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RESEARCH PAPER · Advanced Materials · 2019

Metal‐Complex/Semiconductor Hybrid Photocatalysts and Photoelectrodes for CO2 Reduction Driven by Visible Light

Kazuhiko Maeda

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Metal‐Complex/Semiconductor Hybrid Photocatalysts and Photoelectrodes for CO2 Reduction Driven by Visible LightOriginalImmobilization of Mn( i ) and Ru( ii ) polypyridyl complexes on TiO 2 nanoparticles for selective photoreduction of CO 2 to formic acid13Oxygen‐Doped Ta3N5 Nanoparticles for Enhanced Z‐Scheme Carbon Dioxide Reduction with a Binuclear Ruthenium(II) Complex under Visible Light13Synergetic photocatalysis/piezocatalysis of bismuth oxybromide for degradation of organic pollutants227Three‐Phase Photocatalysis for the Enhanced Selectivity and Activity of CO2 Reduction on a Hydrophobic Surface401Three‐Phase Photocatalysis for the Enhanced Selectivity and Activity of CO2 Reduction on a Hydrophobic Surface57Immobilizing Re(CO)3Br(dcbpy) Complex on CsPbBr3 Nanocrystal for Boosted Charge Separation and Photocatalytic CO2 Reduction68An emerging solar-thermal-electric conversion system based on highly-efficient photothermal nanoabsorber layer5Improved Electrochemical Water Oxidation over Chromium-Substituted Cobalt Aluminate Spinels7In situ fabrication of amorphous TiO2/NH2-MIL-125(Ti) for enhanced photocatalytic CO2 into CH4 with H2O under visible-light irradiation84Photocatalytic and Photoelectrochemical Systems: Similarities and Differences394A leaf-branch TiO2/carbon@MOF composite for selective CO2 photoreduction127Synthesis of Copolymerized Carbon Nitride Nanosheets from Urea and 2‐Aminobenzonitrile for Enhanced Visible Light CO2 Reduction with a Ruthenium(II) Complex Catalyst16Activity and selectivity of CO 2 photoreduction on catalytic materials18Architecting epitaxial-lattice-mismatch-free (LMF) zinc oxide/bismuth oxyiodide nano-heterostructures for efficient photocatalysis29Nano vs. bulk rutile TiO 2 :N,F in Z-scheme overall water splitting under visible light28Photoelectrochemical solar fuels from carbon dioxide, water and sunlight36Self-assembled CoTiO 3 nanorods with controllable oxygen vacancies for the efficient photochemical reduction of CO 2 to CO44Synthesis, crystal structure, and magnetic properties of oxynitride perovskites SrMn 0.2 M 0.8 O 2.6 N 0.4 (M = Nb, Ta)5The influence of inorganic anions on photocatalytic CO 2 reduction16Water Purification Using Subnanostructured Photocatalysts0Molecular Junctions on Polymeric Carbon Nitrides with Enhanced Photocatalytic Performance30Photoelectrochemical Conversion of Carbon Dioxide (CO2) into Fuels and Value-Added Products627Photocatalytic Reduction of CO 2 by Metal‐Free‐Based Materials: Recent Advances and Future Perspective248Visible-Light-Driven Hydrogen Peroxide Synthesis by a Hybrid Photocatalyst Consisting of Bismuth Vanadate and Bis(hexafluoroacetylacetonato)copper(II) Complex22Engineering Active Ni Sites in Ternary Layered Double Hydroxide Nanosheets for a Highly Selective Photoreduction of CO2 to CH4 under Irradiation above 500 nm80Semiconductor/Covalent‐Organic‐Framework Z‐Scheme Heterojunctions for Artificial Photosynthesis513Semiconductor/Covalent‐Organic‐Framework Z‐Scheme Heterojunctions for Artificial Photosynthesis94In-situ hydroxyl modification of monolayer black phosphorus for stable photocatalytic carbon dioxide conversion230Nafion-Assisted Noncovalent Assembly of Molecular Sensitizers and Catalysts for Sustained Photoreduction of CO2 to