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RESEARCH PAPER · Chemical Reviews · 2010

Hybrid Organic−Inorganic Polyoxometalate Compounds: From Structural Diversity to Applications

Anne Dolbecq, Eddy Dumas, Cédric R. Mayer, Pierre Mialane

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Hybrid Organic−Inorganic Polyoxometalate Compounds: From Structural Diversity to ApplicationsOriginalHeterometallic 3d–4f polyoxometalates: still an incipient field97Discrete Covalent Organic–Inorganic Hybrids: Terpyridine Functionalized Polyoxometalates Obtained by a Modular Strategy and Their Metal Complexation93From Platonic Templates to Archimedean Solids: Successive Construction of Nanoscopic {V16As8}, {V16As10}, {V20As8}, and {V24As8} Polyoxovanadate Cages105Elaboration of Covalently Linked Polyoxometalates with Ruthenium and Pyrene Chromophores and Characteriation of Their Photophysical Properties89Polyoxometalate-Based Metal Organic Frameworks (POMOFs): Structural Trends, Energetics, and High Electrocatalytic Efficiency for Hydrogen Evolution Reaction545Inorganic–Organic Hybrid Vesicles with Counterion- and pH-Controlled Fluorescent Properties194First Three-Dimensional Inorganic–Organic Hybrid Material Constructed From an “Inverted Keggin” Polyoxometalate and a Copper(I)-Organic Complex160A polyoxometalate-based single-molecule magnet with an S = 21/2 ground state90A Multifunctional Organic–Inorganic Hybrid Structure Based on MnIII–Porphyrin and Polyoxometalate as a Highly Effective Dye Scavenger and Heterogenous Catalyst420Sensitization of Lanthanoid Luminescence by Organic and Inorganic Ligands in Lanthanoid-Organic-Polyoxometalates132A building block strategy to access sulfur-functionalized polyoxometalate based systems using {Mo2S2O2} and {Mo3S4} as constitutional units, linkers or templates117Assembly of a luminescent core–shell nanocluster featuring a Ag34S26 shell and a W6O216− polyoxoanion core95Diversity in structures and properties of 3d-incorporating polyoxotungstates332Engineering polyoxometalates with emergent properties969Functionalization and post-functionalization: a step towards polyoxometalate-based materials891Functionalized polyoxometalates with covalently linked bisphosphonate, N-donor or carboxylate ligands: from electrocatalytic to optical properties126Ionic liquids as crystallisation media for inorganic materials114One-dimensional growth of MoOx-based organic–inorganic hybrid nanowires with tunable photochromic properties110Polyoxometalate water oxidation catalysts and the production of green fuel775Polyoxometalate-decorated nanoparticles254Recent advances in paramagnetic-TM-substituted polyoxometalates (TM = Mn, Fe, Co, Ni, Cu)614Recent advances on polyoxometalate-based molecular and composite materials909Solution behaviors and self-assembly of polyoxometalates as models of macroions and amphiphilic polyoxometalate–organic hybrids as novel surfactants369Highly dispersed platinum in metal organic framework NH2-MIL-101(Al) containing phosphotungstic acid – Characterization and catalytic performance159Hybrid Assemblies of Eu‐Containing Polyoxometalates and Hydrophilic Block Copolymers with Enhanced Emission in Aqueous Solution105Polyoxometalate–Organic Hybrid Molecules as Amphiphilic Emulsion Catalysts for Deep Desulfurization106An Ionothermal Synthetic Approach to Porous Polyoxometalate‐Based Metal–Organic Frameworks179High‐Nuclearity Silver Ethynide Clusters Assembled with Phosphonate and Metavanadate Precursors114Polyoxometalate-based molecular/nano composites: Advances in environmental remediation by photocatalysis and biomimetic approaches to solar energy conversion154Chiral polyoxometalate-based materials: From design syntheses to functional applications235Series of Inorganic–Organic Hybrid Materials Constructed From Octamolybdates and Metal–Organic Frameworks: Syntheses, Structures, and Physical Properties101Synthesis, electrochemical and photophysical properties of covalently linked porphyrin–polyoxometalates96Polyoxometalates as Versatile Enzyme Inhibitors138Four New Three-Dimensional Polyoxometalate-Based Metal–Organic Frameworks Constructed From [Mo6O18(O3AsPh)2]4– Polyoxoanions and Copper(I)-Organic Fragments: Syntheses, Structures, Electrochemistry, and Photocatalysis Properties128Phosphonate coupling molecules for the control of surface/interface properties and the synthesis of nanomaterials243Polyoxometalate–biomolecule conjugates: A new approach to create hybrid drugs for cancer therapeutics95Three New Imidazole‐Functionalized Hexanuclear Oxidovanadium Clusters with Exceptional Catalytic Oxidation Properties for Alcohols88Engineering Chiral Polyoxometalate Hybrid Metal–Organic Frameworks for Asymmetric Dihydroxylation of Olefins380Covalently Tethered Polyoxometalate–Pyrene Hybrids for Noncovalent Sidewall Functionalization of Single‐Walled Carbon Nanotubes as High‐Performance Anode Material142Hybrid Surfactant Systems with Inorganic Constituents95Tunable, luminescent, and self-healing hybrid hydrogels of polyoxometalates and triblock copolymers based on electrostatic assembly101Polyoxometallates trapped in a zeolitic imidazolate framework leading to high uptake and selectivity of bioactive molecules121Inorganic–organic hybrid polymer with multiple redox for high-density data storage183Polyoxometalate based open-frameworks (POM-OFs)442Polyoxoniobate-based 3D framework materials with photocatalytic hydrogen evolution activity126Recent advances in porous polyoxometalate-based metal–organic framework materials969The organic ligands with mixed N-/O-donors used in construction of functional metal–organic frameworks134Molecular Nanoparticles Are Unique Elements for