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RESEARCH PAPER · Coordination Chemistry Reviews · 2012

Chiral polyoxometalate-based materials: From design syntheses to functional applications

Dong‐Ying Du, Li‐Kai Yan, Zhong‐Min Su, Shun‐Li Li, Ya‐Qian Lan, Enbo Wang

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Chiral polyoxometalate-based materials: From design syntheses to functional applicationsOriginalA 3d–4f heterometallic 3D POMOF based on lacunary Dawson polyoxometalates36Assembly and spontaneous resolution of the chiral inorganic polyoxometalates-based frameworks via helical chains association22Metal–organic frameworks as platforms for clean energy970Monolacunary Keggin polyoxometalates connected to ten 4d or 4f metal atoms21Structure and bifunctional electrocatalytic activity of a novel 3D framework based on dimeric monocopper-substituted polyoxoanions as ten-connected linkages37Interdigitated architectures assembled from α-metatungstates and lanthanide–organic complexes11A New Organic-Paradodecatungstate Hybrid Compound: Synthesis, Characterization and Crystal Structure2A flexible chelate ligand in dodecatungstoborate-based supramolecular compounds1Recent advances on polyoxometalates intercalated layered double hydroxides: From synthetic approaches to functional material applications283An unprecedented (3,4,24)-connected heteropolyoxozincate organic framework as heterogeneous crystalline Lewis acid catalyst for biodiesel production47A 3D Polyoxometalate Network Based on the Tetra-CoII Sandwiched Phosphotungstate Units Linked by Cs+ Cations2Ethylenediammonium sodium tetrakis[bis(ethylenediamine-κ2N,N′)(oxalato-κ2O1,O2)cobalt(III)] [pentahydrogen di(phosphatooctadecatungstate)] tetradecahydrate0Rubidium pentaaqua( L -serine)cobalt(II) hexahydrogenhexamolybdocobaltate(III) L -serine monosolvate decahydrate2Disproportionation of Achiral Nickel(II) Centers into Two Kinds of Chiral Nickel(II) Centers Caused by an Achiral Diimine Ligand16Assembly of co-bimb-polyoxotungstate hybrids: from 1D chain to 3D framework influenced by the charge of Keggin anions25Synthesis, structure, and photocatalytic hydrogen of three environmentally friendly titanium oxo-clusters28Two Organic–Inorganic Hybrids Assembled by Carboxylate-Bridging Lanthanide-Substituted Polyoxometalate Dimers with Copper–ethylendiamine Cations5Hydrothermal Syntheses and Structural Characterization of Two 3-D Supramolecular Networks Constructed from Tetra-CoII Sandwiched Polyoxometalates2Tuning the dimension of POM-based inorganic–organic hybrids from 3D self-penetrating framework to 1D poly-pendant chain via changing POM clusters and introducing secondary spacers34Chirality meets visible-light photocatalysis in a molecular cerium vanadium oxide cluster59A new 3D framework based on reduced Wells-Dawson arsenotungstates as eight-connected linkages26Complexation of metal carbonyl units with [α-PW 11 O 39 ] 7− and [α 2 -P 2 W 17 O 61 ] 10− : insights into the chiral “twisted-sandwich” dimeric structures12Polyoxometalate complexes for oxidative kinetic resolution of secondary alcohols: unique effects of chiral environment, immobilization and aggregation27Recent advances in porous polyoxometalate-based metal–organic framework materials969Solvent-controlled 3D lanthanide–polyoxometalate frameworks: reduction and stabilization of Ag nanocomposites and catalytic properties11The coexistence of interconnected and interweaved double helices in an octamolybdate-based compound: synthesis, structure, and photocatalytic properties11Solvothermal Synthesis of Four Polyoxometalate-Based Coordination Polymers Including Diverse Ag(I)···π Interactions61Two Hexa-Ni-Substituted AsW9O34 Clusters Functionalized by Organic Ligands2Superhydrophobic Polyoxometalate/Calixarene Inorganic–Organic Hybrid Materials with Highly Efficient Desulfurization Ability20Novel One-Dimensional Organic–Inorganic Polyoxometalate Hybrids Constructed from Heteropolymolybdate Units and Copper–Aminoacid Complexes49Synthesis and electrochemical properties of an interdigitated architecture based on Keggin phosphotungstates7Anhydrous Lanthanide MOFs and Direct Photoluminescent Sensing for Polyoxometalates in Aqueous Solution75A Microporous Anionic Metal–Organic Framework for Sensing Luminescence of Lanthanide(III) Ions and Selective Absorption of Dyes by Ionic Exchange164Diamondoid Hydrazones and Hydrazides: Sterically Demanding Ligands for Sn/S Cluster Design31Entangled structures in polyoxometalate-based coordination