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RESEARCH PAPER · Angewandte Chemie International Edition · 2022

Conversion of Polyethylenes into Fungal Secondary Metabolites

Chris Rabot, Yuhao Chen, Swati Bijlani, Yi‐Ming Chiang, C. Elizabeth Oakley, Berl R. Oakley, Travis J. Williams, Clay C. C. Wang

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Conversion of Polyethylenes into Fungal Secondary MetabolitesOriginalFrom green to circular chemistry paved by biocatalysis92Polystyrene Upcycling into Fungal Natural Products and a Biocontrol Agent82Distribution, sources, transportation and biodegradation of microplastics in the soil environment33Upcycling of polyethylenes by catalysis0Degradable and Recyclable Polyesters from Multiple Chain Length Bio‐ and Waste‐Sourceable Monomers54Degradable and Recyclable Polyesters from Multiple Chain Length Bio‐ and Waste‐Sourceable Monomers4A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds12Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis6Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Emerging green approaches for valorization of plastics with saturated carbon backbones42Synthesis and Deconstruction of Polyethylene-type Materials194Comparison of Methodologies for Microplastic Isolation through Multicriteria Analysis (AHP)7Sustainable Harnessing of Waste Polycarbonate for Synthesizing Activated Furans to Generate Stenhouse Adducts on Polymer Surface3Biological Upcycling of Plastics Waste37Bottlenecks in biobased approaches to plastic degradation114Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Circular Melt-Spun Textile Fibers from Polyethylene-like Long-Chain Polyesters7Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste70Catalytic Upcycling of Polyolefins316Oxidative degradation and upcycling of polyethylene wastes40The current progress of tandem chemical and biological plastic upcycling20Oxidative Upcycling of Polyolefin Wastes into the Dynamically Cross-Linked Elastomer25Deconstruction of carbon-carbon bonded polymers for biological conversion through COOH-functionalization and Fenton chemistry1Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds14Chemical bio-manufacture from diverse C-rich waste polymeric feedstocks using engineered microorganisms7Circular plastic economy for sustainable development: current advances and future perspectives49Co-upcycling of mixed polypropylene and polyesters5Phosphoramidates as promising low-loading flame retardants for low density polyethylene4Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization3Recycling homocarbon backbone polymers toward a circular materials economy12Aliphatic–Aromatic Copolyesters with Waste-Sourceable Multiple Chain-Length Building Blocks11A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown4Planetary sustainability science and technology: Integrating Astro-soil, Astro-environmental engineering and Astro-habitat engineering for space exploration9Recent progress in upcycling of plastic-derived intermediates into value-added chemicals via electrocatalytic strategies – A review1Mixed polyamide and polyester upcycling via chemical autoxidation and engineered Pseudomonas putida4Engineering microbial consortia for mixed plastic upcycling27A Multi‐step Synergistic Strategy for Upgrading Plastic Waste into Circular Economy Feedstocks1Carbon–carbon bond cleavage for lignin and plastics deconstruction0Environmental Applications of Fungal Secondary Metabolites0Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Catalytic Autoxidation for Depolymerization of Multilayer Plastic Films0Recent Advancements in Chemical Valorization of Legacy and Emerging Fiber‐Reinforced Polymer Composites2Plastic Waste Upgrading by Biological Funneling: The Case for Fungal Platforms0The Biosynthesis of a Fungal Flavonoid, Chlorflavonin, Precisely Controlled by Two Types of Equilibrium States0

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  1. From green to circular chemistry paved by biocatalysis

    Green Chemistry · 2023-01-01

    Pedro Lozano, Eduardo García‐Verdugo

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  2. Polystyrene Upcycling into Fungal Natural Products and a Biocontrol Agent

    Journal of the American Chemical Society · 2023-02-13

    Chris Rabot, Yuhao Chen, Shu-Yi Lin, Ben Miller, Yi‐Ming Chiang, C. Elizabeth Oakley, Berl R. Oakley, Clay C. C. Wang, Travis J. Williams

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  3. Distribution, sources, transportation and biodegradation of microplastics in the soil environment

    TrAC Trends in Analytical Chemistry · 2023-05-19

    Yizheng Li, Qinghui Liu, Muhammad Junaid, Guanglong Chen, Jun Wang

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  4. Upcycling of polyethylenes by catalysis

    Unknown journal · 2023-07-20

    Adamu Aminu Idris

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  5. Degradable and Recyclable Polyesters from Multiple Chain Length Bio‐ and Waste‐Sourceable Monomers

