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RESEARCH PAPER · Small · 2021

A Fluoride‐Ion‐Conducting Solid Electrolyte with Both High Conductivity and Excellent Electrochemical Stability

Jinzhu Wang, Jipeng Hao, Chaomin Duan, Xinchao Wang, Kai Wang, Cheng Ma

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A Fluoride‐Ion‐Conducting Solid Electrolyte with Both High Conductivity and Excellent Electrochemical StabilityOriginalDegrees of freedom for energy storage material14Superior room-temperature cycling stability of fluoride-ion batteries enabled by solid electrolytes synthesized by the solid-state reaction27Electrolyte design for rechargeable anion shuttle batteries50Point Defect Engineering Enabled the High Ionic Conductivity of BaSnF4 for Solid-State Fluoride-Ion Batteries at Room Temperature25Constructing a BiF3/Bi7F11O5 multiple-phase composite as advanced cathode for room-temperature all-solid-state fluoride-ion batteries7Effects of Mixed Phases on Electrical Conductivities for (CeF 3 ) 1– m (CaF 2 ) m Fast-Fluoride-Ion-Conducting Solid Electrolytes8Mn2+ doped BaSnF4-based solid state electrolyte for room-temperature fluoride ion batteries18Near‐Room‐Temperature Quasi‐Solid‐State F‐Ion Batteries with High Conversion Reversibility Based on Layered Structured Electrolyte67Mechanochemical synthesis, microstructure and electrochemical properties of solid electrolytes with stabilized fluorite-type structure in the PbF2-SrF2-KF system for solid-state fluoride-ion batteries23Challenges for fluoride superionic conductors: fundamentals, design, and applications22Growth and Characterization of All-Inorganic Halide Perovskite CsPbF3 Single Crystals12Fluorosulfide La 2+ x Sr 1– x F 4+ x S 2 with a Triple-Fluorite Layer Enabling Interstitial Fluoride-Ion Conduction20Construction and Interfacial Modification of a β-PbSnF4 Electrolyte with High Intrinsic Ionic Conductivity for a Room-Temperature Fluoride-Ion Battery42Synthesis and characterization of Sn-based electrolytes for F-ion batteries0Accelerated Exploration of Fast Fluoride-Ion Conductors Based on Compositional Descriptors11Ion Mobility in Crystalline Battery Materials63Studies on fluoride ion conductivity of the mechanochemically synthesized β-KSbF4 for all-solid-state fluoride-ion batteries16Composite anode for fluoride-ion batteries using alloy formation and phase separation in charge and discharge processes14Effect of Pb 6s 2 lone pair on the potential flattening of fluoride-ion conduction in perovskite-type fluoride18Effects of mixed phases on ionic conductivities for (LaF 3 ) 1– x (PbF 2 ) x fast-fluoride-ion-conducting solid electrolytes10Fluorosulfide La 2.7 Ba 6.3 F 8.7 S 6 with a double-layer honeycomb structure enabling fluoride-ion conduction3Long-cycle stable operation of fluoride-ion batteries at room temperature enabled by an advanced interface engineering and ion diffusion kinetics regulation strategy3Mechanochemical Synthesis of Fluorine-Conducting Solid Electrolytes Based on Tysonite and Fluorite Structures7Recent advances in aqueous and non-aqueous alkali metal hybrid ion capacitors36Structure design of a BiOF solid electrolyte with remarkably outstanding fluoride ion diffusion performance induced by Ga doping3TlSn 2 F 5 , a SnF 2 -based solid electrolyte with high ionic conductivity and electrochemical stability for all-solid-state fluoride ion batteries11Versatile metal fluorides in ion battery application18Inorganic lithium-ion conductors for fast-charging lithium batteries: a review9High-Capacity and Long-Cycling F-Ion Pouch Cells Enabled by Green Electrolytes42Fluorine Chemistry in Rechargeable Batteries: Challenges, Progress, and Perspectives254Rocking‐Chair Aqueous Fluoride‐Ion Batteries Enabled by Hydrogen Bonding Competition22Rocking‐Chair Aqueous Fluoride‐Ion Batteries Enabled by Hydrogen Bonding Competition11Recent progress, challenges and prospects of electrolytes for fluoride-ion batteries59Atomically engineered Al-doped LaOCl for chlorine-ion batteries4Pressure Tuning and Sn Particle Size Optimization for Enhanced Performance