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RESEARCH PAPER · Journal of the American Chemical Society · 2020

Layered and Cubic Semiconductors AGaM′Q4 (A+ = K+, Rb+, Cs+, Tl+; M′4+ = Ge4+, Sn4+; Q2– = S2–, Se2–) and High Third-Harmonic Generation

Daniel Friedrich, Hye Ryung Byun, Shiqiang Hao, Shane Patel, Chris M. Wolverton, Joon Ik Jang, Mercouri G. Kanatzidis

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Layered and Cubic Semiconductors AGaM′Q4 (A+ = K+, Rb+, Cs+, Tl+; M′4+ = Ge4+, Sn4+; Q2– = S2–, Se2–) and High Third-Harmonic GenerationOriginalSynthesis, crystal structure and physical properties of a new chalcogenides Rb3Ga3Ge7S208Step by Step Bisacrificial Templates Growth of Bimetallic Sulfide QDs‐Attached MOF Nanosheets for Nonlinear Optical Limiting39ВЗАЄМОДІЯ У СИСТЕМАХ Tl2Sе–Ga(In)2Sе3–SnSе20Vast Structural and Polymorphic Varieties of Semiconductors AMM′Q4 (A = K, Rb, Cs, Tl; M = Ga, In; M′ = Ge, Sn; Q = S, Se)10Investigation into Structural Variation from 3D to 1D and Strong Second Harmonic Generation of the AHgPS4 (A+ = Na+, K+, Rb+, Cs+) Family26Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor8Hg-based chalcogenides: An intriguing class of infrared nonlinear optical materials129Structural modification from centrosymmetric Rb 4 Hg 2 Ge 2 S 8 to noncentrosymmetric (Na 3 Rb)Hg 2 Ge 2 S 8 : mixed alkali metals strategy for infrared nonlinear optical material design28Building-block approach to the discovery of Na8Mn2(Ge2Se6)2: A polar chalcogenide exhibiting promising harmonic generation signals with a high laser-induced damage threshold9First polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties16Infrared nonlinear optical performances of a new sulfide β-PbGa2S415New quaternary sulfide LiGaSiS4: Synthesis, structure and optical properties0AInSn2S6 (A = K, Rb, Cs)─Layered Semiconductors Based on the SnS2 Structure6AIB3IIC3IIIQ8VI: A New Family for the Design of Infrared Nonlinear Optical Materials by Coupling Octahedra and Tetrahedra Units152Ba3.5Cu7.55In1.15Se9: A Wide-Bandgap Copper Indium Selenide Reveals Strong Luminescence and Third-Harmonic Generation1Universal Method for Determining the Principal Optical Indicatrix Axes in Triclinic Crystals1Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 423Structure, Second-, and Third-Harmonic Generation of Li4P2S6: A Wide Gap Material with a High Laser-Induced Damage Threshold15“Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect80CsY2M3Se5: The first quaternary chalcogenides of the A–Y–M–Q (A = Rb/Cs; M = Cu/Ag; Q = S/Se) system0Pseudotetrahedral Organotin-Capped Chalcogenidometalate Supermolecules with Optical Limiting Performance16Alkali Metal-Ion Binding by a Model Macrocycle Containing a C-I···N Halogen Bonded Network: A DFT Study of C-I···M+ and N···M+ Binding Interactions, M+ = Li+, Na+, K+, and Rb+9Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications1AI2Mg3Ga12S22 (AI = K, Rb): T2-type supertetrahedra coupled with [MgS6] octahedra for designing wide-band gap infrared nonlinear optical materials with well-balanced properties16Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)6SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation7CsGaGe₃Se₈: Enhanced optical anisotropy and bandgap via cation-substitution-driven dimensionality reduction0Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion6Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion12

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  1. Synthesis, crystal structure and physical properties of a new chalcogenides Rb3Ga3Ge7S20

    Journal of Solid State Chemistry · 2021-01-07

    Shu‐Fang Li, Dong Yan

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  2. Step by Step Bisacrificial Templates Growth of Bimetallic Sulfide QDs‐Attached MOF Nanosheets for Nonlinear Optical Limiting

    Advanced Optical Materials · 2021-02-01

    Yin‐Di Zhu, Yao Kang, Zhi‐Gang Gu, Jian Zhang

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  3. ВЗАЄМОДІЯ У СИСТЕМАХ Tl2Sе–Ga(In)2Sе3–SnSе2