    Angewandte Chemie International Edition · 2023-09-07

    Taylor F. Nelson, Dario Rothauer, Michael Sander, Stefan Mecking

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  6. Degradable and Recyclable Polyesters from Multiple Chain Length Bio‐ and Waste‐Sourceable Monomers

    Angewandte Chemie · 2023-09-07

    Taylor F. Nelson, Dario Rothauer, Michael Sander, Stefan Mecking

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  7. A facile methodology for side- and upcycling of HDPE waste via partial creation of unsaturated double bonds

    Green Chemistry · 2024-01-01

    Wenyu Wu, Lucie Perret, Patrick Rupper, Sandro Lehner, Xiaoyu Zhou, Henrik Eliasson, Rico Muff, Manfred Paul Heuberger, Sabyasachi Gaan

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  8. Controlled degradation of chemically stable poly(aryl ethers) via directing group-assisted catalysis

    Chemical Science · 2024-01-01

    Satoshi Ogawa, Hiroki Morita, Yu‐I Hsu, Hiroshi Uyama, Mamoru Tobisu

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  9. Catalytic conversion of mixed polyolefins under mild atmospheric pressure

    The Innovation · 2024-02-03

    Binzhi Zhao, Hui Tan, Jie Yang, Xiaohui Zhang, Zidi Yu, Han‐Li Sun, Jialiang Wei, Xinyi Zhao, Yufeng Zhang, Lili Chen, Dali Yang, Jin Deng, Yao Fu, Zheng Huang, Ning Jiao

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  10. Emerging green approaches for valorization of plastics with saturated carbon backbones

    Trends in Chemistry · 2024-02-05

    Bao‐Nguyen T. Nguyen, Jason Y. C. Lim

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  11. Synthesis and Deconstruction of Polyethylene-type Materials

    Chemical Reviews · 2024-02-26

    Simon Timm Schwab, Maximilian Baur, Taylor F. Nelson, Stefan Mecking

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  12. Comparison of Methodologies for Microplastic Isolation through Multicriteria Analysis (AHP)

    Microplastics · 2024-03-10

    Valentina Phinikettou, Iliana Papamichael, Irene Voukkali, Antonis A. Zorpas

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  13. Sustainable Harnessing of Waste Polycarbonate for Synthesizing Activated Furans to Generate Stenhouse Adducts on Polymer Surface

    Chemistry - An Asian Journal · 2024-04-10

    Lisa Zeußel, Shefali Chowdhary, Haocheng Wu, Vipan Kumar, Sukhdeep Singh

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  14. Biological Upcycling of Plastics Waste

    Annual Review of Chemical and Biomolecular Engineering · 2024-04-15

    Ross R. Klauer, D. Alex Hansen, Derek Wu, Lummy Maria Oliveira Monteiro, Kevin Solomon, Mark Blenner

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  15. Bottlenecks in biobased approaches to plastic degradation

    Nature Communications · 2024-06-03

    Amelia R. Bergeson, Ashli J. Silvera, Hal S. Alper

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  16. Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling

    Advanced Materials · 2024-06-13

    Shuangqiao Yang, Yijun Li, Min Nie, Xingang Liu, Qi Wang, Ning Chen, Chuhong Zhang

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  17. Circular Melt-Spun Textile Fibers from Polyethylene-like Long-Chain Polyesters

    ACS Applied Polymer Materials · 2024-07-30

    Katrin Wurst, Melissa Birkle, Katharina J. Scherer, Stefan Mecking

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  18. Industrial and Laboratory Technologies for the Chemical Recycling of Plastic Waste

    ACS Catalysis · 2024-08-05

    Mason T. Chin, Tianning Diao

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  19. Catalytic Upcycling of Polyolefins

    Chemical Reviews · 2024-08-16

    Jia‐Kai Sun, Jinhu Dong, Lijun Gao, Yu‐Quan Zhao, Hyunjin Moon, Susannah L. Scott

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  20. Oxidative degradation and upcycling of polyethylene wastes

    Science China Chemistry · 2024-08-23

    Yizhen Che, Yanfen Wu, Zhiqiang Niu

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  21. The current progress of tandem chemical and biological plastic upcycling

    Biotechnology Advances · 2024-10-10

    Yifeng Hu, Yuxin Tian, Chenghao Zou, Tae Seok Moon

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  22. Oxidative Upcycling of Polyolefin Wastes into the Dynamically Cross-Linked Elastomer

    Macromolecules · 2024-10-23

    Yinlong Chang, Yangke Xiao, Minghao Sun, Weiqiang Gao, Liqian Zhu, Qingyue Wang, Wenjun Wang, Bo‐Geng Li, Pingwei Liu

