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RESEARCH PAPER · Journal of the American Chemical Society · 2019

Modular Design via Multiple Anion Chemistry of the High Mobility van der Waals Semiconductor Bi4O4SeCl2

Quinn Gibson, Troy D. Manning, Marco Zanella, Tianqi Zhao, Philip A. E. Murgatroyd, Craig M. Robertson, Leanne A. H. Jones, Fiona McBride, Rasmita Raval, Furio Corà, Ben Slater, John B. Claridge, V.R. Dhanak, Matthew Stephen Dyer, Jonathan Alaria, Matthew J. Rosseinsky

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Modular Design via Multiple Anion Chemistry of the High Mobility van der Waals Semiconductor Bi4O4SeCl2OriginalBi2+2nO2+2nCu2−δSe2+n–δXδ (X = Cl, Br): A Three-Anion Homologous Series19M-IDAs: A Scalable and Droppable Big Data Intelligent Platform Based on Modular Design0Shift–Twin Option in Eight-Layer Hexagonal Perovskite Niobates Ba8MNb6O246Fast lithium-ion conductivity in the ‘empty-perovskite’ n = 2 Ruddlesden–Popper-type oxysulphide Y 2 Ti 2 S 2 O 514Visible-light photoelectric response in semiconducting quaternary oxysulfide FeOCuS with anti-PbO-type structure9First-Principles Hydrothermal Synthesis Design to Optimize Conditions and Increase the Yield of Quaternary Heteroanionic Oxychalcogenides28Low thermal conductivity in a modular inorganic material with bonding anisotropy and mismatch202Van Der Waals gap-rich BiOCl atomic layers realizing efficient, pure-water CO2-to-CO photocatalysis326Fabrication and enhanced photoelectric properties of a novel Bi 9 O 7.5 S 6 /CdS composite film2Oxygen vacancies induced narrow band gap of BiOCl for efficient visible-light catalytic performance from double radicals249Multiple Anion Chemistry for Ionic Layer Thickness Tailoring in Bi2+2nO2+2nSenX2 (X = Cl, Br) van der Waals Semiconductors with Low Thermal Conductivities15Expanding multiple anion superlattice chemistry: Synthesis, structure and properties of Bi4O4SeBr2 and Bi6O6Se2Cl212Facet synergy dominant Z-scheme transition in BiOCl with enhanced 1O2 generation9Band Structure Engineering of Bi4O4SeCl2 for Thermoelectric Applications20Sn4+ doping enhanced inner electric field for photocatalytic performance promotion of BiOCl based nanoflowers41Synthesis and improved photoelectrochemical performances of Bi9O7.5S6/CdS heterojunction9Enhanced photocatalytic reduction of CO2 on BiOBr under synergistic effect of Zn doping and induced oxygen vacancy generation90Configuration regulation of active sites by accurate doping inducing self-adapting defect for enhanced photocatalytic applications: A review121Low thermal conductivity in Bi 8 CsO 8 SeX 7 (X = Cl, Br) by combining different structural motifs4Preparation of a novel Bi 9 O 7.5 S 6 /SnS composite film with improved photoelectric properties3Thermoelectric Properties and Phase Alterations in Bi4o4secl2 Synthesized Via Solid-State Reaction and the Post-Ball-Milling Technique0Database Construction of Two-Dimensional Charged Building Blocks for Functional-Oriented Material Design12High-Crystallinity BiOCl Nanosheets as Efficient Photocatalysts for Norfloxacin Antibiotic Degradation28Thermoelectric Properties of n-Type Bi4O4SeX2 (X = Cl, Br)4Bi/Mn-Doped BiOCl Nanosheets Self-Assembled Microspheres toward Optimized Photocatalytic Performance19Tightly bound and room-temperature-stable