CO12Efficient Visible-Light-Driven CO 2 Reduction by a Cobalt Molecular Catalyst Covalently Linked to Mesoporous Carbon Nitride314Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications1050Modulating charge separation and transfer kinetics in carbon nanodots for photoredox catalysis26Formation of Hierarchical FeCoS2–CoS2 Double‐Shelled Nanotubes with Enhanced Performance for Photocatalytic Reduction of CO2245Formation of Hierarchical FeCoS2–CoS2 Double‐Shelled Nanotubes with Enhanced Performance for Photocatalytic Reduction of CO228Revealing the role of oxygen vacancies in bimetallic PbBiO2Br atomic layers for boosting photocatalytic CO2 conversion116Site-Selective Deposition of a Cobalt Cocatalyst onto a Plasmonic Au/TiO2 Photoanode for Improved Water Oxidation41Visible-Light-Induced Photocatalytic Activity of Stacked MXene Sheets of Y2CF2443D Nanostructures for the Next Generation of High‐Performance Nanodevices for Electrochemical Energy Conversion and Storage182An efficient visible-light photocatalyst for CO2 reduction fabricated by cobalt porphyrin and graphitic carbon nitride via covalent bonding71Site- and Spatial-Selective Integration of Non-noble Metal Ions into Quantum Dots for Robust Hydrogen Photogeneration60Selective CO2 reduction into formate using Ln–Ta oxynitrides combined with a binuclear Ru(II) complex under visible light18Construction of Functionally Compartmental Inorganic Photocatalyst–Enzyme System via Imitating Chloroplast for Efficient Photoreduction of CO 2 to Formic Acid1312D PbS Nanosheets with Zigzag Edges for Efficient CO2 Photoconversion12Bismuth‐Decorated Silicon Photocathodes for CO2‐to‐Formate Solar‐Driven Conversion12Engineering photocatalytic and photoelectrocatalytic CO2 reduction reactions: Mechanisms, intrinsic kinetics, mass transfer resistances, reactors and multi-scale modelling simulations195Pyroelectric catalysis157Boosting photocatalytic CO2 reduction over a covalent organic framework decorated with ruthenium nanoparticles172Photochemical In Situ Exfoliation of Metal–Organic Frameworks for Enhanced Visible‐Light‐Driven CO2 Reduction136Photochemical In Situ Exfoliation of Metal–Organic Frameworks for Enhanced Visible‐Light‐Driven CO2 Reduction18Suppression of Nb reduction in high-κ perovskite oxynitrides, BaM Nb1−O2+4N1−4 (M = Li, Na; x ≤ 0.15)6Durable photoelectrochemical CO 2 reduction with water oxidation using a visible-light driven molecular photocathode46Reticular Materials for Artificial Photoreduction of CO 2142Recent Progress in Mixed‐Anion Materials for Solar Fuel Production58Fabrication of non-covalently grafted Cu(acac)2 over two-dimensional graphene oxide nanosheets: An environmentally benign noble photocatalyst for visible-light-driven degradation of phenol6Saw-Tooth Heat-Cycling Nitridation of Metallic Cu Yields First Photoactive p-Cu3N for PEC Applications5Rare-Earth Single-Atom La–N Charge-Transfer Bridge on Carbon Nitride for Highly Efficient and Selective Photocatalytic CO2 Reduction460Highly Efficient and Selective Visible-Light Driven CO2 Reduction by Two Co-Based Catalysts in Aqueous Solution27Encapsulation of Cobalt Oxide into Metal‐Organic Frameworks for an Improved Photocatalytic CO2 Reduction64Nickel-Coordinated Carbon Nitride as a Metallaphotoredox Platform for the Cross-Coupling of Aryl Halides with Alcohols114Visible-light-driven CO2 reduction to ethylene on CdS: Enabled by structural relaxation-induced intermediate dimerization and enhanced by ZIF-8 coating130DFT calculations for single-atom confinement effects of noble metals