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RESEARCH PAPER · Materials Horizons · 2020

Crystal regulation towards rechargeable magnesium battery cathode materials

Shuangshuang Tan, Fangyu Xiong, Junjun Wang, Qinyou An, Liqiang Mai

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Crystal regulation towards rechargeable magnesium battery cathode materialsOriginalAdvances in rechargeable Mg batteries148Multivalent Mg2+-, Zn2+-, and Ca2+-Ion Intercalation Chemistry in a Disordered Layered Structure212D Ti3C2 MXene embedded with Co(II)(OH)n nanoparticles as the cathode material for hybrid magnesium–lithium-ion batteries21Design of new electrode materials by Soft Chemistry for multivalent ion batteries0Does Water Enhance Mg Intercalation in Oxides? The Case of a Tunnel Framework17Unravelling the role of interfacial chemistry evolution in the kinetics of zinc insertion into chevrel phase12The potential application of VS2 as an electrode material for Mg ion battery: A DFT study99Recent Progress and Challenges in the Optimization of Electrode Materials for Rechargeable Magnesium Batteries90A comprehensive review of the development of magnesium anodes for primary batteries162Crystal defect modulation in cathode materials for non-lithium ion batteries: Progress and challenges109MoS2/graphene heterostructure with facilitated Mg-diffusion kinetics for high-performance rechargeable magnesium batteries68Recent Progress in Electrolyte Development and Design Strategies for Next‐Generation Potassium‐Ion Batteries53Interlayer Engineering of Preintercalated Layered Oxides as Cathode for Emerging Multivalent Metal-ion Batteries: Zinc and Beyond182An Overview on Anodes for Magnesium Batteries: Challenges towards a Promising Storage Solution for Renewables130Designing Nanostructured Metal Chalcogenides as Cathode Materials for Rechargeable Magnesium Batteries94Magnesium Deintercalation From the Spinel‐Type MgMn2‐yFeyO4 (0.4≤y≤2.0) by Acid‐Treatment and Electrochemistry11Magnesium Ion Storage Properties in a Layered (NH4)2V6O16·1.5H2O Nanobelt Cathode Material Activated by Lattice Water34A Bismuth-Based Protective Layer for Magnesium Metal Anode in Noncorrosive Electrolytes193High-rate performance magnesium batteries achieved by direct growth of honeycomb-like V2O5 electrodes with rich oxygen vacancies41Interlayer‐Expanded MoS2 Containing Structural Water with Enhanced Magnesium Diffusion Kinetics and Durability9Dual redox groups enable organic cathode material with a high capacity for aqueous zinc-organic batteries41Polyaniline nanoarrays/carbon cloth as binder-free and flexible cathode for magnesium ion batteries64Lattice Expanding by Te-Substitution to Boost Electrochemical Mg Storage of Cu7.2s4 Nanotube Cathode30Low‐strain TiP2O7 with three‐dimensional ion channels as long‐life and high‐rate anode material for Mg‐ion batteries117Anionic Te-Substitution Boosting the Reversible Redox in CuS Nanosheet Cathodes for Magnesium Storage113Solid‐State Electrolytes for Rechargeable Magnesium‐Ion Batteries: From Structure to Mechanism61Strategy of cation/anion co-doping for potential elevating of VS4 cathode for magnesium ion batteries53Ether–Water Hybrid Electrolyte Contributing to Excellent Mg Ion Storage in Layered Sodium Vanadate98Flexible three-dimensional-networked iron vanadate nanosheet arrays/carbon cloths as high-performance cathodes for magnesium ion batteries30Research advances of magnesium and magnesium alloys worldwide in 2021536Vanadium-based cathodes for aqueous zinc-ion batteries: Mechanism, design strategies and challenges329Preparation of conductive Cu1.5Mn1.5O4 and Mn3O4 spinel mixture powders as positive active materials in rechargeable Mg batteries operative at room temperature2RETRACTED: Exploring the application of AlN graphyne in calcium ion