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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2018

CaZnOS:Nd3+ Emits Tissue-Penetrating near-Infrared Light upon Force Loading

Lejing Li, Lothar Wondraczek, Lihua Li, Yu Zhang, Ye Zhu, Mingying Peng, Chuanbin Mao

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CaZnOS:Nd3+ Emits Tissue-Penetrating near-Infrared Light upon Force LoadingOriginalNovel persistent and tribo-luminescence from bismuth ion pairs doped strontium gallate68Recent development of elastico-mechanoluminescent phosphors69Optical and vibrational properties of CaZnOS: The role of intrinsic defects21Piezophotonic effect based on mechanoluminescent materials for advanced flexible optoelectronic applications184Mechanically Excited Multicolor Luminescence in Lanthanide Ions254Coexistence of self-reduction from Mn 4+ to Mn 2+ and elastico-mechanoluminescence in diphase KZn(PO 3 ) 3 :Mn 2+74Intense red photoluminescence and mechanoluminescence from Mn 2+ -activated SrZnSO with a layered structure59Mechanics-induced triple-mode anticounterfeiting and moving tactile sensing by simultaneously utilizing instantaneous and persistent mechanoluminescence161Near infrared mechanoluminescence from the Nd 3+ doped perovskite LiNbO 3 :Nd 3+ for stress sensors95Trap-controlled mechanoluminescent materials446New Theoretical Insights into the Crystal-Field Splitting and Transition Mechanism for Nd3+-Doped Y3Al5O1234Near infrared mechanoluminescence from Sr 3 Sn 2 O 7 : Nd 3+ for in situ biomechanical sensor and dynamic pressure mapping70Artificial Microbial Arenas: Materials for Observing and Manipulating Microbial Consortia47Expanding the toolbox for lanthanide-doped upconversion nanocrystals43Largely enhanced elastico-mechanoluminescence of CaZnOS: Mn2+ by co-doping with Nd3+ ions45Creating visible-to-near-infrared mechanoluminescence in mixed-anion compounds SrZn2S2O and SrZnSO145Force-induced 1540 nm luminescence: Role of piezotronic effect in energy transfer process for mechanoluminescence72In-Depth Determination of the Microstructure and Energy Transition Mechanism for Nd3+-Doped Yttrium Oxide Laser Crystals24A ZnS/CaZnOS Heterojunction for Efficient Mechanical‐to‐Optical Energy Conversion by Conduction Band Offset217Short-Term Non-Decaying Mechanoluminescence in Li2MgGeO4:Mn2+21Tuning Multimode Luminescence in Lanthanide(III) and Manganese(II) Co‐Doped CaZnOS Crystals72Ferroelectric Sr 3 Sn 2 O 7 :Nd 3+ : A New Multipiezo Material with Ultrasensitive and Sustainable Near‐Infrared Piezoluminescence118Efficient color manipulation of zinc sulfide-based mechanoluminescent elastomers for visualized sensing and anti-counterfeiting33Force-induced charge carrier storage: a new route for stress recording141Conversion of mechanical energy into light : understanding the phenomenon in the case of phosphor-elastomer composite materials0Near-infrared mechanoluminescence crystals: a review87Enhanced mechanically induced red-light emitting novel mechanoluminescence materials for ultrasonic visualization and monitoring applications55Regulating the trap distribution to achieve high-contrast mechanoluminescence with an extended saturation threshold through co-doping Nd 3+ into CaZnOS:Bi 3+ ,Li +42Self‐Recoverable Mechanically Induced Instant Luminescence from Cr3+‐Doped LiGa5O8191Mechanoluminescence Rebrightening the Prospects of Stress Sensing: A Review507Near-Infrared Mechanoluminescence Material from Organic Acid-Aided Process6Time‐Resolved Bright Red to Cyan Color Tunable Mechanoluminescence from CaZnOS: Bi 3+ , Mn 2+ for Anti‐Counterfeiting Device and Stress Sensor135Sensing Materials: Lanthanide Materials1A review of mechanochromic polymers and composites: From material design strategy to advanced electronics application97Sensitization of Yb(III), ER(III), and Nd(III) Luminescence by Ligands Based on 3-Formyl-4-Hydroxybenzoic Acid and Transition Metals2Self-Reduction-Related Defects, Long Afterglow, and Mechanoluminescence in Centrosymmetric Li2ZnGeO4:Mn2+83Broadband multimodal emission in Sb-doped CaZnOS-layered semiconductors25Recent Development of Flexible Tactile Sensors and Their Applications97Achieving visible and near-infrared dual-emitting mechanoluminescence