on monolayer g-C 3 N 4 for photocatalytic applications62Effect of Li ions doping into p-type semiconductor NiO as a hole injection/transfer medium in the CO2 reduction sensitized/catalyzed by Zn-porphyrin/Re-complex upon visible light irradiation12Graphdiyne anchored ultrafine Ag nanoparticles for highly efficient and solvent-free catalysis of CO 2 cycloaddition18Immobilising molecular Ru complexes on a protective ultrathin oxide layer of p-Si electrodes towards photoelectrochemical CO 2 reduction17Porphyrin and single atom featured reticular materials: recent advances and future perspective of solar-driven CO 2 reduction62Recent advances in zinc chalcogenide-based nanocatalysts for photocatalytic reduction of CO 242Supramolecular photocatalysts fixed on the inside of the polypyrrole layer in dye sensitized molecular photocathodes: application to photocatalytic CO 2 reduction coupled with water oxidation29Well-defined Co 9 S 8 cages enable the separation of photoexcited charges to promote visible-light CO 2 reduction66Engineering 2D Photocatalysts toward Carbon Dioxide Reduction237Tuning Crystallinity and Surface Hydrophobicity of a Cobalt Phosphide Cocatalyst to Boost CO2 Photoreduction Performance44Synthesis of Au/UiO-66-NH2/Graphene composites as efficient visible-light photocatalysts to convert CO258Hybrid Photocathodes for Carbon Dioxide Reduction: Interfaces for Charge Separation and Selective Catalysis21Dissecting the interfaces of MOF-coated CdS on synergized charge transfer for enhanced photocatalytic CO2 reduction96Irreversible Resistive State Switching in Devices with a Homoleptic Cobalt(II) Complex Active Layer8The roles of polyoxometalates in photocatalytic reduction of carbon dioxide89Recent Progress on Photocatalytic CO2 Reduction with Earth‐abundant Single‐atom Reactive Sites22Chemically Exfoliated Semiconducting Bimetallic Porphyrinylphosphonate Metal–Organic Layers for Photocatalytic CO2 Reduction under Visible Light36Regulating Utilization Efficiency of the Photogenerated Charge Carriers by Constructing Donor–π–Acceptor Polymers for Upgrading Photocatalytic CO2 Reduction20Hybridization of Molecular and Graphene Materials for CO2 Photocatalytic Reduction with Selectivity Control116Light-driven catalytic conversion of CO2 with heterogenized molecular catalysts based on fourth period transition metals78Molecule/Semiconductor Hybrid Materials for Visible-Light CO 2 Reduction: Design Principles and Interfacial Engineering99Interfacial Interactions between Co‐Based Cocatalysts and Semiconducting Light Absorbers for Solar‐Light‐Driven Redox Reactions5Improved photocatalytic CO2 conversion efficiency on Ag loaded porous Ta2O548Cobalt Phosphide Cocatalysts Coated with Porous N‐doped Carbon Layers for Photocatalytic CO 2 Reduction26Integrating Single Atoms with Different Microenvironments into One Porous Organic Polymer for Efficient Photocatalytic CO2 Reduction206Catalytic reduction of CO2 by Al–Sn-CNTs composite for synthesizing formic acid14General framework for enzyme-photo-coupled catalytic system toward carbon dioxide conversion21Hierarchical Double-Shelled CoP Nanocages for Efficient Visible-Light-Driven CO2 Reduction38In situ preparation of polymeric cobalt phthalocyanine–decorated TiO2 nanorods for efficient photocatalytic CO2 reduction36Engineering metal-organic frameworks for efficient photocatalytic conversion of CO2 into solar fuels112A review on progress and perspective of molecular catalysis in photoelectrochemical reduction of CO2110Hexanuclear nickel-based [P4Mo11O50] with