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RESEARCH PAPER · Inorganic Chemistry · 2009

Second-Order Nonlinear Optical Properties of Polyoxometalate Salts of a Chiral Stilbazolium Derivative

Jean‐Daniel Compain, Pierre Mialane, Anne Dolbecq, Jérôme Marrot, Anna Proust, Keitaro Nakatani, Pei Yu, F. Sécheresse

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Second-Order Nonlinear Optical Properties of Polyoxometalate Salts of a Chiral Stilbazolium DerivativeOriginalOrgano-Ruthenium Supported Heteropolytungstates: Synthesis, Structure, Electrochemistry, and Oxidation Catalysis72Synthesis, structure and characterization of three highly-connected 3D inorganic compounds based on paradodecatungstate-B16A new IR non-linear optical material with 2D 3-fold interpenetrated topology21Dual Photochromic/Electrochromic Compounds Based On Cationic Spiropyrans and Polyoxometalates72Synthesis and Optical Properties of a Rod−Coil Diblock Copolymer with Polyoxometalate Clusters Covalently Attached to the Coil Block69Hybrid Organic−Inorganic Polyoxometalate Compounds: From Structural Diversity to Applications1755Quadratic and Cubic Nonlinear Optical Properties of Salts of Diquat-Based Chromophores with Diphenylamino Substituents41Syntheses and Properties of Two-Dimensional, Dicationic Nonlinear Optical Chromophores Based on Pyrazinyl Cores36N-Aryl stilbazolium dyes as sensitizers for solar cells18DFT studies on the electronic properties of organometallic-polyoxomolybdate anions [ Cp n ∗ Mo6O19−](2−)− (n= 1 or 2): Revealing bonding features of Cp∗–Mo3The structure–property relationship of chiral 1,1′-binaphthyl-based polyoxometalates: TDDFT studies on the static first hyperpolarizabilities and the ECD spectra16Charge-transfer salts based on Lindqvist and Keggin polyoxoanion acceptors and ferrocenyl cationic donors9Chiroptical, linear, and second-order nonlinear optical properties of binaphthol derivatives32Functionalization and post-functionalization: a step towards polyoxometalate-based materials891Inorganic–organic hybrid compounds based on octamolybdates and multidentate N-donor ligand: syntheses, structures, photoluminescence and photocatalysis42TDDFT studies on chiral organophosphonate substituted divacant Keggin-type polyoxotungstate: diplex multistep-redox-triggered chiroptical and NLO switch13Tuning the Photochromic Properties of Molybdenum Bisphosphonate Polyoxometalates67TDDFT studies on the structures and ECD spectra of chiral bisarylimidos bearing different lengths of o-alkoxy chain-substituted polyoxomolybdates12Computational study of chiral molecules with high intrinsic hyperpolarizabilities6Fabrication and optical nonlinearities of ultrathin composite films incorporating a Keplerate type polyoxometalate22Luminescence Responsive Charge Transfer Intercluster Crystals37Ruthenium(II) dichloro or dithiocyanato complexes with 4,4′:2′,2″:4″,4‴-quaterpyridinium ligands: Towards photosensitisers with enhanced low-energy absorption properties0Chiral polyoxometalate-based materials: From design syntheses to functional applications235Cs 4 Mo 5 P 2 O 22 : a first Strandberg-type POM with 1D straight chains of polymerized [Mo 5 P 2 O 23 ] 6− units and moderate second harmonic generation response83Theoretical study on the photophysical properties of chiral mononuclear and dinuclear zinc complexes10Chiroptical, linear, and second-order nonlinear optical properties of tetrathiafulvalenylallene: a multifunctional molecular material24Photophysical properties of azaboradibenzo[6]helicene derivatives30Synthesis, Characterizations, and Morphological Studies of Polyoxometalate‐Containing Rod–Coil Diblock Copolymers19Notable third-order optical nonlinearities of a Keplerate-type polyoxometalate in solution and in thin films of PMMA17Spectroscopic readout of polyoxometalates' molecular information via self-assembly8New photoresponsive charge-transfer spiropyran/polyoxometalate assemblies with highly tunable optical properties58Synthesis, growth, crystal structure, spectral, thermal, mechanical and optical studies of stilbazolium derivative single crystal: 2-[2-(4-Diethylamino-phenyl)-vinyl]-1-methyl-pyridinium naphthalene-2-sulfonate (DESNS)15Nonplanar Donor–Acceptor Chiral Molecules with Large Second-Order Optical Nonlinearities: 1,1,4,4-Tetracyanobuta-1,3-diene