polymers112Induced circular dichroism of polyoxometalates via electrostatic encapsulation with chiral organic cations14Symmetry Breaking of α-[H2W12O40]6– Depends on the Transformation of Isopolyoxotungstates19Stepwise synthesis of two inorganic–organic hybrids based on the manganese monosubstituted Keggin polyanion chains1A novel single-side azobenzene-grafted Anderson-type polyoxometalate for recognition-induced chiral migration70Assembly of Six Polyoxometalate-Based Hybrid Compounds from a Simple Supramolecule to a Complicated Pseudorotaxane Framework via Tuning the pH of the Reaction Systems72Structures and Properties of Coordination Polymers based on 5‐Nitroisophthalic Acid and N,N′‐bis(4‐pyridyl‐methyl) Piperazine5Modular Molecules: Site‐Selective Metal Substitution, Photoreduction, and Chirality in Polyoxometalate Hybrids32Spontaneous resolution of polyoxometalate-based inorganic–organic hybrids driven by solvent and common ion33Recent progress in metal-functionalized germanotungstates: from structures to properties15Applications of chiroptical spectroscopy to coordination compounds85Modulating the polyoxometalate-based inorganic–organic hybrids from simple chains to complicated frameworks via changing POM clusters9Preparation, characterization and catalytic activity studies of organoruthenium‐supported polyoxotungstates on SBA‐157Four polyoxometalate-based semiconductive coordination polymers: Syntheses, structures, photoluminescent and photocatalytic properties18Temperature-induced racemic compounds and chiral conglomerates based on polyoxometalates and lanthanides: syntheses, structures and catalytic properties30Kinetics and Mechanism of Oxidation of 2‐Mercaptoethanol by the Heteropolyoxovanadate [MnV13O38]7−8Two new members of the niobium-substituted polytungstophosphate family based on hexalacunary [H 2 P 2 W 12 O 48 ] 12− building blocks37A novel organic–inorganic hybrid polyoxometalate for the selective adsorption/isolation of β-lactoglobulin24Lanthanide-supported molybdenum–vanadium oxide clusters: syntheses, structures and catalytic properties19Moisture-responsive films consisting of luminescent polyoxometalates and agarose26POM-based inorganic–organic hybrid compounds: synthesis, structures, highly-connected topologies and photodegradation of organic dyes17Recent progress in polyoxoniobates decorated and stabilized via transition metal cations or clusters53Synthesis and structural characterization of BINOL-modified chiral polyoxometalates17Tuning the topology structures of polymolybdate-based hybrids from interpenetrated framework to interdigitated architecture via changing polymolybdate clusters14Novel organic–inorganic hybrid monomeric Keggin-type phosphotungstate containing heterometallic {Ni6WNi} clusters8Chiral separation by counter-current chromatography54Heterogeneous Catalysis of Polyoxometalate Based Organic–Inorganic Hybrids108Ultrastable Polymolybdate-Based Metal–Organic Frameworks as Highly Active Electrocatalysts for Hydrogen Generation from Water664A molecular crown analogue templated by Keggin polyanions: synthesis, structure, and electrochemical and luminescent properties3Hybrid polyoxometalate materials for photo(electro-) chemical applications384Supramolecular Chirality in Self-Assembled Systems2242Synthesis and properties of new materials with cobalt(II), iron(III) and manganese(III)-substituted Keggin polyoxotungstates and 1-alkyl-3-methylimidazolium cations13Preparation of green luminescence composite film and study of electrofluorochromic performance7Systematic Investigation of High‐Sensitivity Luminescent Sensing for Polyoxometalates and Iron(III) by MOFs Assembled with a New Resorcin[4]arene‐Functionalized Tetracarboxylate102Chiral Dawson‐Type Hybrid Polyoxometalate Catalyzes Enantioselective Diels–Alder Reactions22Polyoxometalate-Gold(I)/H+ Complexes: Air-Stable, Efficient, Polyvalent, and Bifunctional Catalysts17A {Nb6P2W12}‐Based Hexameric Manganese Cluster with Single‐Molecule Magnet Properties48TDDFT studies on the chiroptical properties of a chiral inorganic polythioanion Möbius strip2A Mn( iii ) polyoxotungstate in the oxidation of organosulfur compounds by H 2 O 2 at room temperature: an environmentally safe catalytic approach21Spontaneous Resolution of Evans–Showell-Type Polyoxometalates in Constructing Chiral Inorganic–Organic Hybrid Architectures33Tuning the microstructures of decavanadate-based supramolecular hybrids via regularly changing the spacers of bis(triazole) ligands9“Pinwheel” subunit-directed