photocatalytic reduction of CO2 activity9Reticular-Chemistry-Inspired Supramolecule Design as a Tool to Achieve Efficient Photocatalysts for CO2 Reduction29Closing the Anthropogenic Chemical Carbon Cycle toward a Sustainable Future via CO2 Valorization86BiOBr Micro–Nanosheets: Controllable Synthesis and Piezoelectric and Photoelectric Properties8Advances in photoelectroreduction of CO2 to hydrocarbons fuels: Contributions of functional materials32Mechanism of the photoreduction of carbon dioxide catalyzed by the benchmarking rhenium dimethylbipyridine complexes; operando measurements by XAFS and FT-IR22Solar-Driven CO2 Reduction Using a Semiconductor/Molecule Hybrid Photosystem: From Photocatalysts to a Monolithic Artificial Leaf129Nanoarchitectonics of Metal-Free Porous Polyketone as Photocatalytic Assemblies for Artificial Photosynthesis39BiZnx/Si Photocathode: Preparation and CO2 Reduction Performance2Current status, research gaps, and future scope for nanomaterials toward visible light photocatalysis2Electrospun 1D-NiO hollow nanowires on glass support for the sunlight-driven photodegradation of methylene blue9Emergent Catalytic Materials Towards CO2 Reduction0High-yield synthesis and hybridizations of Cu microplates for catalytic applications9Organic–inorganic hybrid photocatalyst consisting of a highly conjugated metal complex and graphitic carbon nitride for efficient hydrogen evolution and Cr( vi ) reduction18Synthesis, Structural Distortion, and Magnetic Property of Complex Perovskites Amn0.2m0.8o2.6n0.4 (a = Sr, Ba; M = Nb, Ta)0Synthesis, Structural Distortion, and Magnetic Property of Complex Perovskites Amn0.2m0.8o2.6n0.4 (a = Sr, Ba; M = Nb, Ta)0Highly Efficient Photocatalytic Reduction of CO 2 to CO by In Situ Formation of a Hybrid Catalytic System Based on Molecular Iron Quaterpyridine Covalently Linked to Carbon Nitride87Highly Efficient Photocatalytic Reduction of CO 2 to CO by In Situ Formation of a Hybrid Catalytic System Based on Molecular Iron Quaterpyridine Covalently Linked to Carbon Nitride17Host-guest assemblies of anchoring molecular catalysts of CO2 reduction onto CuInS2/ZnS quantum dots for robust photocatalytic syngas production in water27CO 2 Reduction Using Water as an Electron Donor over Heterogeneous Photocatalysts Aiming at Artificial Photosynthesis258The Importance of the Macroscopic Geometry in Gas‐Phase Photocatalysis55Layered Double Hydroxide Engineering for the Photocatalytic Conversion of Inactive Carbon and Nitrogen Molecules33Protein‐Mediated Biosynthesis of Semiconductor Nanocrystals for Photocatalytic NAD(P)H Regeneration and Chiral Amine Production32Protein‐Mediated Biosynthesis of Semiconductor Nanocrystals for Photocatalytic NAD(P)H Regeneration and Chiral Amine Production2Surface States for Photoelectrodes of Gallium Phosphide (GaP) with Surface-Specific Electronic Spectra and Phase Measurements15Design of some novel dithio π-conjugated ligand-based metal complexes and their semiconductor behavior0Coupling Ruthenium Bipyridyl and Cobalt Imidazolate Units in a Metal–Organic Framework for an Efficient Photosynthetic Overall Reaction in Diluted CO2123Alumina‐Supported Alpha‐Iron(III) Oxyhydroxide as a Recyclable Solid Catalyst for CO2 Photoreduction under Visible Light24Alumina‐Supported Alpha‐Iron(III) Oxyhydroxide as a Recyclable Solid Catalyst for CO2 Photoreduction under Visible Light3Principles, synthesis and applications of dual Z-scheme photocatalysts145In-situ constructing Schottky junction and oxygen vacancy on HNb3O8 nanosheets for rapid charge