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RESEARCH PAPER · Inorganic Chemistry · 2018

Ternary Mixed-Metal Cd4GeS6: Remarkable Nonlinear-Optical Properties Based on a Tetrahedral-Stacking Framework

Mengyue Li, Bingxuan Li, Hua Lin, Yong‐Fang Shi, Zuju Ma, Li‐Ming Wu, Xintao Wu, Qi‐Long Zhu

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Ternary Mixed-Metal Cd4GeS6: Remarkable Nonlinear-Optical Properties Based on a Tetrahedral-Stacking FrameworkOriginalRecent progress on new infrared nonlinear optical materials with application prospect133From CuFeS 2 to Ba 6 Cu 2 FeGe 4 S 16 : rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold22SrCdGeS4 and SrCdGeSe4: Promising Infrared Nonlinear Optical Materials with Congruent-Melting Behavior74Ba10In6Zn7S26-nZnS: An Inorganic Composite System with Interface Phase-Matching Tuned for High-Performance Infrared Nonlinear Optical Materials13Ba10In6Zn7S10Se16 and Ba10In6Zn7Se26: Two new infrared nonlinear optical materials with T2 super tetrahedron6Ba2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains99Sn 2 Ga 2 S 5 : A Polar Semiconductor with Exceptional Infrared Nonlinear Optical Properties Originating from the Combined Effect of Mixed Asymmetric Building Motifs81Rational design of infrared nonlinear optical chalcogenides by chemical substitution287Mixed-metal thiophosphate CuCd 3 PS 6 : an infrared nonlinear optical material activated by its three-in-one tetrahedra-stacking architecture33One-Dimensional Double Chains in Sodium-Based Quaternary Chalcogenides Displaying Intriguing Red Emission and Large Optical Anisotropy17An assessment of the structural, electronic, optical and thermoelectric properties of the BaAg2GeS4 compound11Cd4SiQ6 (Q = S, Se): Ternary Infrared Nonlinear Optical Materials with Mixed Functional Building Motifs21Controlled nano‐crystallization of IR frequency‐doubling Cd 4 GeS 6 crystal in chalcogenide glass3HgCuPS4: An Exceptional Infrared Nonlinear Optical Material with Defect Diamond-like Structure146Functional Chalcogenide Na2HgSn2Se6 and K2MnGe2Se6 Exhibiting Flexible Chain Structure and Intriguing Birefringence Tunability16Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials131A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks53Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials47Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks5α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band Gaps30Rb2CuSb7S12: Quaternary Antimony-Rich Semiconductor Featuring a Three-Dimensional Open Framework and Exhibiting an Intriguing Photocurrent Response31Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184Rb2MGe3S8 (M=Zn, Cd): Non-Centrosymmetry Transformation Led by Structure Change of [MGe3S8]2- Unit※4Optimization on preparation conditions to improve the nonlinear optical response of ZnO/TiO2/ZrO2 ternary nanocomposites under continuous-wave laser irradiation21Li2Mg2Si2S6 and Li2Mg2Ge2S6: Two nonlinear optical sulfides featuring a unique, polar trigonal structure incorporating ethane‐like anions5A novel bifunctional thioarsenate based on unprecedented molecular [Cd 4 As 8 Se 16 (Se 2 ) 2 ] 8− cluster anions11Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance57Regulating the key performance parameters for Hg-based IR NLO chalcogenides via bandgap engineering strategy26Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response28Structural, electronic and optical properties of CdTiX2 (X = N and P): A first principles density functional theory investigation3Nonbonding Electron Inversion‐Driven Structural Engineering: Synergistic Enhancement of Linear and Nonlinear Optical Properties3Nonbonding Electron Inversion‐Driven Structural Engineering: Synergistic Enhancement of Linear and Nonlinear Optical Properties26Synergistic Enhancement of Band Gap and Optical Anisotropy via Functional-Site Cosubstitution in Antiperovskite-Type Chalcohalides [Ba2K][X][MS4] (M = Ge, Si; X = Cl, Br)2Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29Vacancy-driven tetrahedral distortion leading to exceptional second harmonic generation3A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation2Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12From Centrosymmetric Mg 2 GeS 4 to Noncentrosymmetric CdMg 3 Ge 2 S 8 : Cation-Mixing-Driven Symmetry Reduction4NaGa2PS6: A Noncentrosymmetric Thiophosphate with Wide Band Gap and High Laser-Induced Damage Threshold0Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics0

