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RESEARCH PAPER · Chemical Society Reviews · 2018

A critical review of cathodes for rechargeable Mg batteries

Minglei Mao, Tao Gao, Singyuk Hou, Chunsheng Wang

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A critical review of cathodes for rechargeable Mg batteriesOriginalComposition- and size-modulated porous bismuth–tin biphase alloys as anodes for advanced magnesium ion batteries69Emergence of rechargeable seawater batteries115Intercalation chemistry of graphite: alkali metal ions and beyond903Alkali ions pre-intercalated layered vanadium oxide nanowires for stable magnesium ions storage105Rational Design of Preintercalated Electrodes for Rechargeable Batteries108Microstructure Characteristics of Cathode Materials for Rechargeable Magnesium Batteries64Multi-ion strategies towards emerging rechargeable batteries with high performance172Progress in development of electrolytes for magnesium batteries247Monolayer, Bilayer, and Heterostructure Arsenene as Potential Anode Materials for Magnesium-Ion Batteries: A First-Principles Study77Post-Li batteries: promises and challenges103High-Energy-Density Rechargeable Mg Battery Enabled by a Displacement Reaction86Rechargeable Magnesium–Sulfur Battery Technology: State of the Art and Key Challenges116A Pyrazine‐Based Polymer for Fast‐Charge Batteries260Recent advances in electrolytes and cathode materials for magnesium and hybrid-ion batteries172Recent Progress on Layered Cathode Materials for Nonaqueous Rechargeable Magnesium Batteries80Nanosheets assembling hierarchical starfish-like Cu2−xSe as advanced cathode for rechargeable Mg batteries84Novel One-Dimensional Hollow Carbon Nanotubes/Selenium Composite for High-Performance Al-Se Batteries48Ultrahigh Nitrogen Doping of Carbon Nanosheets for High Capacity and Long Cycling Potassium Ion Storage263Layered birnessite MnO2 with enlarged interlayer spacing for fast Mg-ion storage67Exploits, advances and challenges benefiting beyond Li-ion battery technologies236Reversible Electrochemical Interface of Mg Metal and Conventional Electrolyte Enabled by Intermediate Adsorption95Hollow structured cathode materials for rechargeable batteries54A Stable Solid Electrolyte Interphase for Magnesium Metal Anode Evolved from a Bulky Anion Lithium Salt187Challenges and perspectives for manganese‐based oxides for advanced aqueous zinc‐ion batteries411Iodine Vapor Transport-Triggered Preferential Growth of Chevrel Mo6S8 Nanosheets for Advanced Multivalent Batteries1363D printing of structured electrodes for rechargeable batteries163Advances in rechargeable Mg batteries148Crystal regulation towards rechargeable magnesium battery cathode materials102Recent advances in developing organic electrode materials for multivalent rechargeable batteries256Review—Polymer Electrolytes for Magnesium Batteries: Forging Away from Analogs of Lithium Polymer Electrolytes and Towards the Rechargeable Magnesium Metal Polymer Battery88Ni0.85Se hexagonal nanosheets as an advanced conversion cathode for Mg secondary batteries58Morphology-dependent electrochemical performance of VS4 for rechargeable magnesium battery and its magnesiation/demagnesiation mechanism72Hierarchical Copper Sulfide Porous Nanocages for Rechargeable Multivalent-Ion Batteries79Achieving high capacity and long life of aqueous rechargeable zinc battery by using nanoporous-carbon-supported poly(1,5-naphthalenediamine) nanorods as cathode165A Trip to Oz and a Peak Behind the Curtain of Magnesium Batteries128Optimizing Calcium Electrolytes by Solvent Manipulation for Calcium Batteries82Highly Efficient Non-Nucleophilic Mg(CF 3 SO 3 ) 2 -Based Electrolyte for High-Power Mg/S Battery83Highly Reversible