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  23. Deconstruction of carbon-carbon bonded polymers for biological conversion through COOH-functionalization and Fenton chemistry

    Polymer Degradation and Stability · 2024-11-12

    Amit K. Jha, Daniella V. Martinez, Jay E. Salinas, Estevan J. Martinez, Ryan D. Davis, Alberto Rodriguez, Hemant Choudhary, Michael S. Kent, Oleg Davydovich

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  24. Low‐Temperature Catalytic Approaches for Upcycling Plastics into Oxygenated Aromatic Compounds

    ChemCatChem · 2024-11-19

    Jason Y. C. Lim

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  25. Chemical bio-manufacture from diverse C-rich waste polymeric feedstocks using engineered microorganisms

    RSC Sustainability · 2025-01-01

    Maria Franca Pitzalis, Joanna C. Sadler

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  26. Circular plastic economy for sustainable development: current advances and future perspectives

    RSC Sustainability · 2025-01-01

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  27. Co-upcycling of mixed polypropylene and polyesters

    Green Chemistry · 2025-01-01

    Xiangyue Wei, Qiang Zhang, Chengfeng Shen, Pengbo Ye, Jin Xu, Xuehui Liu, Zhishan Su, Shimei Xu, Yu‐Zhong Wang

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  28. Phosphoramidates as promising low-loading flame retardants for low density polyethylene

    Polymer Degradation and Stability · 2025-01-25

    Alejandro Fonseca, Carlos Alberto Márquez, Nikolaos S. Giakoumakis, Ivica Ðuretek, Eleni Pachatouridou, Stylianos D. Stefanidis, Maarten Rubens, Angelos A. Lappas, Thomas Lucyshyn, Dirk E De Vos

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  29. Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization

    Organic Letters · 2025-01-31

    Ryota Shiraki, Yu‐I Hsu, Hiroshi Uyama, Mamoru Tobisu

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  30. Recycling homocarbon backbone polymers toward a circular materials economy

    Chem · 2025-02-10

    Jie Zheng, Zhuang Mao Png, Xin Yi Oh, H.Y. Zuo, Zibiao Li

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  31. Aliphatic–Aromatic Copolyesters with Waste-Sourceable Multiple Chain-Length Building Blocks

    ACS Sustainable Chemistry & Engineering · 2025-02-19

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  32. A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown

    Journal of the American Chemical Society · 2025-05-13

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  33. Planetary sustainability science and technology: Integrating Astro-soil, Astro-environmental engineering and Astro-habitat engineering for space exploration

    The Science of The Total Environment · 2025-06-27

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  34. Recent progress in upcycling of plastic-derived intermediates into value-added chemicals via electrocatalytic strategies – A review

    Next research. · 2025-07-31

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  35. Mixed polyamide and polyester upcycling via chemical autoxidation and engineered Pseudomonas putida

    Reaction Chemistry & Engineering · 2025-09-19

    Ross Eaglesfield, Brandon L. Frey, Ciaran W. Lahive, Amy A. Cuthbertson, Eugene Kuatsjah, Kelsey J. Ramirez, Young-Saeng Cho Avina, Hannah M. Alt, Natalie Banakis, Katrina M. Knauer, Gregg T. Beckham, Allison Z. Werner

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  36. Engineering microbial consortia for mixed plastic upcycling

    Nature Communications · 2025-12-11

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  37. A Multi‐step Synergistic Strategy for Upgrading Plastic Waste into Circular Economy Feedstocks

    ChemPlusChem · 2026-01-01

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  38. Carbon–carbon bond cleavage for lignin and plastics deconstruction

    Chemical Society Reviews · 2026-01-01

    Davide Rigo, Brandon L. Frey, Alison Sy-min Chang, Marcos G. Farpón, Erik T. Ouellette, Yuriy Román‐Leshkov, Gregg T. Beckham, Joseph S. M. Samec

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  39. Environmental Applications of Fungal Secondary Metabolites

    Springer eBooks · 2026-01-01

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  40. Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins

    Chinese Journal of Organic Chemistry · 2026-01-01

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  41. Catalytic Autoxidation for Depolymerization of Multilayer Plastic Films

    ChemSusChem · 2026-04-13

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  42. Recent Advancements in Chemical Valorization of Legacy and Emerging Fiber‐Reinforced Polymer Composites

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  43. Plastic Waste Upgrading by Biological Funneling: The Case for Fungal Platforms

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  44. The Biosynthesis of a Fungal Flavonoid, Chlorflavonin, Precisely Controlled by Two Types of Equilibrium States

    Journal of the American Chemical Society · 2026-08-29

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