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RESEARCH PAPER · Journal of Solid State Chemistry · 2015

Polymorphism and second harmonic generation in a novel diamond-like semiconductor: Li2MnSnS4

Kasey P. Devlin, Andrew J. Glaid, Jacilynn A. Brant, Jian‐Han Zhang, Matthew N. Srnec, Daniel J. Clark, Yong Soo Kim, Joon Ik Jang, Kimberly R. Daley, Meghann A. Moreau, Jeffry D. Madura, Jennifer A. Aitken

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Polymorphism and second harmonic generation in a novel diamond-like semiconductor: Li2MnSnS4OriginalChemInform Abstract: Polymorphism and Second Harmonic Generation in a Novel Diamond‐Like Semiconductor: Li2MnSnS4.0Na 2 Hg 3 M 2 S 8 (M = Si, Ge, and Sn): New Infrared Nonlinear Optical Materials with Strong Second Harmonic Generation Effects and High Laser-Damage Thresholds186Na 2 ZnGe 2 S 6 : A New Infrared Nonlinear Optical Material with Good Balance between Large Second-Harmonic Generation Response and High Laser Damage Threshold302Analysis and prediction of mid-IR nonlinear optical metal sulfides with diamond-like structures336Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship338Li2HgMS4 (M = Si, Ge, Sn): New Quaternary Diamond-Like Semiconductors for Infrared Laser Frequency Conversion64Na2ZnSn2S6: A mixed-metal thiostannate with large second-harmonic generation response activated by penta-tetrahedral [ZnSn4S14]10− clusters10Li2MnSnSe4: A New Quaternary Diamond‐Like Semiconductor with Nonlinear Optical Response and Antiferromagnetic Property16Four new quaternary chalcogenides A 2 Ba 7 Sn 4 Q 16 (A = Li, Na; Q = S, Se): syntheses, crystal structures determination, nonlinear optical performances investigation26Structural insights into T 2 -cluster-containing chalcogenides with vertex-, edge- and face-sharing connection modes of NaQ 6 ligands: Na 3 ZnM III Q 4 (M III = In, Ga; Q = S, Se)13From AgGaS2 to Li2ZnSiS4: Realizing Impressive High Laser Damage Threshold Together with Large Second-Harmonic Generation Response134Synthesis, structure, magnetic and optoelectric properties of layered NaM0.5Sn0.5S2 (M= Mn, Fe)1Electronic, bonding, linear, and nonlinear optical properties of Na2MGe2Q6 (M=Cd, Zn, Hg; Q=S, Se), Na2ZnSi2S6, and Na2ZnSn2S6 two metal-mixed chalcogenide compounds: Insights from an ab initio study21Synthesis and Characterization of Ag2MnSnS4, a New Diamond‐like Semiconductor14Rb10Zn4Sn4S17: A Chalcogenide with Large Laser Damage Threshold Improved from the Mn-Based Analogue28Rational design of infrared nonlinear optical chalcogenides by chemical substitution287Non-centrosymmetric sulfides A 2 Ba 6 MnSn 4 S 16 (A = Li, Ag): syntheses, structures and properties21Infrared Nonlinear Optical Polymorphs α- and β-SrCu 2 SnS 4 Exhibiting Large Second Harmonic Generation Responses with Requisite Phase-Matching Behavior44A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs107Na 6 MQ 4 (M=Zn, Cd; Q=S, Se): Promising New Ternary Infrared Nonlinear Optical Materials24Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184Ba6(CuxZy)Sn4S16 (Z = Mg, Mn, Zn, Cd, In, Bi, Sn): High Chemical Flexibility Resulting in Good Nonlinear-Optical Properties12Defect diamond-like tellurides as infrared nonlinear optical materials with giant second-harmonic generation tensor14BaCu2SiS4: A New Member of the AIIBI2MIVQ4 Chalcogenide Family with a Chiral Crystal Structure6Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates153The centrosymmetric to non-centrosymmetric transformation induced by alkaline-earth cations producing infrared nonlinear optical AeMn6Ga6S16 (Ae = Ca, Sr)13Mechanochemical synthesis of rock salt-type Na 2 CaSnS 4 as a sodium-ion conductor0Modulating Nonlinear Optical Performances in α/β-SnGa2GeS6 Polymorphs via Atomic Coordination Engineering1Structural Evolution and Optical Tunability of Diamond-Like Semiconductors Li 2 Zn 1– x Cd x SnS 4 , Li 2 CdSn(S 1– y Se y ) 4 , and Li 2 ZnSn(S 1– y Se y ) 44A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation2Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals15A Rigid‐Flexible Cooperative Bond‐Engineering Strategy for the Rational Design of Advanced Infrared Nonlinear Optical Crystals2Controlled synthesis, crystal structure, and thermal behavior of the potential smart material γ-Cd(IO3)20d-f synergistic effect contributing record-high second-harmonic generation response in phase-matchable Mn-based chalcogenides0