batteries12Octylamine‐Supporting Interlayer Expanded Molybdenum Diselenide as a High‐Power Cathode for Rechargeable Mg Batteries18Novel Organic Cathode with Conjugated N-Heteroaromatic Structures for High-Performance Aqueous Zinc-Ion Batteries70Kinetically optimized copper sulfide cathodes for rechargeable magnesium batteries40Zinc‐ion hybrid supercapacitors: Design strategies, challenges, and perspectives62A Molybdenum Polysulfide In-Situ Generated from Ammonium Tetrathiomolybdate for High-Capacity and High-Power Rechargeable Magnesium Battery Cathodes41Progress and perspective on rechargeable magnesium-ion batteries38Effects of Position and Quantity of the Cyano Group in Organic Electrode Materials on Electrochemical Performance10Electrochemical properties and crystal and electronic structure changes during charge/discharge of spinel type cathode-materials Mg1.33V1.67-Mn O4 for magnesium secondary batteries8Vanadium-based cathode materials for rechargeable magnesium batteries28A two-dimensional VO 2 /VS 2 heterostructure as a promising cathode material for rechargeable Mg batteries: a first principles study11Hierarchical BiOCl flowerlike microspheres via a room-temperature solid-state chemical reaction as a new anode for rechargeable magnesium-ion batteries22Oxygen – a fatal impurity for reversible magnesium deposition/dissolution16A Single Mg Ion-conductive Polymer-coated MgCo2O4 for Mg Rechargeable Batteries3Cathode Electrolyte Interphase (CEI) Endows Mo 6 S 8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics70Cathode Electrolyte Interphase (CEI) Endows Mo6S8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics8Modulating vacancies concentration ratio of cationic and anionic in WO3 for driving high performance magnesium ions storage45Efficient boron-based electrolytes constructed by anionic and interfacial co-regulation for rechargeable magnesium batteries41Layered buserite Mg-Mn oxide cathode for aqueous rechargeable Mg-ion battery58Localized Ligands Assist Ultrafast Multivalent‐Cation Intercalation Pseudocapacitance4Localized Ligands Assist Ultrafast Multivalent‐Cation Intercalation Pseudocapacitance40Regulating solvation sheath by introducing multifunctional fluoride boronic esters for highly efficient magnesium stripping/plating36Toward Improved Anodic Stability of Ether-Based Electrolytes for Rechargeable Magnesium Batteries24Cu+ redox activation and polyselenide stabilization via strong Se-C interaction for superior magnesium storage33Layered Materials in the Magnesium Ion Batteries: Development History, Materials Structure, and Energy Storage Mechanism24Research advances of magnesium and magnesium alloys worldwide in 20210Research advances of magnesium and magnesium alloys worldwide in 20211Strong solvent coordination effect inducing gradient solid-electrolyte-interphase formation for highly efficient Mg plating/stripping102Magnesium-based energy materials: Progress, challenges, and perspectives181Bi nanoparticles encapsulated in nitrogen-doped carbon as a long-life anode material for magnesium batteries26Nanowires for Multivalent‐ion Batteries0Organic cathode materials for rechargeable magnesium-ion batteries: Fundamentals, recent advances, and approaches to optimization59A Hauser-base modulated boron-based electrolyte empowering superior interfacial chemistry in rechargeable magnesium batteries17Binary Mg‐1 at%Gd alloy anode for high‐performance rechargeable magnesium batteries6A review of metal sulfide cathode materials for non-aqueous multivalent ion (Mg2+, Ca2+, Al3+) batteries19MoS2 for Battery and Supercapacitor Applications0Transition metal oxides and transition metal sulfides as cathodes for magnesium-ion batteries: current status and modification strategies34Mo3S13 Cluster-Based Cathodes for Rechargeable Magnesium Batteries: Reversible