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RESEARCH PAPER · Journal of Materials Chemistry C · 2019

Coexistence of self-reduction from Mn 4+ to Mn 2+ and elastico-mechanoluminescence in diphase KZn(PO 3 ) 3 :Mn 2+

Huimin Chen, Liwei Wu, Liwei Wu, Bo Fang, Jikang Jian, Li Wu, Li Wu, Hongwu Zhang, Lirong Zheng, Yongfa Kong, Yi Zhang, Jingjun Xu

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Coexistence of self-reduction from Mn 4+ to Mn 2+ and elastico-mechanoluminescence in diphase KZn(PO 3 ) 3 :Mn 2+OriginalOptical‐Dielectric Duple Bistable Switches: Photoluminescence of Reversible Phase Transition Molecular Material7Ratiometric Optical Thermometer with High Sensitivity Based on Site-Selective Occupancy of Mn2+ Ions in Li5Zn8Al5Ge9O36 under Controllable Synthesis Atmosphere40Crystal structure, luminescence properties and application performance of color tuning Y 2 Mg 2 Al 2 Si 2 O 12 :Ce 3+ ,Mn 2+ phosphors for warm white light-emitting diodes28Interstitial oxygen defect induced mechanoluminescence in KCa(PO 3 ) 3 :Mn 2+53Intense green elastico-mechanoluminescence from KZn(PO3)3:Tb3+24Surface heterostructure induced by TiO2 modification in Li-rich cathode materials for enhanced electrochemical performances57Tuning the Oxidation States of Dopants: A Strategy for the Modulation of Material Photoluminescence Properties11Scrutinizing and Collating the Broadband Photo-Detection Properties of Isotype n-MnO₂/TiO₂ Nanostructure17Localized Charge Accumulation Driven by Li+ Incorporation for Efficient LED Phosphors with Tunable Photoluminescence77Ultrahigh-Energy-Transfer Efficiency and Efficient Mn2+ Red Emission Realized by Structural Confinement in Ca9LiMn(PO4)7:Eu2+,Tb3+ Phosphor40A promising route for developing yellow long persistent luminescence and mechanoluminescence in CaGa 2 O 4 :Pr 3+ ,Li +47Construction of a novel mechanoluminescent phosphor Li 2 MgGeO 4 : x Mn 2+ by defect control32Intrinsic and extrinsic defects build a novel mechanoluminescent phosphor Na 2 MgGeO 4 :Mn 2+52Low-temperature-synthesized Mn-doped Bi 2 Fe 4 O 9 as an efficient electrode material for supercapacitor applications43Mechanoluminescent materials for tactile sensors11Intense and recoverable piezoluminescence in Pr3+-activated CaTiO3 with centrosymmetric structure33Discovering and Dissecting Mechanically Excited Luminescence of Mn2+ Activators via Matrix Microstructure Evolution47Bright and thermal-stable RGB emission realized by Eu2+-Tb3+/Mn2+ energy transfer in Na3SrMg11(PO4)99Designing a Polyphosphate Polymorph of CsMg(PO3)3 as Host Lattice for Preparing Single Mn2+-Oxidation Doped Phosphor in the Open Environment18Self-Reduction-Related Defects, Long Afterglow, and Mechanoluminescence in Centrosymmetric Li2ZnGeO4:Mn2+83Fundamental luminescence properties of Mn 4+ activated Ca 14 Al 10 Zn 6 O 35 phosphor24High-performance ultra-narrow-band green-emitting phosphor LaMgAl 11 O 19 :Mn 2+ for wide color-gamut WLED backlight displays80Oxygen vacancy content drives self-reduction and anti-thermal quenching40Thermal stability and self-reduction of a new red phosphor NaMg(PO 3 ) 3 :Mn 2+17Ternary-Host and Heterojunction Enabled Eye-Visible Elastic Mechanoluminescence from (Ca0.5Sr0.5)ZnOS/xZnS/Mn2+19Luminescence and interstitial-defect-related self-reduction in Mn2+ activated Ba3BP3O12 phosphor13Multiple Color Emission of Mechanoluminescence and Photoluminescence from SrZnSO: Bi3+ for Multimode Anticounterfeiting65Intense Luminescence and Good Thermal Stability in a Mn2+-Activated Mg-Based Phosphor with Self-Reduction27Structural Confinement and Energetic Matching Synergistic Effect toward a High-Energy Transfer Efficiency and a Significant Red Emission Enhancement in a Eu2+,Ln3+ Co-doped Sr9LiMn(PO4)7 Whitlockite Phosphor14Deep-red to NIR mechanoluminescence in centrosymmetric perovskite MgGeO3: Mn2+ for potential dynamic signature anti-counterfeiting124Elucidating the Multisite and Multivalence Nature of Mn Ions in Solids and Predicting Their Optical Transition Properties: A Case Study on a Series of Garnet Hosts14Smart Mechanoluminescent Phosphors: A Review of Strontium‐Aluminate‐Based Materials, Properties, and Their Advanced Application Technologies202Novel high-saturated red-emitting phosphor Sr9(Mg0.5Mn0.5)K(PO4)7: Eu2+ with great quantum efficiency enhancement by La3+ codoping for white LED application16Near-ultraviolet and deep red dual-band mechanoluminescence for color manipulation and biomechanics detection35Cation-defect-induced self-reduction towards efficient mechanoluminescence in Mn 2+ -activated perovskites57Investigation on Photoluminescence and Mechanoluminescence of Single Tb3＋-doped Intense Green Phosphor3Self-reduction of Mn 4+ to Mn 2+ : NaY 9 Si 6 O 26 :Mn 2+ red phosphors with excellent thermal stability for NUV LEDs36A flexible organic mechanoluminophore device46Unique Self‐Reduction of Transitional Metal Ion in a Borate with Planar [BO3]3− Groups12Single Tb3+ ion doped ratiometric mechanoluminescence for tunable stress visualization52Mechanoluminescent property of bis(phenylethynyl)platinum(II) complexes bearing substituted bipyridine and their application for developing rewritable data recording device4Breaking the balance of chemical ratio in ZnAl2O4 to regulate activators and traps for multimode luminescence – A new strategy13Stimulus response of mechanoluminescence of SrAl2O4:Eu,Dy mixed with epoxy resin using uniaxial load8Dynamic optical information encoding strategy of flexible thin films based on Ba2SiO4 phosphor for ultra-long storage time11Awakening dumb Mn2+ mechanoluminescence site to achieve force, temperature and time-domain induced color tuning via trap-assisted energy transfer14Adjusting luminescence properties of ZnAl2O4:Mn2+(Mn4+), Li+ phosphors through cation substitution1Visible-to-Near-Infrared Mechanoluminescence in Bi-Activated Spinel Compounds for Multiple Information Anticounterfeiting35Advanced luminescence applications of 3d3 transition metal ions6Structure Modulation and Charge Transfer in Self‐Reduction Phosphors: A Review18Shifting d ‐band Center: An Overlooked Factor in Broadening Electromagnetic Wave Absorption Bandwidth38Study on luminescence properties and anti-counterfeiting application of Sr3Y2Ge3O12 doped Mn2+ long afterglow materials9Characterization and luminescence properties of CaMgGe2O6: Mn2+ NIR-I mechanoluminescence phosphor2Fast and sensitive determination of trace penicillin G at nanomolar quantity in environmental and food chains using enzyme-catalysed electrochemical sensing composite4High Defect Tolerance Breaking the Design Limitation of Full‐Spectrum Multimodal Luminescence Materials50Prediction and explanation of the self-reduction of Eu3+ → Eu2+ and Mn4+ → Mn2+ using Site Occupancy Theory (SOT)6Tunable orange-deep red photoluminescence in amorphous KZn 1− x Mn x (PO 3 ) 3 phosphors and anti-counterfeiting applications1Unlocking dual Mn 3+ /Mn 4+ emissions in garnet phosphors for WLED and plant growth lighting applications15Spin-State Effect of Tetrahedron-Coordinated Single-Atom Catalysts on CO2 Electroreduction76Self-reduction-induced Mn heterovalent coexistence for Vis–NIR dual-emission16Thermoluminescence characteristics of Mn doped SrAl2O4 phosphor0Crystal field engineering drives Mn2+ doped CaGeO3 dual-mode luminescence color tunable7POST-based prediction of Ce4 + → Ce3+ self-reduction and luminescence enhancement via energy transfer in BaAl2B2O7: Ce, Gd system5Tunable Defect Engineering in NaYF 4 Nanoparticles:Tailoring Trap States for Enhanced NIR-II Bioimaging2Regulation of high pressure on mechanoluminescence: Summary and Prospects0A novel green-emitting phosphor NaLa 9 Ge 6 O 26 : x Tb 3+ with anti-thermal quenching for WLEDs0Mn valence state transition via Li + structure modulation and charge transfer for multi-modal temperature sensing and optical encryption applications1Dual-functional Ca14Zn6Ga10(1-x)O35: Mn2+ phosphor with integrated mechanoluminescence and full-spectrum long persistent luminescence0Harnessing the predictive power of the POST method for spontaneous Mn4+ → Mn2+ and Ce4+ → Ce3+ self-reduction in Sr2P2O7 with experimental validation1Synergistic co-doping strategy in KZn(PO3)3 for multimodal anti-counterfeiting, stress visualization, and self-powered lighting2Defect‐Controlled Photo‐Thermo‐Mechanical Responsive Luminescence in Self‐Activated Phosphor2Peculiarities of the electronic structure of phosphors possessing Mn2+ ions either in octahedral Oh or tetrahedral Td coordination: A first-principles study0On the luminescence enhancement of SrSb2O6:Mn4+ phosphor via Ln3+ (Ln = La, Ce, Gd, Y, Lu) addition for plant growth lighting0

