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RESEARCH PAPER · Nature Reviews Chemistry · 2022

A unified view on catalytic conversion of biomass and waste plastics

Kyungho Lee, Yaxuan Jing, Yanqin Wang, Ning Yan

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A unified view on catalytic conversion of biomass and waste plasticsOriginalA state-of-the-art review on waste plastics-derived aviation fuel: Unveiling the heterogeneous catalytic systems and techno-economy feasibility of catalytic pyrolysis78Understanding the Structure–Activity Relationships in Catalytic Conversion of Polyolefin Plastics by Zeolite-Based Catalysts: A Critical Review269Recent progress in photoelectrocatalysis beyond water oxidation46Hydrogenolysis‐Isomerization of Waste Polyolefin Plastics to Multibranched Liquid Alkanes59Catalytic hydroconversion processes for upcycling plastic waste to fuels and chemicals94A room temperature dissolution solvent and its mechanism for natural biopolymers: hydrogen bonding interaction investigation47Acid hydrolysis of chitin in calcium chloride solutions30Catalytic conversion of chitin as a nitrogen-containing biomass45Electroreforming injects a new life into solid waste39From vanillin to biobased aromatic polymers70Microwave-enhanced hydrogen production: a review56Recent advances in plastic recycling and upgrading under mild conditions147Waste to wealth: direct utilization of spent materials for electrocatalysis and energy storage43Cooperative catalysis of Co single atoms and nanoparticles enables selective CAr−OCH3 cleavage for sustainable production of lignin-based cyclohexanols86Machine-learning atomic simulation for heterogeneous catalysis90RETRACTED: Metal-organic framework-based nanostructured catalysts: Applications in biomass conversion30A novel method for industrial production of clean hydrogen (H2) from mixed plastic waste42Heterolytic dissociation of H2 and bond activation: Spotting new opportunities from a unified view38Debromination with Bromine Recovery from Pyrolysis of Waste Printed Circuit Boards Offers Economic and Environmental Benefits45Catalytic Amounts of an Antibacterial Monomer Enable the Upcycling of Poly(Ethylene Terephthalate) Waste59Photoredox-Catalyzed Plastic Waste Conversion: Nonselective Degradation versus Selective Synthesis110Analysis of the Scale of Global Human Needs and Opportunities for Sustainable Catalytic Technologies42Artificial photosynthesis bringing new vigor into plastic wastes63Rational design of photo− /electro−catalytic systems for the transformation of plastic wastes51Heterogeneous Interface Catalysts with Electron Local Exchange toward Highly Selective Oxidation of Biomass Platform Compounds62Photocatalysis as an Effective Tool for Upcycling Polymers into Value‐Added Molecules87Electrochemical Production of Glycolate Fuelled By Polyethylene Terephthalate Plastics with Improved Techno‐Economics136Net Zero Transition: Possible Implications for Catalysis36TiO2 nanoparticle supported Ru catalyst for chemical upcycling of polyethylene terephthalate to alkanes29Design of a bifunctional catalyst by alloying Ni with Ru-supported H-beta for selective hydrodeoxygenation of bisphenol A and polycarbonate plastic waste94Effects of cellulose addition on the physicochemical properties, pore structure and iodine adsorption of lignin-based biochar28Acetalization strategy in biomass valorization: a review64Ni/HZSM-5 catalysts for hydrodeoxygenation of polycarbonate plastic wastes into cycloalkanes for sustainable aviation fuels77Insight into pyrolysis mechanism of plastic waste with C-O/C-N bonds in the backbone58Waste to wealth: H2S-free fabrication of Fe-ZnS/NC by industrial lignin self S-doping for efficient lignin aerobic oxidation32Ni-catalyzed carbon–carbon bonds cleavage of mixed polyolefin plastics waste42Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers94Regulating the Interaction within Pd-Cu Dual Metal Sites for Selective Hydrogenation of Furfural Using Ambient H2 Pressure41Chemical Upcycling of PET into a Morpholine Amide as a Versatile Synthetic Building Block27Partial hydrogenation of anisole to cyclohexanone in water medium catalyzed by atomically dispersed Pd anchored in the micropores of zeolite36Conversion of organic solid waste into energy and functional materials using biochar catalyst: Bibliometric analysis, research progress, and directions81Outlooks for zeolite catalysts in a low-carbon scenario32Hydrocracking of polyethylene to hydrocarbon fuels over Pt/USY catalysts: Assessment of the hydrogen donors28From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100IrOx-MoO3 nano-heterostructure electrocatalysts for efficient acidic water oxidation27Unraveling the potential-dependent structure evolution in CuO for electrocatalytic biomass valorization55Solar-driven photocatalysis for recycling and upcycling plastics122Co-upcycling of polyvinyl chloride and polyesters199Advances in Biocarbon and Soft Material Assembly for Enthalpy Storage: Fundamentals, Mechanisms, and Multimodal Applications26Enhancing polyethylene terephthalate conversion through efficient microwave-assisted deep eutectic solvent-catalyzed glycolysis29Catalytic Conversion of Lignin into Valuable Chemicals: Full Utilization of Aromatic Nuclei and Side Chains99Precise activation of C–C bonds for recycling and upcycling of plastics81Spin Polarization: A New Frontier in Efficient Photocatalysis for Environmental Purification and Energy Conversion26Boosting strong metal-support interactions between Ru and sodium titanate nanowire for hydrogenolysis of polyolefins under mild conditions44Selective C–C and C–O bond cleavage strategies for the thermochemical upgrading of (hemi)cellulosic biomass44A review of comprehensive utilization of biomass to synthesize carbon nanotubes: From chemical vapor deposition to microwave pyrolysis44Transition metals-catalyzed amination of biomass feedstocks for sustainable construction of N-heterocycles130Recent advancement on photocatalytic plastic upcycling90Synthesis of JP-10 analogues high-density fuels via one-pot Diels-Alder/hydrodeoxygenation reaction25Acid catalyst screening for hydrolysis of post-consumer PET waste and exploration of acidolysis69Heterogeneous catalysis for the environment92Multivalent cobalt nanoparticles supported on silica for efficient and sustainable methanolysis of commercial polyethylene terephthalate waste bottles34Recent catalytic innovations in furfural transformation97Polyethylene Upgrading to Liquid Fuels Boosted by Atomic Ce Promoters74Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Sustainable microwave-driven CO2 gasification of plastic waste for high-yield H2 and CO production47The forefront of chemical engineering research43Synergy of heterogeneous Co/Ni dual atoms enabling selective C–O bond scission of lignin coupling with in-situ N-functionalization60Solar reforming as an emerging technology for circular chemical industries182A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30Research advances on the catalytic conversion of biomass-derived furfural into pentanediols35Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Carbon deposition behavior on biochar during chemical vapor deposition process30Synergy between Cu and Lewis Acidic Sites in Cu/Zn-FeOx Catalysts for the Selective Conversion of Poly(ethylene terephthalate) Waste to p-Xylene and Ethylene Glycol36Chemical recycling of waste plastics: Current challenges and perspectives37Upgrading waste plastics to value-added aromatics30Tandem catalysis enables chlorine-containing waste as chlorination reagents48Food waste management and sustainable waste to energy: Current efforts, anaerobic digestion, incinerator and hydrothermal carbonization with a focus in Malaysia91Stable Interfacial Ruthenium Species for Highly Efficient Polyolefin Upcycling104Perspectives on sustainable plastic treatment: A shift from linear to circular economy39Studies on hydrolysis/alcoholysis/ammonolysis mechanisms of ethylene terephthalate dimer using DFT method29Catalytic Hydrogenolysis by Atomically Dispersed Iron Sites Embedded in Chemically and Redox Non-innocent N-Doped Carbon28Layered Double Hydroxide Derivatives for Polyolefin Upcycling103Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Catalytic Consequences of Hierarchical Pore Architectures within MFI and FAU Zeolites for Polyethylene Conversion54Selective Photoreforming of Waste Plastics into Diesel Olefins via Single Reactive Oxygen Species51Photocatalysis toward Microplastics Conversion: A Critical Review148Microwave‐Assisted Pyrolysis‐A New Way for the Sustainable Recycling and Upgrading of Plastic and Biomass: A Review46Counterintuitive chemoselectivity in the reduction of carbonyl compounds27Progress and Perspective for “Green” Strategies of Catalytic Plastics Conversion into Fuels by Regulating Half-Reactions102Municipal Solid and Plastic Waste Co‐pyrolysis Towards Sustainable Renewable Fuel and Carbon Materials: A Comprehensive Review38Photorefinery of Biomass and Plastics to Renewable Chemicals using Heterogeneous Catalysts96Atomic Co/Cu Dual‐Metal for Rapid Conversion of 5‐Hydroxymethylfurfural under Ambient Pressure45From Ethylene Glycol to Glycolic Acid: Electrocatalytic Conversion on Pt-Group Metal Surfaces41Advancing Recyclable Thermosets through C═C/C═N Dynamic Covalent Metathesis Chemistry36Unlocking opportunities: Supported metal catalysts for the chemical upcycling of waste plastics26Waste plastics upcycled for high-efficiency H2O2 production and lithium recovery via Ni-Co/carbon nanotubes composites63Chemoselective Hydrogenolysis of Urethanes to Formamides and Alcohols in the Presence of More Electrophilic Carbonyl Compounds27Two-dimensional single-crystalline mesoporous high-entropy oxide nanoplates for efficient electrochemical biomass upgrading77Catalytic Upcycling of Polyolefins316Catalytic recycling of plastics into value-added products28Visible Light‐Switchable Lattice Oxygen Sites for Selective C−H and C(O)−C Bond