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RESEARCH PAPER · Journal of Power Sources · 2019

Exsolution and electrochemistry in perovskite solid oxide fuel cell anodes: Role of stoichiometry in Sr(Ti,Fe,Ni)O3

Tenglong Zhu, Horacio Esteban Troiani, Liliana Mogni, Mariano Santaya, Minfang Han, Scott Alexander Barnett

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Exsolution and electrochemistry in perovskite solid oxide fuel cell anodes: Role of stoichiometry in Sr(Ti,Fe,Ni)O3OriginalStudy of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part B: Conditions of Ni exsolution28Cobalt and Titanium substituted SrFeO3 based perovskite as efficient symmetrical electrode for solid oxide fuel cell34Progress and Opportunities for Exsolution in Electrochemistry26Review on exsolution and its driving forces in perovskites138Exceptional Tunability over Size and Density of Spontaneously Formed Nanoparticles via Nucleation Dynamics38In Situ Exsolved Metal Nanoparticles: A Smart Approach for Optimization of Catalysts163Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part C: Electrical and electrochemical behavior8In-situ Ni exsolution from NiTiO3 as potential anode for solid oxide fuel cells14Exsolution of Ni nanoparticles on the surface of cerium and nickel co-doped lanthanum strontium titanate as a new anodic layer for DIR-SOFC. Anti-coking potential and H2S poisoning resistance of the prepared material18A highly active and carbon-tolerant anode decorated with in situ grown cobalt nano-catalyst for intermediate-temperature solid oxide fuel cells88Ternary Ni–Co–Fe Exsolved Nanoparticles/Perovskite System for Energy Applications: Nanostructure Characterization and Electrochemical Activity23Sr(Ti,Fe)O 3− δ Based Intermediate Temperature Solid Oxide Fuel Cell Anode with Self-precipitated (Ni,Fe) and Gd 0.1 Ce 0.9 O 2− δ Nano Particles2Metal Exsolution to Enhance the Catalytic Activity of Electrodes in Solid Oxide Fuel Cells55Stability and activity controls of Cu nanoparticles for high-performance solid oxide fuel cells66Defective Sr 0.9 Mo 0.9 O 3−δ perovskites with exsolved Ni nanoparticles as high-performance composite anodes for solid-oxide fuel cells9Excellent kinetics of single-phase Gd-doped ceria fuel electrodes in solid oxide cells60Coupling decreased polarization resistance Sr0.95Ti0.3Fe0.6Ni0.1O3-δ cathode with efficient metal supported Solid Oxide Fuel Cell31Progress of Exsolved Metal Nanoparticles on Oxides as High Performance (Electro)Catalysts for the Conversion of Small Molecules120Exsolution of Embedded Nanoparticles in Defect Engineered Perovskite Layers54Nanoparticle exsolution in perovskite oxide and its sustainable electrochemical energy systems43Emergence and Future of Exsolved Materials214Improvement of Ni-Cermet performance of protonic ceramic fuel cells by catalyst11A New in-situ Exsolution Supporting Framework for Metal Nanoparticle Growth0(La,Sr)(Ti,Fe)O 3− δ perovskite with in‐situ constructed FeNi 3 nanoparticles as fuel electrode for reversible solid oxide cell17Exploring point defects and trap states in undoped SrTiO3 single crystals26Plasma Driven Exsolution for Nanoscale Functionalization of Perovskite Oxides50Performance modulation through selective, homogenous surface doping of lanthanum strontium ferrite electrodes revealed by in situ PLD impedance measurements9Co-improving the electrocatalytic performance and H 2 S tolerance of a Sr 2 Fe 1.5 Mo 0.5 O 6− δ based anode for solid oxide fuel cells23Tracking the nanoparticle exsolution/reoxidation processes of Ni-doped SrTi 0.3 Fe 0.7 O 3− δ electrodes for intermediate temperature symmetric solid oxide fuel cells47A Robust Approach to In Situ Exsolve Highly Dispersed and Stable Electrocatalysts3The metal/oxide heterointerface delivered by solid-based exsolution strategy: A review53Effect of nickel addition on the physicochemical properties of SrTiO3-based materials7Comparative study on the electrochemical performance of Sr(Ti0.3Fe0.7)O3-δ fuel electrode in different fuel gases for solid oxide electrochemical cells11Rapid Plasma Exsolution from an A‐site Deficient Perovskite Oxide at Room Temperature57Metal exsolution engineering on perovskites for electrocatalysis: a perspective35La0.3Sr0.7Ti0.3Fe0.7O3-δ-Based Electrodes for Symmetrical Solid Oxide Fuel Cells by A-Site Deficiency Manipulation25Exsolved catalyst particles as a plaything of atmosphere and electrochemistry11Recent advances in exsolved perovskite oxide construction: exsolution theory, modulation, challenges, and prospects86Surface reconstruction of defective SrTi0.7Cu0.2Mo0.1O3-δ perovskite oxide induced by in-situ copper nanoparticle exsolution for high-performance direct CO2 electrolysis18Electrocatalytic Oxidative Coupling of Methane on NiFe Exsolved Perovskite Anode: Effect of Water11Emerging