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RESEARCH PAPER · Angewandte Chemie International Edition · 2018

High‐Pressure Synthesis of A 2 NiO 2 Ag 2 Se 2 (A=Sr, Ba) with a High‐Spin Ni 2+ in Square‐Planar Coordination

Yuki Matsumoto, Takafumi Yamamoto, Kousuke Nakano, Hiroshi Takatsu, Taito Murakami, Kenta Hongo, Ryo Maezono, Hiraku Ogino, Dongjoon Song, Craig M. Brown, Cédric Tassel, Hiroshi Kageyama

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High‐Pressure Synthesis of A 2 NiO 2 Ag 2 Se 2 (A=Sr, Ba) with a High‐Spin Ni 2+ in Square‐Planar CoordinationOriginalSynthesis and Magnetism of Extended Solids Containing Transition-Metal Cations in Square-Planar, MO4 Coordination Sites18Manipulating metal spin states for biomimetic, catalytic and molecular materials chemistry41Structure of the water-splitting photocatalyst oxysulfide α-LaOInS 2 and ab initio prediction of new polymorphs28High-pressure Synthesis of Ba2CoO2Ag2Te2 with Extended CoO2 Planes16Magnetic and electronic properties of layered Sr2NiO2Cl2 with square planar coordination5Proposed ordering of textured spin singlets in a bulk infinite-layer nickelate14Computational Discovery of Stable Heteroanionic Oxychalcogenides ABXO (A, B = Metals; X = S, Se, and Te) and Their Potential Applications41The dawn of the nickel age of superconductivity50Electronic structure and magnetism in infinite-layer nickelates RNiO2 ( R=La−Lu )59Designing new polar materials1Low Valence Nickelates: Launching the Nickel Age of Superconductivity32Magnetism of competing high-spin/low-spin states in Ba2NiO2(AgSe)2 and related two-orbital two-electron systems4Superconductivity in infinite-layer nickelates130A d 8 anti-Hund’s singlet insulator in an infinite-layer nickelate1High-Pressure Synthesis and Order–Disorder Transition of Layered Oxytelluride Ba2ZnO2Ag2Te29Field-induced Bose-Einstein condensation and supersolid in the two-dimensional Kondo necklace7Magnetic structure of oxygen-deficient perovskite nickelates with ordered vacancies17Coherent approach to two-dimensional heterolayered oxychalcogenides using molten hydroxides21Mixed anion materials0High- versus Low-Spin Ni2+ in Elongated Octahedral Environments: Sr2NiO2Cu2Se2, Sr2NiO2Cu2S2, and Sr2NiO2Cu2(Se1–xSx)212High pressure chemistry1Thermoelectric properties of layered oxyselenides with 3d transition metal ions15Comprehensive review on multiple mixed-anion ligands, physicochemical performances and application prospects in metal oxysulfides32Infinite-layer nickelates as Ni-eg Hund’s metals39Magnetic ordering in the layered oxyhalide Sr2NiO2Cl23Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Observation and enhancement through alkali metal doping of p-type conductivity in the layered oxyselenides Sr 2 ZnO 2 Cu 2 Se 2 and Ba 2 Zn 1− x O 2− x Cu 2 Se 24Decompression-Induced In-Plane Lone Pair Electrons in BiSF Synthesized under High Pressure7High-pressure X-ray study of NbON oxynitride: direct transition from baddeleyite to cotunnite structure0Novel Co2+ and Cd2+ Complexes Derived From a New N‐Donor Pyridyl‐Functionalized Thiophosphoric Triamide Ligand: Structural Investigation, DNA/COVID‐19/Monkeypox Molecular Docking, and Biological Assays6Emergence of Tetragonal Phase and Reentrant Transition in Tensile-Strained Bi2(La1–xBix)O4Cl Solid Solution5Structural stability and polymorphic transitions in LnSI (Ln = lanthanides)2A comprehensive theoretical study of structural and electronic features in LaOInS 2 polymorphs for photocatalytic applications0Superconductivity in the spin-state crossover materials: Nickelates with planar-coordinated low-spin Ni 2 + ions1Chemistry and physics of layered oxychalcogenides containing an anti-cuprate type square lattice2Pressure-Induced Three- to Two-Dimensional Structural Transition in Light Lanthanide Trichlorides0High-pressure synthesis and physical properties of the single-layer nickelate oxychalcogenides B a 2 Ni O 2 C u 2 X 2 ( X = S and Se)0First principles investigation of electronic and optical properties in the thio-apatites series Ba5(VO4−xSx)3X [X=F, Cl, Br, I]: Impact of multiple anionic substitution0Operando Identification of Ni dz 2 Orbital Descriptor Governing Urea Oxidation Electrocatalysis0Spatially Decoupling Co–Ni Centers beyond Sub-Nanometer Distances Enable Auto-Relay Catalysis for C–H Bond Oxidation0

