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RESEARCH PAPER · Chemistry of Materials · 2020

Bi 3 (SeO 3 ) 3 (Se 2 O 5 )F: A Polar Bismuth Selenite Fluoride with Polyhedra of Highly Distortive Lone Pair Cations and Strong Second-Harmonic Generation Response

Jee Yoon Chung, Hongil Jo, Seongbeom Yeon, Hye Ryung Byun, Tae‐Soo You, Joon Ik Jang, Kang Min Ok

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Bi 3 (SeO 3 ) 3 (Se 2 O 5 )F: A Polar Bismuth Selenite Fluoride with Polyhedra of Highly Distortive Lone Pair Cations and Strong Second-Harmonic Generation ResponseOriginalSelenite bromide nonlinear optical materials Pb 2 GaF 2 (SeO 3 ) 2 Br and Pb 2 NbO 2 (SeO 3 ) 2 Br: synthesis and characterization20Sn3B8O15: A Ternary Tin(II) Borate with Flexible [B8O18]12– Fundamental Building Block Formed by [B7O16]11– and [BO3]3– Groups10Facile syntheses of silver thioantimonates exhibiting second-harmonic generation responses and large birefringence18In situ hydrothermal synthesis of polar second-order nonlinear optical selenate Na 5 (SeO 4 )(HSeO 4 ) 3 (H 2 O) 219Role of fluorine on the structure and second-harmonic-generation property of inorganic selenites and tellurites23Unexpected aliovalent cation substitution between two NLO materials LiBa 3 Bi 6 (SeO 3 ) 7 F 11 and Ba 3 Bi 6.5 (SeO 3 ) 7 F 10.5 O 0.518Order and Disorder: Toward the Thermodynamically Stable α-BaMoO2F4 from the Metastable Polymorph31Second-order nonlinear optical property of the ultraviolet transparent alkali metal-rare earth metal carbonate Na3Y(CO3)3.3H2O5Structure, Photoluminescence Emissions, and Photocatalytic Activity of Ag2SeO3: A Joint Experimental and Theoretical Investigation23Solvothermal Syntheses of Three-Dimensional Open-Framework Thioantimonates Displaying Nonlinear Optical Responses5Giant Second-Harmonic Generation Response and Large Band Gap in the Partially Fluorinated Mid-Infrared Oxide RbTeMo 2 O 8 F149The Role of Acidity in the Synthesis of Novel Uranyl Selenate and Selenite Compounds and Their Structures2GaSeCl5O: A Molecular Compound with Very Strong SHG Effect19Harnessing Bismuth Coordination Chemistry to Achieve Bright, Long-Lived Organic Phosphorescence24Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations48Polymorphic Pb14O8I12 and Pb7O4I6 oxyhalides featuring unprecedented [O8Pb14] clusters with broad IR transparency20Nonlinear optical properties of a new polar bismuth tellurium oxide fluoride, Bi3F(TeO3)(TeO2F2)315Complex coordinated functional groups: A great genes for nonlinear optical materials64( R )- and ( S )-[C 8 H 10 NO 3 ] 2 [NbOF 5 ]: noncentrosymmetric niobium oxyfluorides with large optical anisotropy3Metal oxyhalides: an emerging family of nonlinear optical materials124Towards a relationship between photoluminescence emissions and photocatalytic activity of Ag 2 SeO 4 : combining experimental data and theoretical insights10Wide bandgaps and strong SHG responses of hetero-oxyfluorides by dual-fluorination-directed bandgap engineering28Na 3 Ti 3 O 3 (SeO 3 ) 4 F: A Phase-Matchable Nonlinear-Optical Crystal with Enlarged Second-Harmonic-Generation Intensity and Band Gap20Uncovering the Structural Diversity and Excellent Performance of a Deep Ultraviolet Nonlinear Optical System Li(B2O3)nF (n= 1, 1.5, 2, and 3) by Multicomponent Prediction26PbBi(SeO 3 ) 2 F and Pb 2 Bi(SeO 3 ) 2 Cl 3 : Coexistence of Three Kinds of Stereochemically Active Lone-Pair Cations Exhibiting Excellent Nonlinear Optical Properties57Predicting Diamond-like Nitrides as Infrared Nonlinear Optical Materials with High Thermal Conductivity20From CdPb 8 (SeO 3 ) 4 Br 10 to Pb 3 (TeO 3 )Br 4 : the first tellurite bromide exhibiting an SHG response and mid-IR transparency21Second-harmonic-generation of [(Se,Te)Cl 3 ] + [GaCl 4 ] − with aligned ionic tetrahedra6Polar Bismuth