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RESEARCH PAPER · Angewandte Chemie International Edition · 2018

Undoped Layered Perovskite Oxynitride Li2LaTa2O6N for Photocatalytic CO2 Reduction with Visible Light

Takayoshi Oshima, Tom Ichibha, Ken Sinkou Qin, Kanemichi Muraoka, Junie Jhon M. Vequizo, Keisuke Hibino, Ryo Kuriki, Shunsuke Yamashita, Kenta Hongo, Tomoki Uchiyama, Kotaro Fujii, Daling Lu, Ryo Maezono, Akira Yamakata, Hideki Kato, Koji Kimoto, Masatomo Yashima, Yoshiharu Uchimoto, Masato Kakihana, Osamu Ishitani, Hiroshi Kageyama, Kazuhiko Maeda

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Undoped Layered Perovskite Oxynitride Li2LaTa2O6N for Photocatalytic CO2 Reduction with Visible LightOriginalLayered Heterostructures of Ultrathin Polymeric Carbon Nitride and ZnIn 2 S 4 Nanosheets for Photocatalytic CO 2 Reduction146Synthesis and X-ray absorption spectroscopic analysis of exfoliated perovskite oxynitride nanosheets obtained from LiLaTa2O6.15N0.57 precursor3Two-Dimensional Metal Oxide Nanosheets as Building Blocks for Artificial Photosynthetic Assemblies192A Visible-Light-Driven Z-Scheme CO2 Reduction System Using Ta3N5 and a Ru(II) Binuclear Complex30Ultrathin Conductor Enabling Efficient IR Light CO2 Reduction201Switching on efficient photocatalytic water oxidation reactions over CaNbO2N by Mg modifications under visible light illumination29Polydopamine and Barbituric Acid Co‐Modified Carbon Nitride Nanospheres for Highly Active and Selective Photocatalytic CO2 Reduction23Argonne Leadership Computing Facility (2018 Annual Report)2Highly selective conversion of CO 2 to C 2 H 6 on graphene modified chlorophyll Cu through multi-electron process for artificial photosynthesis28In situ topotactic formation of 2D/2D direct Z-scheme Cu 2 S/Zn 0.67 Cd 0.33 S in-plane intergrowth nanosheet heterojunctions for enhanced photocatalytic hydrogen production34Surface strategies for catalytic CO 2 reduction: from two-dimensional materials to nanoclusters to single atoms904Cocatalysts for Selective Photoreduction of CO 2 into Solar Fuels23011．金属錯体光触媒を用いた二酸化炭素還元と複合系への展開0Two‐Dimensional Layered Zinc Silicate Nanosheets with Excellent Photocatalytic Performance for Organic Pollutant Degradation and CO 2 Conversion110Two‐Dimensional Layered Zinc Silicate Nanosheets with Excellent Photocatalytic Performance for Organic Pollutant Degradation and CO2 Conversion11Homogeneous Doping of Substitutional Nitrogen/Carbon in TiO2 Plates for Visible Light Photocatalytic Water Oxidation75Synthesis of a Layered Niobium Oxynitride, Rb2NdNb2O6N·H2O, Showing Visible-Light Photocatalytic Activity for H2 Evolution34Metal‐Complex/Semiconductor Hybrid Photocatalysts and Photoelectrodes for CO2 Reduction Driven by Visible Light280Revisiting the materials and mechanism of metal oxynitrides for photocatalysis53Oxygen‐Doped Ta3N5 Nanoparticles for Enhanced Z‐Scheme Carbon Dioxide Reduction with a Binuclear Ruthenium(II) Complex under Visible Light13Built-in electric field induced CeO2/Ti3C2-MXene Schottky-junction for coupled photocatalytic tetracycline degradation and CO2 reduction220Improved Photoactivities of Large‐surface‐area g‐C3N4 for CO2 Conversion by Controllably Introducing Co‐ and Ni‐Species to Effectively Modulate Photogenerated Charges20A [001]‐Oriented Hittorf's Phosphorus Nanorods/Polymeric Carbon Nitride Heterostructure for Boosting Wide‐Spectrum‐Responsive Photocatalytic Hydrogen Evolution from Pure Water232A [001]‐Oriented Hittorf's Phosphorus Nanorods/Polymeric Carbon Nitride Heterostructure for Boosting Wide‐Spectrum‐Responsive Photocatalytic Hydrogen Evolution from Pure Water43ThCr2Si2-type quaternary chalcogenides as efficient Pt-free counter electrodes for dye-sensitized solar cells10Integrating photocatalytic reduction of CO2 with selective oxidation of tetrahydroisoquinoline over InP–In2O3 Z-scheme p-n junction53Simultaneous Ni nanoparticles decoration and Ni doping of CdS nanorods for synergistically promoting photocatalytic H2 evolution54Synthesis of Copolymerized Carbon Nitride Nanosheets from Urea and 2‐Aminobenzonitrile for Enhanced Visible Light CO2 Reduction with a Ruthenium(II) Complex Catalyst16Anion Ordered and Ferroelectric Ruddlesden–Popper Oxynitride Ca3Nb2N2O5 for Visible-Light-Active Photocatalysis28Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 Evolution57Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 Evolution6Recent advances of bismuth oxychloride photocatalytic material: Property, preparation and performance enhancement83Selective CO2 reduction into formate using Ln–Ta oxynitrides combined with a binuclear Ru(II) complex under visible light18Synthesis of Three-Layer Perovskite Oxynitride K2Ca2Ta3O9N·2H2O and Photocatalytic Activity for H2 Evolution under Visible Light35Ruddlesden–Popper Perovskite Oxides for Photocatalysis-Based Water Splitting and Wastewater Treatment105Perovskite Oxide Based Materials for Energy and Environment-Oriented Photocatalysis636Inside‐and‐Out Semiconductor Engineering for CO 2 Photoreduction: From Recent Advances to New Trends411The In-situ Growth NiFe-layered Double Hydroxides/g-C3N4 Nanocomposite 2D/2D Heterojunction for Enhanced Photocatalytic CO2 Reduction Performance49Recent Progress in Mixed‐Anion Materials