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  1. Recent progress on new infrared nonlinear optical materials with application prospect

    Journal of Solid State Chemistry · 2018-12-20

    Xiaoyu Luo, Zhuang Li, Yangwu Guo, Jiyong Yao, Yicheng Wu

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  2. From CuFeS 2 to Ba 6 Cu 2 FeGe 4 S 16 : rational band gap engineering achieves large second-harmonic-generation together with high laser damage threshold

    Chemical Communications · 2019-01-01

    Wangzhu Cao, Dajiang Mei, Yi Jin Yang, Yuanwang Wu, Ling‐Yun Zhang, Yuandong Wu, Xiao Dong He, Zheshuai Lin, Fuqiang Huang

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  3. SrCdGeS4 and SrCdGeSe4: Promising Infrared Nonlinear Optical Materials with Congruent-Melting Behavior

    Crystal Growth & Design · 2019-01-07

    Yunwei Dou, Ying Chen, Zhuang Li, Abishek K. Iyer, Bin Kang, Wenlong Yin, Jiyong Yao, Arthur Mar

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  4. Ba10In6Zn7S26-nZnS: An Inorganic Composite System with Interface Phase-Matching Tuned for High-Performance Infrared Nonlinear Optical Materials

    Inorganic Chemistry · 2019-03-01

    Anyi Zhou, Weilong Zhang, Chensheng Lin, Fang-Yu Yuan, Yongyu Pang, Hao Zhang, Wen‐Dan Cheng, Jing Zhu, Guoliang Chai

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  5. Ba10In6Zn7S10Se16 and Ba10In6Zn7Se26: Two new infrared nonlinear optical materials with T2 super tetrahedron

    Journal of Alloys and Compounds · 2019-05-11

    Yongyu Pang, Anyi Zhou, Chensheng Lin, Wendan Cheng, Guoliang Chai

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  6. Ba2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains

    Journal of the American Chemical Society · 2019-07-05

    Justin Mark, Jian Wang, Kui Wu, Jeane Gladys Lo, Shannon Lee, Kirill A. Kovnir

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  7. Sn 2 Ga 2 S 5 : A Polar Semiconductor with Exceptional Infrared Nonlinear Optical Properties Originating from the Combined Effect of Mixed Asymmetric Building Motifs

    Chemistry of Materials · 2019-07-26

    Mengyue Li, Bingxuan Li, Hua Lin, Zuju Ma, Li‐Ming Wu, Xin‐Tao Wu, Qi‐Long Zhu

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  8. Rational design of infrared nonlinear optical chalcogenides by chemical substitution

    Coordination Chemistry Reviews · 2019-12-21

    Hua Lin, Wenbo Wei, Hong Chen, Xintao Wu, Qi‐Long Zhu

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  9. Mixed-metal thiophosphate CuCd 3 PS 6 : an infrared nonlinear optical material activated by its three-in-one tetrahedra-stacking architecture

    Journal of Materials Chemistry C · 2020-01-01

    Zhuang Li, Shengzi Zhang, Wenhao Xing, Yangwu Guo, Chunxiao Li, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  10. One-Dimensional Double Chains in Sodium-Based Quaternary Chalcogenides Displaying Intriguing Red Emission and Large Optical Anisotropy

    Inorganic Chemistry · 2020-01-30

    Ya Feng Yang, Kui Wu, Bingbing Zhang, Xiaowen Wu, Ming‐Hsien Lee

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  11. An assessment of the structural, electronic, optical and thermoelectric properties of the BaAg2GeS4 compound

    Journal of Solid State Chemistry · 2020-02-14

    Mosayeb Naseri, D.M. Hoat, Rodrigo Ponce-Pérez, Juan Francisco Rivas-Silva, Gregorio H. Cocoletzi