Derivatives22Solution Properties and Effect of Anions on Third-Order Optical Nonlinearity of Porphyrin–Heteropolyoxometalate Hybrid System41Enantiomerically Pure Lanthanide–Organic Polytungstates Exhibiting Two-Photon Absorption Properties49Symmetry Breaking of α-[H2W12O40]6– Depends on the Transformation of Isopolyoxotungstates19Third-order optical nonlinearities of a series of compounds derived from a Keplerate type molybdenum-oxide-based polyoxometalate2Base promoted successive dealkylation steps of molybdenum alkoxides leading to a row of novel 1D and 2D polymeric frameworks of potassium–molybdenum oxomethoxides2Temperature-induced racemic compounds and chiral conglomerates based on polyoxometalates and lanthanides: syntheses, structures and catalytic properties30Functional helquats: helical cationic dyes with marked, switchable chiroptical properties in the visible region50Influence of electronic vs. steric factors on the solid-state photochromic performances of new polyoxometalate/spirooxazine and spiropyran hybrid materials16Synthesis and structural characterization of BINOL-modified chiral polyoxometalates17Luminescent Polythiophene‐Based Main‐Chain Polyoxometalate‐Containing Conjugated Polymers with Improved Solar‐Cell Performance17Iodonium‐polyoxometalate and thianthrenium‐polyoxometalate as new one‐component UV photoinitiators for radical and cationic polymerization40Encapsulation of polyoxometalates into supramolecular cages based on flexible ligands: Synthesis, structure and properties10Dawson-type polyoxometalate-based oligomeric Hg(II)-acetylide hybrid: Synthesis, characterization and materials properties5Spontaneous Resolution of Evans–Showell-Type Polyoxometalates in Constructing Chiral Inorganic–Organic Hybrid Architectures33A series of Anderson-type polyoxometalate-based metal–organic complexes: their pH-dependent electrochemical behaviour, and as electrocatalysts and photocatalysts62Chiral polyoxomolybdate-based hybrid compounds obtained by spontaneous resolution: syntheses, structures and non-linear optical properties10Controlled chiral electrochromism of polyoxometalates incorporated in supramolecular complexes20Donor–acceptor organo-imido polyoxometalates: high transparency, high activity redox-active NLO chromophores44Spontaneous chiral resolution and hierarchical directing effects of two-winged propeller-like SDAs on the construction of noncentrosymmetric iodoargentates/iodocuprates15Optical Properties of Hybrid Organic‐Inorganic Materials and their Applications345“Closer is Better and Two is Superior to One”: Third-Order Optical Nonlinearities of a Family of Porphyrin–Anderson Type Polyoxometalate Hybrid Compounds40Ligand-controlled formation of covalently modified antimoniomolybdates and their photochromic properties20Optical Properties of Hybrid Organic–inorganic Materials and their Applications – Part II : Nonlinear Optics and Plasmonics2Photophysical properties of chiral covalent organic cages3Induced chirality and reversal of phosphomolybdate cluster via modulating its interaction with cyclodextrins44Theoretical studies on the chiral polyoxoanions [P 2 Mo 18 O 62 ] 6− and [PMo 9 O 31 (OH 2 ) 3 ] 3− with histidine: chiral inversion and chiral induction0Anderson-Type Polyoxometalates Functionalized by Tetrathiafulvalene Groups: Synthesis, Electrochemical Studies, and NLO Properties51Optically Active Polyoxometalate‐Based Silica Nanohelices: Induced Chirality from Inorganic Nanohelices to Achiral POM Clusters26Combination of N-Arylstilbazolium Organic Nonlinear Optical Chromophores with Iodoargentates: Structural Diversities and Optical Properties19Synthèse de polyoxométallates hybrides et étude de leurs propriétés en biologie et en optique0Theoretical Assessment of the Second-Order Nonlinear Optical Responses of Lindqvist-Type Organoimido Polyoxometalates49Application of temperature-controlled chiral hybrid structures constructed from copper( ii )-monosubstituted Keggin polyoxoanions and copper( ii )-organoamine complexes in enantioselective sensing of tartaric acid8Organic–Inorganic Hybrids Composed of Keggin-Type [PMo10V2O40]5– Anions and Porphyrins: The Synthesis, Characterization, and Influence of Porphyrin Substituents on Optical Nonlinearities24Crystalline Porous Materials for Nonlinear Optics91

