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RESEARCH PAPER · Inorganic Chemistry · 2017

Ba5Zn4(BO3)6: A Nonlinear-Optical Material with Reinforced Interlayer Connections and Large Second-Harmonic-Generation Response

Meihong Duan, Mingjun Xia, Rukang K. Li

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Ba5Zn4(BO3)6: A Nonlinear-Optical Material with Reinforced Interlayer Connections and Large Second-Harmonic-Generation ResponseOriginalBa 2 ZnSc(BO 3 ) 3 and Ba 4 Zn 5 Sc 2 (BO 3 ) 8 : first examples of borates in the Zn–Sc–B–O system featuring special structure configurations15Flexible coordination of Pb atoms and variable zinc–borate frameworks to construct three Pb 5 Zn 4 B 6 O 18 polymorphs8LiCs 2 La(BO 3 ) 2 and Li 3 K 9 La 3 (BO 3 ) 7 : new mixed alkali metal lanthanum borates with three-dimensional open frameworks and short cut-off edges10A Member of Fluorooxoborates: Li2Na0.9K0.1B5O8F2 with the Fundamental Building Block B5O10F2 and a Short Cutoff Edge27The role of cations in second-order nonlinear optical materials based on π-conjugated [BO 3 ] 3− groups195Beryllium-Free Nonlinear-Optical Crystals A 3 Ba 3 Li 2 Ga 4 B 6 O 20 F (A = K and Rb): Members of the Sr 2 Be 2 (BO 3 ) 2 O Family with a Strong Covalent Connection between the ∞ 2 [Li 2 Ga 4 B 6 O 20 F] 9– Double Layers27BaLiZn3B3O9: a Mixed‐Cation KBe2BO3F2‐Type Zinc‐Borate with a (LiZn3B3O9)∞ Network9Mo6+ Cation Enrichment of the Structure Chemistry of Iodates: Syntheses, Structures, and Calculations of Ba(MoO2)2(IO3)4O, Ba3[(MoO2)2(IO3)4O(OH)4]·2H2O, and Sr[(MoO2)6(IO4)2O4]·H2O24Hybridization-activated new deep ultraviolet transparent nonlinear optical material Ba 11 [Al(PO 4 ) 4 ](P 2 O 7 )(PO 4 ) 3 with balanced overall performance and parsimony-forbidden structure23Two Polar Molybdenum(VI) Iodates(V) with Large Second-Harmonic Generation Responses67Research and Development of Zincoborates: Crystal Growth, Structural Chemistry and Physicochemical Properties20Hydroisocyanurates X 2 Y(H 2 C 3 N 3 O 3 ) 4 ·4H 2 O (X = K, Cs; Y = Zn, Cd) with large birefringence stemming from π-conjugated (H 2 C 3 N 3 O 3 ) − anions28Synthesis, Crystal Structure, and Characterization of a Noncentrosymmetric Sulfate Cs2Ca2(SO4)320Aliovalent-substituted synthesis for a non-centrosymmetric phosphate with enhanced nonlinear-optical response5Borates: A Rich Source for Optical Materials1089Ba 2.5 Pb 1.5 B 12 O 22 : structural transformation from a centrosymmetric to a noncentrosymmetric space group by introducing Pb into Ba 2 B 6 O 117From K[ZnBP2O8] to K[(Zn0.5Al0.5)2P2O8]: Substitution-Induced Microporous Zincoaluminophosphate with a Congruent-Melting Behavior5The First Mixed Calcium Zinc Borate with a Flexible [B8O17] Fundamental Building Block and Short UV Cutoff Edge7Effect of Zinc Fluoride addition on structure of barium Borate glasses for nonlinear optical applications27Na 3 AEZn 2 B 3 O 9 (AE = Mg, Ca): two new short-wave ultraviolet beryllium-free Sr 2 Be 2 B 2 O 7 -type zincoborates designed by chemical cosubstitution9NaZnAlP2O8: A New KZnBP2O8‐Type Congruent‐Melting Microporous Zincoaluminophosphate Accessed by Substitution Design Strategy and Molten Salt Method2NaK5Zn2(B5O10)2 and β-K3ZnB5O10: Two Zincoborates with Deep-UV Cutoff Edge9Ba6Zn6(B3O6)6(B6O12): Barium Zinc Borate Contains π-Conjugated [B3O6]3– Anions and [B6O12]6– Anion with Edge-Sharing BO4 Tetrahedra36Exploring Short-Wavelength Phase-Matching Nonlinear Optical Crystals by Employing KBe2BO3F2 as the Template95Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration0Mg assists in modulating the dimensionalities of the anionic frameworks of borates1Two Acentric Zn-Based l -Tartrates with Moderate Second Harmonic Generation Responses and Large Birefringence6Unraveling Superior Elasticity and Controlled Thermal Expansion in Trigonal MBO3 (M=Al, Ga) with Isolated [BO3] Group: A Theoretical Perspective9(C5H12N2S)Hg(NO3)2: A Mercury Nitrate Nonlinear Optical Crystal Motivated by Heteroatom Coordination Strategy9A Promising Short-Wave UV NLO Crystal with an Optimized KBBF-like Structure and Well-Balanced Properties Achieved via a Chemical Substitution Strategy6Four zinc borates: From acentric chain to centric porous layer0Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 42Two transition metal borates built from unprecedented {B11} clusters with nonlinear optical properties0

