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RESEARCH PAPER · Advanced Optical Materials · 2021

Time‐Resolved Bright Red to Cyan Color Tunable Mechanoluminescence from CaZnOS: Bi 3+ , Mn 2+ for Anti‐Counterfeiting Device and Stress Sensor

Yun‐Ling Yang, Xuechun Yang, Jia‐Yong Yuan, Ting Li, Yuting Fan, Lin Wang, Zheng Deng, Qianli Li, Dongyun Wan, Jing‐Tai Zhao, Zhijun Zhang

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Time‐Resolved Bright Red to Cyan Color Tunable Mechanoluminescence from CaZnOS: Bi 3+ , Mn 2+ for Anti‐Counterfeiting Device and Stress SensorOriginalMultiple Color Emission of Mechanoluminescence and Photoluminescence from SrZnSO: Bi3+ for Multi-mode Anti-counterfeiting1Enabling narrowband cyan photoluminescence and long-lasting ultraviolet-A persistent luminescence in Bi 3+ single-doped Sr 3 Sc 2 Ge 3 O 12 phosphors by selective site occupation48Significant enhancement of scintillation performance by inducing oxygen vacancies in alkali metal ion (A + = Li + , Na + , K + )-incorporated (Lu, Sc)BO 3 :Ce2Stress memory for the visualization detection of complicated mechanical structures via trap structure manipulation14Temporal @ Spatial Anti-Counterfeiting with Mn2+/Bi3+/Er3+ Doped Baznos Phosphors61Ternary-Host and Heterojunction Enabled Eye-Visible Elastic Mechanoluminescence from (Ca0.5Sr0.5)ZnOS/xZnS/Mn2+19Design of Ratiometric Dual‐Emitting Mechanoluminescence: Lanthanide/Transition‐Metal Combination Strategy63Tunable luminescent chromaticity of CaZnOS: Bi3+, Eu3+ with white emitting based on energy transfer29Interfacial triboelectrification-modulated self-recoverable and thermally stable mechanoluminescence in mixed-anion compounds106Multiple Color Emission of Mechanoluminescence and Photoluminescence from SrZnSO: Bi3+ for Multimode Anticounterfeiting65Dynamic organic mechanoluminescence (ML): The roles of Mechano-induced conformational isomer and energy transfer from ML to photoluminescence (PL)35Sensitive mechanoluminescence from Eu2+, Tm3+ co-doped Sr3Al2O5Cl2 phosphors21Alkaline‐Earth‐Metal‐Ions Blending Enhanced Self‐Activated and Bi3+‐Activated Mechanoluminescence from Ca1‐xBaxZnOS45Magnetic properties and photocatalytic activity of Bi1-xSmxFe1-yNiyO3 nanoparticles for methyl red degradation2Multi-color mechano-luminescence of LaGaO3:Sm3+,Tb3+ via trap sharing for anti-counterfeiting and encryption30Ratiometric Mechanoluminescence of Double‐Activator Doped Phosphatic Phosphors: Color‐Resolved Visualization of Stress‐Sensing and Quantified Evaluation for Sensing Performance58Variable luminnescence chromaticity and energy transfer in CaZnOS: Pr3+, Mn2+ by ultraviolet and blue excitations8Mechanoluminescence ratiometric thermometry via MgF 2 :Tb 3+17A multi-color persistent luminescent phosphor Ca3Al2Ge3O12:Re3+ (Re3+=Tb3+, Pr3+, Dy3+) for dynamic anti-counterfeiting34Bismuth‐Activated Persistent Phosphors65Opto-mechano-thermo-sensitive allochroic luminescence based on coupled dual activators in tantalate towards multidimensional stimulus sensing12Alkaline-earth-metal-ion blending enhanced mechanoluminescence of lanthanide ions in MZnOS hosts for stress sensing and anticounterfeiting19Cation-defect-induced self-reduction towards efficient mechanoluminescence in Mn 2+ -activated perovskites57Color-tunable emissions realized by Tb 3+ to Eu 3+ energy transfer in ZnGdB 5 O 10 under near-UV excitation9Principles, properties, and sensing applications of mechanoluminescence materials61Recent advances in the design of afterglow materials: mechanisms, structural regulation strategies and applications475Significantly enhanced mechanoluminescence from Nb 5+ co-doped ZrO 2 :Sm 3+ via a high valence ion doping strategy11Site occupation and upconversion process enabled multicolor emission in a Gd 3 GaO 6 :Bi 3+ ,Er 3+ phosphor for quad-mode anti-counterfeiting23Strengthening the non-pre-irradiated near-infrared mechanoluminescence of CaZnOS:Nd 3+ by Mn 2+ coactivation for biomechanical imaging31Trap-regulated highly efficient mechanoluminescence and persistent mechanoluminescence of Ca 2 MgSi 2 O 