excitons in van der Waals degenerate-semiconductor Bi4O4SeCl2 with high charge-carrier density5High ZT Value and Ultralow Lattice Thermal Conductivity Induced by Edge Dislocations Coupled with the Superlattice Structure in Ag-Doped BST Alloy8Glass-like Transport Dominates Ultralow Lattice Thermal Conductivity in Modular Crystalline Bi 4 O 4 SeCl 260Ultralow thermal conductivity and high thermoelectric performance induced by multiscale lattice defects in Cu-doped BST alloys10Band engineering of layered oxyhalide photocatalysts for visible-light water splitting42Data-Driven Materials Informatics for Novel Piezoelectric Janus-Type Nanomaterials Discovery4Synthesis, crystal and electronic structures of two novel tunnel bismuth oxychlorides Bi18O22Cl8.5(BO3)0.5 and Bi18O22Cl8Se2High In-Plane Thermoelectric Performance of Layered Bi4O4SeCl211Crystal facet/interface anchored Janus activity of BiOBr in driving photocatalytic water splitting27Enhanced thermoelectric properties of bismuth telluride via Ultra-Low thermal conductivity BOSC compound addition4Thermal transport properties of polycrystalline Bi4SeCl2O4 with various texturizations and densities3Tuning the band gap and structure from wide gap SrBi 3 O 4 Cl 3 to narrow gap Bi 4 O 4 SeCl 2 by aliovalent anion substitution2Post-ball-milling-assisted solid-state synthesis of Bi4O4SeCl2: A low thermal conductivity material1Layered Ordered Multianion Semiconductor Bi18O21.6Se1.8Cl7.2 with Low c-Axial Thermal Conductivity0Grain boundary‐mediated reversible insulator‐to‐semiconductor transition in layered heteroanionic Bi 4 O 4 SeCl 22Enhanced photoactivity of Sn-doped BiOI microspheres for antibiotic degradation2Chemistry and physics of layered oxychalcogenides containing an anti-cuprate type square lattice2Self‐Powered Polarization‐Sensitive Near‐Infrared Photodetection Based on 2D Bi 4 O 4 SeCl 20Unlocking Selective Electrochemical Regulation via Interlayer Anion Competition for Nitrate Extraction from Wastewater2Unlocking Selective Electrochemical Regulation via Interlayer Anion Competition for Nitrate Extraction from Wastewater2Advances in bismuth oxyhalide-based photocatalytic CO 2 reduction: from materials design to reaction mechanisms0Coupled Effects of Cation and Halogen Substitution on Electronic Structure, Phonon Transport, and Thermoelectric Performance of Layered M₄O₄SeX₂ (M = Bi, Sb; X = Cl, Br)0Growth of large crystals of Janus phase RhSeCl using self-selecting vapour growth1Structural origins of photocatalytic properties in Ruddlesden–Popper Sr n +1 Ti n O 3 n +1 ( n = 1, 2) and their topochemically fluorinated phases Sr n +1 Ti n O (3 n +1)− x F 2 x ( x ≈ n )3Te Substitution-Induced Structural Evolution and Thermoelectric Properties of Quasi-1D BiSeI0Cu 7.62 Bi 6 Se 12 Cl 6 I: Discovery of a Low Band Gap, Low Thermal Conductivity Mixed-Anion Material0Post-annealing effects on (00l) texture, Cl/Se ratio, and electrical and glass-like thermal transport in Bi₄O₄SeCl₂0Efficient photothermoelectric detection by layered Bi2 + 2 n O2 + 2 n Se n Cl2 superlattices with ultralow thermal conductivity0Bi4O4SeCl2 nanoinclusions enable heat-charge transport decoupling in Cu2Se thermoelectric composites0Enhancing Quasi‐Two‐Dimensional Electronic Structure in Bi 2 O 2 Se via Chlorine Substitution0