Magnesium Association/Dissociation at the Bridging Disulfur along with Sulfur–Sulfur Bond Break/Formation9A perspective on the key factors of safety for rechargeable magnesium batteries32Large-Scale Integration of the Ion-Reinforced Phytic Acid Layer Stabilizing Magnesium Metal Anode47Utilization of Delithiation-Induced Amorphous Oxide as a Cathode for Rechargeable Magnesium Batteries11Interfacial chemistry of anode/electrolyte interface for rechargeable magnesium batteries49Fine nanostructure design of metal chalcogenide conversion-based cathode materials for rechargeable magnesium batteries14Initiating cationic-anionic chemistry with stepwise surface-to-inner conversion in copper selenide superstructures for high-energy rechargeable magnesium batteries15The Enormous Potential of Sodium/Potassium‐Ion Batteries as the Mainstream Energy Storage Technology for Large‐Scale Commercial Applications190BP-biphenylene monolayers: A promising anode material for high-performance magnesium-ion batteries13Electron-injection-engineering induced dual-phase MoO2.8F0.2/MoO2.4F0.6 heterostructure for magnesium storage11Cu3VSe4 Cathode for Rechargeable Magnesium Batteries: Favorable Chemical and Electronic Structures Inducing Intercalation and Displacement Reactions16Organic Heterophase Composites Induced Sulfur Vacancies and Internal Electric Field Enhancement for Advanced Magnesium Storage of Copper Sulfide Cathodes233D Tunnel Copper Tetrathiovanadate Nanocube Cathode Achieving Ultrafast Magnesium Storage Reactions through a Charge Delocalization and Displacement Mechanism23Co-intercalation of solvated Mg2+ in amine-chain-expanded VOPO4 cathodes with fast kinetics under high-voltage condition8Physical and chemical interfacial engineering of Mg anodes for rechargeable magnesium batteries24Boosting anionic-cationic redox chemistry in anion-rich CuSe2 cathode toward high-energy magnesium batteries9In Situ Electrochemical Atomic Force Microscopy Study of Interfacial Reactions on a Graphite Negative Electrode for Magnesium-Ion Batteries0Insertion-type cathode materials in magnesium ion batteries: Research progress and application potential4High voltage cathode materials for rechargeable magnesium batteries: Structural aspects and electrochemical perspectives13Comparison of the insertion-extraction of Ca and Mg ions in amorphous CaMn2O4 post-spinel-based cathodes in aqueous media3Interface Engineering Endowing High Reversibility of SPAN Cathode and Mg Metal Anode for Mg‐SPAN Batteries1Mechanistic Insights into Magnesium Metal Anodes: Interfacial Challenges and Design Principles in Organic and Aqueous Electrolytes17Polyaniline-Pyrrole as a Potential Cathode Modifier in Magnesium-Sulfur Battery: An Ab Initio Study0Multi‐Step Data‐Driven High‐Voltage MgMn 2 O 4 with Inorganic‐Rich Cathode‐Electrolyte Interphase for Stable Mg 2+ Storage0A perspective on practical rechargeable magnesium batteries0Enabling 3 V magnesium-sodium hybrid battery by fluorinated alkoxyborate-based double-salt electrolytes3Tailoring electrochemical kinetics in Mg-ion batteries using defect-rich Mg-doped iron vanadium oxide as cathode material0Synthesis of DOTAB assisted nickel manganese ferrite nanoparticles for neurotransmitter detection and energy storage applications1Manganese-Based Oxide Cathode Materials for Aqueous Magnesium-Ion Batteries1Bioinspired Solvation‐Interfacial Dual Regulation for Subzero‐Tolerant and Long‐Cycling Aqueous Zinc Metal Batteries1Anion-cation coordination reconstruction enables a regulated Helmholtz layer for stable chloride-free rechargeable magnesium metal batteries0Defect‐Mediated Mg 2+ Transport and Structural Stability in the Sulfide Cathodes for Rechargeable Magnesium Batteries0Advances of metal-organic framework based materials for aqueous multivalent metal-ion batteries0