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  1. Ba 2 ZnSc(BO 3 ) 3 and Ba 4 Zn 5 Sc 2 (BO 3 ) 8 : first examples of borates in the Zn–Sc–B–O system featuring special structure configurations

    Inorganic Chemistry Frontiers · 2018-01-01

    Yanna Chen, Min Zhang, Cong Hu, Zhihua Yang, Shilie Pan

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  2. Flexible coordination of Pb atoms and variable zinc–borate frameworks to construct three Pb 5 Zn 4 B 6 O 18 polymorphs

    Inorganic Chemistry Frontiers · 2018-01-01

    Xiaobo Pan, Hongping Wu, Ming Wen, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  3. LiCs 2 La(BO 3 ) 2 and Li 3 K 9 La 3 (BO 3 ) 7 : new mixed alkali metal lanthanum borates with three-dimensional open frameworks and short cut-off edges

    Dalton Transactions · 2018-01-01

    Ruru Ma, Yun Mo Yang, Cong Hu, Xiaoyu Dong, Zhihua Yang, Shilie Pan

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  4. A Member of Fluorooxoborates: Li2Na0.9K0.1B5O8F2 with the Fundamental Building Block B5O10F2 and a Short Cutoff Edge

    Inorganic Chemistry · 2018-01-02

    Shujuan Han, Ying Wang, Bingbing Zhang, Zhihua Yang, Shilie Pan

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  5. The role of cations in second-order nonlinear optical materials based on π-conjugated [BO 3 ] 3− groups

    Coordination Chemistry Reviews · 2018-04-06

    Yaoguo Shen, Sangen Zhao, Junhua Luo

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  6. Beryllium-Free Nonlinear-Optical Crystals A 3 Ba 3 Li 2 Ga 4 B 6 O 20 F (A = K and Rb): Members of the Sr 2 Be 2 (BO 3 ) 2 O Family with a Strong Covalent Connection between the ∞ 2 [Li 2 Ga 4 B 6 O 20 F] 9– Double Layers

    Inorganic Chemistry · 2018-04-20

    Xianghe Meng, Fei Liang, Mingjun Xia, Zheshuai Lin

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  7. BaLiZn3B3O9: a Mixed‐Cation KBe2BO3F2‐Type Zinc‐Borate with a (LiZn3B3O9)∞ Network

    European Journal of Inorganic Chemistry · 2018-06-20

    Meihong Duan, Mingjun Xia, Rukang K. Li

    Read original paper ↗ ·

  8. Mo6+ Cation Enrichment of the Structure Chemistry of Iodates: Syntheses, Structures, and Calculations of Ba(MoO2)2(IO3)4O, Ba3[(MoO2)2(IO3)4O(OH)4]·2H2O, and Sr[(MoO2)6(IO4)2O4]·H2O

