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RESEARCH ARTICLE · Angewandte Chemie International Edition · 2026

Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion

Meng‐Na Jing, Si‐Fan Lu, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice DistortionOriginalA promising mid-infrared nonlinear optical crystal with well-balanced properties0KGdSiSe 4 and KGdGeSe 4 : two rare earth-based selenides with wide bandgaps and large nonlinear optical responses0Series of phosphate nonlinear optical materials containing active metal ions with short cut-off edges0The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 116Engineering Multiple Hydrogen‐Bond Sites With D‐π‐A Motifs for Strong Optical Nonlinearity and Giant Birefringence in Organic‐Inorganic Halides4Linear [ICl 2 ] Units Induced Giant Optical Anisotropy in AICl 2 (A = NH 4 , Rb): A Pathway to Advanced Birefringent Materials4LiMn(IO 3 ) 3 : A Noncentrosymmetric Iodate Synthesized by Polyhedral Volume Ratio Modulation0Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0A Two‐Dimensional Organic Salt With a Deep‐Ultraviolet Cutoff Edge and Strong Second‐Harmonic Generation0Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity0From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0A Composition-Matched Intermediate Reveals Site-Specific Symmetry Evolution with Retained Second-Harmonic Generation in Supertetrahedral Sulfides0

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  1. A promising mid-infrared nonlinear optical crystal with well-balanced properties

    Inorganic Chemistry Frontiers · 2026

    Yujun Wang, Yuning Qi, Yongkuan Xu, Ning Ye, Zhanggui Hu, Conggang Li

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  2. KGdSiSe 4 and KGdGeSe 4 : two rare earth-based selenides with wide bandgaps and large nonlinear optical responses

    Dalton Transactions · 2026

    Zhenglong Li, Guansong Zheng, Chen Bai, Leyan Nian, Shilie Pan, Junjie Li

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  3. Series of phosphate nonlinear optical materials containing active metal ions with short cut-off edges

    Dalton Transactions · 2026

    Xiaoqin Ma, Xianmeng He, Jialong Wang, Lei Wu, Yu Xue, Qun Jing, Zhaohui Chen

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  4. The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 11

    Angewandte Chemie International Edition · 2026

    Hongshan Wang, Miriding Mutailipu, Shilie Pan, Junjie Li

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  5. Engineering Multiple Hydrogen‐Bond Sites With D‐π‐A Motifs for Strong Optical Nonlinearity and Giant Birefringence in Organic‐Inorganic Halides

    Angewandte Chemie International Edition · 2026

    Y Z Zhang, Yuchao Li, Y N Wu, Bing Teng, Hongting Lu, Xingxing Jiang, Shijia Sun, C Hu, Dongwei Zhai, Lifeng Cao, Jinkang Ma, R K Li, Degang Xu, Zheshuai Lin, Degao Zhong

    Read original paper ↗ ·

  6. Linear [ICl 2 ] Units Induced Giant Optical Anisotropy in AICl 2 (A = NH 4 , Rb): A Pathway to Advanced Birefringent Materials

    Advanced Functional Materials · 2026

    Du Yinxia, C J Huang, Hongshan Wang, Linan Wang, Z Chen, Miriding Mutailipu, Shilie Pan, Junjie Li

    Read original paper ↗ ·

  7. LiMn(IO 3 ) 3 : A Noncentrosymmetric Iodate Synthesized by Polyhedral Volume Ratio Modulation

    Inorganic Chemistry · 2026

    Ruilan Kong, Weitong Wang, Shuoxing Yang, S W, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yizhi Wu, HS Wu

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  8. Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects

    Advanced Optical Materials · 2026

    Xiangran Kong, Jingdong Yan, Zi Wang, Hongwei Leng, Shichao Cheng, Sue Hao, Xiaoran Niu, Zuotao Lei, Chunhui Yang

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  9. A Two‐Dimensional Organic Salt With a Deep‐Ultraviolet Cutoff Edge and Strong Second‐Harmonic Generation

    Angewandte Chemie International Edition · 2026

    Xiaotian Zhang, Xingxing Jiang, Shaohua Xiao, Wenzhi Song, Chao Wu, Zheshuai Lin, Zhipeng Huang, Jinhu Yang, Mark Graeme Humphrey, Chi Zhang

    Read original paper ↗ ·

  10. Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity

    Angewandte Chemie International Edition · 2026

    Qichao Zhao, Bingxuan Li, Guang Peng, Ning Ye, Jindong Chen

    Read original paper ↗ ·

  11. From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance

    Chinese Journal of Structural Chemistry · 2026

    Hong Chen, Zheng-Tao Hu, Mao‐Yin Ran, 马祖驹, Xin-Tao Wu, Hua Lin

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  12. A Composition-Matched Intermediate Reveals Site-Specific Symmetry Evolution with Retained Second-Harmonic Generation in Supertetrahedral Sulfides

    Inorganic Chemistry · 2026

    KuiXian Cai, Ximeng Lv, Chuang Liu, Shuchang Wu, Zichang Wang, Yang Liu, Bin Luo, Xiao‐Ming Jiang, Dajiang Mei

    Read original paper ↗ ·
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