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  1. Bi2+2nO2+2nCu2−δSe2+n–δXδ (X = Cl, Br): A Three-Anion Homologous Series

    Inorganic Chemistry · 2018-09-26

    Quinn Gibson, Matthew Stephen Dyer, Craig M. Robertson, C. Delacotte, Troy D. Manning, Michael J. Pitcher, Matthew J. Rosseinsky, Marco Zanella, Jonathan Alaria, John B. Claridge, Matthew J. Rosseinsky

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  2. M-IDAs: A Scalable and Droppable Big Data Intelligent Platform Based on Modular Design

    International Conference on High Performance Big Data and Intelligent Systems (HPBD&IS) · 2020-05-01

    Haitian Zeng, Chao Wang, Ruili Ye, Yan Wang, Nan Yang, Yibo Xue

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  3. Shift–Twin Option in Eight-Layer Hexagonal Perovskite Niobates Ba8MNb6O24

    Inorganic Chemistry · 2020-11-02

    Congling Yin, Fengqiong Tao, Lei Zhao, Xiaoming Wang, Xing Ming, Chaoping Liang, Xiaojun Kuang

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  4. Fast lithium-ion conductivity in the ‘empty-perovskite’ n = 2 Ruddlesden–Popper-type oxysulphide Y 2 Ti 2 S 2 O 5

    Journal of Materials Chemistry A · 2021-01-01

    Kit McColl, Furio Corà

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  5. Visible-light photoelectric response in semiconducting quaternary oxysulfide FeOCuS with anti-PbO-type structure

    Chemical Communications · 2021-01-01

    Wei Du, Ganghua Zhang, Ping Chen, Pingying Tang, Jing Wang, Dezeng Li, Jingshan Hou, Yongzheng Fang

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  6. First-Principles Hydrothermal Synthesis Design to Optimize Conditions and Increase the Yield of Quaternary Heteroanionic Oxychalcogenides

    Chemistry of Materials · 2021-04-05

    Lauren N. Walters, Chi Zhang, Vinayak P. Dravid, Kenneth Reinhard Poeppelmeier, James M. Rondinelli

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  7. Low thermal conductivity in a modular inorganic material with bonding anisotropy and mismatch

    Science · 2021-07-15

    Quinn Gibson, Tianqi Zhao, Matthew J. Rosseinsky, Helen C. Walker, Ramzy Daou, S. Hébert, Marco Zanella, Matthew Stephen Dyer, John B. Claridge, Ben Slater, Michael W. Gaultois, Furio Corà, Jonathan Alaria, Matthew J. Rosseinsky

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  8. Van Der Waals gap-rich BiOCl atomic layers realizing efficient, pure-water CO2-to-CO photocatalysis

    Nature Communications · 2021-10-11

    Yanbiao Shi, Jie Li, Chengliang Mao, Song Liu, Xiaobing Wang, Xiufan Liu, Shengxi Zhao, Xiao Liu, Yanqiang Huang, Lizhi Zhang

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  9. Fabrication and enhanced photoelectric properties of a novel Bi 9 O 7.5 S 6 /CdS composite film

    Dalton Transactions · 2022-01-01

    Yongzheng Fang, Jing Wang, Zhanqiang Liu, Guoying Zhao, Yanwei Huang, Jingshan Hou, Ganghua Zhang

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  10. Oxygen vacancies induced narrow band gap of BiOCl for efficient visible-light catalytic performance from double radicals

    Journal of Material Science and Technology · 2022-01-21

    Changyan Chen, Ting Jiang, Jianhua Hou, Tingting Zhang, Geshan Zhang, Yongcai Zhang, Xiaozhi Wang

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  11. Multiple Anion Chemistry for Ionic Layer Thickness Tailoring in Bi2+2nO2+2nSenX2 (X = Cl, Br) van der Waals Semiconductors with Low Thermal Conductivities

    Chemistry of Materials · 2022-05-05

    Ruiwen Ji, Meng Lei, Cécile Genevois, Wenda Zhang, Xing Ming, Lunhua He, Mathieu M. B. Allix, Congling Yin, Xiaojun Kuang, Xianran Xing

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  12. Expanding multiple anion superlattice chemistry: Synthesis, structure and properties of Bi4O4SeBr2 and Bi6O6Se2Cl2

    Journal of Solid State Chemistry · 2022-05-19

    Quinn Gibson, Jon A. Newnham, Matthew Stephen Dyer, Craig M. Robertson, Marco Zanella, Todd Wesley Surta, Matthew J. Rosseinsky, Jonathan Alaria, John B. Claridge, Matthew J. Rosseinsky

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  13. Facet synergy dominant Z-scheme transition in BiOCl with enhanced 1O2 generation

    Chemosphere · 2022-07-11

    Chongshang Guan, Tian Hou, Wuyang Nie, Qian Zhang, Libing Duan, Xiaoru Zhao

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  14. Band Structure Engineering of Bi4O4SeCl2 for Thermoelectric Applications