7 :Eu 2+41Recent Progress in Inorganic Afterglow Materials: Mechanisms, Persistent Luminescent Properties, Modulating Methods, and Bioimaging Applications143Highly-efficient cyan-emitting phosphor enabling high-color-quality lighting and transparent anticounterfeiting64Environmentally Stable and Self-Recovery Flexible Composite Mechanical Sensor Based on Mechanoluminescence52Ratiometric mechanoluminescence in LiSrPO4:Eu2+/Eu3+ for stress sensing: Dopant concentration dependent sensitivity15Stress-Induced Photoluminescence Change of Monolayer Nanosheet Prepared by Delamination of Aurivillius-Phase Layered Perovskite8Stress‐Triggered Mechanoluminescence in ZnO‐Based Heterojunction for Flexible and Stretchable Mechano‐Optics70Light Delivery, Acoustic Read‐Out, and Optical Thermometry Using Ultrasound‐Induced Mechanoluminescence and the Near‐Infrared Persistent Luminescence of CaZnOS:Nd3+44Pressure- and Rate-Dependent Mechanoluminescence with Maximized Efficiency and Tunable Wavelength in ZnS: Mn2+, Eu3+28Interface-Mediated Mechanoluminescence Enhancement from Heterojunction Phosphors: Experiment and Theory15Mechanically induced photons from ultraviolet-C to near-infrared in Tm3+-doped MgF28Mechanoluminescence and Photoluminescence Heterojunction for Superior Multimode Sensing Platform of Friction, Force, Pressure, and Temperature in Fibers and 3D‐Printed Polymers186Strain-sensitive mechanoluminescence with high stability and self-recovery toward stretchable strain sensor17Multicolor Mechanoluminescence in Sr2Ga2GeO7: Pr3+ for Stress Sensing and Anticounterfeiting62Unraveling Mechanoluminescent Mechanisms in Doped CaZnOS Materials: Co‐Mediation of Trap‐Controlled and Non‐Trap‐Controlled Processes55Multicolor luminescence from CaZnOS: Bi3+, Eu3+ for stress sensing and multimode anti-counterfeiting29Inkjet‐Printed and Nanopatterned Photonic Phosphor Motifs with Strongly Polarized and Directional Light‐Emission4Stress‐Induced Multi‐Stimulus‐Responsive Mechanoluminescence in Mn2+ Doped Double Perovskite Compound34Unusual Thermal Quenching of Photoluminescence from an Organic–Inorganic Hybrid [MnBr 4 ] 2− ‐based Halide Mediated by Crystalline–Crystalline Phase Transition79Unusual Thermal Quenching of Photoluminescence from an Organic–Inorganic Hybrid [MnBr4]2−‐based Halide Mediated by Crystalline–Crystalline Phase Transition10Achieving room-temperature self-healing of mechanoluminescent materials by dynamic borate ester bonding23High-temperature dynamic luminescence of MgGa2O4: Tb3+, Er3+ phosphors for advanced anti-counterfeiting and information encryption24Isolated Coordination Polyhedron Confinement in ABP2O7:Mn2+ (A = Ba/Sr; B = Mg/Zn)5Defect-management-induced multi-stimulus-responsive mechanoluminescence in Mn2+ doped gallate compound50Multi-mode mechanoluminescence of fluoride glass ceramics from rigid to flexible media toward multi-scene mechanical sensors22Designing Ratiometric Mechanoluminescence via Threshold Manipulation in Sandwich Structures15Mechanoluminescence for display devices1Novel dual spectral conversion via Eu 2+ , Cu + -coactivated core–shell-structured CaS@CaZnOS phosphors for efficient photosynthesis of plants10Efficient blue mechanoluminescence in Eu2+-Activated Sr5(PO4)3Cl for advanced anticounterfeiting with mildew-resistant behavior12Mechanoluminescent functional devices: Developments, applications and prospects92Intense green mechanoluminescence from rare-earth doped gallium gehlenite for multimode anti-counterfeiting9The determining role of stacking fault in the mechanoluminescence properties of ZnS: Mn thin films11Structural and optical properties of Cr ion-doped near-infrared long persistent luminescence silicogermanate phosphors with broad emission bands21A promising route for developing green phosphor with mechanoluminescence and long persistent luminescence in Sr2Ga2GeO7: Tb3+12Highly efficient mechanoluminescence of SrAl2–Y O4:Eu2+,Dy3+ via trap regulation for dynamic signature anticounterfeiting13A Review of Mechanoluminescence Based on Quaternary Oxysulfides: Research Progress, Mechanism and