dynamic molecular pockets on one-dimensional channels for splitting ethylene from C2–C4 alkynes47Flexible–robust MOFs/HOFs for challenging gas separations137Scalable Synthesis of Robust MOF for Challenging Ethylene Purification and Propylene Recovery with Record Productivity77An Ultra‐stable Supramolecular Framework Based on Consecutive Side‐by‐side Hydrogen Bonds for One‐step C 2 H 4 /C 2 H 6 Separation50Electro‐field alignment in a novel metal–organic framework for benchmark separation of ethylene from a ternary gas mixture47Enabling C2H2/CO2 Separation Under Humid Conditions with a Methylated Copper MOF52Machine Learning-Assisted Discovery of Propane-Selective Metal–Organic Frameworks85Effective C 4 Separation by Zeolite Metal–Organic Framework Composite Membranes47Isoreticular Contraction of Cage-like Metal–Organic Frameworks with Optimized Pore Space for Enhanced C2H2/CO2 and C2H2/C2H4 Separations121A Layered Hydrogen-Bonded Organic Framework with C3H6-Preferred Pores for Efficient One-Step Purification of Methanol-to-Olefins (MTO) Products54Recent Advances of Multidentate Ligand-Based Anion-Pillared MOFs for Enhanced Separation and Purification Processes44Ideal Cage‐like Pores for Molecular Sieving of Butane Isomers with High Purity and Record Productivity40Toward Scalable and Sustainable Synthesis of Metal–Organic Frameworks61An innovative NH2-UiO-66/NH2-MIL-125 MOF-on-MOF structure to improve the performance and antifouling properties of ultrafiltration membranes70Metal–Organic Framework with Space-Partition Pores by Fluorinated Anions for Benchmark C2H2/CO2 Separation137Synergistic C 2 H 2 Binding Sites in Hydrogen‐Bonded Supramolecular Framework for One‐Step C 2 H 4 Purification from Ternary C2 Mixture39A Stable Layered Microporous MOF Assembled with Y–O Chains for Separation of MTO Products39Controlling Guest Diffusion by Local Dynamic Motion in Soft Porous Crystals to Separate Water Isotopologues and Similar Gases40Host-guest interactions in the confined spaces of metal–organic frameworks: Design principles, characterizations, and applications51Aromatic-aliphatic hydrocarbon separation with oriented monolayer polyhedral membrane111Accurate stacking engineering of MOF nanosheets as membranes for precise H2 sieving59Ionic porous materials: from synthetic strategies to applications in gas separation and catalysis45Pore engineering in metal–organic frameworks and covalent organic frameworks: strategies and applications143Recent progress in metal-organic frameworks (Part II—material application)57MOF membranes for gas separations141Architecting Metal–Organic Frameworks at Molecular Level toward Direct Air Capture103Mobile Constituent-Boosted Dynamic Separation of C 2 H 2 /C 2 H 4 /CO 2 Ternary Mixtures in Metal–Organic Frameworks63Nanospace Engineering of Metal–Organic Frameworks for Adsorptive Gas Separation52Efficient One-Step Purification of Methanol-to-Olefin Products Using a Porphyrinyl MOF to Achieve Record C2H4 and C3H6 Productivity42

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