    ACS Organic & Inorganic Au · 2022-07-14

    Jon A. Newnham, Tianqi Zhao, Quinn Gibson, Troy D. Manning, Marco Zanella, Elisabetta Mariani, Matthew J. Rosseinsky, Jonathan Alaria, John B. Claridge, Furio Corà, Matthew J. Rosseinsky

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  15. Sn4+ doping enhanced inner electric field for photocatalytic performance promotion of BiOCl based nanoflowers

    Applied Surface Science · 2022-08-11

    Chongshang Guan, Tian Hou, Wuyang Nie, Qian Zhang, Libing Duan, Xiaoru Zhao

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  16. Synthesis and improved photoelectrochemical performances of Bi9O7.5S6/CdS heterojunction

    Journal of Alloys and Compounds · 2022-09-30

    Jing Wang, Yongzheng Fang, Zhanqiang Liu, Wei Du, Shu Chen, Jingshan Hou, Zhongzhi Wang, Xin Qiao, Ganghua Zhang

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  17. Enhanced photocatalytic reduction of CO2 on BiOBr under synergistic effect of Zn doping and induced oxygen vacancy generation

    Journal of Colloid and Interface Science · 2022-11-23

    Chongshang Guan, Tian Hou, Wuyang Nie, Qian Zhang, Libing Duan, Xiaoru Zhao

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  18. Configuration regulation of active sites by accurate doping inducing self-adapting defect for enhanced photocatalytic applications: A review

    Coordination Chemistry Reviews · 2022-12-23

    Shuqu Zhang, Xingshen Yi, Guanghua Hu, Meixue Chen, H. F. Shen, Bing Jhang Li, Lixia Yang, Weili Dai, Jian‐Ping Zou, Shenglian Luo

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  19. Low thermal conductivity in Bi 8 CsO 8 SeX 7 (X = Cl, Br) by combining different structural motifs

    Journal of Materials Chemistry A · 2023-01-01

    Jon A. Newnham, Quinn Gibson, Todd Wesley Surta, Alexandra Morscher, Troy D. Manning, Matthew J. Rosseinsky, John B. Claridge, Matthew J. Rosseinsky

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  20. Preparation of a novel Bi 9 O 7.5 S 6 /SnS composite film with improved photoelectric properties

    Dalton Transactions · 2023-01-01

    Tianhong Luo, Jing Wang, Zhanqiang Liu, Shu Chen, Jingshan Hou, Yongzheng Fang, Yanwei Huang, Ganghua Zhang

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  21. Thermoelectric Properties and Phase Alterations in Bi4o4secl2 Synthesized Via Solid-State Reaction and the Post-Ball-Milling Technique

    SSRN Electronic Journal · 2023-01-01

    Nattharika Theekhasuk, Nuttakrit Somdock, Athorn Vora–ud, Aparporn Sakulkalavek, Rachsak Sakdanuphab, Pichet Limsuwan

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  22. Database Construction of Two-Dimensional Charged Building Blocks for Functional-Oriented Material Design

    Nano Letters · 2023-05-05

    Jun Deng, Jinbo Pan, Yanfang Zhang, Shixuan Du

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  23. High-Crystallinity BiOCl Nanosheets as Efficient Photocatalysts for Norfloxacin Antibiotic Degradation

    Nanomaterials · 2023-06-12

    Dongxue Song, Mingxia Li, Lijun Liao, Liping Guo, Haixia Liu, Bo Wang, Zhenzi Li

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  24. Thermoelectric Properties of n-Type Bi4O4SeX2 (X = Cl, Br)

    Materials · 2023-06-12

    Tao Wang, Wanghua Hu, Zhefeng Lou, Zhuokai Xu, Xiaohui Yang, Tian Le, Jialu Wang, Xiao Lin

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  25. Bi/Mn-Doped BiOCl Nanosheets Self-Assembled Microspheres toward Optimized Photocatalytic Performance

    Nanomaterials · 2023-08-25

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  26. Tightly bound and room-temperature-stable excitons in van der Waals degenerate-semiconductor Bi4O4SeCl2 with high charge-carrier density

    Communications Materials · 2023-09-04

    Yueshan Xu, Junjie Wang, Bo Su, Jun Deng, Cao Peng, Chunlong Wu, Qinghua Zhang, Lin Gu, Jianlin Luo, Nan Xu, Jiangang Guo, Zhiguo Chen