Cuprous Mediated Cathode Chemistry for Magnesium Batteries103Recent Advances in Rechargeable Magnesium‐Based Batteries for High‐Efficiency Energy Storage241Highly stable magnesium-ion-based dual-ion batteries based on insoluble small-molecule organic anode material164Alloy Anode Materials for Rechargeable Mg Ion Batteries252NiMn-Cl Layered Double Hydroxide/Carbon Nanotube Networks for High-Performance Chloride Ion Batteries68Side by Side Battery Technologies with Lithium‐Ion Based Batteries278Challenges and Recent Progress on Key Materials for Rechargeable Magnesium Batteries295Quest for carbon and vanadium oxide based rechargeable magnesium-ion batteries51Recent advances and perspectives in stable and dendrite-free potassium metal anodes150Intercalated water in aqueous batteries60Unravelling the Mechanism of Rechargeable Aqueous Zn–MnO 2 Batteries: Implementation of Charging Process by Electrodeposition of MnO 2136Capacity Retention Analysis in Aluminum-Sulfur Batteries62Water‐Pillared Sodium Vanadium Bronze Nanowires for Enhanced Rechargeable Magnesium Ion Storage58High Voltage Mg-Ion Battery Cathode via a Solid Solution Cr–Mn Spinel Oxide72Active Materials for Aqueous Zinc Ion Batteries: Synthesis, Crystal Structure, Morphology, and Electrochemistry1788Aluminum electrolytes for Al dual-ion batteries86Ammonium ion intercalated hydrated vanadium pentoxide for advanced aqueous rechargeable Zn-ion batteries162New Insight on Open‐Structured Sodium Vanadium Oxide as High‐Capacity and Long Life Cathode for Zn–Ion Storage: Structure, Electrochemistry, and First‐Principles Calculation88Unexpected discovery of magnesium-vanadium spinel oxide containing extractable Mg2+ as a high-capacity cathode material for magnesium ion batteries67An overview and prospective on Al and Al-ion battery technologies263Pseudocapacitive Ti-Doped Niobium Pentoxide Nanoflake Structure Design for a Fast Kinetics Anode toward a High-Performance Mg-Ion-Based Dual-Ion Battery52Two-Phase Electrochemical Proton Transport and Storage in α-MoO3 for Proton Batteries96Hydrated MgxV5O12 Cathode with Improved Mg2+ Storage Performance58Dendrites in Zn‐Based Batteries1180Exploring Cation–Anion Redox Processes in One-Dimensional Linear Chain Vanadium Tetrasulfide Rechargeable Magnesium Ion Cathodes81Rechargeable aqueous zinc-ion batteries: Mechanism, design strategies and future perspectives281A review on current anode materials for rechargeable Mg batteries123Rechargeable Sodium‐Based Hybrid Metal‐Ion Batteries toward Advanced Energy Storage71High‐Energy Aqueous Magnesium Hybrid Full Batteries Enabled by Carrier‐Hosting Potential Compensation72Recent Advances and Perspectives on Calcium‐Ion Storage: Key Materials and Devices191Electrochemical Mg 2+ Displacement Driven Reversible Copper Extrusion/Intrusion Reactions for High‐Rate Rechargeable Magnesium Batteries90Promises and Challenges of Next-Generation “Beyond Li-ion” Batteries for Electric Vehicles and Grid Decarbonization1612Reaction mechanisms and optimization strategies of manganese-based materials for aqueous zinc batteries76A comprehensive review of the development of magnesium anodes for primary batteries162Advanced electrode materials for nonaqueous calcium rechargeable batteries55Application of expanded graphite-based materials for rechargeable batteries beyond lithium-ions60High-performance magnesium metal batteries via switching the passivation film into a solid electrolyte interphase90Principles of interlayer-spacing regulation of layered vanadium phosphates for superior zinc-ion batteries254Pseudo-solid-state electrolytes utilizing the ionic liquid family for rechargeable batteries110Strategies of structural and defect engineering for high-performance