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RESEARCH PAPER · Nature Reviews Chemistry · 2022

Control of light, spin and charge with chiral metal halide semiconductors

Haipeng Lu, Zeev Valy Vardeny, Matthew C. Beard

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Control of light, spin and charge with chiral metal halide semiconductorsOriginalChiral three-dimensional supramolecular assemblies: colloidal onions, cubosomes, and hexosomes4The chemistry and physics of organic—inorganic hybrid perovskite quantum wells10A chiral lead-free tin(IV)-based halide organic-inorganic semiconductor with dielectric switching and phase transition44Revealing the Intrinsic Chiroptical Activity in Chiral Metal-Halide Semiconductors132Organic-inorganic hybrid perovskites and their heterostructures45Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers56Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers12A chiral two-dimensional perovskite-like lead-free bismuth( iii ) iodide hybrid with high phase transition temperature15A photoluminescent chiral lead-free hybrid ferroelastic semiconductor with switchable second-harmonic generation23Amplification of polarization ratio is observed in monolayer Dion–Jacobson hybrid perovskites6Atomistic modeling of metal–ligand chirality transfer and chiroptical properties of lead and tin hybrid perovskites23Broadband emission originating from the stereochemical expression of 6s 2 lone pairs in two-dimensional lead bromide perovskites11Chiral mesostructured NiFe 2 O 4 films with chirality induced spin selectivity6Circularly polarized luminescence and nonlinear optical harmonic generation based on chiral zinc halides23Linear optical afterglow and nonlinear optical harmonic generation from chiral tin( iv ) halides: the role of lattice distortions37Spin-photogalvanic effect in chiral lead halide perovskites30The rise of halide perovskite semiconductors137Resonant Second Harmonic Generation in Proline Hybrid Lead Halide Perovskites56Materials for chiral light control235An Organic Chiroptical Detector Favoring Circularly Polarized Light Detection from Near‐Infrared to Ultraviolet and Magnetic‐Field‐Amplifying Dissymmetry in Detectivity33Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime41Spin Polarization of Chiral Amorphous Fe‐Ni Electrocatalysts Enabling Efficient Electrochemical Oxygen Evolution67Chirality induced spin selectivity: A classical spin-off3Highly‐Active Chiral Organic Photovoltaic Catalysts with Suppressed Charge Recombination43Highly‐Active Chiral Organic Photovoltaic Catalysts with Suppressed Charge Recombination3Spin selectivity of chiral mesostructured diamagnetic BiOBr films28Research progress in spintronics of chiral perovskite materials4Chiral Perovskite Nanocrystals for Asymmetric Reactions: A Highly Enantioselective Strategy for Photocatalytic Synthesis of N–C Axially Chiral Heterocycles50Achiral Fluorinated Aromatic Ligands Based Chiral Hybrid Antimony Halides with High‐Efficiency Second‐Harmonic Generation18Chirality Versus Symmetry: Electron's Spin Selectivity in Nonpolar Chiral Lead–Bromide Perovskites55Chiral Inorganic Nanomaterials for Photo(electro)catalytic Conversion71High-performance metal halide perovskite transistors160Interlayer Polymerization of 2D Chiral Perovskite Single‐Crystal Films toward High‐Performance Flexible Circularly Polarized Light Detection46Spatially Correlated Chirality in Chiral Two-Dimensional Perovskites Revealed by Second-Harmonic-Generation Circular Dichroism Microscopy56Chiral Ligand‐Induced Inversion and Tuning of Excitonic Optical Activity in Intrinsically Chiral CsPbBr3 Perovskite Nanoplatelets32Fundamentals, Advances, and Artifacts in Circularly Polarized Luminescence (CPL) Spectroscopy165Chirality induced spin selectivity in chiral hybrid organic–inorganic perovskites36Chiral Lead Halide Perovskite Nanocrystals: Construction Strategies and Photophysical Properties11MatGPT: A Vane of Materials Informatics from Past, Present, to Future74Conditions for EPR detection of chirality-induced spin selectivity in spin-polarized radical pairs in isotropic solution7Nonlinear optical properties in chiral copper oxide nanosheets3Synthesis and Optical Properties of One Year Air-Stable Chiral Sb(III) Halide Semiconductors16Spin-dependent electrochemistry and electrochemical enantioselective recognition with chiral methylated bis(ethylenedithio)-tetrathiafulvalenes12Cluster-assembled superatomic crystals for chirality-dependent charge-to-spin conversion2Free Halogen Substitution of Chiral Hybrid Metal Halides for Activating the Linear and Nonlinear Chiroptical Properties140Homochirality in Ferroelectrochemistry32Spin Chiral Anisotropy of Chiral Mesostructured Inorganic Materials with Different Intrinsic Magnetisms30Extended Honeycomb Metal Chloride with Tunable Antiferromagnetic Correlations7Boosting circularly polarized luminescence by optimizing off-centering octahedral distortion in zero-dimensional hybrid indium-antimony halides29Multi-stimuli-responsive luminescence enabled by crown ether anchored chiral antimony halide phosphors55Variable energy transfer in one-dimensional chiral