    Inorganic Chemistry · 2018-07-19

    Yahui Li, Hongping Wu, Bingbing Zhang, Zhihua Yang, Guopeng Han, Shilie Pan

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  9. Hybridization-activated new deep ultraviolet transparent nonlinear optical material Ba 11 [Al(PO 4 ) 4 ](P 2 O 7 )(PO 4 ) 3 with balanced overall performance and parsimony-forbidden structure

    Journal of Materials Chemistry C · 2019-01-01

    Zhi Gang Fang, Bing‐Ping Yang, Chun‐Li Hu, Jiang‐Gao Mao

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  10. Two Polar Molybdenum(VI) Iodates(V) with Large Second-Harmonic Generation Responses

    Chemistry of Materials · 2019-03-29

    Yahui Li, Guopeng Han, Hongwei Yu, Hao Li, Zhihua Yang, Shilie Pan

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  11. Research and Development of Zincoborates: Crystal Growth, Structural Chemistry and Physicochemical Properties

    Molecules · 2019-07-30

    Yanna Chen, Min Zhang, Miriding Mutailipu, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  12. Hydroisocyanurates X 2 Y(H 2 C 3 N 3 O 3 ) 4 ·4H 2 O (X = K, Cs; Y = Zn, Cd) with large birefringence stemming from π-conjugated (H 2 C 3 N 3 O 3 ) − anions

    CrystEngComm · 2020-01-01

    Kaijin Kang, Xianghe Meng, Fei Liang, Jian Tang, Tixian Zeng, Wenlong Yin, Zheshuai Lin, Mingjun Xia

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  13. Synthesis, Crystal Structure, and Characterization of a Noncentrosymmetric Sulfate Cs2Ca2(SO4)3

    European Journal of Inorganic Chemistry · 2020-02-24

    Yaoguo Shen, Xiaoling Xue, Wenyuan Tu, Zhiqun Liu, Renwen Yan, Hong Zhang, Junrong Jia

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  14. Aliovalent-substituted synthesis for a non-centrosymmetric phosphate with enhanced nonlinear-optical response

    Journal of Solid State Chemistry · 2020-04-08

    Yaoguo Shen, Zhiqun Liu, Hualiang Yu, Bi‐Cheng Zhou

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  15. Borates: A Rich Source for Optical Materials

    Chemical Reviews · 2020-12-14

    Miriding Mutailipu, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  16. Ba 2.5 Pb 1.5 B 12 O 22 : structural transformation from a centrosymmetric to a noncentrosymmetric space group by introducing Pb into Ba 2 B 6 O 11

    Dalton Transactions · 2021-01-01

    Kaitong Liu, Jian Wei Han, Shilie Pan

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  17. From K[ZnBP2O8] to K[(Zn0.5Al0.5)2P2O8]: Substitution-Induced Microporous Zincoaluminophosphate with a Congruent-Melting Behavior

    Inorganic Chemistry · 2021-06-01

    Meihong Duan, Bo Kong, Xu-Kui Yang, Yuxin Li, Peixin Ma, Xinyou An, Tixian Zeng, Da-Bin Qin, Zhi Gang Fang

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  18. The First Mixed Calcium Zinc Borate with a Flexible [B8O17] Fundamental Building Block and Short UV Cutoff Edge

    Chemistry - A European Journal · 2021-06-21

    Wenbin Zhang, Siru Guo, Shujuan Han, Zhihua Yang, Shilie Pan

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  19. Effect of Zinc Fluoride addition on structure of barium Borate glasses for nonlinear optical applications

    Optical Materials · 2021-09-30

    M. M. Neethish, Jitendra Nath Acharyya, Gaddam Vijaya Prakash, V.V. Ravi Kanth Kumar

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  20. Na 3 AEZn 2 B 3 O 9 (AE = Mg, Ca): two new short-wave ultraviolet beryllium-free Sr 2 Be 2 B 2 O 7 -type zincoborates designed by chemical cosubstitution