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  1. Advances in rechargeable Mg batteries

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  2. Multivalent Mg2+-, Zn2+-, and Ca2+-Ion Intercalation Chemistry in a Disordered Layered Structure

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  3. 2D Ti3C2 MXene embedded with Co(II)(OH)n nanoparticles as the cathode material for hybrid magnesium–lithium-ion batteries

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  4. Design of new electrode materials by Soft Chemistry for multivalent ion batteries

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  5. Does Water Enhance Mg Intercalation in Oxides? The Case of a Tunnel Framework

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  6. Unravelling the role of interfacial chemistry evolution in the kinetics of zinc insertion into chevrel phase

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  7. The potential application of VS2 as an electrode material for Mg ion battery: A DFT study

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  8. Recent Progress and Challenges in the Optimization of Electrode Materials for Rechargeable Magnesium Batteries

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  9. A comprehensive review of the development of magnesium anodes for primary batteries

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  10. Crystal defect modulation in cathode materials for non-lithium ion batteries: Progress and challenges

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  11. MoS2/graphene heterostructure with facilitated Mg-diffusion kinetics for high-performance rechargeable magnesium batteries

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  14. An Overview on Anodes for Magnesium Batteries: Challenges towards a Promising Storage Solution for Renewables

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  15. Designing Nanostructured Metal Chalcogenides as Cathode Materials for Rechargeable Magnesium Batteries

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  16. Magnesium Deintercalation From the Spinel‐Type MgMn2‐yFeyO4 (0.4≤y≤2.0) by Acid‐Treatment and Electrochemistry

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  17. Magnesium Ion Storage Properties in a Layered (NH4)2V6O16·1.5H2O Nanobelt Cathode Material Activated by Lattice Water

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  18. A Bismuth-Based Protective Layer for Magnesium Metal Anode in Noncorrosive Electrolytes

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  19. High-rate performance magnesium batteries achieved by direct growth of honeycomb-like V2O5 electrodes with rich oxygen vacancies

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  20. Interlayer‐Expanded MoS2 Containing Structural Water with Enhanced Magnesium Diffusion Kinetics and Durability

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  21. Dual redox groups enable organic cathode material with a high capacity for aqueous zinc-organic batteries

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  22. Polyaniline nanoarrays/carbon cloth as binder-free and flexible cathode for magnesium ion batteries

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  23. Lattice Expanding by Te-Substitution to Boost Electrochemical Mg Storage of Cu7.2s4 Nanotube Cathode

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  24. Low‐strain TiP2O7 with three‐dimensional ion channels as long‐life and high‐rate anode material for Mg‐ion batteries

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  25. Anionic Te-Substitution Boosting the Reversible Redox in CuS Nanosheet Cathodes for Magnesium Storage

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  27. Strategy of cation/anion co-doping for potential elevating of VS4 cathode for magnesium ion batteries

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  28. Ether–Water Hybrid Electrolyte Contributing to Excellent Mg Ion Storage in Layered Sodium Vanadate

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  30. Research advances of magnesium and magnesium alloys worldwide in 2021

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  32. Preparation of conductive Cu1.5Mn1.5O4 and Mn3O4 spinel mixture powders as positive active materials in rechargeable Mg batteries operative at room temperature

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  33. RETRACTED: Exploring the application of AlN graphyne in calcium ion batteries

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  34. Octylamine‐Supporting Interlayer Expanded Molybdenum Diselenide as a High‐Power Cathode for Rechargeable Mg Batteries

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  35. Novel Organic Cathode with Conjugated N-Heteroaromatic Structures for High-Performance Aqueous Zinc-Ion Batteries

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  36. Kinetically optimized copper sulfide cathodes for rechargeable magnesium batteries

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  38. A Molybdenum Polysulfide In-Situ Generated from Ammonium Tetrathiomolybdate for High-Capacity and High-Power Rechargeable Magnesium Battery Cathodes

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  39. Progress and perspective on rechargeable magnesium-ion batteries

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  41. Electrochemical properties and crystal and electronic structure changes during charge/discharge of spinel type cathode-materials Mg1.33V1.67-Mn O4 for magnesium secondary batteries

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  42. Vanadium-based cathode materials for rechargeable magnesium batteries

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  43. A two-dimensional VO 2 /VS 2 heterostructure as a promising cathode material for rechargeable Mg batteries: a first principles study

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  44. Hierarchical BiOCl flowerlike microspheres via a room-temperature solid-state chemical reaction as a new anode for rechargeable magnesium-ion batteries

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  45. Oxygen – a fatal impurity for reversible magnesium deposition/dissolution

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  46. A Single Mg Ion-conductive Polymer-coated MgCo2O4 for Mg Rechargeable Batteries

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  47. Cathode Electrolyte Interphase (CEI) Endows Mo 6 S 8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics

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  48. Cathode Electrolyte Interphase (CEI) Endows Mo6S8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics

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  49. Modulating vacancies concentration ratio of cationic and anionic in WO3 for driving high performance magnesium ions storage

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  50. Efficient boron-based electrolytes constructed by anionic and interfacial co-regulation for rechargeable magnesium batteries

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