Selenite Iodate Oxide BiSeIO6 with Three Types of Lone Pair Cations in One Structure6The First UV Nonlinear Optical Selenite Material: Fluorination Control in CaYF(SeO 3 ) 2 and Y 3 F(SeO 3 ) 485The First UV Nonlinear Optical Selenite Material: Fluorination Control in CaYF(SeO3)2 and Y3F(SeO3)47Elucidating the structure-nonlinear optical property relationship of Te2O4(OH)26Y(HSeO3)(SeO3)(H2O)·(H2O) and Y2(SeO3)2(SeO4)(H2O)2·(H2O)0.75: Two yttrium selenites with a short UV cut-off edge explored from pure selenite compounds20Hg3(SeO3)2(SO4): A UV Nonlinear Optical Mercury Selenite Sulfate Constructed by Neat [Hg6O8(SeO3)4]∞ Layers and SO4 Tetrahedra27A survey of stereoactive oxysalts for linear and nonlinear optical applications40Four UV Transparent Linear and Nonlinear Optical Materials Explored from Pure Selenite Compounds22A two-fold interpenetrated mixed-ligands acentric 3D coordination polymer Zn(OBA)(DIB)·0.5H2O: Topological analysis, fluorescent and second-order NLO properties7KBi(SeO4)(IO3)Cl: A mixed-anion oxychloride with three types of building units in one structure2(TeCl) 4 (TiCl 4 ) with isolated Te 4 Cl 16 and TiCl 4 molecules and second-harmonic-generation4Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Reticular chemistry-aided effective design of new second-order nonlinear optical selenites11Hg3Se(SeO3)(SO4): A Mixed-Valent Selenium Compound with Mid-Infrared Transmittance Obtained by In Situ Reaction26Metal Methanesulfonates with Mixed Anionic Groups with Large Band Gaps and Enhanced Birefringence50UV-Transparent SHG Material Explored in an Alkali Metal Sulfate Selenite System16MgHg(SeO3)2(H2O)2: A magnesium mercury selenite with large birefringence6Old tree blossoms anew: Research progress on the structures and optical properties of ultraviolet selenites56Lewis‐Acid‐Base Synthesis of [Se3Cl3]2[SnCl6] and [BMIm]2[Ga8As6Cl16O14]0Analogous Chain Selenite Chlorides Ba 2 M(SeO 3 ) 2 Cl 2 (M = Cu 2+ , Ni 2+ , Co 2+ , Mn 2+ ) and Pb 2 Cu(SeO 3 ) 2 Cl 2 with Tunable Spin S : Syntheses and Characterizations7Polar Layered Magnet Ba 2 Cu 3 (SeO 3 ) 4 F 2 Composed of Bitriangular Chains: Observation of 1/3-Magnetization Plateau5RE(HSeO3)(SeO3)(H2O)·(H2O) (RE = Y, Gd): Two Rare-Earth Selenite Nonlinear Optical Crystals with Wide Band Gaps6Unprecedented v-shaped [SeO2E] units stabilized in KM[Se2O5]2[SeO2] (M= Al and Ga) constructed by nanoconfinement strategy6Superior thermoelectric power factor in BiCuSeO enabled by a ferromagnetic metallic phase and spin entropy effect3Chemical Substitution‐Driven Design of a High‐Performance Noncentrosymmetric Bismuth Molybdenum Selenite10Pb 4 O 3 I 2 : A Lead Oxyhalide IR Optical Crystal with an Unprecedented 1 ∞ [O 3 Pb 4 ] Chain Featuring a Wide Transmittance Range and Large Birefringence3Synthesis of Four Isomeric Phases of CdVO(SeO3)2 and Characterization of Their Structural, Thermal, and Magnetic Properties2Ag3In3(SeO3)3(SO4)F4: A Sulfate Selenite Nonlinear Optical Material with a Wide Bandgap3Stepwise Substitution Strategy for Beryllium-Based Selenites with Enhanced SHG Response, Moderate Birefringence, and Short UV Cutoff Edges6ZnGa(SeO 3 ) 2 F: a UV transparent birefringent crystal explored in M( ii )–IIIA–selenite–F systems2A mercury-based selenite with wide bandgap and moderate birefringence via cation substitution and partial fluorination1InO6X (X = Cl, Br): distinct functional motif family for nonlinear optical materials5Magnetic Copper Selenite-Sulfate Cu 3 O 2 (HSeO 3 )(HSO 4 )(H 2 O) with T26-Type Non-Archimedean Lattice Featuring a Robust 1/3-Magnetization Plateau2Advances in metal selenite nonlinear optical materials: halogens directed structure modulation and property optimization0Three‐dimensional hybrid perovskite heterostructure single crystals toward highly efficient x‐ray detectors0

