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RESEARCH PAPER · Angewandte Chemie · 2020

Designing Silicates as Deep‐UV Nonlinear Optical (NLO) Materials using Edge‐Sharing Tetrahedra

Hongping Wu, Bingbing Zhang, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, P. Shiv Halasyamani

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Designing Silicates as Deep‐UV Nonlinear Optical (NLO) Materials using Edge‐Sharing TetrahedraOriginalCs 3 Pb 2 (CH 3 COO) 2 X 5 (X=I, Br): Halides with Strong Second‐Harmonic Generation Response Induced by Acetate Groups75Cs3Pb2(CH3COO)2X5 (X=I, Br): Halides with Strong Second‐Harmonic Generation Response Induced by Acetate Groups22Prediction of Novel van der Waals Boron Oxides with Superior Deep‐Ultraviolet Nonlinear Optical Performance43Prediction of Novel van der Waals Boron Oxides with Superior Deep‐Ultraviolet Nonlinear Optical Performance6Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application167Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application18Hydrogen‐Bond‐Driven Synergistically Enhanced Hyperpolarizability: Chiral Coordination Polymers with Nonpolar Structures Exhibiting Unusually Strong Second‐Harmonic Generation87Hydrogen‐Bond‐Driven Synergistically Enhanced Hyperpolarizability: Chiral Coordination Polymers with Nonpolar Structures Exhibiting Unusually Strong Second‐Harmonic Generation19Li 4 MgGe 2 S 7 : The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap213Li4MgGe2S7: The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap15Heterobimetallic Cluster‐Based Coordination Polymers: Assembly, Structures and Third‐Order Nonlinear Optical Properties4Strong SHG Responses in a Beryllium‐Free Deep‐UV‐Transparent Hydroxyborate via Covalent Bond Modification89Strong SHG Responses in a Beryllium‐Free Deep‐UV‐Transparent Hydroxyborate via Covalent Bond Modification9A Lead Mixed Halide with Three Different Coordinated Anions and Strong Second‐Harmonic Generation Response10Designing A New Infrared Nonlinear Optical Material, β‐BaGa 2 Se 4 Inspired by the Phase Transition of the BaB 2 O 4 (BBO) Crystal75Designing A New Infrared Nonlinear Optical Material, β‐BaGa2Se4 Inspired by the Phase Transition of the BaB2O4 (BBO) Crystal13A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency15A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency96Chiral Ligand‐Driven Systematic Synthesis of Coordination Polymers with Non‐centrosymmetric Structures12Sulfamide: A Promising Deep‐Ultraviolet Nonlinear Optical Crystal Assembled from Polar Covalent [SO2(NH2)2] Tetrahedra9Sulfamide: A Promising Deep‐Ultraviolet Nonlinear Optical Crystal Assembled from Polar Covalent [SO2(NH2)2] Tetrahedra84Strong Nonlinearity Induced by Coaxial Alignment of Polar Chain and Dense [BO3] Units in CaZn2(BO3)212Strong Nonlinearity Induced by Coaxial Alignment of Polar Chain and Dense [BO3] Units in CaZn2(BO3)2212Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence43SrZnGeS 4 : A Dual‐Waveband Nonlinear Optical Material with a Transparency Spanning UV/Vis and Far‐IR Spectral Regions88SrZnGeS4: A Dual‐Waveband Nonlinear Optical Material with a Transparency Spanning UV/Vis and Far‐IR Spectral Regions12AgGaSe2-Inspired Nonlinear Optical Materials: Tetrel Selenides of Alkali Metals and Mercury34Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance56NaHSO4·H2O: A Promising Deep-Ultraviolet Nonlinear-Optical Bisulfate with Large Birefringence and a Second-Harmonic-Generation Effect16[Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters21Four New Sb‐based Orthophosphates: Cation Regulation to Investigate Diversified Structural Architecture1SrCl2·6H2O: An Alkaline-Earth-Metal Chloride Hexahydrate as Deep-Ultraviolet Nonlinear-Optical Crystal with the {[Sr(H2O)6]2+}∞ Cationic Framework8Design Principles for Noncentrosymmetric Materials23Synthesis, structural, impedance, optical, Mössbauer characterizations and magnetic studies of Pb-containing germanate compounds8La3Ga5M0.5Sn0.5O14, (M = Ge, Si): Design and Synthesis of Two Langasite Nonlinear Optical Materials with Large Second Harmonic Generation and Birefringence Induced by Distorted (Sn/M)O6 Octahedra4Deep-ultraviolet nonlinear-optical crystals LiBePO 4 and BeP 2 O 6 synthesized by ionic potential modulation towards uniform arrangement of PO 4 groups5Pr3+ Visible to Ultraviolet Upconversion for Antimicrobial Applications26The Dugganite Structure as a Host for New Colored Compounds and for Oxygen Evolution Studies1BaAl2MS6 (M = Si and Ge): the rational construction of diamond-like structures with ultrawide band gap by group-optimization approach6Symmetry‐Aware Equivariant Network for Discovering SHG‐Active Materials5Efficient blue-to-UV-B up-conversion in Li2CaSiO4:Pr,Gd,Na1Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates0Cation Distribution in Li 2 CaSiO 4 :Gd, Pr, Na Uncovered Through Anomalous Diffraction0