transfer and enrichment for boosted photocatalytic CO2 reduction towards CH417Photothermal conversion of CO2 to fuel with nickel-based catalysts: A review19Relevance of Rabi splitting effect for tunable enhancement of Raman scattering in self-assembled silver – Fullerene nanocomposite films4Photocatalytic CO2 reduction by a Z-scheme mechanism in an aqueous suspension of particulate (CuGa)0.3Zn1.4S2, BiVO4 and a Co complex operating dual-functionally as an electron mediator and as a cocatalyst35Single‐Atom Catalysts (SACs) for Photocatalytic CO 2 Reduction with H 2 O: Activity, Product Selectivity, Stability, and Surface Chemistry122Electrocatalytic and photocatalytic sustainable conversion of carbon dioxide to value-added chemicals: State-of-the-art progress, challenges, and future directions45Insight into the mechanism of deep NO photo-oxidation by bismuth tantalate with oxygen vacancies50A core-satellite structured type II heterojunction photocatalyst with enhanced CO2 reduction under visible light48Selective CO 2 -to-Formate Conversion Driven by Visible Light over a Precious-Metal-Free Nonporous Coordination Polymer49Effects of a Nanoparticulate TiO2 Modifier on the Visible-Light CO2 Reduction Performance of a Metal-Complex/Semiconductor Hybrid Photocatalyst26Nanoscale reaction monitoring using localized surface plasmon resonance scatterometry4The roles of gold and silver nanoparticles on ZnIn2S4/silver (gold)/tetra(4-carboxyphenyl)porphyrin iron(III) chloride hybrids in carbon dioxide photoreduction21Integrating polyarylether-COFs with TiO2 nanofibers for enhanced visible-light-driven CO2 reduction in artificial photosynthesis28Efficient photocatalytic aerobic oxidations by a molecular cobalt catalyst linked to mesoporous carbon nitride7Advances in Biomimetic Photoelectrocatalytic Reduction of Carbon Dioxide51MIL-68 (In)-derived In2O3@TiO2 S-scheme heterojunction with hierarchical hollow structure for selective photoconversion of CO2 to hydrocarbon fuels26Implanting CoOx Clusters on Ordered Macroporous ZnO Nanoreactors for Efficient CO2 Photoreduction89Toward Excellence in Photocathode Engineering for Photoelectrochemical CO2 Reduction: Design Rationales and Current Progress104Hierarchical ternary layered double hydroxide/graphitic carbon nitride heterostructures as visible-light photocatalysts for efficient reduction of CO212Improved Charge Separation in Poly(heptazine‐triazine) Imides with Semi‐coherent Interfaces for Photocatalytic Hydrogen Evolution33Improved Charge Separation in Poly(heptazine‐triazine) Imides with Semi‐coherent Interfaces for Photocatalytic Hydrogen Evolution136Harnessing Keto‐Enol Tautomerism to Modulate β‐Ketoenamine‐based Covalent Organic Frameworks for Visible‐Light‐Driven CO2 Reduction8Comprehensive Review for an Efficient Charge Transfer in Single Atomic Site Catalyst/Organic Polymers toward Photocatalytic CO2 Reduction26Development of an Integrated System for Highly Selective Photoenzymatic Synthesis of Formic Acid from CO227Engineered 2D Metal Oxides for Photocatalysis as Environmental Remediation: A Theoretical Perspective10Structure-Dependent Surface Molecule-Modified Semiconductor Photocatalysts: Recent Progress and Future Challenges29Exploration of metal organic frameworks and covalent organic frameworks for energy-related applications217An assembled ternary photocatalyst CoPh/CdSe@TiO2 for simultaneous photocatalytic CO 2 and proton reduction13Surface Immobilization of a Re(I) Tricarbonyl Phenanthroline Complex to Si(111) through Sonochemical Hydrosilylation24