Applications14Direct recording and reading of mechanical force by afterglow evaluation of multi-piezo mechanoluminescent material Li0.12Na0.88NbO3 on well-designed morphotropic phase boundary7Piezochromic Behavior of 2,4,6‐Triphenylpyrylium Tetrachloroferrate9Solvothermal Treatment of Micron-Sized Commercial SrAl2O4:Eu2+, Dy3+ Phosphors and One-Step Preparation of Nanophosphors for Fingerprint Imaging7Intense NIR mechanoluminescence from Al3+-regulated MgGa2O4: Cr3+44Controllable Modulation of Trapped Carriers in Mechano/Thermo Dual‐Responsive Particles for Advanced Stress‐Encoded Information Storage27Mn-Doped Ca14Mg4Ga12O36 with the Tululite Mineral Structure for Color-Tunable Emission14Awakening dumb Mn2+ mechanoluminescence site to achieve force, temperature and time-domain induced color tuning via trap-assisted energy transfer14Multi-color and multi-mode luminescence tuning in persistent phosphors by trap engineering6Amorphous to Crystalline Phase Transformation Enables Tunable Persistent Luminescence for Multi‐Mode Optical Information Storage53Visible-to-Near-Infrared Mechanoluminescence in Bi-Activated Spinel Compounds for Multiple Information Anticounterfeiting35Probing multifunctional applications of CeO2:Pr3+ phosphor for optical thermometry, flexible displays, cheiloscopy, anti-counterfeiting applications24Effect of Polymer Encapsulation on the Mechanoluminescence of Mn2+-Doped CaZnOS7Characterization methods for mechanoluminescent materials10A multi-dimensional anti-counterfeiting nanocomposite based on fluorescent CDs and Eu-MOFs with dual function for continuous detection of Cu2+ and Bacillus anthracis9Improvement in mechanoluminescence performance and implementation of dual-mode photoluminescence based on Bi3+ ion non-intrinsic defect control strategy10Design of Visualized Ratiometric Mechanoluminescent Materials for High‐Resolution Pressure Sensing35Multicolor Mechanoluminescence From Lu3Al2Ga3O12: Tb, Eu for Stress and Temperature Visual Sensing22Exploring Mechanoluminescence of Zinc Alkaline Earth Metal Oxysulfides from Fundamentals to Advanced Applications26X-ray/γ-ray/Ultrasound-Activated Persistent Luminescence Phosphors for Deep Tissue Bioimaging and Therapy25Synthesis of SrZnOSe Crystals with Low Phonon Energy for Enhancing Near‐Infrared Mechanoluminescence42Trap Assisted Dynamic Mechanoluminescence Toward Self‐Referencing and Visualized Strain Sensing48Highly efficient and thermally stable cyan-emitting ZnS/ZnO phosphors for full-visible-spectrum LED lighting12Recent advances in multimodal mechanoluminescent sensors enabled by nanostructure design8Consistency of simulated stress distribution with experimental mechanoluminescent intensity distribution facilitating stress visualization device design4Oscillatory mechanoluminescence of Mn2+-doped SrZnOS in dynamic response to rapid compression26Stress Distributions and Luminescent Responses of Mechanoluminescent Cylinders with Various Sizes and Loading Paths2First-Principles Understanding of Mono- and Dual-Emissions in AZnOS:Bi3+ (A = Ba, Ca) Phosphors3Tunable Photoluminescence of LiTaO 3 : Tb 3+ , Sm 3+ for Dynamic Multimode Optical Anti‐Counterfeiting5Multi-color Ca3Ga4O9: Pr3+ phosphors for high-security-level optical information storage6Persistence Luminescence and Mechanoluminescence in Er3+/Eu2+ Co-Doped SrS/SrZnSO Composites4Self‐Recovering Multicolor Calcium Phosphate Mechanoluminescent Materials for Wearable Skin and Biomedical Applications12Multifunctional mechanoluminescent material with enhanced interfacial synergistic effects: 2SrZn2S2O/ZnS heterojunction2Site substitution and tunable luminescence of Eu2+ activated Ba1-Sr LiZn3(PO4)3 phosphor for plant growth6Multi-stimulated far-UVC luminescence for solar-blind imaging30Er/Mn Co‐Activated SrZnOS Multimodal Luminescence Materials for Optical Sensing2Cr 3+ ‐Activated Tunable Near‐Infrared Mechanoluminescence Materials for Potential Water Pollutant Monitoring10Non-pre-irradiation multicolor mechanoluminescence in piezoelectric Ca3Ga4O9 for secure channel encryption2Multimode emission from Bi3+ induced oxygen vacancy engineering in spinel-type phosphor for versatile optical applications6Sr2+-modulated Y3Al5O12: Eu phosphors with high-efficiency mechanoluminescence and color-tunable photoluminescence for multimodal anti-counterfeiting2Luminescent Materials for Emerging Sensing Technologies7Quantifying the Coupling between Mechanoluminescence Intensity and Elastic Strain Energy Power Density1Properties of Ultrasound‐Induced Luminescence of LiTaO 3 : Pr at kHz and MHz Frequencies3Lamellar‐Cleavage‐Induced Triboluminescence in Discrete Chiral Complexes with Lanthanides2Mg4Ga8Ge2O20:Cr3+, Mn2+ phosphors with multicolor persistent luminescence for advanced anti-counterfeiting applications2Dynamic Stimulus‐Responsive Optical Encoding: Principles, Methods, and Multidimensional Applications7Turning on Mn2+ luminescence through linear defect clusters: Harvesting mechanoluminescence and multimodal emission2Regulation of high pressure on mechanoluminescence: Summary and Prospects0Recent Progress in Mechanoluminescence for Multi‐Dimensional Stress Monitoring6Huge Enhancement of Green Persistent Mechanoluminescence of SrAl 2 O 4 :Dy 3+ ‐Eu 2+ by Nd 3+ for Sound‐to‐Light Conversion, Handwriting Visualization, Force Sensing, and Luminescence Thermometry7Tb3+-activated intense mechanoluminescence materials for potential automotive accident alert sensing1Mechanoluminescent Probing of Elastic Moduli in CaZnOS:Mn 2+ , Bi 3+ Composites: Effects of Matrix Modulus and Filler Loading0Red/near-infrared emitting phosphors based on Bi 3+ ions: recent advances, materials design, and applications3Research progress in ratiometric mechanoluminescent materials0Phase‐Manipulated Calcium Borate‐Based Multicolor Mechanoluminescence9Enhanced mechanoluminescence in Pr3+-doped LiNbO3-LiTaO3 ferroelectric phosphors0Dual-functional Ca14Zn6Ga10(1-x)O35: Mn2+ phosphor with integrated mechanoluminescence and full-spectrum long persistent luminescence0Dual-functional application of Ca2GdTaO6: Bi3+, Ln3+ (Ln = Eu, Sm, Dy) phosphors in optical thermometry and anti-counterfeiting2Color‐Resolved Stress Sensing Visualization Based on Ratiometric Mechanoluminescence: A Universal Strategy via Radiative Energy Transfer1Predicting and achieving self-recoverable mechanoluminescence based on contact electrification3Temperature and stress dual-function visual sensing based on Y3GaO6:Tb3+/Eu3+ multicolor mechanoluminescent material2Recent advances on zinc- and/or sulfur-containing mechanoluminescent materials and their spectroscopic properties toward diverse applications1Tm 3+ Activated Dual‐Emission Ratiometric Mechanoluminescence With Energy Transfer‐Induced Dual‐Peak Ratio Change for Secure Sensing and Encryption0Ultra-broadband visible ZnO:Mn phosphors: Photoluminescence properties and Warm-WLED applications0Mechanically driven multimodal luminescence in SrZnOS:Pr3+,Sm3+ for anti-counterfeiting and visual thermometry0Investigation of the Chemical Interactions in the Na2MoO4-Glycerol-ZrOCl2-ErCl3-H2O System and Luminescent Characteristics of the Resulting Solid Precipitate0Self-recoverable multicolor mechanoluminescence in LaBO3-based composites toward self-powered optical platforms and multimode anticounterfeiting0Stimuli‐Selective Charge Trapping in Cs 3 Cd 2 Cl 7 :Mn 2+ Perovskite Enabling Sensitive X‐Ray Imaging and Force Sensing1Deep traps determining long-term sustainable mechanoluminescence for 16-day continuous real time monitoring of mutation load0

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  39. Interface-Mediated Mechanoluminescence Enhancement from Heterojunction Phosphors: Experiment and Theory

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  41. Mechanoluminescence and Photoluminescence Heterojunction for Superior Multimode Sensing Platform of Friction, Force, Pressure, and Temperature in Fibers and 3D‐Printed Polymers

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  42. Strain-sensitive mechanoluminescence with high stability and self-recovery toward stretchable strain sensor

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