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RESEARCH PAPER · Advanced Optical Materials · 2024

Unveiling Charge Dependent Law to Enhance Birefringence in 2‐Aminopyrimidine Family

Muhammad Sharjeel Arif, Xu Liu, Zi‐Jian Li, Hangwei Jia, Yansheng Jiang, Zhihua Yang, Xueling Hou, Shilie Pan

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Unveiling Charge Dependent Law to Enhance Birefringence in 2‐Aminopyrimidine FamilyOriginalOptimizing optical anisotropy in low-dimensional structures via intralayer hydrogen bonding modulation and anionic substitution17Significant enhancement in the birefringence of metal phosphite halides via the introduction of π-conjugated cations17Metal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy17Extended study of crystal structures, optical properties and vibrational spectra of polar 2-aminopyrimidinium hydrogen phosphite and three centrosymmetric salts - bis(2-aminopyrimidinium) sulfate monohydrate and two 2-aminopyrimidinium hydrogen sulfate polymorphs1Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization88Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization13[CON3H6BF4]: An Efficient Metal‐Free Borate with Optimized Birefringence Achieved by Structural Design Strategy15[C( NH2 )3] 2SiF6 : Design of Deep Ultraviolet Crystals with Large Birefringence Based on a Fluorination‐Oriented Strategy13Effect of Multiple Hydrogen Bonding on the π-Conjugated Groups and Optical Properties in Molecular Crystals5Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups3A multi-scale birefringence modulation strategy in DUV/UV crystals induced by organic cations1Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation1Layered perovskite-like nitrates A 2 Ca(NO 3 ) 2 Cl 2 (A = Rb, Cs) as ultraviolet birefringent optical materials3Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution1Synthesis and characterization of hydrated alkali metal calcium nitrates ACa(NO 3 ) 3 ·2H 2 O (A = NH 4 , Rb, Cs) as short ultraviolet birefringent materials0Protonation‐Triggered Structural Transformations in 4‐Hydroxypyridinium Halides for Solar‐Blind UV Functional Crystals3Protonation‐Triggered Structural Transformations in 4‐Hydroxypyridinium Halides for Solar‐Blind UV Functional Crystals8Structural Anion Geometry-Regulated Molecular Alignment in [C 10 H 8 NO 2 ]-Based Crystals for Enhancing Ultraviolet Birefringence0Hydrogen‐Bond‐Directed Assembly of Urea Derivatives: Exceptional Birefringence Achieved by π ‐Conjugated Unit Alignment3Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1[CN4H8]SiF6: Fluorination-guided design of deep-UV crystal with large birefringence0

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  1. Optimizing optical anisotropy in low-dimensional structures via intralayer hydrogen bonding modulation and anionic substitution

    Materials Horizons · 2025-01-01

    Muhammad Sharjeel Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  2. Significant enhancement in the birefringence of metal phosphite halides via the introduction of π-conjugated cations

    Chemical Science · 2025-01-01

    Ru‐Ling Tang, Yue Wang, Yi‐Lei Lv, Bing-Wei Miao, Wenlong Liu, Sheng‐Ping Guo

    Read original paper ↗ ·

  3. Metal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy

    Small · 2025-04-07

    Zichang Wang, Qing‐Yu Liu, Zhihua Yang, Xueling Hou, Minqiang Gai

    Read original paper ↗ ·

  4. Extended study of crystal structures, optical properties and vibrational spectra of polar 2-aminopyrimidinium hydrogen phosphite and three centrosymmetric salts - bis(2-aminopyrimidinium) sulfate monohydrate and two 2-aminopyrimidinium hydrogen sulfate polymorphs

    Optical Materials · 2025-04-10

    Irena Matulková, L. Bohatý, P. Becker, Ivana Cı́sařová, Róbert Gyepes, Michaela Fridrichová, J. Kroupa, Petr Němec, Ivan Němec

    Read original paper ↗ ·

  5. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie International Edition · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

    Read original paper ↗ ·

  6. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

    Angewandte Chemie · 2025-05-22

    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

    Read original paper ↗ ·

  7. [CON3H6BF4]: An Efficient Metal‐Free Borate with Optimized Birefringence Achieved by Structural Design Strategy

    Small · 2025-05-23

    Muhammad Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  8. [C( NH2 )3] 2SiF6 : Design of Deep Ultraviolet Crystals with Large Birefringence Based on a Fluorination‐Oriented Strategy