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  1. Synthesis and Magnetism of Extended Solids Containing Transition-Metal Cations in Square-Planar, MO4 Coordination Sites

    Inorganic Chemistry · 2019-05-28

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  2. Manipulating metal spin states for biomimetic, catalytic and molecular materials chemistry

    Dalton Transactions · 2020-01-01

    Malcolm A. Halcrow

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  3. Structure of the water-splitting photocatalyst oxysulfide α-LaOInS 2 and ab initio prediction of new polymorphs

    Chemical Communications · 2020-01-01

    Houria Kabbour, Adlane Sayede, Sébastien Saitzek, Gauthier Lefèvre, Laurent Cario, Martine Trentesaux, Pascal Roussel

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  4. High-pressure Synthesis of Ba2CoO2Ag2Te2 with Extended CoO2 Planes

    Inorganic Chemistry · 2020-05-21

    Yuki Matsumoto, Yusuke Nambu, Takashi Honda, Kazutaka Ikeda, Toshiya Otomo, Hiroshi Kageyama

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  5. Magnetic and electronic properties of layered Sr2NiO2Cl2 with square planar coordination

    Journal of Magnetism and Magnetic Materials · 2020-06-30

    Wenqi Zhou, Shuwei Li, Shuxiang Wu

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  6. Proposed ordering of textured spin singlets in a bulk infinite-layer nickelate

    Physical Review Research · 2020-08-05

    Hyo-Sun Jin, Warren E. Pickett, Kwan-Woo Lee

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  7. Computational Discovery of Stable Heteroanionic Oxychalcogenides ABXO (A, B = Metals; X = S, Se, and Te) and Their Potential Applications

    Chemistry of Materials · 2020-09-09

    Jiangang He, Zhenpeng Yao, Vinay I. Hegde, S. Shahab Naghavi, Jiahong Shen, Kyle Bushick, Chris M. Wolverton

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  8. The dawn of the nickel age of superconductivity

    Nature Reviews Physics · 2020-11-12

    Warren E. Pickett

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  9. Electronic structure and magnetism in infinite-layer nickelates RNiO2 ( R=La−Lu )

    Physical review. B./Physical review. B · 2020-11-24

    Jesse Kapeghian, Antía S. Botana

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  10. Designing new polar materials

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    Emma E. McCabe

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  11. Low Valence Nickelates: Launching the Nickel Age of Superconductivity

    Frontiers in Physics · 2022-02-02

    Antía S. Botana, Kwan-Woo Lee, Michael R. Norman, Víctor Pardo, Warren E. Pickett

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  12. Magnetism of competing high-spin/low-spin states in Ba2NiO2(AgSe)2 and related two-orbital two-electron systems

    Physical review. B./Physical review. B · 2022-02-04

    Rajiv R. P. Singh

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  13. Superconductivity in infinite-layer nickelates

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  14. A d 8 anti-Hund’s singlet insulator in an infinite-layer nickelate

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  15. High-Pressure Synthesis and Order–Disorder Transition of Layered Oxytelluride Ba2ZnO2Ag2Te2

    Inorganic Chemistry · 2022-04-24

    Yang Yang, Tong Zhu, Yuki Matsumoto, Hiroshi Kageyama

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  16. Field-induced Bose-Einstein condensation and supersolid in the two-dimensional Kondo necklace

    Communications Physics · 2022-05-30

    Wei-Lin Tu, Eun-Gook Moon, Kwan-Woo Lee, Warren E. Pickett, Hyun‐Yong Lee

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  17. Magnetic structure of oxygen-deficient perovskite nickelates with ordered vacancies

    Physical Review Research · 2022-06-30

    Yongjin Shin, James M. Rondinelli

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  18. Coherent approach to two-dimensional heterolayered oxychalcogenides using molten hydroxides