Mn/Cd-based halides and strong stereo-selective fluorescence for chiral recognition5Electron-donating functional groups strengthen ligand-induced chiral imprinting on CsPbBr3 quantum dots22Chiral Multidentate Ligand Facilitating Perovskite Nanocrystals with Circularly Polarized Luminescence and Chiral Assembly27Bright Circularly Polarized Mechanoluminescence from 0D Hybrid Manganese Halides101Topological Nodal-Point Superconductivity in Two-Dimensional Ferroelectric Hybrid Perovskites9Induced Circularly Polarized Luminescence and Exciton Fine Structure Splitting in Magnetic-Doped Chiral Perovskites12Luminescent metal-halide perovskites: fundamentals, synthesis, and light-emitting devices20Chiral photon emission from a chiral–achiral perovskite heterostructure3Inducing Circularly Polarized Single-Photon Emission via Chiral-Induced Spin Selectivity28Perovskite versus Nonperovskite: Modulating the Nature and Optical Properties of One-Dimensional Chiral Lead–Bromide Networks15Structure-Guided Approaches for Enhanced Spin-Splitting in Chiral Perovskite42Spin-polarized white organic light-emitting diodes based on chirality-induced spin selectivity effect2Dimensional and Doping Engineering of Chiral Perovskites with Enhanced Spin Selectivity for Green Emissive Spin Light-Emitting Diodes44Highly Emissive Organic Antimony Halide with Ferromagnetism and Methanol Sensing Properties7Self-Powered Circularly Polarized Light Detection Enabled by Chiral Two-Dimensional Perovskites with Mixed Chiral–Achiral Organic Cations42Experimental Evidence of the Molecular and Macroscopic Origins of Circular Dichroism in Chiral Metal‐Halide Networks10High Field Electrical Polarization and Magnetoelectric Coupling in Chiral Magnet [Cu(pym)(H2O)4]SiF6·H2O4Room-temperature spin injection across a chiral perovskite/III–V interface100A chemical perspective on the chiral induced spin selectivity effect56Chirality‐Induced Memristor of Chiral Nanostructured Half‐Metallic Fe 3 O 4 Films12Fluorinated Organic Cations Derived Chiral 2D Perovskite Enabling Enhanced Spin‐Dependent Oxygen Evolution Reaction11Nonadiabatic Molecular Dynamics in Momentum Space Beyond Harmonic Approximation: Hot Electron Relaxation in Photoexcited Black Phosphorus10Phase Transition of a Chiral Lead‐Free Hybrid Antimony(III) Halide Crystal2Boosted Chirality Transfer in 2D Perovskites through Structural Isomer‐Driven Halogen–Halogen Interaction33Synthesis and growth of solution-processed chiral perovskites12Engineering spin-dependent catalysts: chiral covalent organic frameworks with tunable electroactivity for electrochemical oxygen evolution32Dimensional control of chiral perovskites for high-performance circularly polarized light detection via ligand engineering14Macroscopic Twisting of Chiral Metal Halide Single Crystals Driven by Thermo-Induced Topochemical Dehydration31Review of Polarized Light‐Spin/Dipole Interactions: Fundamental Physics and Application in Circularly Polarized Detecting25Chiral Perovskite Nanowire Optoelectronic Synapse for Full‐Stokes Polarization‐Resolved Perception and Reservoir Computing27Enhancing Chiroptoelectronic Activity in Chiral 2D Perovskites via Chiral–Achiral Cation Mixing11A-Site Cation Chemistry in Halide Perovskites123Remote chirality transfer in low-dimensional hybrid metal halide semiconductors67Regulating Second‐Harmonic Generation in 2D Chiral Perovskites Through Achiral Organic Spacer Cation Alloying Strategy15Is There an Optimal Spacer Cation for Two-Dimensional Lead Iodide Perovskites?18Efficient circularly polarized luminescence from zero-dimensional terbium- and europium-based hybrid metal halides23From the Bulk to the Nanoscale: Strong Evolution in the Structure and Chiroptical Properties of Chiral Halide Double Perovskites5Design of Two-Dimensional Hybrid Perovskites with Giant Spin Splitting and Persistent Spin Textures33Chiroptical Synaptic Perovskite Memristor as Reconfigurable Physical Unclonable Functions53Exciton Transport in Perovskite Materials46Chiral hybrid manganese( ii ) chloride single crystals for achieving second harmonic generation and moderate circularly polarized luminescence4Chirality-driven dimensionality and broadband emission in lead bromide perovskites6Customizing circularly polarized afterglow by stepwise chiral amplification in BINAPs/BINAPOs8Machine learning-driven prediction of ultrafast spin relaxation in metal halide perovskites for spintronic applications5Spin effects in metal halide perovskite semiconductors25Self-assembly of chiroptical ionic co-crystals from silver nanoclusters and organic macrocycles32Green Spin Light-Emitting Diodes Enabled by Perovskite Nanocrystals in Situ Modified with Chiral Ligands42Roadmap on metal-halide perovskite semiconductors and devices17Efficient Spin‐Light‐Emitting Diodes With Tunable Red to Near‐Infrared Emission at Room Temperature39Chiral Inorganic Nanomaterial‐Based Diagnosis and Treatments for Neurodegenerative Diseases32Chiral light–matter interactions in solution-processable semiconductors60High‐Performance Sky‐Blue Perovskite Spin‐Light Emitting Diodes Due to Chiral Ionic Liquid Implantation and Passivation18Chiral-Polar