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RESEARCH PAPER · Journal of the American Chemical Society · 2022

Revealing the Intrinsic Chiroptical Activity in Chiral Metal-Halide Semiconductors

Zixuan Zhang, Zhiyu Wang, Herman H. Y. Sung, Ian Duncan Williams, Zhi Yu, Haipeng Lu

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Revealing the Intrinsic Chiroptical Activity in Chiral Metal-Halide SemiconductorsOriginalCircularly polarized luminescence enlargement from crystals to oriented films of enantiopure 2D hybrid perovskites13Research progress in optical activities and nonlinear optics of chiral perovskites1Unique Chiro-optical Properties of the Weakly-2D (R-/S-MBA)2CuBr4 Hybrid Material31Low Detection Limit Circularly Polarized Light Detection Realized by Constructing Chiral Perovskite/Si Heterostructures16Unprecedented Chiral Three‐dimensional Hybrid Organic‐Inorganic Perovskitoids36Unprecedented Chiral Three‐dimensional Hybrid Organic‐Inorganic Perovskitoids0Can we still measure circular dichroism with circular dichroism spectrometers: The dangers of anisotropic artifacts44Tuning Phase Purity in Chiral 2D Perovskites24Chiral Cation Doping for Modulating Structural Symmetry of 2D Perovskites62Spatially Correlated Chirality in Chiral Two-Dimensional Perovskites Revealed by Second-Harmonic-Generation Circular Dichroism Microscopy56Chiroptical Response Inversion and Enhancement of Room‐Temperature Exciton‐Polaritons Using 2D Chirality in Perovskites18Chiral Ruthenium Halide Semiconductor with Strong Antiferromagnetic Coupling28Chiral Lead Halide Perovskite Nanocrystals: Construction Strategies and Photophysical Properties11Enhanced Circular Dichroism and Polarized Emission in an Achiral, Low Band Gap Bismuth Iodide Perovskite Derivative14Unveiling Chiral Perovskite CD Signal Scaling: Discerning Authentic and Counterfeit Signals through Sample-State Analysis22In Situ Formed Perovskite Nanocrystal Films Toward Efficient Circularly Polarized Electroluminescence33Deciphering the electronic and structural origin of chiroptical activity of chiral 2D perovskites14The role of halogens in structural diversity and chirality enhancement of 1D chiral hybrid metal halides8Ligand‐Induced Chirality in ClMBA2SnI4 2D Perovskite**38Ligand‐Induced Chirality in ClMBA2SnI4 2D Perovskite**6Effect of film morphology on circular dichroism of low-dimensional chiral hybrid perovskites21Highly Circularly Polarized Light‐Sensitive Chiral One‐Dimensional Perovskites Enabled by Antisolvent Engineering26Giant Apparent Optical Circular Dichroism in Thin Films of Bismuth‐Based Hybrid Organic–Inorganic Metal Halide Semiconductor Through Preferred Orientation16Axially Chiral Organic Semiconductors for Visible‐Blind UV‐Selective Circularly Polarized Light Detection35Induced Circularly Polarized Luminescence and Exciton Fine Structure Splitting in Magnetic-Doped Chiral Perovskites12The first chiral cerium halide towards circularly-polarized luminescence in the UV region65Patterned Chiral Perovskite Film for Self‐Driven Stokes Photodetectors32Perovskite versus Nonperovskite: Modulating the Nature and Optical Properties of One-Dimensional Chiral Lead–Bromide Networks15Large exchange-driven intrinsic circular dichroism of a chiral 2D hybrid perovskite41Chiral materials and mechanisms for circularly polarized light-emitting diodes289Understanding and Controlling the Photoluminescence Line Shapes of 2D Perovskites with Chiral Methylbenzylammonium-Based Cations25Lyotropic Chromonic Mesophases of Chiral Organopalladium(II) Complexes for Amplified Circularly Polarized Phosphorescence10Chiral Induction in 2D Borophene Nanoplatelets through Stereoselective Boron–Sulfur