in PbSnF4‐Based All‐Solid‐State Fluoride Ion Batteries17Effect of Uniaxial Stack Pressure on the Performance of Nanocrystalline Electrolytes and Electrode Composites for All‐Solid‐State Fluoride‐Ion Batteries8Solvation engineering of non-aqueous electrolytes for room-temperature fluoride-ion batteries24Electrolyte Design by Synergistic High‐Donor Solvent and Alcohol Anion Acceptor for Reversible Fluoride Ion Batteries31Machine learning potentials for the simulation of fluoride ion batteries electrolytes0Insights into the Micro-Structure-Transport Relationships of the Fluoride-Ion Conductor t -BaSnF 4 Synthesized by Spark Plasma Sintering8Fluoride-Ion Conduction by Synergic Rotation of the Anion Sublattice for Tl4.5SnF8.5 Analogues6Toward Practical Fluoride-Ion Batteries: A Review and Perspective on Liquid Electrolyte Development9Experimental Visualization of F-Ion Diffusion Pathways and Geometric Frustration-Induced Positional Disorder in CaF 2 –BaF 2 Solid Electrolytes13Polymer Electrolyte Based All‐Solid‐State Rechargeable Fluoride Ion Batteries21Shielding Fluoride Ion Basicity through Diurea Coordination for Nonaqueous Fluoride Shuttle Batteries2Shielding Fluoride Ion Basicity through Diurea Coordination for Nonaqueous Fluoride Shuttle Batteries7Fluoride superionic conduction in TlF with the new anti-α-CuBr structure containing intrinsic F vacancies2Design and synthesis of a weakly solvated electrolyte for high-performance fluoride-ion batteries5Highly efficient atomic-scale design of CaF 2 for ultrafast fluoride-ion conduction5Development of all-solid-state fluoride ion battery with enhanced electrochemical stability2Construction of Acceptor‐Multi‐F State Electrolyte to Enable Unprecedented Long‐Life and High‐Capacity Fluoride‐Ion Batteries16Enhanced ionic conductivity and electrochemical stability in fluoride solid electrolyte K0.3Sn1.7F4.72Lewis Acid–Base Synergistically Enhancing Practical Composite Electrolyte for Fluoride‐ion Batteries at Room Temperature9Evidence of High Fluorine Ion Conductivity in SrF2-Rich SrF2–TiO2-Based Compounds0A Comprehensive Review of Sulfide Solid-State Electrolytes: Properties, Synthesis, Applications, and Challenges39Revealing an Intercalation Nature of High‐Capacity Conversion Cathode Materials for Fluoride‐Ion Batteries by Operando Studies3Physicochemical characterization of fluoride solid electrolyte PbSnF4 synthesized via sonochemical reaction0Exploring the structural and conductivity behaviours of mechanochemically and hydrothermally synthesized Ce3+-doped BaSnF4 solid electrolytes for all-solid-state fluoride-ion batteries1Fast Solid-State Defluorination/Fluorination of FeFx (x = 3–0) as Fluoride-Ion Battery Cathode1Advances and Future Perspectives of Solid‐State Electrolytes for Fluoride‐Ion Batteries3Optimizing the dopant concentration of solid electrolyte for room temperature fluoride ion battery applications0Ion‐Pump‐Regulated Highly Conductive Polymer Electrolyte to Enable the First All‐Solid‐State Rechargeable Fluoride‐Ion Pouch Cells8Fluoride-Ion Batteries: A Review of Recent Advances and Future Opportunities5Steric Hindrance-Driven Closed-Loop Conversion of Acceptor Enables Long-Life and High-Capacity Fluoride-Ion Batteries10Role of optical phonon in fluoride-ion conductivity of LaF30Engineering sintering-induced secondary phases in La 0.9 Ba 0.1 F 2.9 -based composite electrolytes for fluoride-ion conduction0K/Sr Dual-Doping Enables Simultaneous Enhancement of Ionic Conductivity and Phase Stability for β-PbF 2 -Based Solid-State Fluoride-Ion Electrolyte0Zr-doped NH4Sn1.96Zr0.04F5.08 electrolyte accelerating fluoride ion transport at room temperature0Intergrowth Fluorite Slabs Modulate Interstitial Fluorine to Enhance Fluoride‐Ion Conductivity0Intergrowth Fluorite Slabs Modulate Interstitial Fluorine to Enhance Fluoride‐Ion Conductivity0Fluoride‐Ion Batteries: Unraveling the Fundamental Science for Next‐Generation Energy Storage0Sulfide Solid Electrolytes for All-Solid-State Batteries: Electrochemical Properties, Ion Transport Mechanisms, and Performance Correlations0

