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RESEARCH PAPER · Journal of Materials Chemistry C · 2017

Anomalous spontaneous-reduction of Mn 7+ /Mn 4+ to Mn 2+ and luminescence properties in Zn 2 GeO 4 :Mn

Jieqi Hu, Enhai Song, Shi Ye, Bo Zhou, Qinyuan Zhang

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Anomalous spontaneous-reduction of Mn 7+ /Mn 4+ to Mn 2+ and luminescence properties in Zn 2 GeO 4 :MnOriginalFabrication, activity and mechanism studies of transition metal molybdate/molybdenum trioxide hybrids as novel CWAO catalysts22A novel Mn(II)-based green phosphor and its self-reduction mechanism21Deep‐red photoluminescence and long persistent luminescence in double perovstkite‐type La 2 MgGeO 6 :Mn 4+90An efficient synthetic strategy for uniform perovskite core–shell nanocubes NaMgF 3 :Mn 2+ ,Yb 3+ @NaMgF 3 :Yb 3+ with enhanced near infrared upconversion luminescence9First-principles calculations of optical properties of Zn2GeO4 under high pressures2Persistent luminescence found in Mg 2+ and Pr 3+ co-doped LiNbO 3 single crystal39Thermometry of red nanoflaked SrAl12O19:Mn4+ synthesized with boric acid flux41Long persistent and photo‐stimulated luminescence in Pr 3+ ‐doped layered perovskite phosphor for optical data storage46Exploring the self-redox reaction mechanism of Mn-doped Mg2(Ti/Sn)O4 with its precise dopant position10Crystal field modulation-control, bandgap engineering and shallow/deep traps tailoring-guided design of a color-tunable long-persistent phosphor (Ca, Sr)Ga 4 O 7 :Mn 2+ ,Bi 3+44Solid state synthesis and luminescence of Zn2GeO4:Mn2+ phosphors using MnO2 as manganese source material: self-reduction of Mn4+ to Mn2+9Characterization of the structural, optical, photocatalytic and in vitro and in vivo anti-inflammatory properties of Mn 2+ doped Zn 2 GeO 4 nanorods29Non-stoichiometric defect-controlled reduction toward mixed-valence Mn-doped hexaaluminates and their optical applications47Photoluminescence and phosphorescence of Mn2+ ion activated green phosphor Na2ZnSiO4:Mn2+ synthesized by self-reduction60Tunable WLED with UV chip based on all-inorganic perovskite quantum dots6Blue-emitting Bi-doped double perovskite Gd2ZnTiO6 phosphor with near-ultraviolet excitation for warm white light-emitting diodes48Luminescent properties of Zn2GeO4:Mn2+ phosphors synthesized by using different manganese sources14Intra-grain polarized infrared spectroscopy realized in domain-engineered Zn2GeO4 ceramics5Novel narrow-band blue-emitting Cs 3 Zn 6 B 9 O 21 :Bi 3+ phosphor with superior thermal stability33UV–Vis-NIR broadband-photostimulated luminescence of LiTaO3:Bi3+ long-persistent phosphor and the optical storage properties143Polarized Raman scattering and infrared dispersion analysis of Na2ZnGeO4 ceramics2Tuning the Oxidation States of Dopants: A Strategy for the Modulation of Material Photoluminescence Properties11Optical-vibration and intrinsic dielectric properties of low-k high-Q Zn2GeO4 ceramics9Localized Charge Accumulation Driven by Li+ Incorporation for Efficient LED Phosphors with Tunable Photoluminescence77Novel UV and X-ray irradiated white-emitting persistent luminescence and traps distribution of Ca5Ga6O14: Pr3+ phosphors41Review: theoretical and experimental investigation of the intrinsic properties of Zn2GeO4 nanocrystals20A review on the structural dependent optical properties and energy transfer of Mn 4+ and multiple ion-codoped complex oxide phosphors36Superior thermally-stable narrow-band green emitter from Mn2+-doped zero