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RESEARCH PAPER · Angewandte Chemie International Edition · 2020

Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 Evolution

Takayoshi Oshima, Tom Ichibha, Kenji Oqmhula, Keisuke Hibino, Hiroto Mogi, Shunsuke Yamashita, Kotaro Fujii, Yugo Miseki, Kenta Hongo, Daling Lu, Ryo Maezono, Kazuhiro Sayama, Masatomo Yashima, Koji Kimoto, Hideki Kato, Masato Kakihana, Hiroshi Kageyama, Kazuhiko Maeda

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Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 EvolutionOriginalSynthesis of Three-Layer Perovskite Oxynitride K2Ca2Ta3O9N·2H2O and Photocatalytic Activity for H2 Evolution under Visible Light35Facile synthesis of difunctional NiV LDH@ZIF-67 p-n junction: Serve as prominent photocatalyst for hydrogen evolution and supercapacitor electrode as well122Perovskite – A wonder catalyst for solar hydrogen production73Recent Progress in Mixed‐Anion Materials for Solar Fuel Production58Bifunctional black phosphorus: coupling with hematite for Z-scheme photocatalytic overall water splitting13Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers9Developing sustainable, high-performance perovskites in photocatalysis: design strategies and applications253Advances in engineering perovskite oxides for photochemical and photoelectrochemical water splitting47Computational discovery of stable and metastable ternary oxynitrides38Research on the Hydrogen Production Technology18Preparation of Multifunctional Metal Oxynitride 2D Crystals and Oriented Transparent Free-Standing Oxynitride Films22Control of the Photocatalytic Activity of Metastable Layered Oxynitride K2LaTa2O6N through Topochemical Transformation of Tuned Oxide Precursors18O/F anion order in Pb$_2$Ti$_4$O$_9$F$_2$ stabilized by the 6$s^2$ lone pair electrons of Pb$^{2+}$0Significantly Enhanced Visible‐Light H2 Evolution of Polyfluorene Polyelectrolyte by Anionic Polyelectrolyte Doping4LaTaON2 Mesoporous Single Crystals for Efficient Photocatalytic Water Oxidation and Z‑Scheme Overall Water Splitting66Recent Progress on Mixed-Anion Materials for Energy Applications110Recent advances in the fabrication of 2D metal oxides111A two-dimensional perovskite oxyfluoride Pb 3 Fe 2 O 5 F 2 as a catalyst for electrochemical oxidation of water to oxygen9Anionic ordering in Pb 2 Ti 4 O 9 F 2 revisited by nuclear magnetic resonance and density functional theory3Low Temperature Synthesis of Oxyfluoride Csti2o2.85f3.15 from a Layered Oxide Cs0.68ti1.83o41Double Perovskite LaFe1−xNixO3 Coated with Sea Urchin-like Gold Nanoparticles Using Electrophoresis as the Photoelectrochemical Electrode to Enhance H2 Production via Surface Plasmon Resonance Effect8Low temperature synthesis of oxyfluoride CsTi2O2.85F3.15 from a layered oxide Cs0.68Ti1.83O43Enhanced Metal–Semiconductor Interaction for Photocatalytic Hydrogen‐Evolution Reaction12Two-dimensional perovskite SrNbO2N with Zr doping for accelerating photoelectrochemical water splitting12Cost-effective preparation of layered tantalum oxynitrides for visible light-driven photocatalysis4Interlayer modification and single-layer exfoliation of the Ruddlesden–Popper perovskite oxynitride K 2 LaTa 2 O 6 N to improve photocatalytic H 2 evolution activity17Bandgap Tunable Oxynitride LaNb 2 O 7–x N x Nanosheets20Photocatalytic Water Splitting Using Layered Zirconium Chloride Nitride8CuS as bifunctional catalyst for enhancing photocatalytic degradation efficiency of Bi4Ti3O1211In Situ X-ray Photoelectron Spectroscopy (XPS) Demonstrated Graphdiyne (g-CnH2n–2) Based GDY-CuI/NiV-LDH Double S-Scheme Heterojunction for Efficient Photocatalytic Hydrogen Evolution27Effect of alkali-metal cations on synthesis of stoichiometric layered perovskite oxynitrides3High-Temperature Synthesis of Ferromagnetic Eu3Ta3(O,N)9 with a Triple Perovskite Structure3Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis19Designed functions of oxide/hydroxide nanosheets via elemental replacement/doping44Tuning 2D perovskite–graphene layered composite for photocatalysis13Two-dimensional nanomaterials based on rare earth elements for biomedical applications36Layered oxide precursor strategy for the synthesizing of titanium oxynitrides2Recent Advances in Redox-Based Z-Scheme Overall Water Splitting under Visible Light Irradiation16Perovskite Oxynitrides and Oxysulfides toward Photocatalytic Green Hydrogen Production: Scalability Prospects5Perovskite materials for highly efficient Photo(electro)catalytic water splitting: A mini-review22A new photocatalyst InGaZn0.3Cu0.7O4 with co-catalyst CuO to decompose tetracycline efficiently1Supra-ceramics: a molecule-driven frontier of inorganic materials45CsCl-flux synthesis of titanium oxynitride (Ti 2.85 O 4 N) for photocatalysis0Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications29Effects of Metal-Cation Doping on Photocatalytic H2 Evolution Activity of Layered Perovskite Oxynitride K2LaTa2O6N7Hybrid Perovskite Solar Cells: A Disruptive Technology for Hydrogen Production through Photocatalytic Water Splitting4Solar-driven photocatalytic and photoelectrocatalytic hydrogen evolution reaction: Advances, challenges, and future directions9Recent progress in two-dimensional materials: From emerging structures and synthesis approaches to electronic and sensing applications75Hydrazine‐Mediated Thermally Assisted Photocatalytic Ammonia Decomposition Over Layered Protonated Perovskites7Bridging Scales in Solar‐Driven Water Splitting: Pathways to System Integration26Topochemical synthesis of mesoporous TiO 2 co-doped with nitrogen and fluorine for improved photocatalytic O 2 evolution under visible light0Topochemical Synthesis and Photocatalytic Activity of Layered K 2 LaTa 2 O 6 N Using CsLaTa 2 O 7 Precursor Prepared by Flux Method0Green synthesis of EuCN S-scheme photocatalysts via Centella asiatica extract for enhanced MB photodegradation and H 2 O 2 photoproduction: DFT investigation and mechanistic insights0Engineering structural variations in oxynitrides to boost photocatalytic hydrogen evolution: current advances and future directions1Tantalum‐Based Perovskite Oxynitride Monolayers Derived From a Charge‐Balanced Nitridation Strategy for Photocatalytic Overall Water Splitting12Topotactic Nitridation Enabled Core–Shell La 4 Ti 3 (O,N) 12 @LaTiO 2 N for Efficient Photoelectrochemical Water Splitting0The Reproducibility Crisis: Shining a Light Where Photo‐Induced Process Descriptions Fall Short0