Electrooxidation30Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Designing 2D carbon dot nanoreactors for alcohol oxidation coupled with hydrogen evolution75Grave-to-cradle dry reforming of plastics via Joule heating64Optimization of PET depolymerization for enhanced terephthalic acid recovery from commercial PET and post consumer PET-bottles via low-temperature alkaline hydrolysis36Novel Feruloyl Esterase for the Degradation of Polyethylene Terephthalate (PET) Screened from the Gut Microbiome of Plastic-Degrading Mealworms ( Tenebrio Molitor Larvae)37Inverse ceria-nickel catalyst for enhanced C–O bond hydrogenolysis of biomass and polyether61Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Evaluation of char properties from co-pyrolysis of biomass/plastics: Effect of different types of plastics42Selective Oxidation of Polyesters via PdCu–TiO 2 Photocatalysts in Flow60Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Polyethylene hydrogenolysis by dilute RuPt alloy to achieve H2-pressure-independent low methane selectivity70Microwave‐Powered Liquid Metal Degradation of Polyolefins30Autogenetic Carbon Oxyanions Enable Interfacial OH − Deconfinement for Reinforced Biomass Electrooxidation over Wide Potential Window39Co-pyrolysis of biomass and plastic waste into carbon materials with environmental applications: a critical review109Optimizing CO 2 electroreduction: theoretical insights for enhancing efficiency across elementary steps65Sustainable thermochemical plastic valorization towards a circular economy: a critical review27Advanced Catalysts for the Chemical Recycling of Plastic Waste90Green coal and lubricant via hydrogen-free hydrothermal liquefaction of biomass30Photocatalytic upcycling of polylactic acid to alanine by sulfur vacancy-rich cadmium sulfide103Recent progress on the synergistic preparation of liquid fuels by co-pyrolysis of lignocellulosic biomass and plastic wastes35Bimetallic synergy in supported Ni–Pd catalyst for selective hydrogenolysis of C–O bonds in epoxy resins39Photocatalytic Upgrading of Plastic Waste into High-Value-Added Chemicals and Fuels: Advances and Perspectives49Highly selective upcycling of plastic mixture waste by microwave-assisted catalysis over Zn/b-ZnO68Catalysis Enhanced by Catalyst Wettability46Photothermocatalytic Wet Reforming of Waste Plastics to Syngas45Photocatalytic and Electrochemical Synthesis of Biofuel via Efficient Valorization of Biomass132Selectively Steering the Retention and Cleavage of C–C Bond in Electrooxidation of PET Plastic and Biomass-Derived Alcohols by Defective Ni(OH)2–x-Supported Pt67High-Performance Nickel Phosphide Confined in SBA-15 for Low-Temperature Hydrogenation of Biomass-Derived Compounds25Singlet‐Oxygen‐Driven Cooperative Photocatalytic Coupling of Biomass Valorization and Hydrogen Peroxide Production Using Covalent Organic Frameworks90Singlet‐Oxygen‐Driven Cooperative Photocatalytic Coupling of Biomass Valorization and Hydrogen Peroxide Production Using Covalent Organic Frameworks28Upcycling waste commodity polymers into high-performance polyarylate materials with direct utilization of capping agent impurities34Selective Asymmetric Hydrogenation of Waste Polyethylene Terephthalate via Controlled Sorption through Precisely Tuned Moderate Acid Sites50Unexpected persistent production of H2O2 during tetrabromobisphenol A photocatalytic degradation based on interface carrier regulation36Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Stable Ni(II) sites in Prussian blue analogue for selective, ampere-level ethylene glycol electrooxidation81Recent advances in pyrolysis upcycling of waste plastics into hydrocarbon fuels on biochar-based catalysts28Co-recycling of plastics and other waste materials70Cost‐Effective and Low‐Carbon Scalable Recycling of Waste Polyethylene Terephthalate Through Bio‐Based Guaiacol‐Enhanced Methanolysis30Hydrogen Spillover‐Induced Brønsted Acidity Enables Controllable Hydrocracking of Polyolefin Waste to Liquid Fuels32Synergistic Catalysis for Recycling and Upcycling of Plastics35Photocatalytic Hydrogen Evolution Driven by Advanced Metal Sulfides from Sustainable Multilevel Biomass and Waste Plastics51Rational Design of Advanced Functional Catalysts for Photo‐Reforming Glucose into Bio‐Derived Fuels and Chemicals29Selective electrified polyethylene upcycling by pore-modulated pyrolysis25Biochar-driven rhizoremediation of soil contaminated with organic pollutants: engineered solutions, microbiome enrichment, and bioeconomic benefits for ecosystem restoration27Low-coordination PtBi heterogeneous interface boosting the selective electrooxidation of ethylene glycol to value-added glycolic acid26Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32Solar-Driven Upcycling of Polylactic Acid to Alanine over Pt/CdS–TiO 2 Heterojunction Single-Atom Photocatalyst35Near-infrared plasmonic activation of molecular oxygen for selective oxidation of biomass derivatives41

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