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RESEARCH PAPER · Journal of the American Chemical Society · 2024

Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions

Qinyuan Hu, Zhixing Zhang, Dongpo He, Jiacong Wu, Jinyu Ding, Qingxia Chen, Xingchen Jiao, Yi Xie

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Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-ReactionsOriginalQuantum tunnelling dominates chloride leaching from polyvinyl chloride3Alloying effect-triggered electron polarization in PdCu metallene for simultaneous electrocatalytic upcycling of nitrate and polyethylene terephthalate to value-added chemicals37Pore Engineering in Biomass-Derived Carbon Materials for Enhanced Energy, Catalysis, and Environmental Applications71Preparation of NiCo hydroxide by chloride corrosion for electrocatalytic upcycling of polyethylene terephthalate plastic waste24Circular Economy and Chemical Conversion for Polyester Wastes23Current Advances in the Photoconversion of Plastics: the Catalysts and Reaction Pathways7Electroreforming of plastic wastes for value-added products20Enhancing the Conversion Efficiency of Polyethylene to Methane through Codoping of Mn Atoms into Ru Centers and CeO2 Supports37Chemical Innovations in Polymer Upcycling: Beyond Traditional Recycling1Advancements and prospects of near-infrared-light driven CO 2 reduction reaction69Chemical upcycling of biodegradable plastic waste: a critical review9Construction of Magnetically Recoverable Fe3o4@Ceo2 Core-Shell Photocatalyst for Efficient Upcycling of Plastic Waste0Deep eutectic solvent-assisted recycling of spent lithium-ion batteries into electrocatalysts for polyethylene terephthalate upcycling8Modulating ion migration realizes both enhanced and long-term-stable nanozyme activity for efficient microplastic degradation13Sustainable thermochemical plastic valorization towards a circular economy: a critical review27Topochemical synthesis of an atomic Pt modified plasmonic yolk–shell nanostructure for enhanced photocatalytic hydrogen evolution15Tunable Syngas Production from Photocatalytic PET Reforming over TiO2/CdZnS S-Scheme Heterojunction0Advanced Catalysts for the Chemical Recycling of Plastic Waste90Pd-doped CoNi-based bifunctional electrodes for upcycling of PET plastic with ultra-long stability19Efficient metallic Ni as a bifunctional electrocatalyst for integrating continuous PET plastic upcycling with hydrogen production65Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles73Advances in Solar-Driven, Electro/Photoelectrochemical, and Photothermal-Assisted Upcycling of Waste Plastics10Ultralow-coordinated Ni species boosting paired electrosynthesis of formate from waste plastic and carbon dioxide22Selective Electrooxidation of Ethylene Glycol to Formate with Hydrogen Cogeneration in Ni3S2 Nanodomains on NiFeMn-LDH Nanosheet Arrays39Asymmetric Atomic Pt–B Dual-Site Catalyst for Efficient Photoreforming of Waste Polylactic Acid Plastics in Seawater56Lattice Hydrogen Involved Electrocatalytic Nitrate Reduction to Hydroxylamine81Turning plastic trash into Energy: Converted MOFs and carbon for energy storage18Regulating second-shell coordination in molybdenum single-atom catalysts for efficient photocatalytic nitrogen fixation30Dynamic Crystal‐Structure and Active‐Site of Defective ZnAl‐Catalysts During CO 2 Photoreduction14Dynamic Crystal‐Structure and Active‐Site of Defective ZnAl‐Catalysts During CO 2 Photoreduction0Plastic waste upcycling through electrocatalysis10Fundamentals and challenges for indirect and direct photocatalytic conversion of plastic wastes into valuable fuels5Electrocatalytic Upcycling of Plastic Waste to Organonitrogen Chemicals via Intercepting Carbon Intermediates20Current developments in multifunctional technology for waste plastic chemical recycling and case studies0Electrochemical Degradation of Plastic Waste Coupled with Hydrogen Evolution in Seawater Using Rosette‐Like High‐Entropy Oxides13Solar-driven plastic waste conversion: A mini-review on photoreforming for Co-producing hydrogen and chemical feedstocks7Lattice‐Matched Iridium on Vanadium Nitride as Efficient Hydrogen Electrocatalyst26Industrial-grade electrocatalytic valorization of waste plastics via reconstructed Ni 2+ -CoOOH nanosheet arrays55Binuclear Metal-Based Covalent Organic Framework Mimicking Metallohydrolases for Direct Photoreforming of PET Plastic48As, Cd and Pb contaminated soil remediation by electrochemical methods: mechanisms, current advances and perspective5Effects of Conduction Band Edge Regulation on the Photoreforming Efficiency of Plastic Waste: Taking BPNS/TiO 2 as a Photocatalyst21Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions3Upcycling Polybutylene Succinate Waste to Succinic Acid via Paired Electrocatalytic using Thiol‐Engineered MOFs and a CO 2 ‐Assisted Precipitation System14Electrostatic Adsorption-Reinforced Carboxymethylated Cellulose Nanofiber-Lignin Sustainable Bioplastic for UV-Blocking and Water-Stable Packaging Materials2Photocatalytic Formamide Synthesis from Plastic Waste and Ammonia via C─N Bond Construction Under Mild Conditions4Photocatalytic Formamide Synthesis from Plastic Waste and Ammonia via C─N Bond Construction Under Mild Conditions23Plasma catalytic hydrogenolysis of polyethylene to gasoline-range fuels over Sm/USY catalysts10Catalytic Upcycling of PET: From Waste to Chemicals and Degradable Polymers48Paired Electrocatalysis: Nitrate Reduction to Ammonia Coupled with Anodic Upcycling of Biomass and