thermal expansion (ZTE) material78Regulating Mn2+/Mn4+ Activators in ZnGa2O4 via Mg2+/Ge4+ Doping to Generate Multimode Luminescence for Advanced Anti-Counterfeiting74Structure and luminescence properties of Ce3+-activated BaLu2Al2Ga2SiO12 persistent phosphors for optical information storage10Controllable Synthesis and Luminescence Properties of Zn 2 GeO 4 : Mn 2+ Nanorod Phosphors13Synthesis of Black-TiO2 and manganese-doped TiO2 nanoparticles and their comparative performance evaluation for photocatalytic removal of phenolic compounds from agro-industrial effluent41Tuning multicolour emission of Zn 2 GeO 4 :Mn phosphors by Li + doping for information encryption and anti-counterfeiting applications46Designing ultra-highly efficient Mn2+-activated Zn2GeO4 green-emitting persistent phosphors toward versatile applications62Broad luminescence tuning in Mn 2+ -doped Rb 2 Zn 3 (P 2 O 7 ) 2 via doping level control based on multiple synergies10Crystal structure and optical performance analysis of a new type of persistent luminescence material with multi-functional application prospects21Advanced Luminescence Anticounterfeiting Based on Dynamic Photoluminescence and Non-Pre-Irradiation Mechanoluminescence44The origin of bright cyan persistent luminescence in Ca2SnO4:La3+15Luminescence and interstitial-defect-related self-reduction in Mn2+ activated Ba3BP3O12 phosphor13Achieving opto-responsive multimode luminescence in Zn1+Ga2−2Ge O4:Mn persistent phosphors for advanced anti-counterfeiting and information encryption87Dual-mode multicolor luminescence anti-counterfeiting based on Mn-doped color-tunable MgGa2O4:Zn2+/Ge4+ phosphors4Recent Advances in Ternary Metal Oxides Modified by N Atom for Photocatalysis25Self-reduction of Mn 4+ to Mn 2+ : NaY 9 Si 6 O 26 :Mn 2+ red phosphors with excellent thermal stability for NUV LEDs36Recent Progress in Inorganic Afterglow Materials: Mechanisms, Persistent Luminescent Properties, Modulating Methods, and Bioimaging Applications143Interstitial Zinc Boosted Light Tunability, Afterglow, and Ultrabright White Emission in Zinc Germanate (Zn 2 GeO 4 )30Abnormal Eu3+ → Eu2+ Reduction in Ca9−xMnxEu(PO4)7 Phosphors: Structure and Luminescent Properties19Suppressed Self‐Reduction of Manganese in Mg 2 SnO 4 via Li + Incorporation with Polychromatic Luminescence for Versatile Applications66H2O2-free strategy derived from Hummers method for preparing graphene oxide with high oxidation degree43Persistent Luminescence Zn2GeO4:Mn2+ Nanoparticles Functionalized with Polyacrylic Acid: One-Pot Synthesis and Biosensing Applications43Anomalous thermal quenching of Ca2-xGe7O16:xMn2+ orange-emitting phosphors11Breaking the balance of chemical ratio in ZnAl2O4 to regulate activators and traps for multimode luminescence – A new strategy13Tunable phosphor properties of the CaAl2SiO6 polycrystals doped with chromium, manganese and vanadium ions4Dual-Mode Optical Thermometers Via the Thermochromic Mn2+/Mn4+ Co-Doped Mg0.388al2.408o4 Phosphors for Real-Time Chip Temperature Monitoring0Modulating Mn self-reduction and multimodal luminescence in CaSb 2 O 6 through La 3+ doping for quadruple-mode dynamic anti-counterfeiting and optical temperature sensing applications18Synthesis of Mn 2+ and Pr 3+ co-doped Zn 2 GeO 4 -graphene quantum dot nanorod bundles as an optical probe for sensing pH and temperature and for information encryption0Multi-color luminescent material with Mn2+/Mn4+ non-stoichiometric ratio doped octahedra and its anti-counterfeiting applications7Regulated