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  2. Ratiometric Optical Thermometer with High Sensitivity Based on Site-Selective Occupancy of Mn2+ Ions in Li5Zn8Al5Ge9O36 under Controllable Synthesis Atmosphere

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  3. Crystal structure, luminescence properties and application performance of color tuning Y 2 Mg 2 Al 2 Si 2 O 12 :Ce 3+ ,Mn 2+ phosphors for warm white light-emitting diodes

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  4. Interstitial oxygen defect induced mechanoluminescence in KCa(PO 3 ) 3 :Mn 2+

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  5. Intense green elastico-mechanoluminescence from KZn(PO3)3:Tb3+

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  6. Surface heterostructure induced by TiO2 modification in Li-rich cathode materials for enhanced electrochemical performances

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  7. Tuning the Oxidation States of Dopants: A Strategy for the Modulation of Material Photoluminescence Properties

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  8. Scrutinizing and Collating the Broadband Photo-Detection Properties of Isotype n-MnO₂/TiO₂ Nanostructure

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  9. Localized Charge Accumulation Driven by Li+ Incorporation for Efficient LED Phosphors with Tunable Photoluminescence

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  13. Intrinsic and extrinsic defects build a novel mechanoluminescent phosphor Na 2 MgGeO 4 :Mn 2+

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  14. Low-temperature-synthesized Mn-doped Bi 2 Fe 4 O 9 as an efficient electrode material for supercapacitor applications

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  17. Discovering and Dissecting Mechanically Excited Luminescence of Mn2+ Activators via Matrix Microstructure Evolution

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  18. Bright and thermal-stable RGB emission realized by Eu2+-Tb3+/Mn2+ energy transfer in Na3SrMg11(PO4)9

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  19. Designing a Polyphosphate Polymorph of CsMg(PO3)3 as Host Lattice for Preparing Single Mn2+-Oxidation Doped Phosphor in the Open Environment

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  20. Self-Reduction-Related Defects, Long Afterglow, and Mechanoluminescence in Centrosymmetric Li2ZnGeO4:Mn2+

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