Macromolecular Science: From “Nanoatoms” to Giant Molecules354Porous Metal–Organic Frameworks for Heterogeneous Biomimetic Catalysis722Solar-induced direct biomass-to-electricity hybrid fuel cell using polyoxometalates as photocatalyst and charge carrier181Polyoxometalate Clusters Integrated into Peptide Chains and as Inorganic Amino Acids: Solution‐ and Solid‐Phase Approaches118Metal–organic framework composites2286Incorporating Polyoxometalates into a Porous MOF Greatly Improves Its Selective Adsorption of Cationic Dyes271Recent developments in the crystal engineering of diverse coordination modes (0–12) for Keggin-type polyoxometalates in hybrid inorganic–organic architectures190Ionic liquids for energy, materials, and medicine509Hybrid Materials Based on the Embedding of Organically Modified Transition Metal Oxoclusters or Polyoxometalates into Polymers for Functional Applications: A Review113Electrostatic Assembly of Peptide Nanofiber–Biomimetic Silver Nanowires onto Graphene for Electrochemical Sensors122Unprecedented Application of Flexible Bis(pyridyl-tetrazole) Ligands To Construct Helix/Loop Subunits To Modify Polyoxometalate Anions126Two-Dimensional Nanocrystals of Molecular Janus Particles125Layer‐by‐Layer Assembly of Light‐Responsive Polymeric Multilayer Systems130Discrete metal-carboxylate self-assembled cages: Design, synthesis and applications176Time‐Resolved Assembly of Cluster‐in‐Cluster {Ag12}‐in‐{W76} Polyoxometalates under Supramolecular Control90Recent advances in polyoxometalate-based heterogeneous catalytic materials for liquid-phase organic transformations225Review: Lanthanide coordination chemistry: from old concepts to coordination polymers306Controlling the Ring Curvature, Solution Assembly, and Reactivity of Gigantic Molybdenum Blue Wheels91Covalent multi-component systems of polyoxometalates and metal complexes: Toward multi-functional organic–inorganic hybrids in molecular and material sciences173Recent progress on supported polyoxometalates for biodiesel synthesis via esterification and transesterification142Visible light sensitive photoinitiating systems: Recent progress in cationic and radical photopolymerization reactions under soft conditions582Green and facile synthesis of an Au nanoparticles@polyoxometalate/ordered mesoporous carbon tri-component nanocomposite and its electrochemical applications88Polyoxometalate-based phase transfer catalysis for liquid–solid organic reactions: a review102Polyoxometalate-functionalized nanocarbon materials for energy conversion, energy storage and sensor systems602Polyoxometalates-based heterometallic organic–inorganic hybrid materials for rapid adsorption and selective separation of methylene blue from aqueous solutions176Photosensitizing Metal–Organic Framework Enabling Visible-Light-Driven Proton Reduction by a Wells–Dawson-Type Polyoxometalate436Polyoxometalate‐Based Organic–Inorganic Hybrids as Antitumor Drugs116Complexation of Polyoxometalates with Cyclodextrins203Heterogeneous Catalysis of Polyoxometalate Based Organic–Inorganic Hybrids108Multifunctional Radical-Doped Polyoxometalate-Based Host–Guest Material: Photochromism and Photocatalytic Activity145Selective assemblies of giant tetrahedra via precisely controlled positional interactions392Enhanced Visible Photovoltaic Response of TiO 2 Thin Film with an All-Inorganic Donor–Acceptor Type Polyoxometalate91The Anderson–Evans polyoxometalate: From inorganic building blocks via hybrid organic–inorganic structures to tomorrows “Bio-POM”320Systematic Investigation of High‐Sensitivity Luminescent Sensing for Polyoxometalates and Iron(III) by MOFs Assembled with a New Resorcin[4]arene‐Functionalized Tetracarboxylate102Polyoxometalate-based metal–organic framework-derived hybrid electrocatalysts for highly efficient hydrogen evolution reaction190Cation-mediated optical resolution and anticancer activity of chiral polyoxometalates built from entirely achiral building blocks107Heterogenization of heteropoly compounds: a review of their structure and synthesis105Immobilization of polyoxometalates in crystalline solids for highly efficient heterogeneous catalysis106Magnetic double-tartaric bridging mono-lanthanide substituted phosphotungstates with photochromic and switchable luminescence properties103Self-assembly of polyoxometalates, Pt nanoparticles and metal–organic frameworks into a hybrid material for synergistic hydrogen evolution101Polyoxometalate-assisted synthesis of transition-metal cubane clusters as artificial mimics of the oxygen-evolving center of photosystem II138Flexible single-layer ionic organic–inorganic frameworks towards precise nano-size separation131Chemistry of Mesoporous Organosilica in Nanotechnology: Molecularly Organic–Inorganic Hybridization into Frameworks356Target Delivery of a Novel Antitumor Organoplatinum(IV)‐Substituted Polyoxometalate Complex for Safer and More Effective Colorectal Cancer Therapy In Vivo94Keggin-type lacunary and transition metal substituted polyoxometalates as heterogeneous catalysts: A recent progress134Ni-Decorated Molybdenum Carbide Hollow Structure Derived from Carbon-Coated Metal–Organic Framework for Electrocatalytic Hydrogen Evolution Reaction237Highly Dispersed Polyoxometalate‐Doped Porous Co3O4 Water Oxidation Photocatalysts Derived from POM@MOF Crystalline Materials101Giant Hollow Heterometallic Polyoxoniobates with Sodalite‐Type Lanthanide–Tungsten–Oxide Cages: Discrete Nanoclusters and Extended Frameworks104High-nuclearity silver(I) chalcogenide clusters: A novel class of supramolecular assembly157Nonlinear Optical Materials for the Smart Filtering of Optical Radiation941Ag/Ag x H 3– x PMo 12 O 40 Nanowires with Enhanced