synthesis of 3D nano-flower-like MnCo2O4.5 catalytic materials to enhance thermal decomposition of ammonium perchlorate5Adjusting luminescence properties of ZnAl2O4:Mn2+(Mn4+), Li+ phosphors through cation substitution1Multi-color and multi-mode luminescence tuning in persistent phosphors by trap engineering6Structure Modulation and Charge Transfer in Self‐Reduction Phosphors: A Review18Synthesis and Structure of Manganese Complexes with N,N'-bis[(2,4,6-trimethylphenyl)imino]acenaphthene2Fiber temperature sensor based on dual-wavelength emitting Mg0.388Al2.408O4: Mn2+/Mn4+ phosphors for real-time temperature monitoring5Super‐Sensitive Multi‐Modal Optical Manometer Based on Huge Pressure‐Induced Spectral Red‐Shift and Broadening of Mn2+ Emission Band in Green‐Emitting Zn2GeO4 Phosphors20Synthesis and Structure of Manganese Complexes with N,N’-bis[(2,4,6-trimethylphenyl)imino]acenaphthene0Prediction and explanation of the self-reduction of Eu3+ → Eu2+ and Mn4+ → Mn2+ using Site Occupancy Theory (SOT)6Zn 2 GeO 4 :Cr,Mn phosphor for visible to NIR luminescence-based applications – a theoretical and experimental investigation2Mn–Mn Dimers Induced Multimode Emitters in Mn2+-Activated AZn4(PO4)3 (A = K, Rb, and Cs) with Unique [Zn4PO12] Chains and [ZnOn] Groups3Consequences of tuning rare-earth element (Eu+3)-doping site and Exchange–Correlation energy U on the optoelectronic and mechanical properties of Ca2SnO4 for optoelectronics applications1Mn2+ and Mn4+ competition in photoluminescence and persistent luminescence4The thermal decomposition of ammonium perchlorate and HTPB-CSP combustion is promoted by the “litchi” core-shell structure of MnCo2O4.51Defect-Induced Self-Reduction of Manganese in Zn2SiO4 via Nonequivalent Doping of Yb3+ and B3+ for Dynamic Multimode Optical Information Storage and Information Encryption2Effect of BaO Content on the Photoluminescence Properties of Mn2+ and Eu2+-Codoped Sr3−xBaxMgSi2O8 Phosphors1Self-reduction-induced Mn heterovalent coexistence for Vis–NIR dual-emission16Site‐Selective Occupation of Mn 2+ Activators for Tunable Luminescence in Well‐Designed CaZnGe 2 O 6 Phosphors7Dual-emitting Mn4+-doped Tb3Al5O12 garnet phosphor for high-sensitive, self-referenced optical thermometry0Mn2+ occupancy luminescence and anti-thermal quenching behavior provoked by Mn4+ self-reduction based on construction luminescent glass-ceramics of silica fume substitution3Strategies to achieve Mn5 + -activated highly efficient phosphor for near infrared-II LED light source2Excitation power dependence and trap density of photo-stimulated luminescence in Zn 2 GeO 4 :Mn 2+ phosphor2MnO-induced network strengthening and tunable red emission in gallium germanophosphate glasses0Temperature sensing, anti-counterfeiting and binary encoded applications of the phosphor (Ca,Zn)2Ge7O16/Zn2GeO4:Mn2 +0Optimization of Doping Concentration for Upconversion Emission from Zn2GeO4:Er3+ Phosphor0

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  4. An efficient synthetic strategy for uniform perovskite core–shell nanocubes NaMgF 3 :Mn 2+ ,Yb 3+ @NaMgF 3 :Yb 3+ with enhanced near infrared upconversion luminescence

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  6. Persistent luminescence found in Mg 2+ and Pr 3+ co-doped LiNbO 3 single crystal

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  13. Non-stoichiometric defect-controlled reduction toward mixed-valence Mn-doped hexaaluminates and their optical applications

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