rechargeable aqueous zinc-ion batteries90The design of Co3S4@MXene heterostructure as sulfur host to promote the electrochemical kinetics for reversible magnesium-sulfur batteries81Cathode Design for Aqueous Rechargeable Multivalent Ion Batteries: Challenges and Opportunities203Sustainable Batteries—Quo Vadis?80Crystal defect modulation in cathode materials for non-lithium ion batteries: Progress and challenges109Through the Maze of Multivalent‐Ion Batteries: A Critical Review on the Status of the Research on Cathode Materials for Mg 2+ and Ca 2+ Ions Insertion49Organic‐Inorganic Superlattices of Vanadium Oxide@Polyaniline for High‐Performance Magnesium‐Ion Batteries72Interlayer Engineering of Preintercalated Layered Oxides as Cathode for Emerging Multivalent Metal-ion Batteries: Zinc and Beyond182Storage mechanisms and improved strategies for manganese-based aqueous zinc-ion batteries66Highly efficient overall-water splitting enabled via grafting boron-inserted Fe-Ni solid solution nanosheets onto unconventional skeleton78Recent advances in vanadium-based materials for aqueous metal ion batteries: Design of morphology and crystal structure, evolution of mechanisms and electrochemical performance65A universal strategy towards high–energy aqueous multivalent–ion batteries244Chemical Heterointerface Engineering on Hybrid Electrode Materials for Electrochemical Energy Storage129Hybrid MgCl 2 /AlCl 3 /Mg(TFSI) 2 Electrolytes in DME Enabling High-Rate Rechargeable Mg Batteries79A Bismuth-Based Protective Layer for Magnesium Metal Anode in Noncorrosive Electrolytes193Uncovering electrochemistries of rechargeable magnesium-ion batteries at low and high temperatures61V 2 CT x MXene and its derivatives: synthesis and recent progress in electrochemical energy storage applications111Electrode materials for aqueous multivalent metal-ion batteries: Current status and future prospect73Sn Alloying to Inhibit Hydrogen Evolution of Zn Metal Anode in Rechargeable Aqueous Batteries312Current Design Strategies for Rechargeable Magnesium-Based Batteries208PBA composites and their derivatives in energy and environmental applications211VS4 anchored on Ti3C2 MXene as a high-performance cathode material for magnesium ion battery76Anatase titanium dioxide as rechargeable ion battery electrode - A chronological review102A review on energy storage devices based on rylene imide dyes: Synthesis, applications and challenges55Recent advances in Mg-Li and Mg-Na hybrid batteries83Polyaniline nanoarrays/carbon cloth as binder-free and flexible cathode for magnesium ion batteries64Hydrated eutectic electrolytes for high-performance Mg-ion batteries129Low‐strain TiP2O7 with three‐dimensional ion channels as long‐life and high‐rate anode material for Mg‐ion batteries117Organic-conjugated polyanthraquinonylimide cathodes for rechargeable magnesium batteries59High‐Voltage Aqueous Mg‐Ion Batteries Enabled by Solvation Structure Reorganization124Nano-sized split V2O5 with H2O-intercalated interfaces as a stable cathode for zinc ion batteries without an aging process75Mainstream Optimization Strategies for Cathode Materials of Sodium‐Ion Batteries175Size‐Controllable Nickel Sulfide Nanoparticles Embedded in Carbon Nanofibers as High‐Rate Conversion Cathodes for Hybrid Mg‐Based Battery52Hierarchical Nanocapsules of Cu-Doped MoS2@H-Substituted Graphdiyne for Magnesium Storage68Ether–Water Hybrid Electrolyte Contributing to Excellent Mg Ion Storage in Layered Sodium Vanadate98Rational Design Strategy of Novel Energy Storage Systems: Toward High‐Performance Rechargeable Magnesium Batteries100Understanding rechargeable magnesium ion batteries via first-principles computations: A comprehensive review64CaV 6 O 16 ·2.8H 2 O with Ca 2+ Pillar and Water Lubrication as a High‐Rate and Long‐Life Cathode Material for Ca‐Ion Batteries83Tellurium: A High-Performance Cathode for Magnesium Ion Batteries Based on a Conversion Mechanism77High-Energy Batteries: Beyond Lithium-Ion and Their Long Road to Commercialisation378Recent advances in kinetic optimizations of cathode materials for rechargeable magnesium batteries56Atomic‐Scale Design of Anode Materials for Alkali Metal (Li/Na/K)‐Ion Batteries: Progress and Perspectives149Prussian blue and its analogues as cathode materials for Na-, K-, Mg-, Ca-, Zn- and Al-ion batteries237Towards better Mg metal anodes in rechargeable Mg batteries: Challenges, strategies, and perspectives126Synchrotron Radiation Spectroscopic Studies of Mg 2+ Storage Mechanisms in High‐Performance Rechargeable Magnesium Batteries with Co‐Doped FeS 2 Cathodes52Multifunctional 1D Nanostructures toward Future Batteries: A Comprehensive Review91Recent progress on cathode materials for rechargeable magnesium batteries82From lithium to emerging mono- and multivalent-cation-based rechargeable batteries: non-aqueous organic electrolyte and interphase perspectives137Fundamentals and advances of ligand field theory in understanding structure-electrochemical property relationship of intercalation-type electrode materials for rechargeable batteries106High-Performance NiS 2 Hollow Nanosphere Cathodes in Magnesium-Ion Batteries Enabled by Tunable Redox Chemistry56Toward High-Performance Mg-S Batteries via a Copper Phosphide Modified Separator57A practical perspective on the potential of rechargeable Mg batteries138Magnesium: properties and rich chemistry for new material synthesis and energy applications118Ultraporous, Ultrasmall MgMn 2 O 4 Spinel Cathode for a Room-Temperature Magnesium Rechargeable Battery56Application of 2D MXene in Organic Electrode Materials for Rechargeable Batteries: Recent Progress and Perspectives56Cathode Electrolyte Interphase (CEI) Endows Mo 6 S 8 with Fast Interfacial Magnesium‐Ion Transfer Kinetics70Organosulfur Materials for Rechargeable Batteries: Structure, Mechanism, and Application228Implanting CuS Quantum Dots into Carbon Nanorods for Efficient Magnesium‐Ion Batteries53Ultrahigh-rate and ultralong-life aqueous batteries enabled by special pair-dancing proton transfer79Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities120Engineered nitrogen doping on VO2(B) enables fast and reversible zinc-ion storage capability for aqueous zinc-ion batteries140Cathode materials for calcium‐ion batteries: Current status and prospects68An Emerging Chemistry Revives Proton Batteries64Magnesium-based energy materials: Progress, challenges, and perspectives181Bottom‐Up Magnesium Deposition Induced by Paper‐Based Triple‐Gradient Scaffolds toward Flexible Magnesium Metal Batteries62Prospects for magnesium ion batteries: A compreshensive materials review92Multivalent‐Ion Electrochromic Energy Saving and Storage Devices68Enhancing Reversibility and Stability of Mg Metal Anodes: High‐Exposure (002) Facets and Nanosheet Arrays for Superior Mg Plating/Stripping53Research advances of magnesium and magnesium alloys globally in 2023206Advanced Mg-based materials for energy storage: fundamental, progresses, challenges and perspectives130Enabling high-performance multivalent metal-ion batteries: current advances and future prospects146Structural codes of organic electrode materials for rechargeable multivalent metal batteries76Electrochemical Energy Storage Devices─Batteries, Supercapacitors, and Battery–Supercapacitor Hybrid Devices220Roadmap for Next-Generation Electrochemical Energy Storage Technologies: Secondary Batteries and Supercapacitors149

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