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RESEARCH PAPER · Energy storage materials · 2022

Recent progress on cathode materials for rechargeable magnesium batteries

Masashi Kotobuki, Binggong Yan, Li Lü

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Recent progress on cathode materials for rechargeable magnesium batteriesOriginalCurrent material design strategies on the copper chalcogenide cathodes for rechargeable magnesium batteries: a review17Strategy for enhancement of magnesium ion diffusion in a vanadium tetra sulfide-layered structure for rechargeable magnesium batteries19Li–Na-based hybrid battery5Modeling of Magnesium Intercalation into Chevrel Phase Mo6S8: Report on Improved Cell Design6Implanting CuS Quantum Dots into Carbon Nanorods for Efficient Magnesium‐Ion Batteries53A review on advanced optimization strategies of separators for aqueous zinc-ion batteries15Nitrogen-doped expanded graphite derived from spent graphite induce uniform growth of lithium peroxide for high-performance Li-oxygen battery16Research advances of magnesium and magnesium alloys worldwide in 2022440Excellent ion storage properties of copper-cobalt composite selenide heterostructure in magnesium/lithium hybrid battery18The Magnesium Insertion Effects into P2‐Type Na2/3Ni1/3Mn2/3O211Molybdenum disulfide (MoS_₂) −based cathode materials for magnesium (Mg2+) and Mg2+/Li+ hybrid-ion batteries: Progress and perspective1A critical review on inconsistency mechanism, evaluation methods and improvement measures for lithium-ion battery energy storage systems235In-situ generated elemental selenium nanograins cooperated with NiSe2 microspheres for significantly enhanced magnesium-storage performance13Recent Research Progress on All-Solid-State Mg Batteries14Oxygen Vacancies Boosted Proton Intercalation Kinetics for Aqueous Aluminum–Manganese Batteries37Challenges and recent progress on anodes and their interfacial optimization towards high-performance rechargeable magnesium batteries43A review of metal sulfide cathode materials for non-aqueous multivalent ion (Mg2+, Ca2+, Al3+) batteries19Copper selenide/amino hyperbranched polymer as an organic/inorganic hybrid composite cathode for rechargeable magnesium batteries7Electrolyte-dependent deposition morphology on magnesium metal utilizing MeMgCl, Mg[B(hfip) 4 ] 2 and Mg(HMDS) 2 –2AlCl 3 electrolytes13Extending the Chevrel-type superatoms to the nitrogen family0Magnesium Ion Embedded and Graphene Modified Vanadium Pentoxide Cathode for Superior Magnesium Storage Performance0Recovery of manganese as spinel MgMn2O4 cathode material from electrolytic manganese residue by Na2CO3 hydrothermal-roasting process10Insights on advanced g‐C 3 N 4 in energy storage: Applications, challenges, and future79Efficient and Stable Magnesium Plating/Stripping in High-Capacity Novel Mg//Ni0.6Co0.4Se2 Batteries Enabled by Interfacial Chemistry Modulation10Advances and Challenges in Electrolyte Development for Magnesium–Sulfur Batteries: A Comprehensive Review20CuS-based composite for high-performance magnesium storage with a clarified charge-discharge mechanism9Understanding the Cathode‐Electrolyte Interfacial Chemistry in Rechargeable Magnesium Batteries57Preferentially in-situ generated copper nanograins boosting fast kinetic conversion magnesium storage of bimetallic copper-cobalt sulfide cathode15Dual-Defect Engineering Strategy Enables High-Durability Rechargeable Magnesium-Metal Batteries28Fine nanostructure design of metal chalcogenide conversion-based cathode materials for rechargeable magnesium batteries14References0Ternary Mg alloy-based artificial interphase enables high-performance rechargeable magnesium batteries29Compatibility of Molybdenum Disulfide and Magnesium Fluorinated Alkoxyaluminate Electrolytes in Rechargeable Mg Batteries1Recent advances in morphological tuning strategies for transition metal carbonate hydroxides and promising potential in lithium-ion batteries and electrolyzers2Progress and Challenges of Vanadium Oxide Cathodes for Rechargeable Magnesium Batteries17Sustainable Cathodic Performances of VS 4 in Rechargeable Magnesium Batteries by Cobalt Substitution15High‐Capacity and Ultra‐Long‐Life Mg‐Metal Batteries Enabled by Intercalation‐Conversion Hybrid Cathode Materials8Challenges and Progress in Rechargeable Magnesium‐Ion Batteries: Materials, Interfaces, and Devices90Defect Engineering: Can it Mitigate Strong Coulomb Effect of Mg2+ in Cathode Materials for Rechargeable Magnesium Batteries?43Se‐Doping on Co4S3 Cathode Based on Soft Anion Chemistry to Enhance Magnesium Storage Performance0Regulating Electric Double Layer via Self‐Assembled Monolayer for Stable Solid/Electrolyte Interphase on Mg Metal Anode6Regulating Electric Double Layer via