    Chinese Journal of Chemistry · 2025-06-24

    Shaohua Liu, Xiaoqin Ma, Xifa Long, Yun Mo Yang

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  9. Effect of Multiple Hydrogen Bonding on the π-Conjugated Groups and Optical Properties in Molecular Crystals

    Inorganic Chemistry · 2025-11-03

    Hangwei Jia, Xiangrong Song, Muhammad Arif, Yaqi Jin, Feng Yu, Xueling Hou

    Read original paper ↗ ·

  10. Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups

    Advanced Functional Materials · 2025-12-12

    Muhammad Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  11. A multi-scale birefringence modulation strategy in DUV/UV crystals induced by organic cations

    Materials Chemistry Frontiers · 2026-01-01

    Zhi Fang, G Xu, Wenhu Wang, Huanhuan Wang, Jian Wei Han

    Read original paper ↗ ·

  12. Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation

    Inorganic Chemistry Frontiers · 2026-01-01

    S AN, Yaqi Jin, Wenhu Wang, Bailin Chen, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  13. Layered perovskite-like nitrates A 2 Ca(NO 3 ) 2 Cl 2 (A = Rb, Cs) as ultraviolet birefringent optical materials

    Inorganic Chemistry Frontiers · 2026-01-01

    Hussin Elkik, Muhammad Mujahid Iqbal, Aqsa Munawar, Zhihua Yang, Fangfang Zhang, Shilie Pan

    Read original paper ↗ ·

  14. Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution

    Inorganic Chemistry Frontiers · 2026-01-01

    Mei Hu, Zhencheng Wu, Xin Su, Hongheng Chen, Qun Jing, Zhaohui Chen, Ming‐Hsien Lee

    Read original paper ↗ ·

  15. Synthesis and characterization of hydrated alkali metal calcium nitrates ACa(NO 3 ) 3 ·2H 2 O (A = NH 4 , Rb, Cs) as short ultraviolet birefringent materials

    Dalton Transactions · 2026-01-01

    Hussin Elkik, Muhammad Mujahid Iqbal, Aqsa Munawar, Zhihua Yang, Fangfang Zhang, Shilie Pan

    Read original paper ↗ ·

  16. Protonation‐Triggered Structural Transformations in 4‐Hydroxypyridinium Halides for Solar‐Blind UV Functional Crystals

    Angewandte Chemie · 2026-01-04

    Jing Lu, Xin Liu, Shuangxiong Zhao, Xuebing Deng, Qundong Fu, Jingyu Guo, Zheng Liu, Li‐Ming Wu, Ling Chen

    Read original paper ↗ ·

  17. Protonation‐Triggered Structural Transformations in 4‐Hydroxypyridinium Halides for Solar‐Blind UV Functional Crystals

    Angewandte Chemie International Edition · 2026-01-04

    Jing Lu, Xin Liu, Shuangxiong Zhao, Xuebing Deng, Qundong Fu, Jingyu Guo, Zheng Liu, Li‐Ming Wu, Ling Chen

    Read original paper ↗ ·

  18. Structural Anion Geometry-Regulated Molecular Alignment in [C 10 H 8 NO 2 ]-Based Crystals for Enhancing Ultraviolet Birefringence

    Crystal Growth & Design · 2026-04-07

    YaoGuo Shen, Yiman Yang, Jiajia Xiong, Xinyi Wang

    Read original paper ↗ ·

  19. Hydrogen‐Bond‐Directed Assembly of Urea Derivatives: Exceptional Birefringence Achieved by π ‐Conjugated Unit Alignment

    Small · 2026-04-14

    Peng Jiang, Yuqi Qin, Junwei Feng, Minqiang Gai, Shilie Pan

    Read original paper ↗ ·

  20. Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals

    Advanced Functional Materials · 2026-06-01

    Hangwei Jia, Yaqi Jin, Muhammad Arif, Bailin Chen, Zhihua Yang, Xueling Hou, Shilie Pan

    Read original paper ↗ ·

  21. [CN4H8]SiF6: Fluorination-guided design of deep-UV crystal with large birefringence

    Inorganic Chemistry Communications · 2026-08-23

    Piaoyu Yan, Bao Jiang, Jing Zhou, Jiawen Liu, Wanxiu Xi, Ensheng Wang, Xiuhua Cui, Zhaohui Chen

    Read original paper ↗ ·
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