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RESEARCH PAPER · Inorganic Chemistry · 2017

Unraveling the Magnesium-Ion Intercalation Mechanism in Vanadium Pentoxide in a Wet Organic Electrolyte by Structural Determination

Sung‐Chul Lim, Jinhee Lee, Hunho H. Kwak, Jongwook W. Heo, Munseok S. Chae, Docheon Ahn, Yun Hee Jang, Hochun Lee, Seung‐Tae Hong

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Unraveling the Magnesium-Ion Intercalation Mechanism in Vanadium Pentoxide in a Wet Organic Electrolyte by Structural DeterminationOriginalElectrochemical Intercalation of Mg 2+ into Anhydrous and Hydrated Crystalline Tungsten Oxides71A critical review of cathodes for rechargeable Mg batteries591Aqueous rechargeable Zn-ion batteries: an imperishable and high-energy Zn 2 V 2 O 7 nanowire cathode through intercalation regulation364Can Multielectron Intercalation Reactions Be the Basis of Next Generation Batteries?108An artificial interphase enables reversible magnesium chemistry in carbonate electrolytes481Ammonium Vanadium Bronze (NH 4 V 4 O 10 ) as a High-Capacity Cathode Material for Nonaqueous Magnesium-Ion Batteries162Solvent Effects on the Reversible Intercalation of Magnesium‐Ions into V2O5 Electrodes55On the strange case of divalent ions intercalation in V2O592Water-Activated VOPO4 for Magnesium Ion Batteries165Unveiling the Intercalation Mechanism in Fe2(MoO4)3 as an Electrode Material for Na-Ion Batteries by Structural Determination25H2V3O8 as a High Energy Cathode Material for Nonaqueous Magnesium-Ion Batteries96Effect of water in electrolyte on the Ca2+ insertion/extraction properties of V2O568Anion Effects on Cathode Electrochemical Activity in Rechargeable Magnesium Batteries: A Case Study of V2O563A room temperature multivalent rechargeable iron ion battery with an ether based electrolyte: a new type of post-lithium ion battery47Preparation and electrochemical performance of VO 2 (A) hollow spheres as a cathode for aqueous zinc ion batteries37Rhombohedral Potassium–Zinc Hexacyanoferrate as a Cathode Material for Nonaqueous Potassium-Ion Batteries54First-principles investigation of Sn doping on the geometric and electronic structures of V2O56Intercalation of Magnesium into a Layered Vanadium Oxide with High Capacity100Ab initio modeling and design of vanadia-based electrode materials for post-lithium batteries10Methods and Protocols for Reliable Electrochemical Testing in Post-Li Batteries (Na, K, Mg, and Ca)141Recent Progress on Layered Cathode Materials for Nonaqueous Rechargeable Magnesium Batteries80High Potassium Storage Capability of H 2 V 3 O 8 in a Non‐Aqueous Electrolyte16Interlayer separation in hydrogen titanates enables electrochemical proton intercalation57Valence-to-core X-ray emission spectroscopy of vanadium oxide and lithiated vanadyl phosphate materials18Dual Effect of Structure and Hydration on Magnesium-Ion Insertion into Electrodeposited V 2 O 5 Thin Films12On battery materials and methods214Theoretical and Experimental Study on the Electrochemical Behavior of Beta-Sodium Vanadate in Rechargeable Magnesium Batteries Using Several Electrolyte Solutions9A theoretical and experimental study of hexagonal molybdenum trioxide as dual-ion electrode for rechargeable magnesium battery31On the challenge of large energy storage by electrochemical devices117Reversible Calcium-Ion Insertion in NASICON-Type NaV2(PO4)374Effect of water in a non-aqueous electrolyte on electrochemical Mg2+ insertion into WO324Does Water Enhance Mg Intercalation in Oxides? The Case of a Tunnel Framework17Hydrated MgxV5O12 Cathode with Improved Mg2+ Storage Performance58Mechanisms of Water-Stimulated Mg2+ Intercalation in Vanadium Oxide: Toward the Development of Hydrated Vanadium Oxide Cathodes for Mg Batteries20Na2ZrCl6 enabling highly stable 3 V all-solid-state Na-ion batteries170The Quest for Functional Oxide Cathodes for Magnesium Batteries: A Critical Perspective77Critical Review on the Unique Interactions and Electroanalytical Challenges Related to Cathodes ‐ Solutions Interfaces in Non‐Aqueous Mg Battery Prototypes3Development and challenges of electrode materials for rechargeable Mg batteries57Hierarchical Mg-Birnessite Nanowall