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RESEARCH PAPER · Chemistry of Materials · 2019

Band Engineering of Double-Layered Sillén–Aurivillius Perovskite Oxychlorides for Visible-Light-Driven Water Splitting

Akinobu Nakada, Masanobu Higashi, Takuma Kimura, Hajime Suzuki, Daichi Kato, Hiroyuki Okajima, Takafumi Yamamoto, Akinori Saeki, Hiroshi Kageyama, Ryu Abe

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Band Engineering of Double-Layered Sillén–Aurivillius Perovskite Oxychlorides for Visible-Light-Driven Water SplittingOriginalPhotoelectrochemical CO2 Reduction to Formate with the Sacrificial Reagent Free System of Semiconductor Photocatalysts and Formate Dehydrogenase27Two bismuth niobates containing Bi2O2 segments0Light Absorption Properties and Electronic Band Structures of Lead‐Vanadium Oxyhalide Apatites Pb5(VO4)3X (X=F, Cl, Br, I)12Triple-layered Sillén–Aurivillius Perovskite Oxychloride Bi5PbTi3O14Cl as a Visible-light-responsive Photocatalyst for Water Splitting152D/2D p‐n Heterojunctions of CaSb2O6/g‐C3N4 for Visible Light‐Driven Photocatalytic Degradation of Tetracycline17Exploring the thickness dependent photocatalytic oxygen evolution performance for Bi4TaO8Cl two-dimensional semiconductor15Recent Progress in Mixed‐Anion Materials for Solar Fuel Production58A Stable Polyoxometalate-Based Metal–Organic Framework with Active CoMoO4 Layers for Electroreduction and Visible-Light-Driven Water Oxidation16Photocatalytic Oxygen Evolution from Water Splitting255Visible-Light-Responsive Oxyhalide PbBiO2Cl Photoelectrode: On-Site Flux Synthesis on a Fluorine-Doped Tin Oxide Electrode5A new lead-free Sillén–Aurivillius oxychloride Bi5SrTi3O14Cl with triple-perovskite layers for photocatalytic water splitting under visible light19Progress and Perspectives on Aurivillius-Type Layered Ferroelectric Oxides in Binary Bi4Ti3O12-BiFeO3 System for Multifunctional Applications70Developing sustainable, high-performance perovskites in photocatalysis: design strategies and applications253Synthesis, band structure and photocatalytic properties of Sillén–Aurivillius oxychlorides BaBi 5 Ti 3 O 14 Cl, Ba 2 Bi 5 Ti 4 O 17 Cl and Ba 3 Bi 5 Ti 5 O 20 Cl with triple-, quadruple- and quintuple-perovskite layers43Conduction Band Control of Oxyhalides with a Triple-Fluorite Layer for Visible Light Photocatalysis109Atomic‐Level Charge Separation Strategies in Semiconductor‐Based Photocatalysts50450 Years of Materials Research for Photocatalytic Water Splitting87Advances in engineering perovskite oxides for photochemical and photoelectrochemical water splitting47Photoelectrochemical biosensor for DNA hydroxymethylation detection based on the enhanced photoactivity of in-situ synthesized Bi4NbO8Cl@Bi2S3 heterojunction53Bi4AO6Cl2 (A = Ba, Sr, Ca) with Double and Triple Fluorite Layers for Visible-Light Water Splitting17Photocatalytic Z‐Scheme Overall Water Splitting: Recent Advances in Theory and Experiments291Liberating photocarriers in mesoporous single-crystalline SrTaO2N for efficient solar water splitting38PbBi3O4X3 (X = Cl, Br) with Single/Double Halogen Layers as a Photocatalyst for Visible-Light-Driven Water Splitting: Impact of a Halogen Layer on the Band Structure and Stability24Crystal and Band Engineering in Photocatalytic Materials0Improved water oxidation activity of a Sillén SrBi 3 O 4 Cl 3 photocatalyst by flux method with an appropriate binary-component molten salt11Manipulation of charge carrier flow in Bi 4 NbO 8 Cl nanoplate photocatalyst with metal loading40pH-regulated hydrothermal synthesis and characterization of Sb 4 O 5 X 2 (X = Br/Cl) and its use for the dye degradation of methyl orange both with and without light illumination25Photoexcited charge manipulation in conjugated polymers bearing a Ru( ii ) complex catalyst for visible-light CO 2 reduction14Structural stability, electronic, optical, and thermoelectric properties of layered perovskite Bi 2 LaO 4 I72D Inorganic Nanosheet-based Hybrid Photocatalysts for Water Splitting0Mesoporous single-crystalline SrNbO2N: Expediting charge transportation to advance solar water splitting35Multi anion-based materials: Synthesis and catalytic applications30Layered bismuth-based photocatalysts297Lone-Pair-Induced Intra- and Interlayer Polarizations in Sillén-Aurivillius Layered Perovskite Bi4NbO8Br23Bi12O17Cl2 with a Sextuple BiO Layer Composed of Rock‐Salt and Fluorite Units and its Structural Conversion through Fluorination to Enhance Photocatalytic Activity31Bi-based layered perovskite oxyhalides: Up-and-coming catalysts for efficient energy harvesting