    Проблеми хімії та сталого розвитку · 2021-05-11

    Oksana Tsisar, Ivan D. Olekseyuk, Larysa Marushko, E. М. Kаdyкаlо, Л.В. Піскач

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  4. Vast Structural and Polymorphic Varieties of Semiconductors AMM′Q4 (A = K, Rb, Cs, Tl; M = Ga, In; M′ = Ge, Sn; Q = S, Se)

    Chemistry of Materials · 2021-08-05

    Daniel Friedrich, Shiqiang Hao, Shane Patel, Chris M. Wolverton, Mercouri G. Kanatzidis

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  5. Investigation into Structural Variation from 3D to 1D and Strong Second Harmonic Generation of the AHgPS4 (A+ = Na+, K+, Rb+, Cs+) Family

    Inorganic Chemistry · 2021-11-12

    Wenhao Xing, Chunlan Tang, Pifu Gong, Jieyun Wu, Zheshuai Lin, Jiyong Yao, Wenlong Yin, Bin Kang

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  6. Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor

    Chemistry - A European Journal · 2021-12-09

    Shannon Lee, Gayatri Viswanathan, Scott L. Carnahan, Colin P. Harmer, Georgiy Akopov, Aaron J. Rossini, Gordon J. Miller, Kirill A. Kovnir

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  7. Hg-based chalcogenides: An intriguing class of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-12-09

    Chunxiao Li, Xianghe Meng, Zhuang Li, Jiyong Yao

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  8. Structural modification from centrosymmetric Rb 4 Hg 2 Ge 2 S 8 to noncentrosymmetric (Na 3 Rb)Hg 2 Ge 2 S 8 : mixed alkali metals strategy for infrared nonlinear optical material design

    Journal of Materials Chemistry C · 2021-12-15

    Chunlan Tang, Wenhao Xing, Fei Liang, Mengran Sun, Jian Tang, Zheshuai Lin, Jiyong Yao, Kaixin Chen, Jieyun Wu, Wenlong Yin, Bin Kang

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  9. Building-block approach to the discovery of Na8Mn2(Ge2Se6)2: A polar chalcogenide exhibiting promising harmonic generation signals with a high laser-induced damage threshold

    Journal of Alloys and Compounds · 2021-12-23

    Srikanth Balijapelly, Andrew J. Craig, Jeong Bin Cho, Joon Ik Jang, K. Ghosh, Jennifer A. Aitken, Aleksandr Chernatynskiy, Amitava Choudhury

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  10. First polar quaternary sulphide CsLiGa 6 S 10 with mixed ordered alkali cations displaying excellent infrared nonlinear optical properties

    Inorganic Chemistry Frontiers · 2022-01-01

    Zi Wang, Bin‐Wen Liu, Guo‐Cong Guo

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  11. Infrared nonlinear optical performances of a new sulfide β-PbGa2S4

    Journal of Alloys and Compounds · 2022-02-02

    Wen‐Fa Chen, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  12. New quaternary sulfide LiGaSiS4: Synthesis, structure and optical properties

    Journal of Solid State Chemistry · 2022-05-10

    Ziyi Chen, Dajiang Mei, Xiao‐Ming Jiang, Jun Zhao, Yuandong Wu, Jihu Wang, Shaoguo Wen

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  13. AInSn2S6 (A = K, Rb, Cs)─Layered Semiconductors Based on the SnS2 Structure

    Inorganic Chemistry · 2022-08-12

    Daniel Friedrich, Michael A. Quintero, Shiqiang Hao, Craig C. Laing, Christopher Wolverton, Mercouri G. Kanatzidis

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  14. AIB3IIC3IIIQ8VI: A New Family for the Design of Infrared Nonlinear Optical Materials by Coupling Octahedra and Tetrahedra Units

    Journal of the American Chemical Society · 2022-11-18

    Ling Luo, Linan Wang, Jianbang Chen, Jiazheng Zhou, Zhihua Yang, Shilie Pan, Junjie Li

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  15. Ba3.5Cu7.55In1.15Se9: A Wide-Bandgap Copper Indium Selenide Reveals Strong Luminescence and Third-Harmonic Generation

    Inorganic Chemistry · 2023-01-19

    Yu-Hsuan Su, Weiliang Chen, Hye Ryung Byun, Yufu Zhang, Min-Rui Zhuang, Yu-Cih Lin, Chung‐Kai Chang, Po-Yuan Wang, Che-Cheng Lin, Kuang‐I Lin, Hsin‐Kuan Liu, Min-Kai Lee, Joon Ik Jang, Yu‐Ming Chang, Kuei‐Fang Hsu