Arrays with Enriched (010) Planes for High Performance Aqueous Mg-Ion Batteries18Facilitating Mg2+ diffusion in high potential LixV2(PO4)3 cathode material with a co-insertion strategy for rechargeable Mg-ion batteries24Enhanced Van-Der Waals Separation in Hydrated Tungsten Oxide Nanoplates Enables Superior Pseudocapacitive Charge Storage16Exploring the Insertion Properties of Mg2+ in H2v3o8 as a Function of the Water Content in the Organic Electrolyte12Investigating the role of structural water on the electrochemical properties of α-V 2 O 5 through density functional theory10Multivalent Ion Conduction in Inorganic Solids38Bilayered Ca 0.28 V 2 O 5 ·H 2 O: High-Capacity Cathode Material for Rechargeable Ca-Ion Batteries and Its Charge Storage Mechanism60Intercalation-type positive electrode materials for nonaqueous calcium-ion batteries10Sodium-pillared vanadium oxides as next-gen materials: Does co-inserted water control the cyclic stability of vanadates in an aqueous electrolyte?8Recent progress on cathode materials for rechargeable magnesium batteries82V2O5 as a versatile electrode material for postlithium energy storage systems29Progress and perspective on rechargeable magnesium-ion batteries38Vanadium-based cathode materials for rechargeable magnesium batteries28Intercalation of bilayered V2O5 by electronically coupled PEDOT for greatly improved kinetic performance of magnesium ion battery cathodes46Refinement of the Crystal Structure of Low-Carbon Polycrystalline AISI 420 Martensitic Steel (C = 0.15%)1Water Vapor Induced Superionic Conductivity in ZnPS323Re‐evaluating the Magnesium‐ion Storage Capability of Vanadium Dioxide, VO2(B): Uncovering the Influence of Water Content on the Previously Overestimated High Capacity10Novel layered iron vanadate as a stable high-voltage cathode material for nonaqueous magnesium-ion batteries19Unraveling the Role of Hydrogen Insertion in Enhancing the Electrochemical Performance of the V2O5 Cathode for Mg-Ion Batteries: A First-Principles Study7Li2GeS3: Lithium Ionic Conductor with an Unprecedented Structural Type10(NH4)2V7O16 as a Cathode Material for Rechargeable Calcium-Ion Batteries: Structural Transformation and Co-Intercalation of Ammonium and Calcium Ions22Transition metal oxides and transition metal sulfides as cathodes for magnesium-ion batteries: current status and modification strategies34Unraveling Polymorphic Crystal Structures of Li4SiS4 for All-Solid-State Batteries: Enhanced Ionic Conductivity via Aliovalent Sb Substitution16Progress and Challenges of Vanadium Oxide Cathodes for Rechargeable Magnesium Batteries17Improving magnetic properties of FeCrCo films by facilitating the internal α-γ phase transition through Pt diffusion2Proton co-intercalation enabled high-performance aqueous multivalent metal-ion batteries5Li 21 Ge 8 P 3 S 34 : New Lithium Superionic Conductor with Unprecedented Structural Type0Li 21 Ge 8 P 3 S 34 : New Lithium Superionic Conductor with Unprecedented Structural Type4Oxygen Vacancy‐Driven High‐Performance V 2 O 5 Cathodes for Aqueous Manganese Metal Batteries35Moisture-Stable Argyrodites with High Ionic Conductivity via Crystal Structure Engineering: Li 6+ x M x As 1– x S 5 I (M = Ge, Sn)4Enhanced Structural Transformation Enabled by Low‐Crystalline Vanadium Oxides in Aqueous Zinc‐Ion Batteries13Self-supporting composite anodes with three-dimensional network by wood-derived hard carbon in rechargeable metallic magnesium batteries3Biochar from renewable wood as an ion-conducting protective layer on stable magnesium metal anodes2High voltage cathode materials for rechargeable magnesium batteries: Structural aspects and electrochemical perspectives13Electrochemical Properties of Aluminum Ion-Doped Vanadium Oxide AlxV2O5 in Magnesium-Containing Propylene Carbonate Electrolytes1Density functional theory study of the electronic, vibrational, thermodynamic, and detonation properties of Difurazo(3,4-h,3,4-l)-1,4,7,10,11-trioxadiazacyclotridec-10-ene0A Molecular Dynamics Study of Aqueous Na+/Mg2+ Intercalation Behavior in Vanadium Oxide Nanopores0Halide-Driven Stabilization of a Hexagonal Polymorph with a Distinct and Disordered Li Substructure in Li3.25GeS3.25Cl0.750

