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RESEARCH PAPER · Angewandte Chemie · 2022

High‐Performance Sulfate Optical Materials Exhibiting Giant Second Harmonic Generation and Large Birefringence

Xuehua Dong, Ling Huang, Hongmei Zeng, Zhien Lin, Kang Min Ok, Guohong Zou

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High‐Performance Sulfate Optical Materials Exhibiting Giant Second Harmonic Generation and Large BirefringenceOriginalHeteroanionic Melilite Oxysulfide: A Promising Infrared Nonlinear Optical Candidate with a Strong Second-Harmonic Generation Response, Sufficient Birefringence, and Wide Bandgap65An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals81An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals22Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance56Large second harmonic generation in a penta-CdO 2 sheet exfoliated from its bulk phase16LiRE(SO 4 ) 2 (RE = Y, Gd, Eu): noncentrosymmetric chiral rare-earth sulfates with very large band gaps21[Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters21Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation41(C 2 H 10 N 2 )[Zn 2 (HPO 4 ) 2 Cl 2 ]: substitution-activated new short-wave ultraviolet phosphate with pivotal dual-property enhancement5Bistable Cholesteric Liquid Crystals: Electro-optic Applications1Detection of high refractive index polymers via spectral Rabi splitting1Designing High-Performance Short-Wave UV Tellurium-Based Mixed Halides Birefringent Crystals via Halogen Substitution Engineering4A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal2Unlocking Strong Second‐Harmonic Generation in Deep‐UV‐Transparent Polar Organic Sulfonates through Connectivity Regulation2Symmetry‐Aware Equivariant Network for Discovering SHG‐Active Materials5Achieving record-high birefringence in a 3D fluorozincoborate via coplanar alignment of π-conjugated [BO 3 ] units0The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides5Anion-Centered Engineering for Simultaneously Enhancing Birefringence and Band Gap in Chalcogenides11D Cobalt‐Cytidine Monophosphate Coordination Polymer Exhibiting Efficient Ultraviolet Second‐Harmonic Generation7Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates0Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids0

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  1. Heteroanionic Melilite Oxysulfide: A Promising Infrared Nonlinear Optical Candidate with a Strong Second-Harmonic Generation Response, Sufficient Birefringence, and Wide Bandgap

    ACS Applied Materials & Interfaces · 2022-05-11

    Ruiqi Wang, Fei Liang, Xin Liu, Yi Xiao, Qianqian Liu, Xian Zhang, Li‐Ming Wu, Ling Chen, Fuqiang Huang

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  2. An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals

    Angewandte Chemie International Edition · 2022-07-29

    Yanqiang Li, Xu Zhang, Zhou Yang, Weiqi Huang, Yipeng Song, Han Wang, Minjuan Li, Maochun Hong, Junhua Luo, Sangen Zhao

    Read original paper ↗ ·

  3. An Optically Anisotropic Crystal with Large Birefringence Arising from Cooperative π Orbitals

    Angewandte Chemie · 2022-07-29

    Yanqiang Li, Xu Zhang, Zhou Yang, Weiqi Huang, Yipeng Song, Han Wang, Minjuan Li, Maochun Hong, Junhua Luo, Sangen Zhao

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  4. Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance

    ACS Applied Materials & Interfaces · 2022-08-11

    Jingjing Xu, Kui Wu, Yan Xiao, Bingbing Zhang, Haohai Yu, Huaijin Zhang

    Read original paper ↗ ·

  5. Large second harmonic generation in a penta-CdO 2 sheet exfoliated from its bulk phase

    Journal of Materials Chemistry A · 2022-11-25

    Changsheng Hou, Yiheng Shen, Qian Wang, Yoshiyuki Kawazoe, Puru Jena

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  6. LiRE(SO 4 ) 2 (RE = Y, Gd, Eu): noncentrosymmetric chiral rare-earth sulfates with very large band gaps

    Materials Chemistry Frontiers · 2022-11-30

    Sunghwan Cho, Kang Min Ok

    Read original paper ↗ ·

  7. [Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters

    Journal of Materials Chemistry C · 2023-01-01

    Chenyao Zhao, Kui Wu, Yan Xiao, Bingbing Zhang, Haohai Yu, Huaijin Zhang

    Read original paper ↗ ·

  8. Nonlinear optical inorganic sulfates: The improvement of the phase matching ability driven by the structural modulation