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  27. High ZT Value and Ultralow Lattice Thermal Conductivity Induced by Edge Dislocations Coupled with the Superlattice Structure in Ag-Doped BST Alloy

    Crystal Growth & Design · 2023-10-04

    Yaohui Liu, Yu Tang, Yonggui Tao, Ying Zhang, Lanxian Shen, Wen Ge, Shukang Deng

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  28. Glass-like Transport Dominates Ultralow Lattice Thermal Conductivity in Modular Crystalline Bi 4 O 4 SeCl 2

    Nano Letters · 2023-10-13

    Zhen Tong, Alessandro Pecchia, ChiYung Yam, Traian Dumitrică, Thomas Frauenheim

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  29. Ultralow thermal conductivity and high thermoelectric performance induced by multiscale lattice defects in Cu-doped BST alloys

    CrystEngComm · 2023-12-01

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  30. Band engineering of layered oxyhalide photocatalysts for visible-light water splitting

    Chemical Science · 2024-01-01

    Daichi Kato, Hajime Suzuki, Ryu Abe, Hiroshi Kageyama

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  31. Data-Driven Materials Informatics for Novel Piezoelectric Janus-Type Nanomaterials Discovery

    The Journal of Physical Chemistry Letters · 2024-06-13

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  32. Synthesis, crystal and electronic structures of two novel tunnel bismuth oxychlorides Bi18O22Cl8.5(BO3)0.5 and Bi18O22Cl8Se

    Journal of Solid State Chemistry · 2024-07-06

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  33. High In-Plane Thermoelectric Performance of Layered Bi4O4SeCl2

    ACS Applied Materials & Interfaces · 2024-07-16

    Wenyan Jiao, Shihao Han, Hongmei Yuan, Wen Lei, Huijun Liu

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  34. Crystal facet/interface anchored Janus activity of BiOBr in driving photocatalytic water splitting

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  35. Enhanced thermoelectric properties of bismuth telluride via Ultra-Low thermal conductivity BOSC compound addition

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  36. Thermal transport properties of polycrystalline Bi4SeCl2O4 with various texturizations and densities

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    Linjie Wu, Xinyue Zhang, Changyuan Li, Qingyu Bai, Zhiwei Chen, Yanzhong Pei

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  37. Tuning the band gap and structure from wide gap SrBi 3 O 4 Cl 3 to narrow gap Bi 4 O 4 SeCl 2 by aliovalent anion substitution

    Journal of Materials Chemistry C · 2025-01-01

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  38. Post-ball-milling-assisted solid-state synthesis of Bi4O4SeCl2: A low thermal conductivity material

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  39. Layered Ordered Multianion Semiconductor Bi18O21.6Se1.8Cl7.2 with Low c-Axial Thermal Conductivity

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  40. Grain boundary‐mediated reversible insulator‐to‐semiconductor transition in layered heteroanionic Bi 4 O 4 SeCl 2

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  41. Enhanced photoactivity of Sn-doped BiOI microspheres for antibiotic degradation

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  42. Chemistry and physics of layered oxychalcogenides containing an anti-cuprate type square lattice

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  43. Self‐Powered Polarization‐Sensitive Near‐Infrared Photodetection Based on 2D Bi 4 O 4 SeCl 2

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  45. Unlocking Selective Electrochemical Regulation via Interlayer Anion Competition for Nitrate Extraction from Wastewater

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  46. Advances in bismuth oxyhalide-based photocatalytic CO 2 reduction: from materials design to reaction mechanisms

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  47. Coupled Effects of Cation and Halogen Substitution on Electronic Structure, Phonon Transport, and Thermoelectric Performance of Layered M₄O₄SeX₂ (M = Bi, Sb; X = Cl, Br)

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  48. Growth of large crystals of Janus phase RhSeCl using self-selecting vapour growth

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  49. Structural origins of photocatalytic properties in Ruddlesden–Popper Sr n +1 Ti n O 3 n +1 ( n = 1, 2) and their topochemically fluorinated phases Sr n +1 Ti n O (3 n +1)− x F 2 x ( x ≈ n )

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  50. Te Substitution-Induced Structural Evolution and Thermoelectric Properties of Quasi-1D BiSeI

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