    Inorganic Chemistry Frontiers · 2022-01-01

    Zhi Gang Fang, Chun‐Li Hu, Wen‐Tong Chen, Jiang‐Gao Mao

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  21. NaZnAlP2O8: A New KZnBP2O8‐Type Congruent‐Melting Microporous Zincoaluminophosphate Accessed by Substitution Design Strategy and Molten Salt Method

    European Journal of Inorganic Chemistry · 2022-08-01

    Meihong Duan, Peixin Ma, Chaoqian Li, Wenhua Ma, Baichuan Wang, Ling Jia, Yanbo Li, Jun Li, Zhi Gang Fang

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  22. NaK5Zn2(B5O10)2 and β-K3ZnB5O10: Two Zincoborates with Deep-UV Cutoff Edge

    Inorganic Chemistry · 2022-10-10

    Wenjuan Ma, Jie Zhang, Feng Yu, Bin Dai

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  23. Ba6Zn6(B3O6)6(B6O12): Barium Zinc Borate Contains π-Conjugated [B3O6]3– Anions and [B6O12]6– Anion with Edge-Sharing BO4 Tetrahedra

    Inorganic Chemistry · 2022-10-28

    Weijie Xie, Zhi Gang Fang, Jiang‐Gao Mao

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  24. Exploring Short-Wavelength Phase-Matching Nonlinear Optical Crystals by Employing KBe2BO3F2 as the Template

    ACS Central Science · 2022-11-11

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  25. Discovery of SrZn 2 B 6 O 12 with an unprecedented quadruple-layered configuration

    New Journal of Chemistry · 2023-01-01

    Xiangyu Long, Yan An Lv, Xueyan Wu

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  26. Mg assists in modulating the dimensionalities of the anionic frameworks of borates

    Dalton Transactions · 2023-01-01

    Qianzhen Zhang, Feixiang Wang, Xifa Long, Yun Mo Yang

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  27. Two Acentric Zn-Based l -Tartrates with Moderate Second Harmonic Generation Responses and Large Birefringence

    Inorganic Chemistry · 2024-03-14

    Ting Yu, Jiahao Wan, Jingye Yang, Xiaokang Luo, Man Xie, Lehui Liu, Hongming Liu

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  28. Unraveling Superior Elasticity and Controlled Thermal Expansion in Trigonal MBO3 (M=Al, Ga) with Isolated [BO3] Group: A Theoretical Perspective

    European Journal of Inorganic Chemistry · 2024-07-24

    Dingfeng Yang, Yurou Tang, Hongxu Xia, Keman Yin, Yuanyuan Li, Yuanyuan Li

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  29. (C5H12N2S)Hg(NO3)2: A Mercury Nitrate Nonlinear Optical Crystal Motivated by Heteroatom Coordination Strategy

    Inorganic Chemistry · 2024-07-31

    Yi‐Lei Lv, Liang Ma, Wenlong Liu, Sheng‐Ping Guo, Ru‐Ling Tang

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  30. A Promising Short-Wave UV NLO Crystal with an Optimized KBBF-like Structure and Well-Balanced Properties Achieved via a Chemical Substitution Strategy

    Inorganic Chemistry · 2025-07-02

    Shuaifeng Li, Mengru Liu, Peng Zhao, Huijian Zhao, Ning Ye, Zhanggui Hu, Conggang Li

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  31. Four zinc borates: From acentric chain to centric porous layer

    Chinese Journal of Structural Chemistry · 2025-10-22

    Juan Chen, Jin-Ni Zhao, Guo‐Yu Yang

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  32. Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 4

    Inorganic Chemistry · 2026-02-05

    Kaitong Liu, Yuan Rao, Zhaoxue Li, Shihang Zhou, Zhizhong Zhang, Yanhui Zhang

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  33. Two transition metal borates built from unprecedented {B11} clusters with nonlinear optical properties

    Science China Chemistry · 2026-09-22

    Juan Chen, Guo-Yu Yang

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