Exsolution Materials for Diverse Energy Applications: Design, Mechanism, and Future Prospects45An active and stable hydrogen electrode of solid oxide cells with exsolved Fe–Co–Ni nanoparticles from Sr2FeCo0.2Ni0.2Mo0.6O6-δ double-perovskite34Roadmap on exsolution for energy applications71Impact of strontium non-stoichiometry of SrxTi0.3Fe0.7O3-δ on structural, electrical, and electrochemical properties for potential oxygen electrode of intermediate temperature solid oxide cells9Exsolution versus particle segregation on (Ni,Co)-doped and undoped SrTi0.3Fe0.7O3-δ perovskites: Differences and influence of the reduction path on the final system nanostructure19Enhanced CO 2 Electrolysis Through Mn Substitution Coupled with Ni Exsolution in Lanthanum Calcium Titanate Electrodes31Development of Promising Flower-like Ag/SrFeO3 Nanosheet Electrode Materials: An Efficient and Selective Electrocatalytic Detection of Caffeic Acid in Coffee and Green Tea12Cu and Co-modified SrTiO3 as materials for environmental applications17Nanoparticle Exsolution on Perovskite Oxides: Insights into Mechanism, Characteristics and Novel Strategies102Nanotechnologies in ceramic electrochemical cells84Construction of high performance fuel electrode in solid oxide electrolysis cells by tuning the surface oxygen defect to promote electrochemical reduction of CO215Electrochemical Oxidative Coupling of Methane: Deciphering the Exceptional Properties of BaMg0.33Nb0.67–xFexO3−δ for Enhanced Electrocatalysis and Durable Operation2Advances in Advanced In Situ Assembled Composite Electrode Materials for Enhanced Solid Oxide Cell Performance33A Single Model for the Thermodynamics and Kinetics of Metal Exsolution from Perovskite Oxides46The effects of nano-socketed metal particles over perovskite surfaces on the electrochemical synthesis of high-value fuels13Transport properties and phase stability of Ni-doped Pr0.6Ba0.4FeO3–δ as potential symmetrical electrodes for proton-conducting electrochemical cells16Different enhancement of Ni doping on La0.3Sr0.7Fe0.9Ti0.1O3-δ electrodes in symmetrical solid oxide cell1Unravelling cobalt incorporation in Ca- and Sr-rich perovskites: How symmetry shapes the phases3Aspects of Fe-Incorporation into CaTiO3-SrTiO3 Perovskites and Their Catalytic Application for Ammonia SCO/SCR12Mapping phase instability to electrochemical degradation in SrTi 1− x Fe x O 3− δ under solid oxide cell fuel-electrode conditions4UHV-based analytics with electrochemical oxygen activity control3Dual doping synergy: Optimizing SrMoO3 perovskite anodes via in-situ Ni exsolution and Cr doping for enhanced SOFC efficiency13A Review of Nanofiber Electrodes and the In Situ Exsolution of Nanoparticles for Solid Oxide Cells6In‐Situ Exsolved Metal Nanoparticles for Solid Oxide Fuel Cell Anode: Mechanism, Design Strategies and Application9Stability and Exsolution of Sr0.98Ti0.7Fe0.25Ni0.05O3 for the Oxygen Evolution Reaction in an Alkaline Environment8Exsolution‐enhanced performance for energy conversion and storage5Synthesis of SrTiO3 perovskite structure for batteries, supercapacitors and fuel cells applications: a review9Optimization of Ni–Fe exsolution in Sr0.93(Ti0.3Fe0.63Ni )O3−δ electrodes: Influence of reduction temperature on hydrogen oxidation reaction kinetics1Perovskite oxide exsolution process and structure regulation strategy: a review2Defects in metal exsolution catalysts: a double-edged role in nanoparticle activity and stability1Highly selective conversion of CO2 to C2–C4 olefins over the bifunctional K/BayFeO33Energy related application of metal oxide-supported metal nanoparticles0A-site deficiency synergistic in situ Fe-Sn alloy exsolution to optimize solid oxide electrolytic cell performance1A novel method for rapidly functionalizing perovskite oxides3In Situ Characterization of Strontium Titanium Ferrite Perovskites for Application as Electrodes of Solid Oxide Cells1Entropy-Assisted B-Site Compositional Engineering in Ruddlesden–Popper La 1.2 Sr 0.8 NiO 4±δ Electrode for Highly Reversible Solid Oxide Cells1Electrode surface engineering for proton-conducting ceramic cells: Advances and perspectives1Impact of La Substitution on SrTi 1-x Fe x O 3- δ Solid Oxide Cell Fuel Electrode Phase Stability and Performance1Comprehensive review of current trends and future directions of metal-supported solid oxide fuel cell: From materials to applications0Multi-effect synergistic design of high-performance Sr0.9Ce0.1Ti0.3Fe0.6Ni0.1O3-δ anode for SOFCs: In situ exsolution and electronic structure modulation0Indium dual role in tuning ionic transport, vacancy ordering, and phase stability in SrFe1–xInxO3–δ: A concentration-dependent effect0Enhancing the performance and stability of perovskite anodes through the interplay of Ni-Fe alloy exsolution and structural reconstruction for SOFCs0