for Solar Fuel Production58Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers9Colocalization of light harvesting and catalytic units in a ‘soft’ coordination polymer hydrogel toward visible-light driven photocatalytic hydrogen production51Enhanced photocatalytic properties of a chemically modified blue phosphorene10Photochemical reduction of carbon dioxide to formic acid115Plasma synthesis of Pt/g-C3N4 photocatalysts with enhanced photocatalytic hydrogen generation92Molecule/Semiconductor Hybrid Materials for Visible-Light CO 2 Reduction: Design Principles and Interfacial Engineering99A roadmap towards the development of superior photocatalysts for solar- driven CO2-to-fuels production43Computational discovery of stable and metastable ternary oxynitrides38Defect-engineered room-temperature ferromagnetism in quasi-two-dimensional nitrided CoTa2O61Preparation of Multifunctional Metal Oxynitride 2D Crystals and Oriented Transparent Free-Standing Oxynitride Films22O/F anion order in Pb$_2$Ti$_4$O$_9$F$_2$ stabilized by the 6$s^2$ lone pair electrons of Pb$^{2+}$0Recent Progress on Mixed-Anion Materials for Energy Applications110Recent advances in the fabrication of 2D metal oxides111Charge-transfer regulated visible light driven photocatalytic H2 production and CO2 reduction in tetrathiafulvalene based coordination polymer gel171Developing Atomically Thin Li1.81H0.19Ti2O5·2H2O Nanosheets for Selective Photocatalytic CO2 Reduction to CO11A two-dimensional perovskite oxyfluoride Pb 3 Fe 2 O 5 F 2 as a catalyst for electrochemical oxidation of water to oxygen9Anionic ordering in Pb 2 Ti 4 O 9 F 2 revisited by nuclear magnetic resonance and density functional theory3High-performance potassium poly(heptazine imide) films for photoelectrochemical water splitting84Creation of SnxNb1−xO2 solid solution through heavy Nb-doping in SnO2 to boost its photocatalytic CO2 reduction to C2+ products under simulated solar illumination41Research progress on the formation, detection methods and application in photocatalytic reduction of CO2 of oxygen vacancy54Interlayer modification and single-layer exfoliation of the Ruddlesden–Popper perovskite oxynitride K 2 LaTa 2 O 6 N to improve photocatalytic H 2 evolution activity17Bandgap Tunable Oxynitride LaNb 2 O 7–x N x Nanosheets20Recent advances in 2D semiconductor nanomaterials for photocatalytic CO2 reduction30Prediction of perovskite structures and thermodynamic stabilities from structural factors0Dark–Light Tandem Catalytic Oxidation of Formaldehyde over SrBi2Ta2O9 Nanosheets7Effect of alkali-metal cations on synthesis of stoichiometric layered perovskite oxynitrides3Sub-50 nm perovskite-type tantalum-based oxynitride single crystals with enhanced photoactivity for water splitting57Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis19Spinel-Type Zn2-2xnbxfexti1-2xo4-2x (00Carbon dioxide reduction utilizing a bismuth halide perovskite as immobilized photocatalyst in a 3D printed microreactor3Layered oxide precursor strategy for the synthesizing of titanium oxynitrides2Doping engineering in S–scheme composite for Regulating the selectivity of photocatalytic CO2 reduction13Theoretical Calculations of Mixed-anion Compounds0A comparative study on carbon neutral hydrogen carrier production: Formic acid from CO2 vs. ammonia32Efficient Visible-Light-Driven Water Oxidation by a Carbon Nitride Modified with Cobalt Polyoxometalate Molecular Catalyst15Molecular-based porous polymers with precise sites for photoreduction of carbon dioxide11Recent advances on surface modification of non-oxide photocatalysts towards efficient CO2 conversion53Advances in perovskite-based photocatalysts: Mechanisms, materials design, and applications0CsCl-flux synthesis of titanium oxynitride (Ti 2.85 O 4 N) for photocatalysis0Tunable optical properties in the (110) p -oriented layered halide perovskite FA 4 Pb 2 I 7.5 (SCN) 0.5 by Br substitution0Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications29Charge Carrier Dynamics at Heterojunction of Semiconductor Nanoheterostructures for Photocatalytic Solar Fuel Generation31Two‐Dimensional Perovskites for Photocatalytic CO 2 Reduction74Two‐Dimensional Perovskites for Photocatalytic CO 2 Reduction21Effects of Metal-Cation Doping on Photocatalytic H2 Evolution Activity of Layered Perovskite Oxynitride K2LaTa2O6N7Multidimensional Engineering of Nanoconfined Catalysis: Frontiers in Carbon-Based Energy Conversion and Utilization171Synergistic Surface Modifications Enable Direct Photocatalytic Overall Water Splitting over a MgTa 2 O 6– x N y /TaON Heterostructure8Tantalum‐Based Perovskite Oxynitride Monolayers Derived From a Charge‐Balanced Nitridation Strategy for Photocatalytic Overall Water Splitting12Synergistic catalysis for promoting photocatalytic CO2 reduction toward C2+ products7Topotactic Nitridation Enabled Core–Shell La 4 Ti 3 (O,N) 12 @LaTiO 2 N for Efficient Photoelectrochemical Water Splitting0Copper-antimony sulfide nanostructures with oriented architecture and their efficient CO2 photoreduction0TiO2/NaBiS2 S-scheme heterostructures for enhanced photoelectrocatalytic degradation of tetracycline0Perovskites for CO 2 Conversion: Active‐Phase Identity, Reconstruction, and the Evidence Behind Mechanistic Claims0