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  16. Universal Method for Determining the Principal Optical Indicatrix Axes in Triclinic Crystals

    Crystal Growth & Design · 2023-02-13

    Jingcheng Feng, Lei Bai, Guochun Zhang

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  17. Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 4

    Inorganic Chemistry · 2023-04-16

    Mengjie Ma, Junhui Dang, Yuandong Wu, Xiao‐Ming Jiang, Dajiang Mei

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  18. Structure, Second-, and Third-Harmonic Generation of Li4P2S6: A Wide Gap Material with a High Laser-Induced Damage Threshold

    Chemistry of Materials · 2023-08-31

    Benjamin M. Oxley, Kyeong‐Hyeon Lee, Thomas S. Ie, Jae Mo Lee, Michael J. Waters, James M. Rondinelli, Joon Ik Jang, Mercouri G. Kanatzidis

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  19. “Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect

    Advanced Functional Materials · 2023-12-28

    Yu Chu, Hongshan Wang, Quan Chen, Xin Su, Zuxin Chen, Zhihua Yang, Junjie Li, Shilie Pan

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  20. CsY2M3Se5: The first quaternary chalcogenides of the A–Y–M–Q (A = Rb/Cs; M = Cu/Ag; Q = S/Se) system

    Journal of Solid State Chemistry · 2023-12-29

    Sweta Yadav, Gopabandhu Panigrahi, Manish K. Niranjan, Jai Prakash

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  21. Pseudotetrahedral Organotin-Capped Chalcogenidometalate Supermolecules with Optical Limiting Performance

    Journal of the American Chemical Society · 2024-03-05

    Ming‐Bu Luo, Heng-Dong Lai, Shan‐Lin Huang, Jian Zhang, Qipu Lin

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  22. Alkali Metal-Ion Binding by a Model Macrocycle Containing a C-I···N Halogen Bonded Network: A DFT Study of C-I···M+ and N···M+ Binding Interactions, M+ = Li+, Na+, K+, and Rb+

    Inorganics · 2024-06-06

    Rubén D. Parra

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  23. Cationic substitution engineering induces a new quaternary chalcogenide in the A–M IIIA –M IVA –Q system for optical crystal applications

    CrystEngComm · 2025-01-01

    Yue Wang, Xuezhong Li, Zihao Lou, Yong‐Fang Shi

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  24. AI2Mg3Ga12S22 (AI = K, Rb): T2-type supertetrahedra coupled with [MgS6] octahedra for designing wide-band gap infrared nonlinear optical materials with well-balanced properties

    Science China Materials · 2025-01-22

    Mengmeng Chen, Xu Liu, Abudukadi Tudi, Cui Chen, Qixian Ren, Zhihua Yang, Yabo Wu, Shilie Pan

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  25. Symmetry over Chemistry: Harmonic Generation of Low-Dimensional Alkali Chalcopnictates RbMP2S6 (M = Sb, Bi)

    Chemistry of Materials · 2025-03-21

    Benjamin M. Oxley, Joshua Lim, Kyeong‐Hyeon Lee, Jeong-Bin Cho, Saugata Sarker, Jadupati Nag, Michael J. Waters, James M. Rondinelli, Venkatraman Gopalan, Joon Ik Jang, Mercouri G. Kanatzidis

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  26. SrZnSiS4: Shattering the 4.0 eV Threshold toward Dual-Optimized Bandgap and Second-Harmonic Generation

    Inorganic Chemistry · 2025-09-04

    Huilin Yin, Xia Wu, Shuchang Wu, Changsheng Sun, Chengxiao Wang, Jiaman Sun, Yang Liu, Xiao‐Ming Jiang, Ximeng Lv, Dajiang Mei

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  27. CsGaGe₃Se₈: Enhanced optical anisotropy and bandgap via cation-substitution-driven dimensionality reduction

    Inorganic Chemistry Communications · 2025-10-01

    Yue Wang, Rongfang Jiang, Zihao Lou, Yong‐Fang Shi

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  28. Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion

    Angewandte Chemie · 2026-01-05

    Meng‐Na Jing, Si‐Fan Lu, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  29. Realizing Phase‐Matching of Nonlinear Optical [ABa 3 Br 2 ][Ga 5 Se 10 ] (A = Cs, Rb, K, Na) Through Large Anisotropic Lattice Distortion

    Angewandte Chemie International Edition · 2026-01-05

    Meng‐Na Jing, Si‐Fan Lu, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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