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RESEARCH PAPER · Chemistry of Materials · 2020

Localized Charge Accumulation Driven by Li+ Incorporation for Efficient LED Phosphors with Tunable Photoluminescence

Yibo Chen, Jinquan Chen, Jinhui Liang, Jin He, Zhao‐Qing Liu, Yadong Yin

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Localized Charge Accumulation Driven by Li+ Incorporation for Efficient LED Phosphors with Tunable PhotoluminescenceOriginalBa 3 YB 3 O 9 based phosphor ceramic plates with excellent thermal stability for wLED applications18Unraveling the valence states of manganese ions and the effects of composition variation and post-processing in YGG1--LuGG :Mn garnet optical sensor14Structural and spectroscopic investigation of an efficient and broadband NIR phosphor InBO3: Cr3+ and its application in NIR pc-LEDs106A Study on the Anti-thermal Dy3+/Eu3+ Co-doped BaLa4Si3O13 Red Phosphors for White-Light-Emitting Diodes and Optical Thermometry Applications41Effect of Li+ doping on the luminescence performance of a novel KAlSiO4:Tb3+ green-emitting phosphor46Combinations of Superior Inorganic Phosphors for Level‐Tunable Information Hiding and Encoding61A novel Eu3+-doped ScCaO(BO3) red phosphor for tricolor-composited high color rendering white light15Thermal Properties of Red Zero-Phonon Luminescence Line from Mn 2+ Ions in Oxide Crystals1Two-step synthetic route towards Er3+/Yb3+ co-doped vernier yttrium oxyfluoride phosphor with high optical temperature sensing sensitivity10Novel Orange Color Pigments Based on La3LiMnO73Achieving highly thermostable red emission in singly Mn 2+ -doped BaXP 2 O 7 (X = Mg/Zn) via self-reduction36Flexible ligand–Gd dye-encapsulated dual-emission metal–organic framework18Lattice-site engineering in ZnGa 2 O 4 :Cr 3+ through Li + doping for dynamic luminescence and advanced optical anti-counterfeiting55Optical spectroscopy of the Sr 4 Al 14 O 25 :Mn 4+ ,Cr 3+ phosphor: pressure and temperature dependences17Perylene diimide derivative dispersed in LDH as a new efficient red-emitting phosphor for LED applications7Thermal stability and self-reduction of a new red phosphor NaMg(PO 3 ) 3 :Mn 2+17Suppression of charge imbalance via Li+-Mn4+ co-incorporated Sr2YSbO6 red phosphors for warm w-LEDs43Site Preference-Driven Mn 4+ Stabilization in Double Perovskite Phosphor Regulating Quantum Efficiency from Zero to Champion53Luminescent properties of Mn4+ in an oxyfluoride complex with ultra-high thermal stability10Luminescence and interstitial-defect-related self-reduction in Mn2+ activated Ba3BP3O12 phosphor13Spectral engineering and thermometric performance of LiIn(Si2-Ge )O6: Cr3+ phosphor for multi-mode NIR thermometry26Highly Efficient Broad-Band Green-Emitting Cerium(III)-Activated Garnet Phosphor Allows the Fabrication of Blue-Chip-Based Warm-White LED Device with a Superior Color Rendering Index69Thermal-responsive dynamic color-tunable persistent luminescence from green to deep red for advanced anti-counterfeiting75Greatly enhanced deep-red luminescence performance of Ca2InSbO6:Mn4+ phosphor via multiple optimization strategies34A selective replacement strategy to a deep-red phosphor for plant growth and optical temperature sensing11The design of the highly active NH3-SCR catalyst Ce-W/UiO-66: Close coupling of active sites and acidic sites28LED-pumped intense red luminescence based on Ba2LaTaO6: Mn4+ double perovskite phosphor39A novel Cr3+-doped stannate far red phosphor for plant lighting: structure evolution, broad-narrow spectrum tuning and application prospect39Mn ions‐activated Gd 3 (Al,Ga) 5 O 12 garnet solid‐solution ceramics: Cation substitution for dual wavelength red‐emission13Recent Developments of Microscopic Study for Lanthanide and Manganese Doped Luminescent Materials8Novel high-saturated red-emitting phosphor Sr9(Mg0.5Mn0.5)K(PO4)7: Eu2+ with great quantum efficiency enhancement by La3+ codoping for white LED application16Enhanced luminescence of Mn4+ equivalently doped fluoride phosphors by reducing defects and impurities16Realization of highly efficient Ba2SrWO6:Mn4+ phosphor via La addition strategy and application for plant cultivation LED40Improving the luminescence performance of far-red-emitting Sr2ScSbO6:Mn4+ phosphor with charge compensation and its application in plant growth LEDs54Achieving excellent thermostable red emission in singly Mn 2+ -doped near-zero thermal expansion (NZTE) material Li 2 Zn 3 (P 2 O 7 ) 26Deep-red-emitting phosphors of Mn 4+ -activated tantalite for high-sensitivity lifetime thermometry and security films10Designing and controlling the Ni 2+ -activated (Zn, Mg)Al 2 O 4 spinel solid-solution for phosphor-converted broadband near-infrared illumination81Enhanced Up-Conversion Persistent Luminescence of Zn2geo4:Mn Phosphors by Non-Equivalent Doping and Sensitization of Up-Conversion Nanocrystals0Equivalent chemical substitution in double–double perovskite-type ALaLiTeO 6 :Mn 4+ (A = Ba 2+ , Sr 2+ , Ca 2+ ) phosphors enabling wide range crystal field strength regulation and efficient far-red emission17Suppressed