Plastic Waste5CdZnS Nanoparticles Supported on an Ultrathin Cu Metal–Organic Layer as an S-Scheme Photocatalyst for Hydrogen Production and Pollutant Degradation5Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12A magnetically recyclable core-shell heterojunction photocatalyst with oxygen vacancies for efficient upcycling of plastic waste6CuO Nanoparticle‐Loaded TiO 2 Catalyst for High‐Performance Photocatalytic Hydrogen Peroxide Generation11Electronic regulation via dual-defect synergy for boosting electro-reforming of polyethylene terephthalate waste to value-added formate and hydrogen4PdNi bimetallic catalyst enables efficient electrochemical upcycling of waste plastics3Tandem depolymerization-electrocatalysis for plastic waste upcycling6A Multi‐step Synergistic Strategy for Upgrading Plastic Waste into Circular Economy Feedstocks1An interfacial W–S bond bridged Bi 2 O 2 S/W 18 O 49 S-scheme heterostructure with rich oxygen vacancies: enhancing charge transfer kinetics for CO 2 photoreduction1Cutting-Edge advances in chemical depolymerization-based recycling of waste polyethylene terephthalate plastics0Electrochemical upgrading of biomass-derived 5-hydroxymethylfurfural over layered double hydroxides: synthesis, mechanisms, and design strategies3Highly selective hydrocracking of polypropylene to gasoline-range fuels over the Pt/MCM-22 catalyst0Photoreforming of plastic waste into value-added chemicals with hydrogen production4Selective two-electron oxygen reduction for H 2 O 2 photosynthesis with anthraquinone-modified UiO-66/Zn 3 In 2 S 6 heterojunctions1Transformation of clinical waste into heteroatom-doped porous carbon materials towards a highly efficient energy storage device0Triad of electrocatalytic strategies for polymer monomer synthesis0Elucidating In Situ Impedance Kinetic Mechanisms for Selective Ethylene Glycol Electrooxidation to Formate Production Regulated by Mo-Doped NiCo 2 O 43Mechanocatalysis: Driving Sustainable Chemical Reactions Under Mild Conditions1Rational design of bifunctional catalysts for hydrocracking of polyethylene waste plastics to narrow-distributed liquid fuels4Designed S‐Scheme FeCo 2 O 4 /g‐C 3 N 4 Heterojunction for Photocatalytic Activation of Peroxymonosulfate to Degrade polyethylene Terephthalate Plastic3Process intensification driven by non-conventional energy fields in emerging plastic recycling: A systematic review2Electrocatalytic degradation strategies for plastic fibers with sustainable resource recovery potential4Rational catalyst design and coupled electrolysis for electrocatalytic upcycling of waste polyester plastics1Photothermal catalysis for plastic upcycling: a review on material design and reaction mechanisms2Tuning Multi‐Active Sites in Ni(OH) 2 Catalyst via V/Ru Doping for Ampere‐Level Upcycling of Polyethylene Terephthalate Plastic0Towards Sustainable C1 Valorization: Coupling Biomass and Waste Plastics Conversion with Renewable Energy0Two-Dimensional Hybrid Framework Based on Weakley-Type POM as a Heterogeneous Catalyst for Glycolysis of PET and Various Polyesters0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Chlorine Ion-Enhanced Efficient Photocatalysis of Polyethylene Plastics1Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Enhanced Seawater High‐Purity Uranium Extraction Coupled With Microplastic Degradation by Quaternary Amine Tuned Microenvironment of COFs0Waste plastic recycling and upgrading via electro- and photocatalytic C−X bond coupling1Electrothermal Strategies for Upcycling Commodity Plastics0Carboxylate vs. phosphonate: Cobalt coordination polymers for enhanced water splitting electrocatalysis0Catalytic Recycling and Upcycling of Bio-Based Waste Plastic0Efficient and mild hydrogenolysis of polyethylene terephthalate to terephthalic acid over a Ni cluster catalyst0Carbothermal-driven lattice iron engineering for synergistic photothermal oxidation of heterogeneous nanoplastics0Photoreforming and Photoelectroreforming of Waste‐Derived Feedstocks for Solar‐Driven Production of Fuels and Chemicals0Regulating •OH generation via an S-scheme TiO2/CdZnS heterojunction for selective photocatalytic PET upcycling to glycolate1Thermochemical conversion of metallized plastic packaging waste: Aluminum in waste enhances polymer pre-cracking and steam-cracker precursor formation over zeolite catalysts1Photoreforming of Waste Plastics into H2 Using Zn x Cd1- x S Nanoplates Synthesized via Cation Exchange Reactions0Electro‐ and Photocatalytic C─X Bond Coupling in Valorization of Waste Plastics/Biomass: Reaction Mechanism and Catalyst Engineering1Multi-site synergy in high-entropy alloys drives integrated biomass valorization and CO2-to-C2 conversion1Electro-reforming of nylon waste plastic into high-value nitrile over Pt-anchored NiCo2O4 nanowires on nickel foam coupled with green hydrogen production0Synthesis of high-purity conductive carbon nanotubes from waste plastics via catalytic pyrolysis: The role of Al2O3 support properties0Photoelectrochemical valorization of inorganic feedstocks for chemical production and environmental remediation0Photocatalytic upcycling of plastic waste coupled with CO2 reduction to high-value chemicals0From Traditional Depolymerization to Value-Added Upgrading: Upcycling of PET Fibers with Sustainable Chemistry and Renewable Energy0Frustrated Lewis Pairs Enable Efficient Polyethylene Oxidative Upcycling0Frustrated Lewis Pairs Enable Efficient Polyethylene Oxidative Upcycling0

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