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  1. Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part B: Conditions of Ni exsolution

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  2. Cobalt and Titanium substituted SrFeO3 based perovskite as efficient symmetrical electrode for solid oxide fuel cell

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  3. Progress and Opportunities for Exsolution in Electrochemistry

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  4. Review on exsolution and its driving forces in perovskites

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  5. Exceptional Tunability over Size and Density of Spontaneously Formed Nanoparticles via Nucleation Dynamics

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  6. In Situ Exsolved Metal Nanoparticles: A Smart Approach for Optimization of Catalysts

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  7. Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part C: Electrical and electrochemical behavior

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  8. In-situ Ni exsolution from NiTiO3 as potential anode for solid oxide fuel cells

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  9. Exsolution of Ni nanoparticles on the surface of cerium and nickel co-doped lanthanum strontium titanate as a new anodic layer for DIR-SOFC. Anti-coking potential and H2S poisoning resistance of the prepared material

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  11. Ternary Ni–Co–Fe Exsolved Nanoparticles/Perovskite System for Energy Applications: Nanostructure Characterization and Electrochemical Activity

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  13. Metal Exsolution to Enhance the Catalytic Activity of Electrodes in Solid Oxide Fuel Cells

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  17. Coupling decreased polarization resistance Sr0.95Ti0.3Fe0.6Ni0.1O3-δ cathode with efficient metal supported Solid Oxide Fuel Cell

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  18. Progress of Exsolved Metal Nanoparticles on Oxides as High Performance (Electro)Catalysts for the Conversion of Small Molecules

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  19. Exsolution of Embedded Nanoparticles in Defect Engineered Perovskite Layers

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  22. Improvement of Ni-Cermet performance of protonic ceramic fuel cells by catalyst

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  23. A New in-situ Exsolution Supporting Framework for Metal Nanoparticle Growth

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  32. Effect of nickel addition on the physicochemical properties of SrTiO3-based materials

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  33. Comparative study on the electrochemical performance of Sr(Ti0.3Fe0.7)O3-δ fuel electrode in different fuel gases for solid oxide electrochemical cells

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  44. Impact of strontium non-stoichiometry of SrxTi0.3Fe0.7O3-δ on structural, electrical, and electrochemical properties for potential oxygen electrode of intermediate temperature solid oxide cells

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  45. Exsolution versus particle segregation on (Ni,Co)-doped and undoped SrTi0.3Fe0.7O3-δ perovskites: Differences and influence of the reduction path on the final system nanostructure

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  46. Enhanced CO 2 Electrolysis Through Mn Substitution Coupled with Ni Exsolution in Lanthanum Calcium Titanate Electrodes

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  48. Cu and Co-modified SrTiO3 as materials for environmental applications

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  49. Nanoparticle Exsolution on Perovskite Oxides: Insights into Mechanism, Characteristics and Novel Strategies

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  50. Nanotechnologies in ceramic electrochemical cells

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