Conjugation12Generation and Enhancement of Chirality-Induced Spin-Polarized Emission in 3D@1D Lead Halide Perovskites4Dimensional and Doping Engineering of Chiral Perovskites with Enhanced Spin Selectivity for Green Emissive Spin Light-Emitting Diodes44Efficient Green Spin Light-Emitting Diodes Enabled by Ultrafast Energy- and Spin-Funneling in Chiral Perovskites94Uniaxial‐Oriented Chiral Perovskite for Flexible Full‐Stokes Polarimeter34Self-Powered Circularly Polarized Light Detection Enabled by Chiral Two-Dimensional Perovskites with Mixed Chiral–Achiral Organic Cations42Experimental Evidence of the Molecular and Macroscopic Origins of Circular Dichroism in Chiral Metal‐Halide Networks10Homochiral and Heterochiral Cation Mixing in 2D Perovskites for Enhanced Structural Asymmetry and Spin Splitting11A chemical perspective on the chiral induced spin selectivity effect56Fluorinated Organic Cations Derived Chiral 2D Perovskite Enabling Enhanced Spin‐Dependent Oxygen Evolution Reaction11Chiral multiferroicity in two-dimensional hybrid organic-inorganic perovskites59Hydrogen Bonding Analysis of Structural Transition-Induced Symmetry Breaking and Spin Splitting in a Hybrid Perovskite Employing a Synergistic Diffraction-DFT Approach18Strain-Amplified Exciton Chirality in Organic-Inorganic Hybrid Materials9Boosted Chirality Transfer in 2D Perovskites through Structural Isomer‐Driven Halogen–Halogen Interaction33Chirality and Solvent Coassist the Structural Evolution of Hybrid Manganese Chlorides with Second-Harmonic-Generation Response7Unraveling the Role of Structural Topology on Chirality Transfer and Chiroptical Properties in Chiral Germanium Iodides31Dimensional control of chiral perovskites for high-performance circularly polarized light detection via ligand engineering14Macroscopic Twisting of Chiral Metal Halide Single Crystals Driven by Thermo-Induced Topochemical Dehydration31Increasing the Magnetic Transition Dipole Moment of Chiral Perovskite Through Eu3+ Doping8Unveiling Chirality Transfer between Chiral Centers and Metal Halides in Chiral Organic–Inorganic Hybrid Metal Halides25Enhancing Chiroptoelectronic Activity in Chiral 2D Perovskites via Chiral–Achiral Cation Mixing11Remote chirality transfer in low-dimensional hybrid metal halide semiconductors67Self-Assembly of Chiral Ligands on 2D Semiconductor Nanoplatelets for High Circular Dichroism8Mechanically Driven, Continuous Synthesis of Chiroplasmonic Assemblies7Deriving Chiroptical Properties from Intrinsically Achiral Building Blocks of One-Dimensional CsPbBr3 Perovskite Nanowires20From the Bulk to the Nanoscale: Strong Evolution in the Structure and Chiroptical Properties of Chiral Halide Double Perovskites5Conformer‐Mediated Helical Chirality in 2D Layered Hybrid Perovskites4Conformer‐Mediated Helical Chirality in 2D Layered Hybrid Perovskites192D/3D Heterostructured Perovskites for Highly Selective Room-Temperature Blue Spin-Polarized Light-Emitting Diodes01D–2D composite perovskite films with self-assembled chiral structure for non-reciprocal circularly polarized emission modulation2Circular dichroism measurement of a single anisotropic chiral nanostructure using scanning circular dichroism microscopy5Regulation of metal valence states for enhancing second harmonic generation performance of chiral tin halides2Tunable chiroptical activity and second-harmonic generation in chiral one-dimensional perovskites2Tuning the visible circularly polarized luminescence in highly emissive chiral terbium and europium chlorides71.5D Chiral Perovskites Mediated by Hydrogen‐Bonding Network with Remarkable Spin‐Polarized Property21.5D Chiral Perovskites Mediated by Hydrogen‐Bonding