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  4. Three‐Phase Photocatalysis for the Enhanced Selectivity and Activity of CO2 Reduction on a Hydrophobic Surface

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  9. In situ fabrication of amorphous TiO2/NH2-MIL-125(Ti) for enhanced photocatalytic CO2 into CH4 with H2O under visible-light irradiation

    Journal of Colloid and Interface Science · 2019-11-04

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  10. Photocatalytic and Photoelectrochemical Systems: Similarities and Differences

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  19. The influence of inorganic anions on photocatalytic CO 2 reduction

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  33. Formation of Hierarchical FeCoS2–CoS2 Double‐Shelled Nanotubes with Enhanced Performance for Photocatalytic Reduction of CO2

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  34. Formation of Hierarchical FeCoS2–CoS2 Double‐Shelled Nanotubes with Enhanced Performance for Photocatalytic Reduction of CO2

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  35. Revealing the role of oxygen vacancies in bimetallic PbBiO2Br atomic layers for boosting photocatalytic CO2 conversion

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  36. Site-Selective Deposition of a Cobalt Cocatalyst onto a Plasmonic Au/TiO2 Photoanode for Improved Water Oxidation

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  37. Visible-Light-Induced Photocatalytic Activity of Stacked MXene Sheets of Y2CF2

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  38. 3D Nanostructures for the Next Generation of High‐Performance Nanodevices for Electrochemical Energy Conversion and Storage

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    Yu‐Ji Gao, Xu‐Bing Li, Xuzhe Wang, Ningjiu Zhao, Yufei Zhao, Yang Wang, Zhi‐Kun Xin, Jianping Zhang, Tierui Zhang, Chen‐Ho Tung, Li‐Zhu Wu

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  41. Selective CO2 reduction into formate using Ln–Ta oxynitrides combined with a binuclear Ru(II) complex under visible light

    Journal of Energy Chemistry · 2020-07-08

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  42. Construction of Functionally Compartmental Inorganic Photocatalyst–Enzyme System via Imitating Chloroplast for Efficient Photoreduction of CO 2 to Formic Acid

    ACS Applied Materials & Interfaces · 2020-07-27

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  43. 2D PbS Nanosheets with Zigzag Edges for Efficient CO2 Photoconversion

    Chemistry - A European Journal · 2020-08-09

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  44. Bismuth‐Decorated Silicon Photocathodes for CO2‐to‐Formate Solar‐Driven Conversion

    ChemCatChem · 2020-08-25

    Dong Fu, Jeoffrey Tourneur, Bruno Fabre, Gabriel Loget, Yao‐Yin Lou, Florence Geneste, Soraya Ababou‐Girard, Cristelle Mériadec

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  45. Engineering photocatalytic and photoelectrocatalytic CO2 reduction reactions: Mechanisms, intrinsic kinetics, mass transfer resistances, reactors and multi-scale modelling simulations

    Chemical Engineering Journal · 2020-08-27

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  46. Pyroelectric catalysis

    Nano Energy · 2020-09-11

    Chunyang Wang, Na Tian, Tianyi Ma, Yihe Zhang, Hongwei Huang

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  47. Boosting photocatalytic CO2 reduction over a covalent organic framework decorated with ruthenium nanoparticles

    Chemical Engineering Journal · 2020-09-12

    Ke Guo, Xiaoli Zhu, Lianlian Peng, Yanghe Fu, Rui Ma, Xinqing Lu, Fu‐Min Zhang, Weidong Zhu, Maohong Fan

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  48. Photochemical In Situ Exfoliation of Metal–Organic Frameworks for Enhanced Visible‐Light‐Driven CO2 Reduction

    Angewandte Chemie International Edition · 2020-09-24

    Hui‐Li Zheng, Shan‐Lin Huang, Ming‐Bu Luo, Wei Qin, Er‐Xia Chen, Liang He, Qipu Lin

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  49. Photochemical In Situ Exfoliation of Metal–Organic Frameworks for Enhanced Visible‐Light‐Driven CO2 Reduction

    Angewandte Chemie · 2020-09-27

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  50. Suppression of Nb reduction in high-κ perovskite oxynitrides, BaM Nb1−O2+4N1−4 (M = Li, Na; x ≤ 0.15)

    Journal of Alloys and Compounds · 2020-10-07

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