Photovoltage-Driven Efficient Self-Powered Circularly Polarized Light Detection in Three-Dimensional Hybrid Perovskites21Circularly polarized electroluminescence from chiral supramolecular semiconductor thin films120Chiral europium halides with high-performance magnetic field tunable red circularly polarized luminescence at room temperature49Humidity Disrupts Structural and Chiroptical Properties of Chiral 2D Perovskites17Two-dimensional organic-inorganic hybrid perovskite quantum-well nanowires enabled by directional noncovalent intermolecular interactions24Elucidating Interfacial Carrier Transfer Dynamics for Circularly Polarized Emission in Self-Assembled Perovskite Heterostructures7Chiral metal halide perovskites toward room temperature spin light-emitting diodes: Insights and perspectives9Two-photon excited spin excitonic properties in two-dimensional chiral perovskite films1Circularly Polarized Luminescence in Achiral Tin-Based Perovskites via Structural Isomer-Driven Coordination Interaction11Controlling the Orientation of Polar Axis in Chiral Metal‐Halides to Reveal Their Intrinsic Circularly Polarized Luminescence5Tuning Interlayer Couplings and Stabilizing 2D Perovskite Lattices through Intercalation Chemistry19Enantiomeric Ferroelectric Chiral Domains18Regulating Circularly Polarized Luminescence in Zero-Dimensional Chiral Hybrid Metal Halides28High Circularly Polarized Luminescence Dissymmetry Factor and Efficient Chiral Second Harmonic Generation in Chiral Hybrid Lead‐Bromide Perovskites13Large propagation-direction-dependent circularly polarized emission and scattering anisotropies of a chiral organic-inorganic semiconductor8Optimizing spin polarization in quantum dot vertical-gain structures through pump wavelength selection1Chiroptical Activities of Low‐Dimensional Lead‐Free Chiral Halide Perovskites with White‐Light Emission3Control over Banded Morphologies and Circular Dichroism in Chiral Halide Perovskites15(R)‐ and (S)‐SbF3(C8H9NO3): Chiral Antimony‐Based Hybrid Materials with Enhanced Second‐Harmonic Generation and Birefringence4Magnetic Organic–Inorganic Hybrid Halide Perovskites: Fundamental Physics, Properties, and Applications14Antimicrobial and Anti-Inflammatory Potentials of Silver Tungstate Nanoparticles, Cytotoxicity and Interference on the Activity of Antimicrobial Drugs2First Chiral Catalan Solid Based on Molybdenum Halide with Efficient Circularly Polarized Luminescence in the Deep‐Red Region10First Chiral Catalan Solid Based on Molybdenum Halide with Efficient Circularly Polarized Luminescence in the Deep‐Red Region2Accurate single-shot full-Stokes detection enabled by heterogeneous grain orientations in polycrystalline films9Multifunctional Chiral Halide Perovskites: Advancing Chiro‐Optics, Chiro‐Optoelectronics, and Spintronics33Amplifying Chirality-Induced Spin Selectivity in Helical Covalent Organic Frameworks through Fullerene Encapsulation17Challenges, Solutions, and Opportunities in Chiral Perovskites: From Synthesis Strategies to Technological Advancements4Spatial mapping of chiral-induced spin selectivity in chiral perovskite via spin-Schottky junction10Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric5Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric1Decoding Chirality Transfer Strengths and Structure–Property Relationships in Bismuth-Containing Chiral Hybrid Organic–Inorganic Semiconductors10Local Symmetry Breaking and Hidden Spin Polarization in 2D Hybrid Perovskites with Nonprimary Ammonium Cations14Chirality-Regulated Spin-Polarization of Perovskite Nanoplates for Photocatalytic CO 2 Reduction Reaction31Circularly polarized laser from three‐dimensional perovskite induced by intramolecular interaction3Record Second‐Harmonic Generation in a Lead‐Free 2D Hybrid Halide Perovskite13Standardizing the characterization of circularly polarized luminescence of chiral materials38Chirality-driven spin dynamics and manipulation in all-inorganic chiral heterostructures7Amplification of Chirality in Self-Assembled Chiral Perovskite Superstructure Films15THz‐Driven Coherent Phonon Fingerprints of Hidden Symmetry Breaking in 2D Layered Hybrid Perovskites7Chiral Metal Halides toward Circularly Polarized Photodetectors13Chiral‐Identified Multicolor‐Tunable Photoluminescence via Excitation‐Wavelength Modulation in 0D Antimony(III) Enantiomers for Multilevel Anti‐Counterfeiting10Molecular Design‐Enabled Pyridinium‐Based Metal Halide Glass Scintillators with Robust Glass‐Forming Ability and Tailorable Radioluminescence18Molecular Design‐Enabled Pyridinium‐Based Metal Halide Glass Scintillators with Robust Glass‐Forming Ability and Tailorable Radioluminescence3Motional narrowing of spin relaxation in 2D perovskites by correlated exciton fluctuations1Recent Advances in Spin‐LEDs Based on Chiral Nanomaterials: Bridging Fundamental Physics, Materials, and Devices Performance9Stable 3D lead bromide hybrid ferroelectric semiconductor enabled by halogen-substitution-induced confinement effect2Principles and advances in spin light-emitting diodes9Lead the Way: Halide Perovskites as Next-Generation Triplet Sensitizers for Photon Upconversion19