in Mn 2+ single-doped magnesium aluminate spinel13Mechanoluminescent Phosphors0Monitoring cardiovascular disease severity using near-infrared mechanoluminescent materials as a built-in indicator43Contact electrification induced mechanoluminescence97Molten Salt Shielded Synthesis of Monodisperse Layered CaZnOS‐Based Semiconductors for Piezophotonic and X‐Ray Detection Applications56Ultrasound‐Induced Mechanoluminescence and Optical Thermometry Toward Stimulus‐Responsive Materials with Simultaneous Trigger Response and Read‐Out Functions73Alkaline‐Earth‐Metal‐Ions Blending Enhanced Self‐Activated and Bi3+‐Activated Mechanoluminescence from Ca1‐xBaxZnOS45Ratiometric Mechanoluminescence of Double‐Activator Doped Phosphatic Phosphors: Color‐Resolved Visualization of Stress‐Sensing and Quantified Evaluation for Sensing Performance58Variable luminnescence chromaticity and energy transfer in CaZnOS: Pr3+, Mn2+ by ultraviolet and blue excitations8Self-recoverable near-infrared mechanoluminescence from ZnS:Mn by controlling manganese clusterization17Near‐Infrared Mechanoluminescence of Cr 3+ Doped Gallate Spinel and Magnetoplumbite Smart Materials135Near-ultraviolet and deep red dual-band mechanoluminescence for color manipulation and biomechanics detection35Alkaline-earth-metal-ion blending enhanced mechanoluminescence of lanthanide ions in MZnOS hosts for stress sensing and anticounterfeiting19Principles, properties, and sensing applications of mechanoluminescence materials61Strengthening the non-pre-irradiated near-infrared mechanoluminescence of CaZnOS:Nd 3+ by Mn 2+ coactivation for biomechanical imaging31NIR Mechanoluminescence from Cr3+ Activated Y3Al5O12 with Intense Zero Phonon line89Light Delivery, Acoustic Read‐Out, and Optical Thermometry Using Ultrasound‐Induced Mechanoluminescence and the Near‐Infrared Persistent Luminescence of CaZnOS:Nd3+44Tuning Oxygen Vacancy in CaZnOS through Cation Substitution for Substantially Enhanced Multimode Luminescence of Mn2+ and Tb3+35Interface-Mediated Mechanoluminescence Enhancement from Heterojunction Phosphors: Experiment and Theory15Transparent Pneumatic Tactile Sensors for Soft Biomedical Robotics14A “Test-to-Treat” Pad for Real-Time Visual Monitoring of Bacterial Infection and On-Site Performing Smart Therapy Strategies78Visualization and Depth Estimation of Inner Crack in High‐Pressure Equipment Based on Organic Mechanochromic Luminescent Materials10Unraveling Mechanoluminescent Mechanisms in Doped CaZnOS Materials: Co‐Mediation of Trap‐Controlled and Non‐Trap‐Controlled Processes55Self-recoverable and cyclically stable near-infrared mechanoluminescence for dual-mode mechanics visualization and biomechanics detection37Cr3+-activated broadband near-infrared mechanoluminescence in garnet compound76A novel long persistent luminescent material CaGeO3:Tb3+ with photo-stimulation properties35Achieving room-temperature self-healing of mechanoluminescent materials by dynamic borate ester bonding23Impact of doping on mechanoluminescence0Mechanoluminescence for infrastructure, health, and safety applications0Synthesis of organic and inorganic mechanoluminescent compounds0A Bifunctional Luminescent Whitening and Sensing Material Based on Photoluminescence and Mechanoluminescence9Efficient blue mechanoluminescence in Eu2+-Activated Sr5(PO4)3Cl for advanced anticounterfeiting with mildew-resistant behavior12Mechanoluminescent functional devices: Developments, applications and prospects92Intense green mechanoluminescence from rare-earth doped gallium gehlenite for multimode anti-counterfeiting9All‐Lanthanide Mechanoluminescence from Transparent Ln‐doped MgF2@Elastomer for Flexible and Stretchable Lighting and Stress Sensing12Near‐Infrared Dual‐Modal Sensing of Force and Temperature in Total Knee Replacement Using Mechanoluminescent Phosphor of Sr 3 Sn 2 O 7 : Nd, Yb33A Review of Mechanoluminescence Based on Quaternary Oxysulfides: Research Progress, Mechanism and Applications14Achieving Tunable Mechanoluminescence in CaZnOS:Tb3+, Sm3+ for Multicolor Stress Sensing10Broadband near-infrared mechanoluminescence in Cr3+ doped Mg3Ga2GeO839Exploring Mechanoluminescence of Zinc Alkaline Earth Metal Oxysulfides from Fundamentals to Advanced