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RESEARCH PAPER · ACS Catalysis · 2025

Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design Principles

Zongyang Ya, Shengbo Zhang, Dong Xu, Hua Wang, Mei Li

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Coupling Plastic Upgrading and Photocatalysis: Catalytic Mechanisms and Design PrinciplesOriginalMOF-Derived CeO₂/Co₃O₄ Heterojunction Photocatalyst:,Synergistic Peroxymonosulfate Activation for PET Degradation0Plastic photoreforming: catalytic production of hydrogen and valuable chemicals15Asymmetric Atomic Pt–B Dual-Site Catalyst for Efficient Photoreforming of Waste Polylactic Acid Plastics in Seawater56Photocatalytic recycling of polyethylene terephthalate: An emerging ecotechnology for environmental sustainability5State-of-the-Art Achievements and Challenges in Photochemical Conversion of Plastics to Chemicals and Composites6Photocatalytic Hydrogen Evolution Driven by Advanced Metal Sulfides from Sustainable Multilevel Biomass and Waste Plastics51Isomer-tailored vinylene-based COFs for photo-enhanced uranium extraction from seawater: Mechanistic insights into carrier dynamics and structural superiority9Catalysis in Renewable Energy: Theoretical Insights and Industrial Applications1Solar Fuels Production from Plastics and Biomass Photoreforming11Photocatalytic Waste Polystyrene Plastic Conversion: Reaction Mechanism and Catalyst Design38Diatomic Zn‐Functionalized Carbon Sphere for Microplastics Remediation in Natural Seawater at Environmentally Relevant Concentration17Bias‐Free Photoelectrochemical System for Scalable Solar‐Driven Hydrogen Peroxide Production via Molecularly Engineered Conjugated Polycarbazole Frameworks11Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions3Solar-powered photothermal-photocatalytic synergistic platform for simultaneous seawater desalination and antibiotic pollutant degradation7Nanocatalytic upcycling of plastic waste: Advances in selective conversion technologies for sustainable high-value products recovery13Advances and Outlook of In Situ Characterization Techniques for Photocatalytic Reforming of Plastic Wastes5Facile construction of HOF@ZnO/TiO2 ternary composite for efficient photocatalytic degradation of dyes15Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Cu‐Doped UiO‐66‐NH 2 Photocatalytic Cross‐Coupling of Arylamine C(sp 2 )‐H with Phenothiazine N─H Bonds0Preparation, Modification, and Application of Graphitic Carbon Nitride in Photocatalytic Degradation of Antibiotics4Design of S-scheme CuO/CeO2 heterojunction for photoreforming of polyethylene terephthalate plastic into value-added chemicals combined with hydrogen evolution9Interfacial engineering of CeO2/Bi19Br3S27 heterojunction for efficient photoreduction of CO2 to CO with nearly 100% selectivity14Depolymerization of polyesters catalyzed by binuclear metal complexes0Tandem depolymerization-electrocatalysis for plastic waste upcycling6Recent Advances in Photocatalytic Conversion of Furfural2Designing interfacial-engineered S-scheme heterostructures with dual-metal sulfides for efficient solar-to-hydrogen conversion3Catalytic Oxidation of Commodity Plastics: Advances in Polyethylene and Polystyrene Valorization5Bio‐Inspired Cascade Photocatalysis on Fe Single‐Atom Carbon Nitride Upcycles Plastic Wastes for Effective Acetic Acid Production7Upcycling Waste Polyethylene and Polypropylene into Carbon Oxides and Hydrocarbons via a Mechanochemistry-Photocatalysis Combined Technology under Mild Conditions1Beyond mechanical recycling: artificial photosynthesis enables polyester plastic upcycling into valuable chemicals5Electrospun Co3O4/CeO2 hollow nanotubes for photocatalytic degradation of PET Plastics with peroxymonosulfate Activation: Performance and DFT Insight0Electrospun nanotubular photocatalysts: Persulfate activation and DFT insight into polyethylene terephthalate degradation0Engineered nanocatalysts for degradation and valorisation of micro/nanoplastics12Ionic liquid photocatalysts in organic transformations1Key components for realistic application of plastic photoreforming coupled with H2 