Self‐Assembled Monolayer for Stable Solid/Electrolyte Interphase on Mg Metal Anode33Engineering Heterointerface to Synergistically Regulate Kinetics and Stress of Copper–Cobalt Selenide toward Reversible Magnesium/Lithium Hybrid Batteries17Amorphous MoS3 Anchored within Hollow Carbon as a Cathode Material for Magnesium-Ion Batteries57Rechargeable magnesium-ion batteries: From mechanism to emerging materials0CaB12H12: A promising salt for aprotic electrolytes in calcium-based secondary batteries6Magnesium Alginate as an Electrolyte for Magnesium Batteries8Ultrafast Synthesis of Oxygen Vacancy-Rich MgFeSiO4 Cathode to Boost Diffusion Kinetics for Rechargeable Magnesium-Ion Batteries19Favorable Orthorhombic Phase Cobalt Diselenide Cathode for Rechargeable Mg Batteries: Elucidating the Significant Impact of Crystal Structure on Conversion‐Type Mg‐Storage Reactions14In Situ Cross‐Linking and Interfacial Engineering via Multifunctional Diamine Additive for High‐Temperature Magnesium Metal Batteries18Advancements in cathode materials for high-performance rechargeable magnesium-ion batteries18Interlayer Cationic Defect Engineering in Lamellar Vanadate Cathodes Enables Ultralong-Lifespan Magnesium-Ion Batteries56Recent advancements in high-performance and durable electrodes materials for magnesium-ion batteries27Advancing Cathode Materials for Rechargeable Magnesium‐Ion Batteries: Sustainable Structures, Ecofriendly Properties, and Enhanced Electrochemical Performance9Simultaneous Enhancement of Interface Stability and Ionic Transport by Li+ and BH4– in Magnesium-Based Energy Storage6Stress release strategy driven by multi-interface structure and dual-ion insertion toward stable hybrid batteries4Unveiling the potential of two morphological Ni0.85Se nanostructures as cathode materials for rechargeable magnesium batteries0Boron‐Doped Hexagonal Boridene‐Derived Sulfides Unlock High Reversible Capacity for Rechargeable Magnesium Batteries4A Concise Overview of the Use of Low-Dimensional Molybdenum Disulfide as an Electrode Material for Li-Ion Batteries and Beyond3Na5YSi4O12-polymer composite coating for hard carbon: a strategy to improve sodium-ion storage performance6Recent Progress in Interlayer Engineering of Layered Materials for High-Performance Magnesium Ion Batteries5Heterointerface Engineering-Induced V–C Bonds and Built-in Electric Field Boosts Mg2+ Storage and Diffusion Kinetics2Life Cycle Assessment (LCA) Challenges in Evaluating Emerging Battery Technologies: A Review6Reassessing Electrolyte Design for Non‐Aqueous Magnesium Batteries: Atomistic Structures and Performance Optimization14Molecular Traffic Control: Fast Mg 2+ Transport via Carbonyl‐Induced Ion‐Dipole Interactions in Covalent Organic Framework Channels6Molecular Traffic Control: Fast Mg 2+ Transport via Carbonyl‐Induced Ion‐Dipole Interactions in Covalent Organic Framework Channels3Cathode properties of MgV 2 O 4 spinel for magnesium rechargeable batteries: effect of synthesis route on structure and electrochemical performance5MgNiP2O7 pyrophosphate as a promising cathode material for magnesium-ion batteries: A computational investigation2Structural stabilization and electronic tuning of CoSe2 via Cu doping toward long-life rechargeable magnesium batteries4Anode-Free Batteries: Pioneering Energy Storage Revolution32Extraction of high-purity magnesium and calcium from phosphate mine waste rocks by a carbon-neutral and circular hydrometallurgy1Ti-doped MgV2O4 spinel for magnesium-ion batteries: Facile carbon-integrated synthesis, experimental study, and theoretical modeling0Multi‐Step Data‐Driven High‐Voltage MgMn 2 O 4 with Inorganic‐Rich Cathode‐Electrolyte Interphase for Stable Mg 2+ Storage0Microstructural regulation in NH4V4O10 with enhanced Mg-ion storage performance for long-life Mg-Ion batteries0Magnesium-ion battery cathode materials: Artificial intelligence applications, research advances, and industrialization0Reaction mechanisms, key challenges, and future prospects of zinc-ion/magnesium-based batteries: from fundamental researches to electrode/electrolyte engineering0Oxygen-deficient TiO2-x(B): A 3D-structured cathode for all-climate magnesium-ion batteries0A Review of Design Strategies and Material Challenges for Magnesium-Based Rechargeable Seawater Batteries: Insights from Sodium-RSB Systems0Cu2+ Pre-Intercalation Enables Fast and Stable Hydrated Vanadium Pentoxide Nanostructure-Based Cathodes for Magnesium–Sodium Hybrid Ion Batteries0Synergistic enhancement via thienyl functionalization and in situ metallic copper formation in porphyrin cathodes for high-energy, long-cycling magnesium batteries0Unlocking sequential H+/Mg2+ co-intercalation chemistry in MgMn2O4 for high-performance aqueous magnesium-ion batteries0