Applications26Piezoelectric-induced mechanoluminescence in centrosymmetric Lu3Al5O12: Properties of self-recoverable and tunable near-infrared luminescence19Synthesis of SrZnOSe Crystals with Low Phonon Energy for Enhancing Near‐Infrared Mechanoluminescence42Rare-earth doped upconversion-photopolymerization hydrogel hybrids for in vivo wound healing8Bioengineered nanomaterials for dynamic diagnostics in vivo17Highly Efficient and Thermally Stable Multifunctional Near-Infrared Emitting Phosphors as Light Source for Multiple Applications0Intense and repeatable orange mechanoluminescence of Mn 2+ activated CaGa 4 O 7 for visualized mechanics sensing7Self-Recoverable Broadband Near-Infrared Mechanoluminescence in Cr3+-Doped Scbo3 Endowing Biological Application1Dynamic and Static Stress Sensing Based on Mechanical Quenching Phenomenon From CaZnOS:Cu+7The elastic properties and strain effects on crystal structures and bandgap of MZnOS (M = Ca, Sr): A first-principles study5Multilevel Trap‐Controlled Bright Mechanoluminescence of Sr/CaGa 2 S 4 : Eu 2+ for Stress Sensing Applications23Tuning Mechanoluminescence From Red to Near‐Infrared Light in CaZnOS:Mn 2+10Flexible Optical Fiber Stress/Temperature Dual‐Mode Sensing Based on CaZnOS:Nd,Er42Defects in Inorganic Mechanoluminescent Phosphors: Insights and Impacts30Mechanoluminescence of Bi‐Activated NaYGeO4 Polycrystals and 3D Printed Scaffolds in the NUV/Blue and NIR Spectral Range3Crystal field engineering drives Mn2+ doped CaGeO3 dual-mode luminescence color tunable7Aliovalent doping strategy toward band structure modulation and enhanced mechanoluminescence of CaZnOS: Mn2+4UV/NUV and BW‐I Mechanoluminescence from Bi‐Activated CaY 2 Ge 4 O 12 Polycrystals2Micro‐Strain Responsive Near‐Infrared Mechanoluminescence for Potential Nondestructive Artificial Joint Stress Imaging21Chemistry and Technology of Upconversion Material-Assisted Near-Infrared Photopolymerization: An Emerging Strategy for Photopolymerization7Mechanoluminescence from Visible to Second Near‐Infrared Region Based on Sr 3 Sn 2 O 7 Matrix4Luminescent Materials for Emerging Sensing Technologies7Design of broadband near-infrared mechanoluminescence for effective mechanical sensing in bright field3Highly biocompatible mechanoluminescent Mn-doped CaZnOS and BaZnOS semiconductor compounds for tactile imaging2Smart Semiconductors: An Overview of AZnOS (A= Ca, Sr, Ba) Based Phosphors, Multi‐Stimuli Responsive Luminescence, and Potential Application Prospects12Mechanoluminescence in borate transparent glass-ceramics: Crystallization of SrAl2B2O7 and rare-earth energy transfer in Eu3+/Tb3+ co-doped systems3Broadband near-infrared luminescence of double perovskite Li3Mg2TaO6 phosphor1Layered-tunnel structure enables high defect tolerance for coexistence of anomalous thermal quenching and mechanoluminescence in Sr2ZnSi2O7:Mn2+0Huge Enhancement of Green Persistent Mechanoluminescence of SrAl 2 O 4 :Dy 3+ ‐Eu 2+ by Nd 3+ for Sound‐to‐Light Conversion, Handwriting Visualization, Force Sensing, and Luminescence Thermometry7Self-recoverable broadband near-infrared mechanoluminescence in Cr3+-doped scandium borate endowing biological application4Ultrastable, Self‐Recoverable and Broadband‐Tunable NIR Mechanoluminescence in Cr 3 + ‐Activated Tantalates3Switchable Ultrasound‐Stimulated Luminescence From Mn 2+ ‐Activated Glass and Nanocrystallized Glass Ceramic1Hydrostatic pressure effects on structural stability, elastic properties and band-gap modulation in SrZn2S2O: A first-principles study0Self-powered near-infrared mechanoluminescence for blood oxygen saturation monitoring0Temperature-regulated evolution of carrier transport driving near-infrared persistent luminescence in Fe3+-activated olivine material1Recent advances on zinc- and/or sulfur-containing mechanoluminescent materials and their spectroscopic properties toward diverse applications1Tunable self-recoverable near-infrared mechanoluminescence from platelike strontium-aluminate: SrAl12O19:Cr3+0Near-infrared mechanoluminescence for non-invasive blood analysis0Sound- and force-driven emission of Mn2+-Nd3+ in ZnS/CaZnOS heterostructures enables excitation-light-free imaging and mechanoluminescence thermometry in biological systems2