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  1. Selenite bromide nonlinear optical materials Pb 2 GaF 2 (SeO 3 ) 2 Br and Pb 2 NbO 2 (SeO 3 ) 2 Br: synthesis and characterization

    Dalton Transactions · 2020-01-01

    Huanke Zhao, Pifu Gong, Xinyuan Zhang, Zheshuai Lin, Zhanggui Hu, Yicheng Wu

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  2. Sn3B8O15: A Ternary Tin(II) Borate with Flexible [B8O18]12– Fundamental Building Block Formed by [B7O16]11– and [BO3]3– Groups

    Inorganic Chemistry · 2020-12-29

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  3. Facile syntheses of silver thioantimonates exhibiting second-harmonic generation responses and large birefringence

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    Gang Yang, Xingxing Jiang, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  4. In situ hydrothermal synthesis of polar second-order nonlinear optical selenate Na 5 (SeO 4 )(HSeO 4 ) 3 (H 2 O) 2

    Inorganic Chemistry Frontiers · 2021-01-01

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  5. Role of fluorine on the structure and second-harmonic-generation property of inorganic selenites and tellurites

    Chemical Communications · 2021-01-01

    Fang Kong, Ting-Kun Jiang, Jiang‐Gao Mao

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  6. Unexpected aliovalent cation substitution between two NLO materials LiBa 3 Bi 6 (SeO 3 ) 7 F 11 and Ba 3 Bi 6.5 (SeO 3 ) 7 F 10.5 O 0.5

    Chemical Communications · 2021-01-01

    Shuangshuang Shi, Chensheng Lin, Dan Zhao, Min Luo, Liling Cao, Guang Peng, Ning Ye

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  7. Order and Disorder: Toward the Thermodynamically Stable α-BaMoO2F4 from the Metastable Polymorph

    Chemistry of Materials · 2021-02-25

    Hongil Jo, Min Hyung Lee, Kang Min Ok

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  8. Second-order nonlinear optical property of the ultraviolet transparent alkali metal-rare earth metal carbonate Na3Y(CO3)3.3H2O

    Journal of Solid State Chemistry · 2021-02-28

    Chao Wu, Lin Lin, Tianhui Wu, Zhipeng Huang, Chi Zhang

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  9. Structure, Photoluminescence Emissions, and Photocatalytic Activity of Ag2SeO3: A Joint Experimental and Theoretical Investigation

    Inorganic Chemistry · 2021-03-26

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  10. Solvothermal Syntheses of Three-Dimensional Open-Framework Thioantimonates Displaying Nonlinear Optical Responses

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  11. Giant Second-Harmonic Generation Response and Large Band Gap in the Partially Fluorinated Mid-Infrared Oxide RbTeMo 2 O 8 F

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  12. The Role of Acidity in the Synthesis of Novel Uranyl Selenate and Selenite Compounds and Their Structures

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  13. GaSeCl5O: A Molecular Compound with Very Strong SHG Effect

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  14. Harnessing Bismuth Coordination Chemistry to Achieve Bright, Long-Lived Organic Phosphorescence

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    Alexander C. Marwitz, Aaron D. Nicholas, Leticia M. Breuer, Jeffery A. Bertke, Karah E. Knope

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  15. Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations

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  16. Polymorphic Pb14O8I12 and Pb7O4I6 oxyhalides featuring unprecedented [O8Pb14] clusters with broad IR transparency

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  17. Nonlinear optical properties of a new polar bismuth tellurium oxide fluoride, Bi3F(TeO3)(TeO2F2)3

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  18. Complex coordinated functional groups: A great genes for nonlinear optical materials

    Chinese Chemical Letters · 2021-12-03

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  19. ( R )- and ( S )-[C 8 H 10 NO 3 ] 2 [NbOF 5 ]: noncentrosymmetric niobium oxyfluorides with large optical anisotropy

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  20. Metal oxyhalides: an emerging family of nonlinear optical materials

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  21. Towards a relationship between photoluminescence emissions and photocatalytic activity of Ag 2 SeO 4 : combining experimental data and theoretical insights

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  22. Wide bandgaps and strong SHG responses of hetero-oxyfluorides by dual-fluorination-directed bandgap engineering