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  1. ChemInform Abstract: Polymorphism and Second Harmonic Generation in a Novel Diamond‐Like Semiconductor: Li2MnSnS4.

    ChemInform · 2015-12-01

    Jennifer A. Aitken, et al.

    Read original paper ↗ ·

  2. Na 2 Hg 3 M 2 S 8 (M = Si, Ge, and Sn): New Infrared Nonlinear Optical Materials with Strong Second Harmonic Generation Effects and High Laser-Damage Thresholds

    Chemistry of Materials · 2016-04-05

    Kui Wu, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  3. Na 2 ZnGe 2 S 6 : A New Infrared Nonlinear Optical Material with Good Balance between Large Second-Harmonic Generation Response and High Laser Damage Threshold

    Journal of the American Chemical Society · 2016-05-19

    Guangmao Li, Kui Wu, Qiong Liu, Zhihua Yang, Shilie Pan

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  4. Analysis and prediction of mid-IR nonlinear optical metal sulfides with diamond-like structures

    Coordination Chemistry Reviews · 2016-11-22

    Fei Liang, Lei Kang, Zheshuai Lin, Yicheng Wu, Chuangtian Chen

    Read original paper ↗ ·

  5. Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship

    Crystal Growth & Design · 2017-03-15

    Fei Liang, Lei Kang, Zheshuai Lin, Yicheng Wu

    Read original paper ↗ ·

  6. Li2HgMS4 (M = Si, Ge, Sn): New Quaternary Diamond-Like Semiconductors for Infrared Laser Frequency Conversion

    Crystals · 2017-04-12

    Kui Wu, Shilie Pan

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  7. Na2ZnSn2S6: A mixed-metal thiostannate with large second-harmonic generation response activated by penta-tetrahedral [ZnSn4S14]10− clusters

    Science China Technological Sciences · 2017-05-12

    Guangmao Li, Kui Wu, Qiong Liu, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  8. Li2MnSnSe4: A New Quaternary Diamond‐Like Semiconductor with Nonlinear Optical Response and Antiferromagnetic Property

    Chemistry - An Asian Journal · 2017-10-07

    Xiaoshuang Li, Chao Li, Molin Zhou, Yicheng Wu, Jiyong Yao

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  9. Four new quaternary chalcogenides A 2 Ba 7 Sn 4 Q 16 (A = Li, Na; Q = S, Se): syntheses, crystal structures determination, nonlinear optical performances investigation

    New Journal of Chemistry · 2018-01-01

    Ailijiang Abudurusuli, Kui Wu, Shilie Pan

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  10. Structural insights into T 2 -cluster-containing chalcogenides with vertex-, edge- and face-sharing connection modes of NaQ 6 ligands: Na 3 ZnM III Q 4 (M III = In, Ga; Q = S, Se)