polyoxometalate-based hybrid compound [Cu(bimb) 2 ] 2 [β-Mo 8 O 26 ] with both helixes and chiral layers11A microporous anionic metal–organic framework for a highly selective and sensitive electrochemical sensor of Cu 2+ ions97An octamolybdate-metal organic framework hybrid for the efficient adsorption of histidine-rich proteins32Asymmetric catalytic sulfoxidation by a novel VIV8 cluster catalyst in the presence of serum albumin: a simple and green oxidation system17Cation-mediated optical resolution and anticancer activity of chiral polyoxometalates built from entirely achiral building blocks107Chiral polyoxomolybdate-based hybrid compounds obtained by spontaneous resolution: syntheses, structures and non-linear optical properties10Controlled chiral electrochromism of polyoxometalates incorporated in supramolecular complexes20Counterion-dominating chirality transfer between chiral and achiral polyoxometalates9Immobilization of polyoxometalates in crystalline solids for highly efficient heterogeneous catalysis106Insight into the reactivity of in situ formed {(NbO 2 ) 3 SiW 9 }: synthesis, structure, and solution properties of a trimeric polytungstosilicate trapping a {MnNb 9 } core16pH-Controlled assembly of two novel Dawson-sandwiched clusters involving the in situ reorganization of trivacant α-[P 2 W 15 O 56 ] 12− into divacant α-[P 2 W 16 O 57 ] 8−26Research progress on polyoxometalate-based transition-metal–rare-earth heterometallic derived materials: synthetic strategies, structural overview and functional applications284The first 3D host–guest structure based on a three-fold interpenetrated Ag-pz coordination polymer network and Keggin-type aluminum tungstates with photo/electro-catalytic properties17Polyoxometalate-assisted synthesis of transition-metal cubane clusters as artificial mimics of the oxygen-evolving center of photosystem II138Heteroanionic Materials Based on Copper Clusters, Bisphosphonates, and Polyoxometalates: Magnetic Properties and Comparative Electrocatalytic NOx Reduction Studies44Synthesis and characterization of a novel polyoxometalate–Cu(II) hybrid catalyst for efficient synthesis of triazols17Improvement of the polyoxometalate's performance in the asymmetric oxidation of styrene via combined with chiral ionic liquid6First Orange Fluorescence Composite Film Based on Sm-Substituted Tungstophosphate and Its Electrofluorochromic Performance29Difference in Chiral Recognition Behavior between AgI3MIII2and AuI3MIII2(M = Co, Rh) Anionic Complexes with l -Cysteinate10Hydrothermal synthesis and electrochemical properties of a coordination polymer based on dinuclear (Pyrazinyl tetrazolate) Copper(II) cations and β-Octamolybdate Anions9Studying mass spectrometric behaviors of {Au 6 Ag 2 (C)[PPh 2 (4‐CH 3 ‐Py)] 6 }(BF 4 ) 4 and {Au 8 [(PPh 3 ) 2 O] 3 (PPh 3 ) 2 }(NO 3 ) 2 by electrospray time‐of‐flight mass spectrometry and electrospray ion trap mass spectrometry0Immobilized polyoxometalate onto the modified magnetic nanoparticle as a photocatalyst for dye degradation34Effect of Directional Hydrogen Bonding on the Self‐Assembly of Anisotropically‐Shaped Macroions16Mixed-Metal Hybrid Polyoxometalates with Amino Acid Ligands: Electronic Versatility and Solution Properties21A wheel-shaped Dy( iii ) single-molecule magnet supported by polyoxotungstates28Chiral metallosupramolecular architectures531Electrochemical and diffuse reflectance study on tetrahedral ε-Keggin-based metal–organic frameworks12Self-assembly of polyoxometalate-based hybrid aggregates: from a monomer to dimers by changing the pH value of reaction systems7Self-organization towards complex multi-fold meso-helices in the structures of Wells–Dawson polyoxometalate-based hybrid materials for lithium-ion batteries71Synthesis, characterization and catalytic epoxidation properties of lanthanide-stabilized peroxoisopolytungstates11Bi-amino surface functionalized polyoxometalate nanocomposite as an environmentally friendly catalyst: synthesis and dye degradation5Introducing Chirality into Hybrid Clusters from an Achiral Ligand: Synthesis and Characterization of Polyoxomolybdates Containing a Benzylarsonate Group7Tetra-nickel substituted polyoxotungsate as an efficient sorbent for the isolation of His6-tagged proteins from cell lysate11Discovery of Heteropolytantalate: Synthesis and Structure of Two 6-Peroxotantalo-4-phosphate Clusters40Exploring the Molecular Growth of Two Gigantic Half‐Closed Polyoxometalate Clusters {Mo180} and {Mo130Ce6}66Exploring the Molecular