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  2. Synthesis and X-ray absorption spectroscopic analysis of exfoliated perovskite oxynitride nanosheets obtained from LiLaTa2O6.15N0.57 precursor

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  3. Two-Dimensional Metal Oxide Nanosheets as Building Blocks for Artificial Photosynthetic Assemblies

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  4. A Visible-Light-Driven Z-Scheme CO2 Reduction System Using Ta3N5 and a Ru(II) Binuclear Complex

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  6. Switching on efficient photocatalytic water oxidation reactions over CaNbO2N by Mg modifications under visible light illumination

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  18. Metal‐Complex/Semiconductor Hybrid Photocatalysts and Photoelectrodes for CO2 Reduction Driven by Visible Light

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  19. Revisiting the materials and mechanism of metal oxynitrides for photocatalysis

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  20. Oxygen‐Doped Ta3N5 Nanoparticles for Enhanced Z‐Scheme Carbon Dioxide Reduction with a Binuclear Ruthenium(II) Complex under Visible Light

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  30. Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 Evolution

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  31. Two‐Dimensional Perovskite Oxynitride K2LaTa2O6N with an H+/K+ Exchangeability in Aqueous Solution Forming a Stable Photocatalyst for Visible‐Light H2 Evolution

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  33. Selective CO2 reduction into formate using Ln–Ta oxynitrides combined with a binuclear Ru(II) complex under visible light

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  45. Molecule/Semiconductor Hybrid Materials for Visible-Light CO 2 Reduction: Design Principles and Interfacial Engineering

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  46. A roadmap towards the development of superior photocatalysts for solar- driven CO2-to-fuels production

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  47. Computational discovery of stable and metastable ternary oxynitrides

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  48. Defect-engineered room-temperature ferromagnetism in quasi-two-dimensional nitrided CoTa2O6

    Physical review. B./Physical review. B · 2021-07-19

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  49. Preparation of Multifunctional Metal Oxynitride 2D Crystals and Oriented Transparent Free-Standing Oxynitride Films

    Chemistry of Materials · 2021-07-29

    Chu‐Wei Hsu, Takumi Ideta, Keisuke Awaya, Masayuki Tsushida, Tetsuya Sato, Kei-ichi Yanagisawa, Koji Kimoto, Kazuto Hatakeyama, Michio Koinuma, Shintaro Ida

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  50. O/F anion order in Pb$_2$Ti$_4$O$_9$F$_2$ stabilized by the 6$s^2$ lone pair electrons of Pb$^{2+}$

    arXiv (Cornell University) · 2021-09-28

    Kengo Oka, Tom Ichibha, Daichi Kato, Mitsunobu Iwasaki, Naoki Noma, Kenta Hongo, Ryo Maezono, Fernando Agustín Reboredo

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