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  2. Synthesis, structure and characterization of three highly-connected 3D inorganic compounds based on paradodecatungstate-B

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  3. A new IR non-linear optical material with 2D 3-fold interpenetrated topology

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  4. Dual Photochromic/Electrochromic Compounds Based On Cationic Spiropyrans and Polyoxometalates

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  5. Synthesis and Optical Properties of a Rod−Coil Diblock Copolymer with Polyoxometalate Clusters Covalently Attached to the Coil Block

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  6. Hybrid Organic−Inorganic Polyoxometalate Compounds: From Structural Diversity to Applications

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  7. Quadratic and Cubic Nonlinear Optical Properties of Salts of Diquat-Based Chromophores with Diphenylamino Substituents

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  8. Syntheses and Properties of Two-Dimensional, Dicationic Nonlinear Optical Chromophores Based on Pyrazinyl Cores

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  9. N-Aryl stilbazolium dyes as sensitizers for solar cells

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  10. DFT studies on the electronic properties of organometallic-polyoxomolybdate anions [ Cp n ∗ Mo6O19−](2−)− (n= 1 or 2): Revealing bonding features of Cp∗–Mo

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  11. The structure–property relationship of chiral 1,1′-binaphthyl-based polyoxometalates: TDDFT studies on the static first hyperpolarizabilities and the ECD spectra

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  12. Charge-transfer salts based on Lindqvist and Keggin polyoxoanion acceptors and ferrocenyl cationic donors

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  14. Functionalization and post-functionalization: a step towards polyoxometalate-based materials

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  15. Inorganic–organic hybrid compounds based on octamolybdates and multidentate N-donor ligand: syntheses, structures, photoluminescence and photocatalysis

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  16. TDDFT studies on chiral organophosphonate substituted divacant Keggin-type polyoxotungstate: diplex multistep-redox-triggered chiroptical and NLO switch

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  17. Tuning the Photochromic Properties of Molybdenum Bisphosphonate Polyoxometalates

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  18. TDDFT studies on the structures and ECD spectra of chiral bisarylimidos bearing different lengths of o-alkoxy chain-substituted polyoxomolybdates

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  19. Computational study of chiral molecules with high intrinsic hyperpolarizabilities

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  20. Fabrication and optical nonlinearities of ultrathin composite films incorporating a Keplerate type polyoxometalate

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  21. Luminescence Responsive Charge Transfer Intercluster Crystals

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  22. Ruthenium(II) dichloro or dithiocyanato complexes with 4,4′:2′,2″:4″,4‴-quaterpyridinium ligands: Towards photosensitisers with enhanced low-energy absorption properties

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  27. Photophysical properties of azaboradibenzo[6]helicene derivatives

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  32. Synthesis, growth, crystal structure, spectral, thermal, mechanical and optical studies of stilbazolium derivative single crystal: 2-[2-(4-Diethylamino-phenyl)-vinyl]-1-methyl-pyridinium naphthalene-2-sulfonate (DESNS)

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  33. Nonplanar Donor–Acceptor Chiral Molecules with Large Second-Order Optical Nonlinearities: 1,1,4,4-Tetracyanobuta-1,3-diene Derivatives

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  34. Solution Properties and Effect of Anions on Third-Order Optical Nonlinearity of Porphyrin–Heteropolyoxometalate Hybrid System

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  35. Enantiomerically Pure Lanthanide–Organic Polytungstates Exhibiting Two-Photon Absorption Properties

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  36. Symmetry Breaking of α-[H2W12O40]6– Depends on the Transformation of Isopolyoxotungstates

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  37. Third-order optical nonlinearities of a series of compounds derived from a Keplerate type molybdenum-oxide-based polyoxometalate

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  39. Temperature-induced racemic compounds and chiral conglomerates based on polyoxometalates and lanthanides: syntheses, structures and catalytic properties

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  45. Encapsulation of polyoxometalates into supramolecular cages based on flexible ligands: Synthesis, structure and properties

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  48. A series of Anderson-type polyoxometalate-based metal–organic complexes: their pH-dependent electrochemical behaviour, and as electrocatalysts and photocatalysts

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