    Coordination Chemistry Reviews · 2023-08-02

    Yanran Shang, Junxin Xu, Hongyuan Sha, Zujian Wang, Chao He, Rongbing Su, Xiaoming Yang, Xifa Long

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  9. (C 2 H 10 N 2 )[Zn 2 (HPO 4 ) 2 Cl 2 ]: substitution-activated new short-wave ultraviolet phosphate with pivotal dual-property enhancement

    Journal of Materials Chemistry C · 2024-01-01

    Zhi Gang Fang, Yu-Ming Pan, Pei Han, Bing‐Ping Yang, Meihong Duan

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  10. Bistable Cholesteric Liquid Crystals: Electro-optic Applications

    Engineering materials · 2025-01-01

    Ridhima Gahrotra, Pankaj Kumar, Vandna Sharma

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  11. Detection of high refractive index polymers via spectral Rabi splitting

    Optics Communications · 2025-04-14

    Peihao Su, Wei Li, Yuxiang Peng, Yuanyuan Liu, Kaijun Wang, Jianqiang Liu, Dengyun Lu, Meng‐Dong He

    Read original paper ↗ ·

  12. Designing High-Performance Short-Wave UV Tellurium-Based Mixed Halides Birefringent Crystals via Halogen Substitution Engineering

    Crystal Growth & Design · 2025-06-24

    Xiang Mao, Yu Yan, Yingzi Zhang, Xuehua Dong, Ling Huang, Liling Cao, Daojiang Gao, Guohong Zou

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  13. A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal

    Angewandte Chemie · 2025-10-17

    Haochen Li, Haotian Tian, Pifu Gong, Tianyu Wang, Hongyu Liu, Bing Li, Qian Wu, Mingjun Xia

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  14. Unlocking Strong Second‐Harmonic Generation in Deep‐UV‐Transparent Polar Organic Sulfonates through Connectivity Regulation

    Angewandte Chemie · 2025-11-10

    Feiyuan Gong, Xingxing Jiang, Kaining Duanmu, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  15. Symmetry‐Aware Equivariant Network for Discovering SHG‐Active Materials

    Advanced Functional Materials · 2025-11-20

    Liudmila A. Klimova, Ivan S. Trofimov, Wenqi Jin, Qi Song, Aleksey V. Arsenin, Congwei Xie, Ivan A. Kruglov, Valentyn S. Volkov

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  16. Achieving record-high birefringence in a 3D fluorozincoborate via coplanar alignment of π-conjugated [BO 3 ] units

    Inorganic Chemistry Frontiers · 2026-01-01

    Yucheng Hao, Qiuhui Zhang, Haoran Yu, Xikai Miu, Simin Cai, Xinnan Li, Fengshan Yu, Yuan Lin, Mingyang Cao

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  17. The modulation of structural polarity facilitating the gradient enhancement of second harmonic generation effects in hybrid metal halides

    Science China Chemistry · 2026-01-04

    Ru‐Ling Tang, Die-Xue Yang, Jian-Dong Guo, C. Z. Chen, Wenlong Liu, Sheng‐Ping Guo

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  18. Anion-Centered Engineering for Simultaneously Enhancing Birefringence and Band Gap in Chalcogenides

    Chemistry of Materials · 2026-01-19

    Chao-Hong Xie, Lu Liu, Xiao‐Ming Jiang, Bin-Wen Liu, Guo‐Cong Guo

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  19. 1D Cobalt‐Cytidine Monophosphate Coordination Polymer Exhibiting Efficient Ultraviolet Second‐Harmonic Generation

    Chemistry - A European Journal · 2026-02-09

    Mubashar Ilyas, Lin Xiong, Li Zhang, Maida, Maroof Ahmad Khan, Muhammad Abbas, Nagesh Manurkar, Mudassar Ilyas, Niu Zhang, Hui Li

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  20. Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates

    Angewandte Chemie · 2026-02-17

    Jin Li, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  21. Lateral‐Site Unblocking Enables Bilateral π ‐Chromophore Organization for Giant Birefringence in One‐Dimensional Lead Hybrids

    Angewandte Chemie · 2026-08-07

    Yu Yan, Yingzi Zhang, Liyi Zhang, Ling Huang, Yuqiao Zhou, Xuehua Dong, Guohong Zou

    Read original paper ↗ ·
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