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  1. Degrees of freedom for energy storage material

    Carbon Energy · 2022-04-29

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  2. Superior room-temperature cycling stability of fluoride-ion batteries enabled by solid electrolytes synthesized by the solid-state reaction

    Science China Materials · 2022-08-23

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  3. Electrolyte design for rechargeable anion shuttle batteries

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  4. Point Defect Engineering Enabled the High Ionic Conductivity of BaSnF4 for Solid-State Fluoride-Ion Batteries at Room Temperature

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  5. Constructing a BiF3/Bi7F11O5 multiple-phase composite as advanced cathode for room-temperature all-solid-state fluoride-ion batteries

    Journal of Electroanalytical Chemistry · 2022-12-12

    Jiali Liu, Zihao Zang, Lingguang Yi, Peng Zeng, Changfei Zou, Xiaoyi Chen, Xiyuan Tao, Li Yang, Baobao Chang, Yongqiang Shen, Xianyou Wang

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  6. Effects of Mixed Phases on Electrical Conductivities for (CeF 3 ) 1– m (CaF 2 ) m Fast-Fluoride-Ion-Conducting Solid Electrolytes

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    Kazuhiro John Mori, Shuki Torii, Kenji Iwase, Takeshi Abe, Toshiharu Fukunaga

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  7. Mn2+ doped BaSnF4-based solid state electrolyte for room-temperature fluoride ion batteries

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  8. Near‐Room‐Temperature Quasi‐Solid‐State F‐Ion Batteries with High Conversion Reversibility Based on Layered Structured Electrolyte

    Advanced Energy Materials · 2023-01-20

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  9. Mechanochemical synthesis, microstructure and electrochemical properties of solid electrolytes with stabilized fluorite-type structure in the PbF2-SrF2-KF system for solid-state fluoride-ion batteries

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    Qianlong Ji, Natalia A. Mel’nikova, Oleg V. Glumov, Ivan Trefilov, Svetlana N. Eliseeva, Igor V. Murin

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  10. Challenges for fluoride superionic conductors: fundamentals, design, and applications

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  11. Growth and Characterization of All-Inorganic Halide Perovskite CsPbF3 Single Crystals

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  12. Fluorosulfide La 2+ x Sr 1– x F 4+ x S 2 with a Triple-Fluorite Layer Enabling Interstitial Fluoride-Ion Conduction

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  13. Construction and Interfacial Modification of a β-PbSnF4 Electrolyte with High Intrinsic Ionic Conductivity for a Room-Temperature Fluoride-Ion Battery

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  14. Synthesis and characterization of Sn-based electrolytes for F-ion batteries

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  15. Accelerated Exploration of Fast Fluoride-Ion Conductors Based on Compositional Descriptors