evolution9Microwave-synthesized Cu-modified g-C 3 N 4 for efficient mold resistance of woods and bamboo0Plastic Upcycling via Artificial Photosynthesis: A Green Conversion From Waste to Value‐Added Chemicals3Glycine photosynthesis via C−N coupling of waste plastic and nitrate over diatomic Pd−B catalyst17Modulating S-scheme charge transfer in Ag2Mo2O7/TiO2 nanobelt heterojunctions via interface engineering for enhanced photocatalysis and antimicrobial activity1Sustainable co-upcycling of waste PET plastic and ethylene glycol to high-value carboxylic acids on a carbon-encapsulated RuNi bimetallic catalyst4Enhanced electrochemical degradation of microcystin-lysine-arginine (MC-LR) using novel nickel oxide anodes in real water matrices1Process intensification driven by non-conventional energy fields in emerging plastic recycling: A systematic review2Electrocatalytic degradation strategies for plastic fibers with sustainable resource recovery potential4Sustainable photoreforming polyethylene terephthalate plastics into valuable chemicals with hydrogen generation over TiO2-carbon nanotubes composite0Photocatalyzed relay cleavage for the upcycling of gem-dimethyl-type plastics3Solar reforming of plastics using acid-catalyzed depolymerization20Unveiling roles of electron migration pathway supported by ion bridging and electron gain/loss properties of organic matter in peroxydisulfate activation for radicals boosted generation and dual nonradicals formation1Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Selective Photocatalytic Upcycling of Polystyrene Plastic to High-Value Chemicals by a Single-Atom Fe Catalyst7Dynamic coordination transformation from single-to dual-metal sites in MOFs for cascaded photoreforming of plastics into CO1Toward Standardized and Comparable Reporting for Sacrificial Photocatalytic Hydrogen Evolution2A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Waste plastic recycling and upgrading via electro- and photocatalytic C−X bond coupling1Advances in photocatalytic systems integrating CO2 reduction with value-added oxidation reactions0Atomic layer deposition technology and its applications in the synthesis of photocatalysts for organic reactions0Enhancing plastic photoreforming by modulating active radicals via lattice-matched heterointerfaces for frustrated Lewis pair formation1Harnessing Mechanical Energy for Catalysis: Mechanisms, Materials, and Applications of the Emerging Piezocatalysis Frontier0Interfacial Hydrophilicity Engineering in Photocatalysts: From Surface Reconstruction to Functional Applications0Tailoring alloy catalysts for electrocatalytic conversion of pollutants to value-added chemicals: ammonia synthesis, CO2 reduction, Ures synthesis and plastic upcycling1Regulating •OH generation via an S-scheme TiO2/CdZnS heterojunction for selective photocatalytic PET upcycling to glycolate1Solar-Driven Synergistic Photoreforming of PET and H2 Evolution over a ZnIn2S4–MoS2 Heterostructure04CzIPN-Br as an Effective Photoredox Organocatalyst for Visible-Light Aerobic Upcycling of Waste Polystyrene0Unconstrained Coordination of Pt Single Atoms on Distorted g‐C 3 N 4 Enables Electronic Flexibility and Enhanced Microplastics Photoreforming0Chemical Recycling of Polyester Wastes: Emerging Upcycling Technologies, Fundamental Mechanisms, Process Analysis, and Machine Learning1Photoreforming of Waste Plastics into H2 Using Zn x Cd1- x S Nanoplates Synthesized via Cation Exchange Reactions0Recent advances in catalytic technologies for plastic conversion: a review0Electro‐ and Photocatalytic C─X Bond Coupling in Valorization of Waste Plastics/Biomass: Reaction Mechanism and Catalyst Engineering1Transition-metals photocatalysts for lignin valorization toward sustainable biofuel production1Catalytic pyrolysis of waste plastics to liquid fuels: pathways, mechanisms, and challenges0From Traditional Depolymerization to Value-Added Upgrading: Upcycling of PET Fibers with Sustainable Chemistry and Renewable Energy0In Situ Hydrogen Utilization in Plastic Waste Recycling and Upcycling0Artificial Photoreforming Technology for Plastic Waste Valorization0