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  1. Electrochemical Intercalation of Mg 2+ into Anhydrous and Hydrated Crystalline Tungsten Oxides

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  2. A critical review of cathodes for rechargeable Mg batteries

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  3. Aqueous rechargeable Zn-ion batteries: an imperishable and high-energy Zn 2 V 2 O 7 nanowire cathode through intercalation regulation

    Journal of Materials Chemistry A · 2018-01-01

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  4. Can Multielectron Intercalation Reactions Be the Basis of Next Generation Batteries?

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  5. An artificial interphase enables reversible magnesium chemistry in carbonate electrolytes

    Nature Chemistry · 2018-04-02

    Seoung‐Bum Son, Tao Gao, Steve P. Harvey, K. Xerxes Steirer, Adam Stokes, Andrew G. Norman, Chunsheng Wang, Arthur von Wald Cresce, Kang Xu, Chunmei Ban

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  6. Ammonium Vanadium Bronze (NH 4 V 4 O 10 ) as a High-Capacity Cathode Material for Nonaqueous Magnesium-Ion Batteries

    Chemistry of Materials · 2018-05-10

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  7. Solvent Effects on the Reversible Intercalation of Magnesium‐Ions into V2O5 Electrodes

    ChemElectroChem · 2018-08-17

    Ran Attias, Michael Salama, Baruch Hirsch, Yosef Gofer, Doron Aurbach

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  8. On the strange case of divalent ions intercalation in V2O5

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  9. Water-Activated VOPO4 for Magnesium Ion Batteries

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  10. Unveiling the Intercalation Mechanism in Fe2(MoO4)3 as an Electrode Material for Na-Ion Batteries by Structural Determination

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  11. H2V3O8 as a High Energy Cathode Material for Nonaqueous Magnesium-Ion Batteries

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  12. Effect of water in electrolyte on the Ca2+ insertion/extraction properties of V2O5

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  13. Anion Effects on Cathode Electrochemical Activity in Rechargeable Magnesium Batteries: A Case Study of V2O5

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  14. A room temperature multivalent rechargeable iron ion battery with an ether based electrolyte: a new type of post-lithium ion battery

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  15. Preparation and electrochemical performance of VO 2 (A) hollow spheres as a cathode for aqueous zinc ion batteries

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  16. Rhombohedral Potassium–Zinc Hexacyanoferrate as a Cathode Material for Nonaqueous Potassium-Ion Batteries

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  17. First-principles investigation of Sn doping on the geometric and electronic structures of V2O5

    Integrated ferroelectrics · 2019-05-04

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  18. Intercalation of Magnesium into a Layered Vanadium Oxide with High Capacity

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  19. Ab initio modeling and design of vanadia-based electrode materials for post-lithium batteries

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  20. Methods and Protocols for Reliable Electrochemical Testing in Post-Li Batteries (Na, K, Mg, and Ca)

    Chemistry of Materials · 2019-10-15

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  21. Recent Progress on Layered Cathode Materials for Nonaqueous Rechargeable Magnesium Batteries

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  22. High Potassium Storage Capability of H 2 V 3 O 8 in a Non‐Aqueous Electrolyte

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  23. Interlayer separation in hydrogen titanates enables electrochemical proton intercalation

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  24. Valence-to-core X-ray emission spectroscopy of vanadium oxide and lithiated vanadyl phosphate materials

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  25. Dual Effect of Structure and Hydration on Magnesium-Ion Insertion into Electrodeposited V 2 O 5 Thin Films

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  27. Theoretical and Experimental Study on the Electrochemical Behavior of Beta-Sodium Vanadate in Rechargeable Magnesium Batteries Using Several Electrolyte Solutions

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  28. A theoretical and experimental study of hexagonal molybdenum trioxide as dual-ion electrode for rechargeable magnesium battery

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  30. Reversible Calcium-Ion Insertion in NASICON-Type NaV2(PO4)3

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  31. Effect of water in a non-aqueous electrolyte on electrochemical Mg2+ insertion into WO3

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  32. Does Water Enhance Mg Intercalation in Oxides? The Case of a Tunnel Framework

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  33. Hydrated MgxV5O12 Cathode with Improved Mg2+ Storage Performance

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  34. Mechanisms of Water-Stimulated Mg2+ Intercalation in Vanadium Oxide: Toward the Development of Hydrated Vanadium Oxide Cathodes for Mg Batteries

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  35. Na2ZrCl6 enabling highly stable 3 V all-solid-state Na-ion batteries

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  36. The Quest for Functional Oxide Cathodes for Magnesium Batteries: A Critical Perspective

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  37. Critical Review on the Unique Interactions and Electroanalytical Challenges Related to Cathodes ‐ Solutions Interfaces in Non‐Aqueous Mg Battery Prototypes

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  38. Development and challenges of electrode materials for rechargeable Mg batteries

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  39. Hierarchical Mg-Birnessite Nanowall Arrays with Enriched (010) Planes for High Performance Aqueous Mg-Ion Batteries

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  40. Facilitating Mg2+ diffusion in high potential LixV2(PO4)3 cathode material with a co-insertion strategy for rechargeable Mg-ion batteries

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  41. Enhanced Van-Der Waals Separation in Hydrated Tungsten Oxide Nanoplates Enables Superior Pseudocapacitive Charge Storage

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  42. Exploring the Insertion Properties of Mg2+ in H2v3o8 as a Function of the Water Content in the Organic Electrolyte

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  43. Investigating the role of structural water on the electrochemical properties of α-V 2 O 5 through density functional theory

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  46. Intercalation-type positive electrode materials for nonaqueous calcium-ion batteries

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  47. Sodium-pillared vanadium oxides as next-gen materials: Does co-inserted water control the cyclic stability of vanadates in an aqueous electrolyte?

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  48. Recent progress on cathode materials for rechargeable magnesium batteries

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  49. V2O5 as a versatile electrode material for postlithium energy storage systems

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