    Dalton Transactions · 2018-01-01

    Ruijiao Chen, Xiaowen Wu, Zhi Su

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  11. From AgGaS2 to Li2ZnSiS4: Realizing Impressive High Laser Damage Threshold Together with Large Second-Harmonic Generation Response

    Chemistry of Materials · 2018-01-17

    Guangmao Li, Yu Chu, Zhongxiang Zhou

    Read original paper ↗ ·

  12. Synthesis, structure, magnetic and optoelectric properties of layered NaM0.5Sn0.5S2 (M= Mn, Fe)

    Journal of Alloys and Compounds · 2018-02-23

    Jianqiao He, Xian Zhang, Chong Zheng, Fuqiang Huang

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  13. Electronic, bonding, linear, and nonlinear optical properties of Na2MGe2Q6 (M=Cd, Zn, Hg; Q=S, Se), Na2ZnSi2S6, and Na2ZnSn2S6 two metal-mixed chalcogenide compounds: Insights from an ab initio study

    Journal of Physics and Chemistry of Solids · 2018-04-12

    R. Mahiaoui, Tarik Ouahrani, A. Chikhaoui, Ángel Morales‐García, A.H. Reshak

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  14. Synthesis and Characterization of Ag2MnSnS4, a New Diamond‐like Semiconductor

    Zeitschrift für anorganische und allgemeine Chemie · 2018-08-02

    Daniel Friedrich, Sebastian Greil, Theresa Block, Lukas Heletta, Rainer Pöttgen, Arno Pfitzner

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  15. Rb10Zn4Sn4S17: A Chalcogenide with Large Laser Damage Threshold Improved from the Mn-Based Analogue

    Inorganic Chemistry · 2019-10-14

    Jun Zhao, Dajiang Mei, Yi Jin Yang, Wangzhu Cao, Chuang Liu, Yuandong Wu, Zheshuai Lin

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  16. Rational design of infrared nonlinear optical chalcogenides by chemical substitution

    Coordination Chemistry Reviews · 2019-12-21

    Hua Lin, Wenbo Wei, Hong Chen, Xintao Wu, Qi‐Long Zhu

    Read original paper ↗ ·

  17. Non-centrosymmetric sulfides A 2 Ba 6 MnSn 4 S 16 (A = Li, Ag): syntheses, structures and properties

    Dalton Transactions · 2020-01-01

    Ruihuan Duan, Hua Lin, Yue Wang, Yuqiao Zhou, Li‐Ming Wu

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  18. Infrared Nonlinear Optical Polymorphs α- and β-SrCu 2 SnS 4 Exhibiting Large Second Harmonic Generation Responses with Requisite Phase-Matching Behavior

    Chemistry of Materials · 2020-01-21

    Ya Feng Yang, Kui Wu, Bingbing Zhang, Xiaowen Wu, Ming‐Hsien Lee

    Read original paper ↗ ·

  19. A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs

    Coordination Chemistry Reviews · 2020-05-25

    Kui Wu, Ya Feng Yang, Lihua Gao

    Read original paper ↗ ·

  20. Na 6 MQ 4 (M=Zn, Cd; Q=S, Se): Promising New Ternary Infrared Nonlinear Optical Materials

    Chemistry - A European Journal · 2021-01-27

    Yi Huang, Le Gao, Haohai Yu, Zhihua Yang, Junjie Li, Shilie Pan

    Read original paper ↗ ·

  21. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

    Hong Chen, Wenbo Wei, Hua Lin, Xintao Wu

    Read original paper ↗ ·

  22. Ba6(CuxZy)Sn4S16 (Z = Mg, Mn, Zn, Cd, In, Bi, Sn): High Chemical Flexibility Resulting in Good Nonlinear-Optical Properties

    Inorganic Chemistry · 2022-01-26

    Bingheng Ji, Kui Wu, Yunhua Chen, Fei Wang, Aaron J. Rossini, Bingbing Zhang, Jian Wang