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  1. MOF-Derived CeO₂/Co₃O₄ Heterojunction Photocatalyst:,Synergistic Peroxymonosulfate Activation for PET Degradation

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  2. Plastic photoreforming: catalytic production of hydrogen and valuable chemicals

    Green Chemistry · 2025-01-01

    Heng Li, Yeqiong Huang, Yueyang Zhang, Haiyan Li, Chengcheng Shen, Dong Sheng Xia, Yanmei Zheng

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  3. Asymmetric Atomic Pt–B Dual-Site Catalyst for Efficient Photoreforming of Waste Polylactic Acid Plastics in Seawater

    ACS Nano · 2025-04-18

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  4. Photocatalytic recycling of polyethylene terephthalate: An emerging ecotechnology for environmental sustainability

    Journal of environmental chemical engineering · 2025-05-20

    Yuanbo Shi, Ziqi Yu, Sijia Bao, Xuenan Yang, Yuan Lu

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  5. State-of-the-Art Achievements and Challenges in Photochemical Conversion of Plastics to Chemicals and Composites

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    Arindam Modak, Jiamin Zheng, Fanyu Wang, Ailijiang Tuerdi, Abdukader Abdukayum, Xiao Liu

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  6. Photocatalytic Hydrogen Evolution Driven by Advanced Metal Sulfides from Sustainable Multilevel Biomass and Waste Plastics

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  7. Isomer-tailored vinylene-based COFs for photo-enhanced uranium extraction from seawater: Mechanistic insights into carrier dynamics and structural superiority

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  8. Catalysis in Renewable Energy: Theoretical Insights and Industrial Applications

    Renewable and Sustainable Energy Technology · 2025-07-16

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  9. Solar Fuels Production from Plastics and Biomass Photoreforming

    Energy & Fuels · 2025-07-22

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  10. Photocatalytic Waste Polystyrene Plastic Conversion: Reaction Mechanism and Catalyst Design

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  11. Diatomic Zn‐Functionalized Carbon Sphere for Microplastics Remediation in Natural Seawater at Environmentally Relevant Concentration

    Advanced Materials · 2025-07-29

    Shengbo Zhang, Penghui Li, Qikun Hu, Yingying Xue, Yanfen Wu, Helai Huang, Yu‐Xiao Zhang, Zongyang Ya, Ting Tan, Jingfu Liu, Zhiqiang Niu

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  12. Bias‐Free Photoelectrochemical System for Scalable Solar‐Driven Hydrogen Peroxide Production via Molecularly Engineered Conjugated Polycarbazole Frameworks

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    Lei Wang, Yuting Wu, Shengming Mao, Ji Zhou, Ying Zhang, Xusheng Zheng, Xiaojun Wu, Hangxun Xu

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  13. Solar‐Driven Plastic Upcycling Coupled with Valuable Reduction Reactions

    Advanced Sustainable Systems · 2025-08-20

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  14. Solar-powered photothermal-photocatalytic synergistic platform for simultaneous seawater desalination and antibiotic pollutant degradation

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  15. Nanocatalytic upcycling of plastic waste: Advances in selective conversion technologies for sustainable high-value products recovery

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  16. Advances and Outlook of In Situ Characterization Techniques for Photocatalytic Reforming of Plastic Wastes

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  17. Facile construction of HOF@ZnO/TiO2 ternary composite for efficient photocatalytic degradation of dyes