Self‐Reduction of Manganese in Mg 2 SnO 4 via Li + Incorporation with Polychromatic Luminescence for Versatile Applications66Synthesis and luminescent properties of Mn4+-doped Li2.06Nb0.18Ti0.76O3 high color purity red-emission phosphor6Downconverted significant luminescence enhancement and structural confinement of a dichromatic nanophosphor for potential applications in NUV-triggered cool pc-WLEDs9Precisely Manipulating the Self‐Reduction of Manganese in MgGa2O4 through Lithium Incorporation for Optical Thermometry and Anti‐Counterfeiting64Breaking the balance of chemical ratio in ZnAl2O4 to regulate activators and traps for multimode luminescence – A new strategy13Be 2+ ‐Induced Red Emission Enhancement in CaAl 12 O 19 :Mn 4+ for Wide Color Gamut Display: Suppressing Self‐Reduction of Mn 4+ to Mn 2+26Luminescence properties and high energy transfer of Ca9MgNa (PO4)7: Eu2+, Mn2+ blue-red dual emission phosphor for plant growth LEDs17Enhanced up-conversion persistent luminescence of Zn2GeO4:Mn phosphors by non-equivalent doping and sensitization of up-conversion nanocrystals12Mechanistic Insight into the Defect-Engineered White Light Emission from the Single-Phase Orthovanadate Phosphor Synthesized by a Facile Rapid Microwave-Assisted Synthesis17Mg4InSbO8 Spinel: Double 2:1 Ordering in Tetrahedral and Octahedral Sublattices and Perspective Application as an Optical Thermometer via Mn2+/4+ Doping19Charge compensators achieve controlled self-reduction of Europium in BaMgP2O730Blue Ca4MgAl2Si3O14:Ce3+, Li+ phosphor with excellent performance for human-centered green plant growth lighting12Abnormal anti-thermal quenching of Mn 2+ and reverse thermal response of Mn 2+ /Mn 4+ luminescence in garnet phosphor for wide-range temperature sensing26Structural confinement helps achieve more accurate energy transfer: studies on garnet structural NYGlG:Tb 3+ ,Eu 3+ phosphors17Structure and photoluminescence of Mn 2+/4+ -activated doubly ordered spinel Mg 4 (Ga/Al)SbO 8 : site-selective Al 3+ -to-Ga 3+ substitution enabling Mn 4+ accumulation, excellent anti-thermal quenching of Mn 2+ green emission, and optical thermometry17Unravelling the white light emission in a single-phase new stoichiometric vanadate phosphor synthesized by rapid low-temperature one-pot synthesis and its W-LED prototype with high CRI and luminous efficacy13Multicolor regulation of trivalent lanthanide ions-codoped boggildite-type phosphor toward superb warm white luminescence for white light-emitting diodes13Grafting Carbon Dots on Persistent Luminescence Phosphors to Generate Remarkably Improved NIR Afterglow for Microenvironment Fluorescence Detection5High temperature sensing performance based on optical thermometry in ZnAl2O4:Eu3+-ZnTiO3:Mn4+ mixed composites4Structural and luminescence properties of MgO: Li nanocrystals5Cation Occupation Engineering Realizes Valence Modulation of Manganese-Activated ZnGa2O414Enhanced color rendering index and thermal stability of Ca2GdNbO6: Dy3+ phosphors by co-doping Sm3+ ions28Toward Controllable Self‐Reduction of Mn4+ to Mn2+ by Lanthanide Ions for Luminescence Based Colorimetric Sensing of Temperature16Solid-state lighting and anti-counterfeiting applications based on double perovskite Ca2GdNbO6:Dy3+, Eu3+ phosphors17A Ca 7 Mg 1.8 Zn 0.2 Ga 6 O 18 :Bi 3+ /Mn 4+ phosphor: energy transfer enables tuneable colour emission and high sensitivity in optical thermometry3Preparation, adsorption and structure of Ce doped layered manganese ion-sieve based on Li2MnO3 spatial structure12Intensive Enhancement of Near‐Infrared Emission in ZnAl 2 O 4 :Fe 3+ via Li‐Substitution for Application in Identifying Lithium Bearing Ores19Enlarging Environmental Asymmetry by the Site Tailoring to Enhance Luminescence Properties of Sm3+ in the (Gd,Na)3(Ga,In)2(Ga,Ge)3O12 Garnet21Time- and temperature-dependent dynamic fluorescence of non-stoichiometric induced defective phosphors and multiple applications33Tb3+/Eu3+ doped Y3GaO6 phosphors for color tunable emission11Self-reduction-induced Mn heterovalent coexistence for Vis–NIR dual-emission16Tm3+/Dy3+ activated single-component niobate phosphors with low correlated color temperature and high thermal stability for white LEDs applications5Manganese valence modulation in ZnGa2O4 via simultaneously localized charge accumulation and oxygen vacancy engineering controlled by Li+ and F− substitutions for tailored applications2Preparation and enhanced photoluminescence features of white-emitting single-phased Ba3Sc(PO4)3: Dy3+ phosphors for light-emitting diodes though the use of flux1Suppressing oxygen vacancies and boosting Fe3+ near-infrared emission via charge compensation0Color-tunable Luminescence via Valence-state modulation in Mn-doped Zn2Sn1-xTixO40Dual‑substitution strategy for highly efficient Far‑red Mn4+‑doped double perovskite phosphors toward plant growth lighting0Achieving Far-Red Emission with Ultrahigh Quantum Efficiency in Mn4+-Activated Sr4AlNbO8 Phosphors Derived from Ge-Induced Valence State Modulation and Crystal Field Engineering0

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