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  4. Revealing the Intrinsic Chiroptical Activity in Chiral Metal-Halide Semiconductors

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  6. Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers

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  7. Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers

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  8. A chiral two-dimensional perovskite-like lead-free bismuth( iii ) iodide hybrid with high phase transition temperature

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  9. A photoluminescent chiral lead-free hybrid ferroelastic semiconductor with switchable second-harmonic generation

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  10. Amplification of polarization ratio is observed in monolayer Dion–Jacobson hybrid perovskites

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  11. Atomistic modeling of metal–ligand chirality transfer and chiroptical properties of lead and tin hybrid perovskites

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  12. Broadband emission originating from the stereochemical expression of 6s 2 lone pairs in two-dimensional lead bromide perovskites

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  13. Chiral mesostructured NiFe 2 O 4 films with chirality induced spin selectivity

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  14. Circularly polarized luminescence and nonlinear optical harmonic generation based on chiral zinc halides

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  17. The rise of halide perovskite semiconductors

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  18. Resonant Second Harmonic Generation in Proline Hybrid Lead Halide Perovskites

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  19. Materials for chiral light control

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  21. Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime

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  24. Highly‐Active Chiral Organic Photovoltaic Catalysts with Suppressed Charge Recombination

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  26. Spin selectivity of chiral mesostructured diamagnetic BiOBr films

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  35. Chiral Ligand‐Induced Inversion and Tuning of Excitonic Optical Activity in Intrinsically Chiral CsPbBr3 Perovskite Nanoplatelets

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  37. Chirality induced spin selectivity in chiral hybrid organic–inorganic perovskites

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  38. Chiral Lead Halide Perovskite Nanocrystals: Construction Strategies and Photophysical Properties

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  39. MatGPT: A Vane of Materials Informatics from Past, Present, to Future

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  40. Conditions for EPR detection of chirality-induced spin selectivity in spin-polarized radical pairs in isotropic solution

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  41. Nonlinear optical properties in chiral copper oxide nanosheets

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  42. Synthesis and Optical Properties of One Year Air-Stable Chiral Sb(III) Halide Semiconductors

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  43. Spin-dependent electrochemistry and electrochemical enantioselective recognition with chiral methylated bis(ethylenedithio)-tetrathiafulvalenes

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  44. Cluster-assembled superatomic crystals for chirality-dependent charge-to-spin conversion

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  45. Free Halogen Substitution of Chiral Hybrid Metal Halides for Activating the Linear and Nonlinear Chiroptical Properties

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  46. Homochirality in Ferroelectrochemistry

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  47. Spin Chiral Anisotropy of Chiral Mesostructured Inorganic Materials with Different Intrinsic Magnetisms

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  48. Extended Honeycomb Metal Chloride with Tunable Antiferromagnetic Correlations

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  49. Boosting circularly polarized luminescence by optimizing off-centering octahedral distortion in zero-dimensional hybrid indium-antimony halides

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  50. Multi-stimuli-responsive luminescence enabled by crown ether anchored chiral antimony halide phosphors

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