    Applied Surface Science · 2025-10-08

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  18. Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling

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  19. Cu‐Doped UiO‐66‐NH 2 Photocatalytic Cross‐Coupling of Arylamine C(sp 2 )‐H with Phenothiazine N─H Bonds

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  20. Preparation, Modification, and Application of Graphitic Carbon Nitride in Photocatalytic Degradation of Antibiotics

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  21. Design of S-scheme CuO/CeO2 heterojunction for photoreforming of polyethylene terephthalate plastic into value-added chemicals combined with hydrogen evolution

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  22. Interfacial engineering of CeO2/Bi19Br3S27 heterojunction for efficient photoreduction of CO2 to CO with nearly 100% selectivity

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  23. Depolymerization of polyesters catalyzed by binuclear metal complexes

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  24. Tandem depolymerization-electrocatalysis for plastic waste upcycling

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  25. Recent Advances in Photocatalytic Conversion of Furfural

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  26. Designing interfacial-engineered S-scheme heterostructures with dual-metal sulfides for efficient solar-to-hydrogen conversion

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  28. Bio‐Inspired Cascade Photocatalysis on Fe Single‐Atom Carbon Nitride Upcycles Plastic Wastes for Effective Acetic Acid Production

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  29. Upcycling Waste Polyethylene and Polypropylene into Carbon Oxides and Hydrocarbons via a Mechanochemistry-Photocatalysis Combined Technology under Mild Conditions

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  30. Beyond mechanical recycling: artificial photosynthesis enables polyester plastic upcycling into valuable chemicals

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  31. Electrospun Co3O4/CeO2 hollow nanotubes for photocatalytic degradation of PET Plastics with peroxymonosulfate Activation: Performance and DFT Insight

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  32. Electrospun nanotubular photocatalysts: Persulfate activation and DFT insight into polyethylene terephthalate degradation

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  33. Engineered nanocatalysts for degradation and valorisation of micro/nanoplastics

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  34. Ionic liquid photocatalysts in organic transformations

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  35. Key components for realistic application of plastic photoreforming coupled with H2 evolution

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  36. Microwave-synthesized Cu-modified g-C 3 N 4 for efficient mold resistance of woods and bamboo

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  37. Plastic Upcycling via Artificial Photosynthesis: A Green Conversion From Waste to Value‐Added Chemicals

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  38. Glycine photosynthesis via C−N coupling of waste plastic and nitrate over diatomic Pd−B catalyst

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  39. Modulating S-scheme charge transfer in Ag2Mo2O7/TiO2 nanobelt heterojunctions via interface engineering for enhanced photocatalysis and antimicrobial activity

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  40. Sustainable co-upcycling of waste PET plastic and ethylene glycol to high-value carboxylic acids on a carbon-encapsulated RuNi bimetallic catalyst

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  41. Enhanced electrochemical degradation of microcystin-lysine-arginine (MC-LR) using novel nickel oxide anodes in real water matrices

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  42. Process intensification driven by non-conventional energy fields in emerging plastic recycling: A systematic review

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  43. Electrocatalytic degradation strategies for plastic fibers with sustainable resource recovery potential

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  44. Sustainable photoreforming polyethylene terephthalate plastics into valuable chemicals with hydrogen generation over TiO2-carbon nanotubes composite

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  45. Photocatalyzed relay cleavage for the upcycling of gem-dimethyl-type plastics

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  46. Solar reforming of plastics using acid-catalyzed depolymerization

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  47. Unveiling roles of electron migration pathway supported by ion bridging and electron gain/loss properties of organic matter in peroxydisulfate activation for radicals boosted generation and dual nonradicals formation

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  48. Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis

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  49. Selective Photocatalytic Upcycling of Polystyrene Plastic to High-Value Chemicals by a Single-Atom Fe Catalyst

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  50. Dynamic coordination transformation from single-to dual-metal sites in MOFs for cascaded photoreforming of plastics into CO

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