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  1. Synthesis of Three-Layer Perovskite Oxynitride K2Ca2Ta3O9N·2H2O and Photocatalytic Activity for H2 Evolution under Visible Light

    Inorganic Chemistry · 2020-07-19

    Ya Nan Tang, Kosaku Kato, Takayoshi Oshima, Hiroto Mogi, Akinobu Miyoshi, Kotaro Fujii, Kei-ichi Yanagisawa, Koji Kimoto, Akira Yamakata, Masatomo Yashima, Kazuhiko Maeda

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  2. Facile synthesis of difunctional NiV LDH@ZIF-67 p-n junction: Serve as prominent photocatalyst for hydrogen evolution and supercapacitor electrode as well

    Renewable Energy · 2020-08-19

    Guorong Wang, Yanbing Li, Lin Xu, Zhiliang Jin, Yanbin Wang

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  3. Perovskite – A wonder catalyst for solar hydrogen production

    Journal of Energy Chemistry · 2020-09-08

    Hui Bian, Deng Li, Junqing Yan, Shengzhong Frank Liu

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  4. Recent Progress in Mixed‐Anion Materials for Solar Fuel Production

    Solar RRL · 2020-10-24

    Akinobu Miyoshi, Kazuhiko Maeda

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  5. Bifunctional black phosphorus: coupling with hematite for Z-scheme photocatalytic overall water splitting

    Catalysis Science & Technology · 2020-11-12

    Ming Wang, Di Li, Yong Zhao, Hao Shen, Biyi Chen, Xiaojie Wu, Xiaolei Qiao, Weidong Shi

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  6. Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers

    Chemical Science · 2021-01-01

    Takuya Hasegawa, Naoki Yamasaki, Yusuke Asakura, Tadaharu Ueda, Shu Yin

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  7. Developing sustainable, high-performance perovskites in photocatalysis: design strategies and applications

    Chemical Society Reviews · 2021-01-01

    Haoxin Mai, Dehong Chen, Yasuhiro Tachibana, Hajime Suzuki, Ryu Abe, Rachel A. Caruso