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  12. Cd4SiQ6 (Q = S, Se): Ternary Infrared Nonlinear Optical Materials with Mixed Functional Building Motifs

    Crystal Growth & Design · 2020-03-11

    Jindong Chen, Chensheng Lin, Shunda Yang, Xiaotian Jiang, Shuangshuang Shi, Yingshuang Sun, Bingxuan Li, Shenghao Fang, Ning Ye

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  13. Controlled nano‐crystallization of IR frequency‐doubling Cd 4 GeS 6 crystal in chalcogenide glass

    Journal of the American Ceramic Society · 2020-03-16

    Qilin Ye, Kaibo Weng, Dan Chen, Changgui Lin

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  14. HgCuPS4: An Exceptional Infrared Nonlinear Optical Material with Defect Diamond-like Structure

    Chemistry of Materials · 2020-04-24

    Mengyue Li, Zuju Ma, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  15. Functional Chalcogenide Na2HgSn2Se6 and K2MnGe2Se6 Exhibiting Flexible Chain Structure and Intriguing Birefringence Tunability

    Inorganic Chemistry · 2020-05-15

    Zhuang Li, Youquan Liu, Shengzi Zhang, Wenhao Xing, Wenlong Yin, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  16. Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2020-06-29

    Weikang Wang, Dajiang Mei, Fei Liang, Jun Zhao, Yuandong Wu, Zheshuai Lin

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  17. A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks

    Inorganic Chemistry Frontiers · 2021-01-01

    Yu Xiao, Man-Man Chen, Yaying Shen, Pengfei Liu, Hua Lin, Yi Liu

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  18. Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials

    Journal of Materials Chemistry C · 2021-01-01

    Chang Liu, Shenghua Zhou, Yu Xiao, Chao Zhang, Hua Lin, Yi Liu

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  19. Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks

    Unknown journal · 2021-04-19

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  20. α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band Gaps

    Inorganic Chemistry · 2021-05-03

    Yingshuang Sun, Chensheng Lin, Jindong Chen, Feng Xu, Shunda Yang, Bingxuan Li, Guangsai Yang, Min Luo, Ning Ye

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  21. Rb2CuSb7S12: Quaternary Antimony-Rich Semiconductor Featuring a Three-Dimensional Open Framework and Exhibiting an Intriguing Photocurrent Response

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    Yu Xiao, Shenghua Zhou, Rui Yu, Yaying Shen, Zuju Ma, Hua Lin, Yi Liu

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  22. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

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  23. Rb2MGe3S8 (M=Zn, Cd): Non-Centrosymmetry Transformation Led by Structure Change of [MGe3S8]2- Unit※

    化学学报 · 2022-01-01

    Xiandan Chai, Wen‐Fa Chen, Qiu-Nan Yan, Binwen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  24. Optimization on preparation conditions to improve the nonlinear optical response of ZnO/TiO2/ZrO2 ternary nanocomposites under continuous-wave laser irradiation

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  25. Li2Mg2Si2S6 and Li2Mg2Ge2S6: Two nonlinear optical sulfides featuring a unique, polar trigonal structure incorporating ethane‐like anions

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  26. A novel bifunctional thioarsenate based on unprecedented molecular [Cd 4 As 8 Se 16 (Se 2 ) 2 ] 8− cluster anions

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  27. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

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  28. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

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  29. Regulating the key performance parameters for Hg-based IR NLO chalcogenides via bandgap engineering strategy

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  30. Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response

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  31. Structural, electronic and optical properties of CdTiX2 (X = N and P): A first principles density functional theory investigation

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  34. Synergistic Enhancement of Band Gap and Optical Anisotropy via Functional-Site Cosubstitution in Antiperovskite-Type Chalcohalides [Ba2K][X][MS4] (M = Ge, Si; X = Cl, Br)

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  35. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

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  36. Vacancy-driven tetrahedral distortion leading to exceptional second harmonic generation

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  37. A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation

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  39. From Centrosymmetric Mg 2 GeS 4 to Noncentrosymmetric CdMg 3 Ge 2 S 8 : Cation-Mixing-Driven Symmetry Reduction

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