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  1. Current material design strategies on the copper chalcogenide cathodes for rechargeable magnesium batteries: a review

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  2. Strategy for enhancement of magnesium ion diffusion in a vanadium tetra sulfide-layered structure for rechargeable magnesium batteries

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  3. Li–Na-based hybrid battery

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  4. Modeling of Magnesium Intercalation into Chevrel Phase Mo6S8: Report on Improved Cell Design

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  5. Implanting CuS Quantum Dots into Carbon Nanorods for Efficient Magnesium‐Ion Batteries

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  6. A review on advanced optimization strategies of separators for aqueous zinc-ion batteries

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  7. Nitrogen-doped expanded graphite derived from spent graphite induce uniform growth of lithium peroxide for high-performance Li-oxygen battery

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  8. Research advances of magnesium and magnesium alloys worldwide in 2022

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  9. Excellent ion storage properties of copper-cobalt composite selenide heterostructure in magnesium/lithium hybrid battery

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  10. The Magnesium Insertion Effects into P2‐Type Na2/3Ni1/3Mn2/3O2

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  11. Molybdenum disulfide (MoS_₂) −based cathode materials for magnesium (Mg2+) and Mg2+/Li+ hybrid-ion batteries: Progress and perspective

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  12. A critical review on inconsistency mechanism, evaluation methods and improvement measures for lithium-ion battery energy storage systems

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  13. In-situ generated elemental selenium nanograins cooperated with NiSe2 microspheres for significantly enhanced magnesium-storage performance

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  14. Recent Research Progress on All-Solid-State Mg Batteries

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  15. Oxygen Vacancies Boosted Proton Intercalation Kinetics for Aqueous Aluminum–Manganese Batteries

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  16. Challenges and recent progress on anodes and their interfacial optimization towards high-performance rechargeable magnesium batteries

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  17. A review of metal sulfide cathode materials for non-aqueous multivalent ion (Mg2+, Ca2+, Al3+) batteries