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  8. Advances in engineering perovskite oxides for photochemical and photoelectrochemical water splitting

    Applied Physics Reviews · 2021-06-01

    Zheyan Wang, Hao Huang, Gang Li, Xiaohui Yan, Zhichao Yu, Kaiying Wang, Yucheng Wu

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  9. Computational discovery of stable and metastable ternary oxynitrides

    The Journal of Chemical Physics · 2021-06-17

    Abhishek Sharan, Stephan Lany

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  10. Research on the Hydrogen Production Technology

    IOP Conference Series Earth and Environmental Science · 2021-07-01

    Niu Jianghao

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  11. Preparation of Multifunctional Metal Oxynitride 2D Crystals and Oriented Transparent Free-Standing Oxynitride Films

    Chemistry of Materials · 2021-07-29

    Chu‐Wei Hsu, Takumi Ideta, Keisuke Awaya, Masayuki Tsushida, Tetsuya Sato, Kei-ichi Yanagisawa, Koji Kimoto, Kazuto Hatakeyama, Michio Koinuma, Shintaro Ida

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  12. Control of the Photocatalytic Activity of Metastable Layered Oxynitride K2LaTa2O6N through Topochemical Transformation of Tuned Oxide Precursors

    Chemistry of Materials · 2021-08-03

    Hiroto Mogi, Kosaku Kato, Shuhei Yasuda, Tomoki Kanazawa, Akinobu Miyoshi, Shunta Nishioka, Takayoshi Oshima, Ya Nan Tang, Toshiyuki Yokoi, Shunsuke Nozawa, Akira Yamakata, Kazuhiko Maeda

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  13. O/F anion order in Pb$_2$Ti$_4$O$_9$F$_2$ stabilized by the 6$s^2$ lone pair electrons of Pb$^{2+}$

    arXiv (Cornell University) · 2021-09-28

    Kengo Oka, Tom Ichibha, Daichi Kato, Mitsunobu Iwasaki, Naoki Noma, Kenta Hongo, Ryo Maezono, Fernando Agustín Reboredo

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  14. Significantly Enhanced Visible‐Light H2 Evolution of Polyfluorene Polyelectrolyte by Anionic Polyelectrolyte Doping

    Macromolecular Chemistry and Physics · 2021-10-05

    Yue Deng, Chao Liu Zeng, Xiaoman Yang, Zhonglin Liu, Chunhui Dai

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  15. LaTaON2 Mesoporous Single Crystals for Efficient Photocatalytic Water Oxidation and Z‑Scheme Overall Water Splitting

    ACS Nano · 2021-10-22

    Shufang Chang, Jinxing Yu, Ran Wang, Qingyang Fu, Xiaoxiang Xu

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  16. Recent Progress on Mixed-Anion Materials for Energy Applications

    Bulletin of the Chemical Society of Japan · 2021-11-15

    Kazuhiko Maeda, Fumitaka Takeiri, Genki Kobayashi, Satoru Matsuishi, Hiraku Ogino, Shintaro Ida, Takao Mori, Yoshiharu Uchimoto, Setsuhisa Tanabe, Tetsuya Hasegawa, Nobuhito Imanaka, Hiroshi Kageyama

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  17. Recent advances in the fabrication of 2D metal oxides

    iScience · 2021-12-10

    Huaguang Xie, Zhong Li, Liang Cheng, Azhar Ali Haidry, Jiaqi Tao, Yi Xu, Kai Xu, Jian Zhen Ou

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  18. A two-dimensional perovskite oxyfluoride Pb 3 Fe 2 O 5 F 2 as a catalyst for electrochemical oxidation of water to oxygen

    Sustainable Energy & Fuels · 2022-01-01

    Ryusuke Mizuochi, Kengo Oka, Yoshiyuki Inaguma, Kazuhiko Maeda

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  19. Anionic ordering in Pb 2 Ti 4 O 9 F 2 revisited by nuclear magnetic resonance and density functional theory

    Dalton Transactions · 2022-01-01

    Kengo Oka, Tom Ichibha, Daichi Kato, Yasuto Noda, Yusuke Tominaga, Kosei Yamada, Mitsunobu Iwasaki, Naoki Noma, Kenta Hongo, Ryo Maezono, Fernando Agustín Reboredo

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  20. Low Temperature Synthesis of Oxyfluoride Csti2o2.85f3.15 from a Layered Oxide Cs0.68ti1.83o4