and conversion18Sustainable Production of Layered Bismuth Oxyhalides for Photocatalytic H 2 Production26Flux-assisted synthesis of tungsten-doped layered perovskite oxychloride with promoted visible-light-responsive O 2 evolution performance7Perovskites in photoelectrochemical water splitting0Single-Crystalline Bi2YO4Cl with Facet-Aided Photocarrier Separation for Robust Solar Water Splitting27Band shifting triggered ·OH evolution and charge separation enhanced H2O2 generation in piezo-photocatalysis of Silleń-Aurivillius-structured Bi4W0.5Ti0.5O8Cl81Molten Salts‐Driven Discovery of a Polar Mixed‐Anion 3D Framework at the Nanoscale: Zn4Si2O7Cl2, Charge Transport and Photoelectrocatalytic Water Splitting1Molten Salts‐Driven Discovery of a Polar Mixed‐Anion 3D Framework at the Nanoscale: Zn4Si2O7Cl2, Charge Transport and Photoelectrocatalytic Water Splitting0Synthesis and Structure of the Double-Layered Sillén–Aurivillius Perovskite Oxychloride La2.1Bi2.9Ti2O11Cl as a Potential Photocatalyst for Stable Visible Light Solar Water Splitting19Synthesis of multi-layered perovskite oxyiodides: Impact of number of perovskite layers and type of halide layer for band levels and photocatalytic properties14Orbital Engineering in Sillén–Aurivillius Phase Bismuth Oxyiodide Photocatalysts through Interlayer Interactions37Accurate design of spatially separated double active site in Bi4NbO8Cl single crystal to promote Z - Scheme photocatalytic overall water splitting40Combined Analyses on Electronic Structure and Molecular Orbitals of d10 Bimetal Oxide In2Ge2O7 and Photocatalytic Performances for Overall Water Splitting and CO2 Reduction8Artificial Photosynthesis for H2 Generation and CO2 Conversion0Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis19Band engineering of layered oxyhalide photocatalysts for visible-light water splitting42Layered 2D material heterostructures – a colloidal perspective23Nanoscale engineering of semiconductor photocatalysts boosting charge separation for solar-driven H 2 production: Recent advances and future perspective10Recent Advances in Redox-Based Z-Scheme Overall Water Splitting under Visible Light Irradiation16Manufacturing porous BaTaO2N nanosheet via nitridation of a novel oxyhalide precursor for boosted photocatalytic water oxidation reaction5Perovskite Oxynitrides and Oxysulfides toward Photocatalytic Green Hydrogen Production: Scalability Prospects5Double-Layered Sillen–Aurivillius Perovskite Oxybromide Sr2Bi3Nb2O11Br as a Fatigue-Free Piezocatalyst with Ultrahigh Hydrogen Evolution Performance12Constructing 2D bismuth-based heterostructure for highly efficient photocatalytic CO2 reduction20Synthetically Enforced Cation Migration in Sillén–Aurivillius Hybrid Perovskites Boosts Photocatalytic Hydrogen Evolution4Electrostatic Control of Electronic Structure in Modular Inorganic Crystals8Conduction Band and Defect Engineering for the Prominent Visible‐Light Responsive Photocatalysts10Conduction Band and Defect Engineering for the Prominent Visible‐Light Responsive Photocatalysts0Emergence of Tetragonal Phase and Reentrant Transition in Tensile-Strained Bi2(La1–xBix)O4Cl Solid Solution5Interfacial heterophase BaTa 2 O 6 :N with spatial CoO x /Pt cocatalysts for stable water oxidation in pH-unadjusted Fe 3+ redox media toward solar energy storage1Strong impacts of inter-π-chain charge transfer accelerating CO 2 reduction photocatalysis of carbazole–diimine-based linear conjugated polymer/Ru complex hybrids3Engineering (001) crystallinity for efficient photocatalytic water splitting in strontium-rich A3X1 Type-Bi4Sr2Ti2NbO14Cl perovskites0Enhanced Photocatalytic O2 Evolution over Layered Perovskite Oxyiodide Ba2Bi3Nb2O11I through Flux Synthesis and Surface Modifications7Emerging Mixed-Anion Semiconductors for Particulate Photocatalytic Water Splitting: Remarkable Structures and Innovative Fabrication Methods7From micro to subnano scale: Insights into the dielectric properties of BiOI nanoplates1Functional Materials for Water Splitting0Synergistic Effect of Ultrasonication-Induced Surface Activation and A-Site Sr/Ba Distribution Unlocks Cocatalyst-Free Hydrogen Evolution in Sillén–Aurivillius Photocatalysts0Interfacial defective engineering boosted charge transfer over armored Bi4NbO8Cl@C plate-like heterostructures for photocatalytic acidic Cr(VI) removal0Synergistic One-Dimensional Conductive Pathways and Local Polarization Fields for Intrinsic Bulk Charge Separation in Nonpolar Oxide Photocatalysts0Suppressing Second-Order Jahn–Teller Distortion of Bi3+ by Smaller Y3+-Substitution in Bi3O4Cl0