Visible-Light-Driven Photocatalytic Performance92A survey of the different roles of polyoxometalates in their interaction with amino acids, peptides and proteins135Four‐Shell Polyoxometalates Featuring High‐Nuclearity Ln 26 Clusters: Structural Transformations of Nanoclusters into Frameworks Triggered by Transition‐Metal Ions172MoP/Mo 2 C@C: A New Combination of Electrocatalysts for Highly Efficient Hydrogen Evolution over the Entire pH Range214Anion-Dependent Assembly of Heterometallic 3d–4f Clusters Based on a Lacunary Polyoxometalate92Polyoxometalate, Cationic Cluster, and γ-Cyclodextrin: From Primary Interactions to Supramolecular Hybrid Materials188Design and synthesis of polyoxometalate-framework materials from cluster precursors270Rare Earth Polyoxometalates205Polyoxometalate/TiO2/Ag composite nanofibers with enhanced photocatalytic performance under visible light177A Polyoxovanadate–Resorcin[4]arene-Based Porous Metal–Organic Framework as an Efficient Multifunctional Catalyst for the Cycloaddition of CO2 with Epoxides and the Selective Oxidation of Sulfides108Nonconventional Three-Component Hierarchical Host–Guest Assembly Based on Mo-Blue Ring-Shaped Giant Anion, γ-Cyclodextrin, and Dawson-type Polyoxometalate116Evolutionary Metal Oxide Clusters for Novel Applications: Toward High‐Density Data Storage in Nonvolatile Memories137Record High‐Nuclearity Polyoxoniobates: Discrete Nanoclusters {Nb114}, {Nb81}, and {Nb52}, and Extended Frameworks Based on {Cu3Nb78} and {Cu4Nb78}117Recent advances in alkoxylation chemistry of polyoxometalates: From synthetic strategies, structural overviews to functional applications324Photochromism into nanosystems: towards lighting up the future nanoworld766Polyoxovanadate-alkoxide clusters as multi-electron charge carriers for symmetric non-aqueous redox flow batteries158A Co2P/WC Nano‐Heterojunction Covered with N‐Doped Carbon as Highly Efficient Electrocatalyst for Hydrogen Evolution Reaction94Highly Efficient Catalysts Based on Divanadium-Substituted Polyoxometalate and N-Doped Carbon Nanotubes for Selective Oxidation of Alkylphenols90Highly Efficient, Near-Infrared and Visible Light Modulated Electrochromic Devices Based on Polyoxometalates and W 18 O 49 Nanowires227Copper Iodide Based Hybrid Phosphors for Energy‐Efficient General Lighting Technologies306Designed fabrication of biomimetic metal–organic frameworks for catalytic applications172Carboxylate covalently modified polyoxometalates: From synthesis, structural diversity to applications291Polyoxometalate-Based Metal–Organic Frameworks for Selective Oxidation of Aryl Alkenes to Aldehydes91Water-Soluble Redox-Active Cage Hosting Polyoxometalates for Selective Desulfurization Catalysis314Trapping an octahedral Ag6 kernel in a seven-fold symmetric Ag56 nanowheel152Polyoxometalate-based materials for advanced electrochemical energy conversion and storage131Metal–Organic Framework Based Microcapsules104Electrochromic Sensors Based on Conducting Polymers, Metal Oxides, and Coordination Complexes102Polyoxometalate Photocatalysis for Liquid-Phase Selective Organic Functional Group Transformations281Aerobic oxidative desulfurization coupling of Co polyanion catalysts and p -TsOH-based deep eutectic solvents through a biomimetic approach118Chirality-Selected Chemical Modulation of Amyloid Aggregation124Self-Assembly of Anionic Polyoxometalate–Organic Architectures Based on Lacunary Phosphomolybdates and Pyridyl Ligands134Recent advances in transition-metal-containing Keggin-type polyoxometalate-based coordination polymers219Polyoxometalate-based materials for sustainable and clean energy conversion and storage302Hybrid polyoxometalates as post-functionalization platforms: from fundamentals to emerging applications444Anderson polyoxometalate built-in covalent organic frameworks for enhancing catalytic performances101Electron transfer in the confined environments of metal–organic coordination supramolecular systems147Heterometallic 3d-4f polyoxometalates: An emerging field with structural diversity to multiple applications112Polyoxometalate functionalized architectures332Polyoxometalate Clusters: Sub-nanometer Building Blocks for Construction of Advanced Materials182Self‐Assembly of Photoresponsive Molecular Amphiphiles in Aqueous Media177The rise of metal–organic polyhedra271A polyoxometalate@covalent triazine framework as a robust electrocatalyst for selective benzyl alcohol oxidation coupled with hydrogen production96Heterogenisation of polyoxometalates and other metal-based complexes in metal–organic frameworks: from synthesis to characterisation and applications in catalysis262The roles of polyoxometalates in photocatalytic reduction of carbon dioxide89Supramolecular assemblies of organo-functionalised hybrid polyoxometalates: from functional building blocks to hierarchical nanomaterials260Plasmonic Ag Modified Ag3vo4/Agpmo S-Scheme Heterojunction Photocatalyst for Boosted Cr(Vi) Reduction Under Visible Light: Performance and Mechanism128Catalytic application of polyoxovanadates in the selective oxidation of organic molecules110State-of-the-art advances in the syntheses, structures, and applications of polyoxometalate-based metal–organic frameworks123Platonic and Archimedean solids in discrete metal-containing clusters138Recent progress in polyoxometalate–viologen photochromic hybrids: structural design, photochromic mechanism, and applications96Hierarchically stabilized Pt single-atom catalysts induced by an atomic substitution strategy for an efficient hydrogen evolution reaction121S-scheme towards interfacial charge transfer between POMs and MOFs for efficient visible-light photocatalytic Cr (VI) reduction96