    SSRN Electronic Journal · 2022-01-01

    Ya Nan Tang, Qinshang Xu, Yu Su, Zihan Wang, Lanlu Lu, Liang Tang

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  21. Double Perovskite LaFe1−xNixO3 Coated with Sea Urchin-like Gold Nanoparticles Using Electrophoresis as the Photoelectrochemical Electrode to Enhance H2 Production via Surface Plasmon Resonance Effect

    Nanomaterials · 2022-02-12

    Hsiang-Wei Tsai, Yen‐Hsun Su

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  22. Low temperature synthesis of oxyfluoride CsTi2O2.85F3.15 from a layered oxide Cs0.68Ti1.83O4

    Journal of Solid State Chemistry · 2022-06-30

    Qinshang Xu, Yu Su, Ya Nan Tang, Zihan Wang, Lanlu Lu, Liang Tang

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  23. Enhanced Metal–Semiconductor Interaction for Photocatalytic Hydrogen‐Evolution Reaction

    Chemistry - A European Journal · 2022-07-27

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  24. Two-dimensional perovskite SrNbO2N with Zr doping for accelerating photoelectrochemical water splitting

    Journal of Material Science and Technology · 2022-11-11

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  25. Cost-effective preparation of layered tantalum oxynitrides for visible light-driven photocatalysis

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  26. Interlayer modification and single-layer exfoliation of the Ruddlesden–Popper perovskite oxynitride K 2 LaTa 2 O 6 N to improve photocatalytic H 2 evolution activity

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  27. Bandgap Tunable Oxynitride LaNb 2 O 7–x N x Nanosheets

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  28. Photocatalytic Water Splitting Using Layered Zirconium Chloride Nitride

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  29. CuS as bifunctional catalyst for enhancing photocatalytic degradation efficiency of Bi4Ti3O12

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  30. In Situ X-ray Photoelectron Spectroscopy (XPS) Demonstrated Graphdiyne (g-CnH2n–2) Based GDY-CuI/NiV-LDH Double S-Scheme Heterojunction for Efficient Photocatalytic Hydrogen Evolution

    Energy & Fuels · 2023-03-20

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  31. Effect of alkali-metal cations on synthesis of stoichiometric layered perovskite oxynitrides

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  32. High-Temperature Synthesis of Ferromagnetic Eu3Ta3(O,N)9 with a Triple Perovskite Structure

    Inorganic Chemistry · 2023-10-12

    Jhonatan R. Guarín, Carlos Frontera, Judith Oró‐Solé, Jaume Gàzquez, C. Ritter, J. Fontcuberta, Amparo Fuertes

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  33. Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis

    Materials Chemistry Frontiers · 2023-12-05

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  34. Designed functions of oxide/hydroxide nanosheets via elemental replacement/doping

    Chemical Society Reviews · 2024-01-01

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  35. Tuning 2D perovskite–graphene layered composite for photocatalysis

    Sustainable Energy & Fuels · 2024-01-01

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  36. Two-dimensional nanomaterials based on rare earth elements for biomedical applications

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  37. Layered oxide precursor strategy for the synthesizing of titanium oxynitrides

    Journal of Solid State Chemistry · 2024-01-08

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  38. Recent Advances in Redox-Based Z-Scheme Overall Water Splitting under Visible Light Irradiation

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  39. Perovskite Oxynitrides and Oxysulfides toward Photocatalytic Green Hydrogen Production: Scalability Prospects

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  40. Perovskite materials for highly efficient Photo(electro)catalytic water splitting: A mini-review

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  41. A new photocatalyst InGaZn0.3Cu0.7O4 with co-catalyst CuO to decompose tetracycline efficiently

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  42. Supra-ceramics: a molecule-driven frontier of inorganic materials

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  43. CsCl-flux synthesis of titanium oxynitride (Ti 2.85 O 4 N) for photocatalysis

    Dalton Transactions · 2025-01-01

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  44. Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications

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  45. Effects of Metal-Cation Doping on Photocatalytic H2 Evolution Activity of Layered Perovskite Oxynitride K2LaTa2O6N

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  46. Hybrid Perovskite Solar Cells: A Disruptive Technology for Hydrogen Production through Photocatalytic Water Splitting

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  47. Solar-driven photocatalytic and photoelectrocatalytic hydrogen evolution reaction: Advances, challenges, and future directions

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  48. Recent progress in two-dimensional materials: From emerging structures and synthesis approaches to electronic and sensing applications

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  49. Hydrazine‐Mediated Thermally Assisted Photocatalytic Ammonia Decomposition Over Layered Protonated Perovskites

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  50. Bridging Scales in Solar‐Driven Water Splitting: Pathways to System Integration

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