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  2. Two bismuth niobates containing Bi2O2 segments

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  3. Light Absorption Properties and Electronic Band Structures of Lead‐Vanadium Oxyhalide Apatites Pb5(VO4)3X (X=F, Cl, Br, I)

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  4. Triple-layered Sillén–Aurivillius Perovskite Oxychloride Bi5PbTi3O14Cl as a Visible-light-responsive Photocatalyst for Water Splitting

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  5. 2D/2D p‐n Heterojunctions of CaSb2O6/g‐C3N4 for Visible Light‐Driven Photocatalytic Degradation of Tetracycline

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  6. Exploring the thickness dependent photocatalytic oxygen evolution performance for Bi4TaO8Cl two-dimensional semiconductor

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  7. Recent Progress in Mixed‐Anion Materials for Solar Fuel Production

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  8. A Stable Polyoxometalate-Based Metal–Organic Framework with Active CoMoO4 Layers for Electroreduction and Visible-Light-Driven Water Oxidation

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  15. Conduction Band Control of Oxyhalides with a Triple-Fluorite Layer for Visible Light Photocatalysis

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  17. 50 Years of Materials Research for Photocatalytic Water Splitting

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  18. Advances in engineering perovskite oxides for photochemical and photoelectrochemical water splitting

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  19. Photoelectrochemical biosensor for DNA hydroxymethylation detection based on the enhanced photoactivity of in-situ synthesized Bi4NbO8Cl@Bi2S3 heterojunction

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  41. Band shifting triggered ·OH evolution and charge separation enhanced H2O2 generation in piezo-photocatalysis of Silleń-Aurivillius-structured Bi4W0.5Ti0.5O8Cl

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  44. Synthesis and Structure of the Double-Layered Sillén–Aurivillius Perovskite Oxychloride La2.1Bi2.9Ti2O11Cl as a Potential Photocatalyst for Stable Visible Light Solar Water Splitting

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  47. Accurate design of spatially separated double active site in Bi4NbO8Cl single crystal to promote Z - Scheme photocatalytic overall water splitting

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  48. Combined Analyses on Electronic Structure and Molecular Orbitals of d10 Bimetal Oxide In2Ge2O7 and Photocatalytic Performances for Overall Water Splitting and CO2 Reduction

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  49. Artificial Photosynthesis for H2 Generation and CO2 Conversion

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  50. Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis

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