Growth of Two Gigantic Half‐Closed Polyoxometalate Clusters {Mo180} and {Mo130Ce6}10A New Three-Dimensional Framework Based on K2Zr3-Substituted Sandwich-Type Polyoxometalate Clusters and K–O Chains7Inorganic-organic hybrid supramolecular material based on the highest connection of a Keggin arsenotungstate with electro-/photo-catalytic properties3A Ag-La heterometallic 2D layer based on mono-lacunary Keggin polyoxometalate: Synthesis, structure, and photocatalytic property8Metal–Organic Frameworks and Their Composites: Synthesis and Electrochemical Applications198Selective Isolation of Myosin Subfragment-1 with a DNA-Polyoxovanadate Bioconjugate15Induced chirality and reversal of phosphomolybdate cluster via modulating its interaction with cyclodextrins44An inorganic–organic hybrid supramolecular framework as a high-performance anode for lithium-ion batteries24An isotetramolybdate-supported rhenium carbonyl derivative: synthesis, characterization, and use as a catalyst for sulfoxidation23Coordination-driven self-assembly of chiral palladium( ii )-based supramolecular triangle structures6Efficient and robust photocatalysts based on {P 2 W 18 } modified by an Ag complex26Epimerization of glucose over ionic liquid/phosphomolybdate hybrids: structure–activity relationship17Pyridine boronic acid-polyoxometalate based porous hybrid for efficient depletion of high abundant glycoproteins in plasma14Theoretical studies on the chiral polyoxoanions [P 2 Mo 18 O 62 ] 6− and [PMo 9 O 31 (OH 2 ) 3 ] 3− with histidine: chiral inversion and chiral induction0Three new high-nuclear transition-metal-substituted heteropolytungstates: syntheses, crystal structures, magnetic studies and NLO properties22Synthesis and polypyrrole-loading study of antifungal medicine fluconazole functionalized Keggin polyoxotungstates5Isomeric organic ligand dominating polyoxometalate-based hybrid compounds: synthesis and as electrocatalysts and pH-sensitive probes9Embonic Acid Functionalized Niobium Complexes with Selective Dye Sorption Properties12A new phenylthiourea grafted Mn-Anderson polyoxometalate cluster: Synthesis, crystal structure and characterization4A Nonclassical Polyoxoanion [P3W6(O2)6(OH)2O22]7– Constructed by Two {PW3(O2)3(OH)O9} Subunits and a {PO4} Group5Synthesis, Characterization and Catalytic Activity of NHC Gold(I) Polyoxometalate Complexes14Tuning the electronic structure of organic–inorganic hybrid polyoxometalates: The crucial role of the covalent linkage55Self-Assembly of Ln(III)-Containing Tungstotellurates(VI): Correlation of Structure and Photoluminescence51Two New Tetra-Zr(IV)-Substituted Sandwich-Type Polyoxometalates Functionalized by Different Organic Amine Ligands8A Series of Compounds Based on [P2W18O62]6–and Transition Metal Mixed Organic Ligand Complexes with High Catalytic Properties for Styrene Epoxidation23The role of the counter-ion in metal-organic frameworks’ chemistry and applications204A Magnetic Adsorbent for the Removal of Cationic Dyes from Wastewater38A Series of Unprecedented Linear Mixed‐Metal‐Substituted Polyoxometalate Trimers: Syntheses, Structures, Luminescence, and Proton Conductivity Properties22Chirality Induction in Crystalline Solids Containing Sandwich-type [Ln(α2-P2W17O61)2]17– Polyoxotungstates and Proline13Recent advances in isopolyoxotungstates and their derivatives13Preparation, characterization and catalytic performance of polyoxometalate immobilized on the surface of halloysite10Stereoselective Assembly of Gigantic Chiral Molybdenum Blue Wheels Using Lanthanide Ions and Amino Acids97Inorganic–organic hybrid high-dimensional polyoxotantalates and their structural transformations triggered by water27Multi-stimuli-responsive induced chirality of polyoxometalates in natural polysaccharide hydrogels10Polyoxometalate-supported metal carbonyl derivatives: from synthetic strategies to structural diversity and applications22Pyrazine dicarboxylate-bridged arsenotungstate: synthesis, characterization, and catalytic activities in epoxidation of olefins and oxidation of alcohols18Recent Progress in Selective Oxidations with Hydrogen Peroxide Catalyzed by Polyoxometalates6Well-confined polyoxometalate-ionic liquid in silicic framework for environmentally friendly asymmetric di-hydroxylation of olefins5Polyoxometalate-Based Well-Defined Rodlike Structural Multifunctional Materials: Synthesis, Structure, and Properties54Enantiomeric Polyoxometalates Based on Malate Chirality-Inducing Tetra-ZrIV–Substituted Keggin Dimeric Clusters29