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  3. Optical and vibrational properties of CaZnOS: The role of intrinsic defects

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  8. Mechanics-induced triple-mode anticounterfeiting and moving tactile sensing by simultaneously utilizing instantaneous and persistent mechanoluminescence

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  9. Near infrared mechanoluminescence from the Nd 3+ doped perovskite LiNbO 3 :Nd 3+ for stress sensors

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  16. Creating visible-to-near-infrared mechanoluminescence in mixed-anion compounds SrZn2S2O and SrZnSO

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  17. Force-induced 1540 nm luminescence: Role of piezotronic effect in energy transfer process for mechanoluminescence

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  36. Self-Reduction-Related Defects, Long Afterglow, and Mechanoluminescence in Centrosymmetric Li2ZnGeO4:Mn2+

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  37. Broadband multimodal emission in Sb-doped CaZnOS-layered semiconductors

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  39. Achieving visible and near-infrared dual-emitting mechanoluminescence in Mn 2+ single-doped magnesium aluminate spinel

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  41. Monitoring cardiovascular disease severity using near-infrared mechanoluminescent materials as a built-in indicator

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  45. Alkaline‐Earth‐Metal‐Ions Blending Enhanced Self‐Activated and Bi3+‐Activated Mechanoluminescence from Ca1‐xBaxZnOS

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  47. Variable luminnescence chromaticity and energy transfer in CaZnOS: Pr3+, Mn2+ by ultraviolet and blue excitations

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  48. Self-recoverable near-infrared mechanoluminescence from ZnS:Mn by controlling manganese clusterization

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  49. Near‐Infrared Mechanoluminescence of Cr 3+ Doped Gallate Spinel and Magnetoplumbite Smart Materials

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  50. Near-ultraviolet and deep red dual-band mechanoluminescence for color manipulation and biomechanics detection

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