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  1. Cs 3 Pb 2 (CH 3 COO) 2 X 5 (X=I, Br): Halides with Strong Second‐Harmonic Generation Response Induced by Acetate Groups

    Angewandte Chemie International Edition · 2020-10-14

    Qirui Shui, Hong‐Xin Tang, Ruibiao Fu, Yuan‐Bin Fang, Zuju Ma, Xintao Wu

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  2. Cs3Pb2(CH3COO)2X5 (X=I, Br): Halides with Strong Second‐Harmonic Generation Response Induced by Acetate Groups

    Angewandte Chemie · 2020-10-15

    Qirui Shui, Hong‐Xin Tang, Ruibiao Fu, Yuan‐Bin Fang, Zuju Ma, Xintao Wu

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  3. Prediction of Novel van der Waals Boron Oxides with Superior Deep‐Ultraviolet Nonlinear Optical Performance

    Angewandte Chemie International Edition · 2021-02-25

    Hao Li, Jingmei Min, Zhihua Yang, Zhenhai Wang, Shilie Pan, Артем Ромаевич Оганов

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  4. Prediction of Novel van der Waals Boron Oxides with Superior Deep‐Ultraviolet Nonlinear Optical Performance

    Angewandte Chemie · 2021-02-25

    Hao Li, Jingmei Min, Zhihua Yang, Zhenhai Wang, Shilie Pan, Артем Ромаевич Оганов

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  5. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie International Edition · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

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  6. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

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  7. Hydrogen‐Bond‐Driven Synergistically Enhanced Hyperpolarizability: Chiral Coordination Polymers with Nonpolar Structures Exhibiting Unusually Strong Second‐Harmonic Generation

    Angewandte Chemie International Edition · 2021-06-07

    Joonhyuk Kee, Kang Min Ok

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  8. Hydrogen‐Bond‐Driven Synergistically Enhanced Hyperpolarizability: Chiral Coordination Polymers with Nonpolar Structures Exhibiting Unusually Strong Second‐Harmonic Generation

    Angewandte Chemie · 2021-06-07

    Joonhyuk Kee, Kang Min Ok

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  9. Li 4 MgGe 2 S 7 : The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap

    Angewandte Chemie International Edition · 2021-07-24

    Ailijiang Abudurusuli, Junben Huang, Peng Wang, Zhihua Yang, Shilie Pan, Junjie Li

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  10. Li4MgGe2S7: The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap

    Angewandte Chemie · 2021-07-24

    Ailijiang Abudurusuli, Junben Huang, Peng Wang, Zhihua Yang, Shilie Pan, Junjie Li

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  11. Heterobimetallic Cluster‐Based Coordination Polymers: Assembly, Structures and Third‐Order Nonlinear Optical Properties