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  23. Na 3 Ti 3 O 3 (SeO 3 ) 4 F: A Phase-Matchable Nonlinear-Optical Crystal with Enlarged Second-Harmonic-Generation Intensity and Band Gap

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  24. Uncovering the Structural Diversity and Excellent Performance of a Deep Ultraviolet Nonlinear Optical System Li(B2O3)nF (n= 1, 1.5, 2, and 3) by Multicomponent Prediction

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  25. PbBi(SeO 3 ) 2 F and Pb 2 Bi(SeO 3 ) 2 Cl 3 : Coexistence of Three Kinds of Stereochemically Active Lone-Pair Cations Exhibiting Excellent Nonlinear Optical Properties

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  26. Predicting Diamond-like Nitrides as Infrared Nonlinear Optical Materials with High Thermal Conductivity

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  27. From CdPb 8 (SeO 3 ) 4 Br 10 to Pb 3 (TeO 3 )Br 4 : the first tellurite bromide exhibiting an SHG response and mid-IR transparency

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  28. Second-harmonic-generation of [(Se,Te)Cl 3 ] + [GaCl 4 ] − with aligned ionic tetrahedra

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  29. Polar Bismuth Selenite Iodate Oxide BiSeIO6 with Three Types of Lone Pair Cations in One Structure

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  30. The First UV Nonlinear Optical Selenite Material: Fluorination Control in CaYF(SeO 3 ) 2 and Y 3 F(SeO 3 ) 4

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  31. The First UV Nonlinear Optical Selenite Material: Fluorination Control in CaYF(SeO3)2 and Y3F(SeO3)4

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  32. Elucidating the structure-nonlinear optical property relationship of Te2O4(OH)2

    Materials Today Physics · 2023-04-05

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  33. Y(HSeO3)(SeO3)(H2O)·(H2O) and Y2(SeO3)2(SeO4)(H2O)2·(H2O)0.75: Two yttrium selenites with a short UV cut-off edge explored from pure selenite compounds

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  34. Hg3(SeO3)2(SO4): A UV Nonlinear Optical Mercury Selenite Sulfate Constructed by Neat [Hg6O8(SeO3)4]∞ Layers and SO4 Tetrahedra

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  35. A survey of stereoactive oxysalts for linear and nonlinear optical applications

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  36. Four UV Transparent Linear and Nonlinear Optical Materials Explored from Pure Selenite Compounds

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  37. A two-fold interpenetrated mixed-ligands acentric 3D coordination polymer Zn(OBA)(DIB)·0.5H2O: Topological analysis, fluorescent and second-order NLO properties

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  38. KBi(SeO4)(IO3)Cl: A mixed-anion oxychloride with three types of building units in one structure

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  39. (TeCl) 4 (TiCl 4 ) with isolated Te 4 Cl 16 and TiCl 4 molecules and second-harmonic-generation

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  40. Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics

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  41. Reticular chemistry-aided effective design of new second-order nonlinear optical selenites

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  42. Hg3Se(SeO3)(SO4): A Mixed-Valent Selenium Compound with Mid-Infrared Transmittance Obtained by In Situ Reaction

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  43. Metal Methanesulfonates with Mixed Anionic Groups with Large Band Gaps and Enhanced Birefringence

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  44. UV-Transparent SHG Material Explored in an Alkali Metal Sulfate Selenite System

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  45. MgHg(SeO3)2(H2O)2: A magnesium mercury selenite with large birefringence

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  46. Old tree blossoms anew: Research progress on the structures and optical properties of ultraviolet selenites

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  47. Lewis‐Acid‐Base Synthesis of [Se3Cl3]2[SnCl6] and [BMIm]2[Ga8As6Cl16O14]

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  48. Analogous Chain Selenite Chlorides Ba 2 M(SeO 3 ) 2 Cl 2 (M = Cu 2+ , Ni 2+ , Co 2+ , Mn 2+ ) and Pb 2 Cu(SeO 3 ) 2 Cl 2 with Tunable Spin S : Syntheses and Characterizations

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  49. Polar Layered Magnet Ba 2 Cu 3 (SeO 3 ) 4 F 2 Composed of Bitriangular Chains: Observation of 1/3-Magnetization Plateau

    Chemistry of Materials · 2024-08-12

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  50. RE(HSeO3)(SeO3)(H2O)·(H2O) (RE = Y, Gd): Two Rare-Earth Selenite Nonlinear Optical Crystals with Wide Band Gaps

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