    Read original paper ↗ ·

  23. Defect diamond-like tellurides as infrared nonlinear optical materials with giant second-harmonic generation tensor

    Materials Today Physics · 2023-07-10

    Mengran Sun, Chunxiao Li, Jinlong Shi, Ming‐Hsien Lee, Jiyong Yao

    Read original paper ↗ ·

  24. BaCu2SiS4: A New Member of the AIIBI2MIVQ4 Chalcogenide Family with a Chiral Crystal Structure

    Zeitschrift für anorganische und allgemeine Chemie · 2023-09-08

    Arka Sarkar, Gayatri Viswanathan, Kui Wu, Gordon J. Miller, Kirill A. Kovnir

    Read original paper ↗ ·

  25. Recent advances in rational structure design for nonlinear optical crystals: leveraging advantageous templates

    Chemical Society Reviews · 2024-01-01

    Ziting Yan, Jinbin Fan, Shilie Pan, Min Zhang

    Read original paper ↗ ·

  26. The centrosymmetric to non-centrosymmetric transformation induced by alkaline-earth cations producing infrared nonlinear optical AeMn6Ga6S16 (Ae = Ca, Sr)

    Science China Chemistry · 2024-07-10

    Yangping Zhang, Shao‐Min Pei, Wen‐Fa Chen, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  27. Mechanochemical synthesis of rock salt-type Na 2 CaSnS 4 as a sodium-ion conductor

    RSC Mechanochemistry · 2024-12-03

    Hamdi Ben Yahia, Atsushi Sakuda, Akitoshi Hayashi

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  28. Modulating Nonlinear Optical Performances in α/β-SnGa2GeS6 Polymorphs via Atomic Coordination Engineering

    Inorganic Chemistry · 2025-09-20

    Jingjing Xu, Yan Xiao, Dazhi Lu, Bingbing Zhang, Kui Wu, Haohai Yu, Huaijin Zhang

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  29. Structural Evolution and Optical Tunability of Diamond-Like Semiconductors Li 2 Zn 1– x Cd x SnS 4 , Li 2 CdSn(S 1– y Se y ) 4 , and Li 2 ZnSn(S 1– y Se y ) 4

    Chemistry of Materials · 2025-10-16

    Pritam Das, Diganta Sarkar, Vidyanshu Mishra, Mengran Sun, Dundappa Mumbaraddi, Mohammed Jomaa, Vladimir K. Michaelis, Jiyong Yao, Arthur Mar

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  30. A high-performance IR nonlinear optical material Sr 3 MnGe 2 S 8 achieved via partial cation substitution-induced structural transformation

    Inorganic Chemistry Frontiers · 2025-11-14

    A-Lan Xu, Mao‐Yin Ran, Zuju Ma, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

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  31. Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals

    Coordination Chemistry Reviews · 2026-02-02

    Ailijiang Abudurusuli, Linan Wang, Junben Huang, Xueling Hou, Miriding Mutailipu, Shilie Pan, Junjie Li

    Read original paper ↗ ·

  32. A Rigid‐Flexible Cooperative Bond‐Engineering Strategy for the Rational Design of Advanced Infrared Nonlinear Optical Crystals

    Laser & Photonics Review · 2026-05-27

    Zhihui Xiong, Qian Wu, Pifu Gong, Haotian Tian, Yufei Wei, Zhixi Li, Fang Ding, Mingjun Xia

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  33. Controlled synthesis, crystal structure, and thermal behavior of the potential smart material γ-Cd(IO3)2

    Journal of the Iranian Chemical Society · 2026-07-13

    Zoulikha Hebboul, Djamal Benbertal, Benbadis Benmoulai, Ahmed Draoui

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  34. d-f synergistic effect contributing record-high second-harmonic generation response in phase-matchable Mn-based chalcogenides

    Chinese Chemical Letters · 2026-09-01

    Yu‐Xuan Zhang, Sheng-Xian Xiao, Zhen-Cheng Wu, Mao‐Yin Ran, Sheng‐Ping Guo

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