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  18. Copper selenide/amino hyperbranched polymer as an organic/inorganic hybrid composite cathode for rechargeable magnesium batteries

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  19. Electrolyte-dependent deposition morphology on magnesium metal utilizing MeMgCl, Mg[B(hfip) 4 ] 2 and Mg(HMDS) 2 –2AlCl 3 electrolytes

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  21. Magnesium Ion Embedded and Graphene Modified Vanadium Pentoxide Cathode for Superior Magnesium Storage Performance

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  22. Recovery of manganese as spinel MgMn2O4 cathode material from electrolytic manganese residue by Na2CO3 hydrothermal-roasting process

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  24. Efficient and Stable Magnesium Plating/Stripping in High-Capacity Novel Mg//Ni0.6Co0.4Se2 Batteries Enabled by Interfacial Chemistry Modulation

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  25. Advances and Challenges in Electrolyte Development for Magnesium–Sulfur Batteries: A Comprehensive Review

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  27. Understanding the Cathode‐Electrolyte Interfacial Chemistry in Rechargeable Magnesium Batteries

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  28. Preferentially in-situ generated copper nanograins boosting fast kinetic conversion magnesium storage of bimetallic copper-cobalt sulfide cathode

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  29. Dual-Defect Engineering Strategy Enables High-Durability Rechargeable Magnesium-Metal Batteries

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  30. Fine nanostructure design of metal chalcogenide conversion-based cathode materials for rechargeable magnesium batteries

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  31. References

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  32. Ternary Mg alloy-based artificial interphase enables high-performance rechargeable magnesium batteries

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  33. Compatibility of Molybdenum Disulfide and Magnesium Fluorinated Alkoxyaluminate Electrolytes in Rechargeable Mg Batteries

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  34. Recent advances in morphological tuning strategies for transition metal carbonate hydroxides and promising potential in lithium-ion batteries and electrolyzers

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  35. Progress and Challenges of Vanadium Oxide Cathodes for Rechargeable Magnesium Batteries

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  36. Sustainable Cathodic Performances of VS 4 in Rechargeable Magnesium Batteries by Cobalt Substitution

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  37. High‐Capacity and Ultra‐Long‐Life Mg‐Metal Batteries Enabled by Intercalation‐Conversion Hybrid Cathode Materials

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  38. Challenges and Progress in Rechargeable Magnesium‐Ion Batteries: Materials, Interfaces, and Devices

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  39. Defect Engineering: Can it Mitigate Strong Coulomb Effect of Mg2+ in Cathode Materials for Rechargeable Magnesium Batteries?

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  40. Se‐Doping on Co4S3 Cathode Based on Soft Anion Chemistry to Enhance Magnesium Storage Performance

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  42. Regulating Electric Double Layer via Self‐Assembled Monolayer for Stable Solid/Electrolyte Interphase on Mg Metal Anode

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  43. Engineering Heterointerface to Synergistically Regulate Kinetics and Stress of Copper–Cobalt Selenide toward Reversible Magnesium/Lithium Hybrid Batteries

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  44. Amorphous MoS3 Anchored within Hollow Carbon as a Cathode Material for Magnesium-Ion Batteries

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  45. Rechargeable magnesium-ion batteries: From mechanism to emerging materials

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  46. CaB12H12: A promising salt for aprotic electrolytes in calcium-based secondary batteries

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  47. Magnesium Alginate as an Electrolyte for Magnesium Batteries

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  48. Ultrafast Synthesis of Oxygen Vacancy-Rich MgFeSiO4 Cathode to Boost Diffusion Kinetics for Rechargeable Magnesium-Ion Batteries

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  49. Favorable Orthorhombic Phase Cobalt Diselenide Cathode for Rechargeable Mg Batteries: Elucidating the Significant Impact of Crystal Structure on Conversion‐Type Mg‐Storage Reactions

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  50. In Situ Cross‐Linking and Interfacial Engineering via Multifunctional Diamine Additive for High‐Temperature Magnesium Metal Batteries

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