Network with Remarkable Spin‐Polarized Property18Unprecedented Ultraviolet Circularly Polarized Light‐Dependent Anomalous Photovoltaics in Chiral Hybrid Perovskites12Spontaneous Formation of Single-Crystalline Spherulites in a Chiral 2D Hybrid Perovskite6Efficient Spin‐Light‐Emitting Diodes With Tunable Red to Near‐Infrared Emission at Room Temperature39Dark-Field Absorbance Circular Dichroism of Oriented Chiral Thin Films8Chirality-Induced Spin Selectivity in Hybrid Organic-Inorganic Perovskite Semiconductors36Emergent Nonreciprocal Dual Circularly Polarized Luminescence from an Iridescent Cellulose Nanocrystalline Film0Electrical Control of Spin Polarization in a Multiferroic Heterojunction Based on One-Dimensional Chiral Hybrid Metal Halide10Two-photon excited spin excitonic properties in two-dimensional chiral perovskite films1Controlling the Orientation of Polar Axis in Chiral Metal‐Halides to Reveal Their Intrinsic Circularly Polarized Luminescence5Orientation-Driven Chirality Funnels in Chiral Low-Dimensional Lead-Halide Perovskite Heterostructures15Large propagation-direction-dependent circularly polarized emission and scattering anisotropies of a chiral organic-inorganic semiconductor8Control over Banded Morphologies and Circular Dichroism in Chiral Halide Perovskites153D Chiral Metal Halide Semiconductors16Unraveling the Impact of Organic Cation Dipole Moment on Rashba Spin‐Splitting in 2D Hybrid Organic–Inorganic Perovskites14Unraveling the Impact of Organic Cation Dipole Moment on Rashba Spin‐Splitting in 2D Hybrid Organic–Inorganic Perovskites0Polymerization‐Induced Crystallization to Form Stretchable Hydrogels with Banded Spherulites and Circularly Polarized Luminescence24Differential absorption of circularly polarized light by a centrosymmetric crystal42Achiral Cation-Induced Chirality Tuning in Cycloalkyl Chiral Cation-Based Quasi-1D and 2D Perovskites6Challenges, Solutions, and Opportunities in Chiral Perovskites: From Synthesis Strategies to Technological Advancements4Decoding Chirality Transfer Strengths and Structure–Property Relationships in Bismuth-Containing Chiral Hybrid Organic–Inorganic Semiconductors10Apparent circular dichroism in centrosymmetric crystals2Anisotropic Second‐Harmonic Generation in Chiral Hybrid Palladium Halides2Anisotropic Second‐Harmonic Generation in Chiral Hybrid Palladium Halides10Natural optical activity in quasi-2D hybrid organic–inorganic perovskites: Band and molecular contributions1Activating the Chiroptical Properties of High-Fold Axial Chiral Perovskite by a Chiral Induction Strategy11Dimensional Engineering in Hybrid Transition Metal Halide Materials through the Introduction of Chiral Organic Cations5Hierarchical chiral supramolecular assemblies with strong and invertible chiroptical properties81Standardizing the characterization of circularly polarized luminescence of chiral materials38Vortex‐Enabled Nonreciprocal Circularly Polarized Luminescence in Achiral Polymer Systems7Amplification of Chirality in Self-Assembled Chiral Perovskite Superstructure Films15Symmetry Breaking Induced by Chiral Phosphonic Acids in a 2D Tin-Halide Perovskite12Chiral Metal Halides toward Circularly Polarized Photodetectors13A monolithic chiral perovskite crystal enables self-powered, full-Stokes detection of ultra-weak light1Structural Engineering for Chirality-Induced Spin Control in Metal–Halide Perovskites10Bright Cyan Circularly Polarized Luminescence and Efficient Second Harmonic Generation in Zero‐Dimensional Silver‐Based Halides with Achiral Cations3Bright Cyan Circularly Polarized Luminescence and Efficient Second Harmonic Generation in Zero‐Dimensional Silver‐Based Halides with Achiral