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  4. Monolacunary Keggin polyoxometalates connected to ten 4d or 4f metal atoms

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  5. Structure and bifunctional electrocatalytic activity of a novel 3D framework based on dimeric monocopper-substituted polyoxoanions as ten-connected linkages

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  10. An unprecedented (3,4,24)-connected heteropolyoxozincate organic framework as heterogeneous crystalline Lewis acid catalyst for biodiesel production

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  11. A 3D Polyoxometalate Network Based on the Tetra-CoII Sandwiched Phosphotungstate Units Linked by Cs+ Cations

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  12. Ethylenediammonium sodium tetrakis[bis(ethylenediamine-κ2N,N′)(oxalato-κ2O1,O2)cobalt(III)] [pentahydrogen di(phosphatooctadecatungstate)] tetradecahydrate

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  14. Disproportionation of Achiral Nickel(II) Centers into Two Kinds of Chiral Nickel(II) Centers Caused by an Achiral Diimine Ligand

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  22. Complexation of metal carbonyl units with [α-PW 11 O 39 ] 7− and [α 2 -P 2 W 17 O 61 ] 10− : insights into the chiral “twisted-sandwich” dimeric structures

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  33. A Microporous Anionic Metal–Organic Framework for Sensing Luminescence of Lanthanide(III) Ions and Selective Absorption of Dyes by Ionic Exchange

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  34. Diamondoid Hydrazones and Hydrazides: Sterically Demanding Ligands for Sn/S Cluster Design

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  35. Entangled structures in polyoxometalate-based coordination polymers

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  36. Induced circular dichroism of polyoxometalates via electrostatic encapsulation with chiral organic cations

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  37. Symmetry Breaking of α-[H2W12O40]6– Depends on the Transformation of Isopolyoxotungstates

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  38. Stepwise synthesis of two inorganic–organic hybrids based on the manganese monosubstituted Keggin polyanion chains

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  39. A novel single-side azobenzene-grafted Anderson-type polyoxometalate for recognition-induced chiral migration

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  40. Assembly of Six Polyoxometalate-Based Hybrid Compounds from a Simple Supramolecule to a Complicated Pseudorotaxane Framework via Tuning the pH of the Reaction Systems

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  41. Structures and Properties of Coordination Polymers based on 5‐Nitroisophthalic Acid and N,N′‐bis(4‐pyridyl‐methyl) Piperazine

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  42. Modular Molecules: Site‐Selective Metal Substitution, Photoreduction, and Chirality in Polyoxometalate Hybrids

    Chemistry - A European Journal · 2014-09-09

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  43. Spontaneous resolution of polyoxometalate-based inorganic–organic hybrids driven by solvent and common ion

    Dalton Transactions · 2014-09-16

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  44. Recent progress in metal-functionalized germanotungstates: from structures to properties

    RSC Advances · 2014-09-23

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  45. Applications of chiroptical spectroscopy to coordination compounds

    Coordination Chemistry Reviews · 2014-09-28

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  46. Modulating the polyoxometalate-based inorganic–organic hybrids from simple chains to complicated frameworks via changing POM clusters

    RSC Advances · 2014-09-30

    Yan Ping Yu, Huiyuan Ma, Haijun Pang, Li Zhang, Shaobin Li, Chunyan Zhao, Zhuanfang Zhang

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  47. Preparation, characterization and catalytic activity studies of organoruthenium‐supported polyoxotungstates on SBA‐15

    Applied Organometallic Chemistry · 2014-10-02

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  48. Four polyoxometalate-based semiconductive coordination polymers: Syntheses, structures, photoluminescent and photocatalytic properties

    Synthetic Metals · 2014-10-11

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  49. Temperature-induced racemic compounds and chiral conglomerates based on polyoxometalates and lanthanides: syntheses, structures and catalytic properties

    CrystEngComm · 2014-11-07

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  50. Kinetics and Mechanism of Oxidation of 2‐Mercaptoethanol by the Heteropolyoxovanadate [MnV13O38]7−

    International Journal of Chemical Kinetics · 2014-11-10

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