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  46. From Platonic Templates to Archimedean Solids: Successive Construction of Nanoscopic {V16As8}, {V16As10}, {V20As8}, and {V24As8} Polyoxovanadate Cages

    Journal of the American Chemical Society · 2011-06-18

    Lei Zhang, Wolfgang Schmitt

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  47. Polyoxométallates et chimie verte : molécules et matériaux nanostructurés pour la conversion de l’énergie et l’environnement

    Unknown journal · 2011-06-27

    Rosa Ngo Biboum

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  48. Route for the Elaboration of Functionalized Hybrid 3d-Substituted Trivacant Keggin Anions

    Inorganic Chemistry · 2011-07-13

    Guillaume Rousseau, Olivier Oms, Anne Dolbecq, Jérôme Marrot, Pierre Mialane

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  49. Predicting the UV spectrum of polyoxometalates by TD‐DFT

    Journal of Computational Chemistry · 2011-07-18

    Davide Ravelli, Daniele Dondi, Maurizio Fagnoni, Angelo Albini, Alessandro Bagno

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  50. Elaboration of Covalently Linked Polyoxometalates with Ruthenium and Pyrene Chromophores and Characteriation of Their Photophysical Properties

    Inorganic Chemistry · 2011-07-20

    Benjamin Matt, Christophe Coudret, Christine Viala, Damien Jouvenot, Frédérique Loiseau, Guillaume Izzet, Anna Proust

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