Cations1Chirality amplification in semiconductors for advanced optoelectronics23Halogenated Chiral Spacer Integration in Silver Bismuth Double Perovskites for Efficient and Selective CPL Photodetection2Internally and externally induced chiral hybrid metal halide materials for advanced chiroptoelectronic applications23Organic circularly polarized lasers0Integrated Photon Ellipticity Recognition with Chiral Nanomaterials1Strain-relaxed chiral hybrid bismuth halides for spin selectivity and magnetoresistance0Chiral-deformation-induced polarons as a design principle for white-light emission in 2D organic halide perovskites0Homocentric Chirality and Magnetism Enable Strong NIR Magneto-Optical Activity in a Chiral DyFe 3 Cluster5Highly efficient circularly polarized electroluminescence in 3D perovskites passivated by chiral phosphonium halides0Absorption dissymmetry factor enhancement: A data-driven approach to unravel the synthesis knobs of chiral 2D perovskites1On the Origin of Circularly Polarized Luminescence in Chiral One-Dimensional (A)PbBr 3 Single Crystals1Large-Area Three-Dimensional Displaced Overlapping Wing Perovskite Metamaterials with Giant Optical Chirality12D chirality in organic thin films: advances in nonreciprocal chiroptical properties3Achieving Bright White Emission in Chiral 2D Organic Metal Halide Hybrids by Modulating Noncovalent Interactions0Dual‐Color Tunable Circularly Polarized Luminescence With Anti‐Thermal‐Quenching Enabled by Asymmetric Hydrogen‐Bonding Networks in Hybrid Manganese Halides32D/3D perovskite heterostructures for highly selective room-temperature blue spin-polarized light-emitting diodes0Chiral Antimony‐Based Halides With Temperature‐Responsive Multimodal Emission0Chirality Engineering and Properties in Two‐Dimensional Layered Materials2Atomically thin two-dimensional AIIBVI semiconductors with organic ligands: synthesis, optical properties, and applications0Chiral CsPbBr 3 Nanorods With Effective Circularly Polarized Luminescence via Vacancy‐Mediated Regrowth Directed by Chiral Ligands0Mutual Amplification of Chirality Driven by Interfacial Interactions in In Situ Synthesized Perovskite/Polymer Composites0Synergistic Paramagnetic, Piezoelectric, and Chiral Optical Effects in Fe- and Mn- Hybrid Metal Halides0Direction‐Dependent Plasmonic Chiroptical Response With High Asymmetry and Dynamic Tunability0Non-reciprocal linearly polarized light in simple media0A step-by-step workflow to account for linear polarization artifacts in circular dichroism of thin films0Impartation of Optical Activity from Chiral Ligands to Hybrid Perovskites via Virtual Photons0Chiral Lattice Distortion Enables Bright Near-Infrared Circularly Polarized Luminescence in Lead-Free Metal Halides0Data-driven design of ultra-wide band gap chiral metal halides for deep-ultraviolet optoelectronics0

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  41. A chemical perspective on the chiral induced spin selectivity effect

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  43. Chiral multiferroicity in two-dimensional hybrid organic-inorganic perovskites

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  44. Hydrogen Bonding Analysis of Structural Transition-Induced Symmetry Breaking and Spin Splitting in a Hybrid Perovskite Employing a Synergistic Diffraction-DFT Approach

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  45. Strain-Amplified Exciton Chirality in Organic-Inorganic Hybrid Materials

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    Jin Xiao, Haofeng Zheng, Yanan Liu, Fang Li, Jing Li, Jongchan Kim, Yanlong Wang, Qi Liu, Xuyu Ma, Shaocong Hou

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