    Chemistry - An Asian Journal · 2021-07-27

    Chen Cao, Shu‐Jin Bao, Xiao‐Yan Tang, Ze‐Ming Xu, Chun‐Yan Ni, Jian‐Ping Lang

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  12. Strong SHG Responses in a Beryllium‐Free Deep‐UV‐Transparent Hydroxyborate via Covalent Bond Modification

    Angewandte Chemie International Edition · 2021-10-11

    Chao Wu, Xingxing Jiang, Lin Lin, Wenyan Dan, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  13. Strong SHG Responses in a Beryllium‐Free Deep‐UV‐Transparent Hydroxyborate via Covalent Bond Modification

    Angewandte Chemie · 2021-10-11

    Chao Wu, Xingxing Jiang, Lin Lin, Wenyan Dan, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  14. A Lead Mixed Halide with Three Different Coordinated Anions and Strong Second‐Harmonic Generation Response

    Chemistry - A European Journal · 2021-10-15

    Qirui Shui, Ruibiao Fu, Ziqi Zhou, Zuju Ma, Hong‐Xin Tang, Xin‐Tao Wu

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  15. Designing A New Infrared Nonlinear Optical Material, β‐BaGa 2 Se 4 Inspired by the Phase Transition of the BaB 2 O 4 (BBO) Crystal

    Angewandte Chemie International Edition · 2021-11-16

    Yu-Jie Zhang, Qiang Bian, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  16. Designing A New Infrared Nonlinear Optical Material, β‐BaGa2Se4 Inspired by the Phase Transition of the BaB2O4 (BBO) Crystal

    Angewandte Chemie · 2021-11-16

    Yu-Jie Zhang, Qiang Bian, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  17. A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency

    Angewandte Chemie · 2021-12-11

    Chao Wu, Xingxing Jiang, Yilei Hu, Chunbo Jiang, Tianhui Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  18. A Lanthanum Ammonium Sulfate Double Salt with a Strong SHG Response and Wide Deep‐UV Transparency

    Angewandte Chemie International Edition · 2021-12-11

    Chao Wu, Xingxing Jiang, Yilei Hu, Chunbo Jiang, Tianhui Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  19. Chiral Ligand‐Driven Systematic Synthesis of Coordination Polymers with Non‐centrosymmetric Structures

    Chemistry - A European Journal · 2022-01-27

    Yunseung Kuk, Joonhyuk Kee, Kang Min Ok

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  20. Sulfamide: A Promising Deep‐Ultraviolet Nonlinear Optical Crystal Assembled from Polar Covalent [SO2(NH2)2] Tetrahedra

    Angewandte Chemie · 2022-02-18

    Haotian Tian, Ning Ye, Min Luo

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  21. Sulfamide: A Promising Deep‐Ultraviolet Nonlinear Optical Crystal Assembled from Polar Covalent [SO2(NH2)2] Tetrahedra

    Angewandte Chemie International Edition · 2022-02-18

    Haotian Tian, Ning Ye, Min Luo

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  22. Strong Nonlinearity Induced by Coaxial Alignment of Polar Chain and Dense [BO3] Units in CaZn2(BO3)2

    Angewandte Chemie · 2022-03-08

    Miriding Mutailipu, Fuming Li, Congcong Jin, Zhihua Yang, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  23. Strong Nonlinearity Induced by Coaxial Alignment of Polar Chain and Dense [BO3] Units in CaZn2(BO3)2

    Angewandte Chemie International Edition · 2022-03-08

    Miriding Mutailipu, Fuming Li, Congcong Jin, Zhihua Yang, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  24. Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence

    Chemistry of Materials · 2022-03-22

    Wenli Zhao, Conggang Li, Tao Han, Jinmiao Jiao, Yuheng She, Dianxing Ju, Fei Liang, Ning Ye, Zhanggui Hu, Yicheng Wu

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  25. SrZnGeS 4 : A Dual‐Waveband Nonlinear Optical Material with a Transparency Spanning UV/Vis and Far‐IR Spectral Regions