    Nature Synthesis · 2022-08-15

    Xiuquan Zhou, Christos D. Malliakas, Andrey Andreevich Yakovenko, Brandon Wilfong, Suyin G. Wang, Yu‐Sheng Chen, Lei Yu, Jianguo Wen, Mahalingam Balasubramanian, Hsien‐Hau Wang, Duck Young Chung, Mercouri G. Kanatzidis

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  19. Mixed anion materials

    Elsevier eBooks · 2022-08-24

    Tong Zhu, Daichi Kato, Shenghan Gao, Hiroshi Kageyama

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  20. High- versus Low-Spin Ni2+ in Elongated Octahedral Environments: Sr2NiO2Cu2Se2, Sr2NiO2Cu2S2, and Sr2NiO2Cu2(Se1–xSx)2

    Chemistry of Materials · 2022-10-18

    Robert D. Smyth, Jack N. Blandy, Ziyu Yu, Shuai Liu, Craig V. Topping, Simon J. Cassidy, Catherine F. Smura, Daniel N. Woodruff, Pascal Manuel, Craig L. Bull, Nicholas P. Funnell, Christopher J. Ridley, John E. McGrady, Simon J. Clarke

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  21. High pressure chemistry

    Elsevier eBooks · 2022-10-31

    Ulrich T. Schwarz, Kristina Spektor, Ulrich Häußermann

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  22. Thermoelectric properties of layered oxyselenides with 3d transition metal ions

    Journal of the American Ceramic Society · 2022-12-28

    Yueyang Yang, Zhifang Zhou, Bin Wei, Junyan Liu, Jinle Lan, Mingchu Zou, Yushuai Xu, Yunpeng Zheng, Ce‐Wen Nan, Yuanhua Lin

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  23. Comprehensive review on multiple mixed-anion ligands, physicochemical performances and application prospects in metal oxysulfides

    Coordination Chemistry Reviews · 2023-04-05

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  24. Infinite-layer nickelates as Ni-eg Hund’s metals

    npj Quantum Materials · 2023-07-12

    Byungkyun Kang, Corey Melnick, P. Sémon, Siheon Ryee, Myung Joon Han, Gabriel Kotliar, Sangkook Choi

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  25. Magnetic ordering in the layered oxyhalide Sr2NiO2Cl2

    Solid State Sciences · 2023-08-28

    Robert D. Smyth, Dmitry D. Khalyavin, Yoshihiro Tsujimoto, Kazunari Yamaura, Simon J. Clarke

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  26. Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics

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  27. Observation and enhancement through alkali metal doping of p-type conductivity in the layered oxyselenides Sr 2 ZnO 2 Cu 2 Se 2 and Ba 2 Zn 1− x O 2− x Cu 2 Se 2

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  28. Decompression-Induced In-Plane Lone Pair Electrons in BiSF Synthesized under High Pressure

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  29. High-pressure X-ray study of NbON oxynitride: direct transition from baddeleyite to cotunnite structure

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  30. Novel Co2+ and Cd2+ Complexes Derived From a New N‐Donor Pyridyl‐Functionalized Thiophosphoric Triamide Ligand: Structural Investigation, DNA/COVID‐19/Monkeypox Molecular Docking, and Biological Assays

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  31. Emergence of Tetragonal Phase and Reentrant Transition in Tensile-Strained Bi2(La1–xBix)O4Cl Solid Solution

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  32. Structural stability and polymorphic transitions in LnSI (Ln = lanthanides)

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  35. Chemistry and physics of layered oxychalcogenides containing an anti-cuprate type square lattice

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  36. Pressure-Induced Three- to Two-Dimensional Structural Transition in Light Lanthanide Trichlorides

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  37. High-pressure synthesis and physical properties of the single-layer nickelate oxychalcogenides B a 2 Ni O 2 C u 2 X 2 ( X = S and Se)

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  38. First principles investigation of electronic and optical properties in the thio-apatites series Ba5(VO4−xSx)3X [X=F, Cl, Br, I]: Impact of multiple anionic substitution

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  40. Spatially Decoupling Co–Ni Centers beyond Sub-Nanometer Distances Enable Auto-Relay Catalysis for C–H Bond Oxidation

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