    ACS Applied Energy Materials · 2023-11-09

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  16. Ion Mobility in Crystalline Battery Materials

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  17. Studies on fluoride ion conductivity of the mechanochemically synthesized β-KSbF4 for all-solid-state fluoride-ion batteries

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  18. Composite anode for fluoride-ion batteries using alloy formation and phase separation in charge and discharge processes

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  19. Effect of Pb 6s 2 lone pair on the potential flattening of fluoride-ion conduction in perovskite-type fluoride

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  20. Effects of mixed phases on ionic conductivities for (LaF 3 ) 1– x (PbF 2 ) x fast-fluoride-ion-conducting solid electrolytes

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  21. Fluorosulfide La 2.7 Ba 6.3 F 8.7 S 6 with a double-layer honeycomb structure enabling fluoride-ion conduction

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  22. Long-cycle stable operation of fluoride-ion batteries at room temperature enabled by an advanced interface engineering and ion diffusion kinetics regulation strategy

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  23. Mechanochemical Synthesis of Fluorine-Conducting Solid Electrolytes Based on Tysonite and Fluorite Structures

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  24. Recent advances in aqueous and non-aqueous alkali metal hybrid ion capacitors

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  25. Structure design of a BiOF solid electrolyte with remarkably outstanding fluoride ion diffusion performance induced by Ga doping

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  26. TlSn 2 F 5 , a SnF 2 -based solid electrolyte with high ionic conductivity and electrochemical stability for all-solid-state fluoride ion batteries

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  28. Inorganic lithium-ion conductors for fast-charging lithium batteries: a review

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  29. High-Capacity and Long-Cycling F-Ion Pouch Cells Enabled by Green Electrolytes

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  30. Fluorine Chemistry in Rechargeable Batteries: Challenges, Progress, and Perspectives

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  31. Rocking‐Chair Aqueous Fluoride‐Ion Batteries Enabled by Hydrogen Bonding Competition

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  32. Rocking‐Chair Aqueous Fluoride‐Ion Batteries Enabled by Hydrogen Bonding Competition

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  33. Recent progress, challenges and prospects of electrolytes for fluoride-ion batteries

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  34. Atomically engineered Al-doped LaOCl for chlorine-ion batteries

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  35. Pressure Tuning and Sn Particle Size Optimization for Enhanced Performance in PbSnF4‐Based All‐Solid‐State Fluoride Ion Batteries

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  36. Effect of Uniaxial Stack Pressure on the Performance of Nanocrystalline Electrolytes and Electrode Composites for All‐Solid‐State Fluoride‐Ion Batteries

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  37. Solvation engineering of non-aqueous electrolytes for room-temperature fluoride-ion batteries

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  38. Electrolyte Design by Synergistic High‐Donor Solvent and Alcohol Anion Acceptor for Reversible Fluoride Ion Batteries

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  39. Machine learning potentials for the simulation of fluoride ion batteries electrolytes

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  40. Insights into the Micro-Structure-Transport Relationships of the Fluoride-Ion Conductor t -BaSnF 4 Synthesized by Spark Plasma Sintering

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  41. Fluoride-Ion Conduction by Synergic Rotation of the Anion Sublattice for Tl4.5SnF8.5 Analogues

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  44. Polymer Electrolyte Based All‐Solid‐State Rechargeable Fluoride Ion Batteries

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  45. Shielding Fluoride Ion Basicity through Diurea Coordination for Nonaqueous Fluoride Shuttle Batteries

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  47. Fluoride superionic conduction in TlF with the new anti-α-CuBr structure containing intrinsic F vacancies

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  48. Design and synthesis of a weakly solvated electrolyte for high-performance fluoride-ion batteries

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  49. Highly efficient atomic-scale design of CaF 2 for ultrafast fluoride-ion conduction

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  50. Development of all-solid-state fluoride ion battery with enhanced electrochemical stability

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