    Angewandte Chemie International Edition · 2022-05-05

    Qianqian Liu, Xin Liu, Li‐Ming Wu, Ling Chen

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  26. SrZnGeS4: A Dual‐Waveband Nonlinear Optical Material with a Transparency Spanning UV/Vis and Far‐IR Spectral Regions

    Angewandte Chemie · 2022-05-05

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  27. AgGaSe2-Inspired Nonlinear Optical Materials: Tetrel Selenides of Alkali Metals and Mercury

    Chemistry of Materials · 2022-06-26

    Lihua Gao, Jingjing Xu, Xinyu Tian, Bingbing Zhang, Xiaowen Wu, Kui Wu

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  28. Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance

    ACS Applied Materials & Interfaces · 2022-08-11

    Jingjing Xu, Kui Wu, Yan Xiao, Bingbing Zhang, Haohai Yu, Huaijin Zhang

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  29. NaHSO4·H2O: A Promising Deep-Ultraviolet Nonlinear-Optical Bisulfate with Large Birefringence and a Second-Harmonic-Generation Effect

    Inorganic Chemistry · 2022-11-30

    Han Li, Haotian Tian, Chensheng Lin, Xin Lei Zhao, Chao Wang, Ning Ye, Min Luo

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  30. [Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters

    Journal of Materials Chemistry C · 2023-01-01

    Chenyao Zhao, Kui Wu, Yan Xiao, Bingbing Zhang, Haohai Yu, Huaijin Zhang

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  31. Four New Sb‐based Orthophosphates: Cation Regulation to Investigate Diversified Structural Architecture

    Chemistry - A European Journal · 2023-04-10

    Hongyu Huang, Na Li, Ruixin Zhang, Xinmei Wang, Xianmeng He, Lei Wu, Lili Liu, Qun Jing, Zhaohui Chen

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  32. SrCl2·6H2O: An Alkaline-Earth-Metal Chloride Hexahydrate as Deep-Ultraviolet Nonlinear-Optical Crystal with the {[Sr(H2O)6]2+}∞ Cationic Framework

    Inorganic Chemistry · 2023-06-23

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  33. Design Principles for Noncentrosymmetric Materials

    Annual Review of Materials Research · 2023-07-03

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  34. Synthesis, structural, impedance, optical, Mössbauer characterizations and magnetic studies of Pb-containing germanate compounds

    Materials Chemistry and Physics · 2023-08-25

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  35. La3Ga5M0.5Sn0.5O14, (M = Ge, Si): Design and Synthesis of Two Langasite Nonlinear Optical Materials with Large Second Harmonic Generation and Birefringence Induced by Distorted (Sn/M)O6 Octahedra

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  36. Deep-ultraviolet nonlinear-optical crystals LiBePO 4 and BeP 2 O 6 synthesized by ionic potential modulation towards uniform arrangement of PO 4 groups

    Inorganic Chemistry Frontiers · 2025-01-01

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  37. Pr3+ Visible to Ultraviolet Upconversion for Antimicrobial Applications

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  38. The Dugganite Structure as a Host for New Colored Compounds and for Oxygen Evolution Studies

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  39. BaAl2MS6 (M = Si and Ge): the rational construction of diamond-like structures with ultrawide band gap by group-optimization approach

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  40. Symmetry‐Aware Equivariant Network for Discovering SHG‐Active Materials

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  41. Efficient blue-to-UV-B up-conversion in Li2CaSiO4:Pr,Gd,Na

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  42. Confinement π‐Conjugated Moiety Tailoring to Achieve Record Deep‐UV Nonlinearity in Sulfates

    Angewandte Chemie · 2026-03-05

    Yujie Fan, Cheng Hu, Li Wu, Chensheng Lin, Chao Wang, Huixin Fan, Tao Yan, Min Luo

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  43. Cation Distribution in Li 2 CaSiO 4 :Gd, Pr, Na Uncovered Through Anomalous Diffraction

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