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RESEARCH PAPER · Chemical Reviews · 2017

Lanthanide-Activated Phosphors Based on 4f-5d Optical Transitions: Theoretical and Experimental Aspects

Xian Qin, Xiaowang Liu, Xiaowang Liu, Wei Huang, Marco Bettinelli, Xiaogang Liu, Xiaogang Liu

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Lanthanide-Activated Phosphors Based on 4f-5d Optical Transitions: Theoretical and Experimental AspectsOriginalA 980 nm laser-activated upconverted persistent probe for NIR-to-NIR rechargeable in vivo bioimaging93Selective Aerobic Oxidation of Methylarenes to Benzaldehydes Catalyzed by N ‐Hydroxyphthalimide and Cobalt(II) Acetate in Hexafluoropropan‐2‐ol245Tunable Optical Properties and Increased Thermal Quenching in the Blue-Emitting Phosphor Series: Ba2(Y1–xLux)5B5O17:Ce3+ (x = 0–1)185Temperature and Eu2+-Doping Induced Phase Selection in NaAlSiO4 Polymorphs and the Controlled Yellow/Blue Emission95Upconversion nanoprobes for biodetections138Binary temporal upconversion codes of Mn2+-activated nanoparticles for multilevel anti-counterfeiting386Critical Review—Narrow-Band Emission of Nitride Phosphors for Light-Emitting Diodes: Perspectives and Opportunities72Upconversion manipulation by local electromagnetic field127Bluish-White Luminescence in Rare-Earth-Free Vanadate Garnet Phosphors: Structural Characterization of LiCa3MV3O12 (M = Zn and Mg)108A pre-protective strategy for precise tumor targeting and efficient photodynamic therapy with a switchable DNA/upconversion nanocomposite67Controllable two-dimensional luminescence tuning in Eu 2+ ,Mn 2+ doped (Ca,Sr) 9 Sc(PO 4 ) 7 based on crystal field regulation and energy transfer61Efficient rare-earth free red-emitting Ca 2 YSbO 6 :Mn 4+ ,M(M = Li + , Na + , K + , Mg 2+ ) phosphors for white light-emitting diodes117Photoluminescence and energy transfer properties of a novel molybdate KBaY(MoO 4 ) 3 :Ln 3+ (Ln 3+ = Tb 3+ , Eu 3+ , Sm 3+ , Tb 3+ /Eu 3+ , Tb 3+ /Sm 3+ ) as a multi-color emitting phosphor for UV w-LEDs143Photoluminescence tuning in a novel Bi 3+ /Mn 4+ co-doped La 2 ATiO 6 :(A = Mg, Zn) double perovskite structure: phase transition and energy transfer78Remote manipulation of upconversion luminescence275Deciphering the Role of Charge Compensator in Optical Properties of SrWO4:Eu3+:A (A = Li+, Na+, K+): Spectroscopic Insight Using Photoluminescence, Positron Annihilation, and X-ray Absorption115Understanding and Controlling the Emission Brightness and Color of Molecular Cerium Luminophores87Understanding the Interactions between Vibrational Modes and Excited State Relaxation in Y3–xCexAl5O12: Design Principles for Phosphors Based on 5d–4f Transitions72Long-Lived Emissive Probes for Time-Resolved Photoluminescence Bioimaging and Biosensing923Inherently Eu2+/Eu3+ Codoped Sc2O3 Nanoparticles as High‐Performance Nanothermometers268Highly Efficient Blue Emission and Superior Thermal Stability of BaAl 12 O 19 :Eu 2+ Phosphors Based on Highly Symmetric Crystal Structure388Ba3Y2B6O15:Ce3+—A High Symmetry, Narrow-Emitting Blue Phosphor for Wide-Gamut White Lighting188Exploring Lanthanide Doping in UiO-66: A Combined Experimental and Computational Study of the Electronic Structure67Advances in highly doped upconversion nanoparticles1115Efficient Blue-emitting Phosphor SrLu2O4:Ce3+ with High Thermal Stability for Near Ultraviolet (~400 nm) LED-Chip based White LEDs67Domino-like multi-emissions across red and near infrared from solid-state 2-/2,6-aryl substituted BODIPY dyes109Eu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable Luminescence577Lanthanide Doped Near Infrared Active Upconversion Nanophosphors: Fundamental Concepts, Synthesis Strategies, and Technological Applications156Structural Confinement toward Giant Enhancement of Red Emission in Mn2+‐Based Phosphors165Persistent luminescence instead of phosphorescence: History, mechanism, and perspective680Achieving Thermo‐Mechano‐Opto‐Responsive Bitemporal Colorful Luminescence via Multiplexing of Dual Lanthanides in Piezoelectric Particles and its Multidimensional Anticounterfeiting283Identifying an efficient, thermally robust inorganic phosphor host via machine learning362Lanthanide Photocatalysis281Graphene quantum dots from chemistry to applications895X-ray-activated long persistent phosphors featuring strong UVC afterglow emissions252Are lanthanide-doped upconversion materials good candidates for photocatalysis?110Recent advances in near-infrared emitting lanthanide-doped nanoconstructs: Mechanism, design and application for bioimaging310Energy Flux Manipulation in Upconversion Nanosystems108Broadband NIR photostimulated luminescence nanoprobes based on CaS:Eu 2+ ,Sm 3+ nanocrystals96Crystal structure and photoluminescence tuning of novel single-phase Ca 8 ZnLu(PO 4 ) 7 :Eu 2+ ,Mn 2+ phosphors for near-UV converted white light-emitting diodes61Density-functional theory calculations, luminescence properties and fluorescence ratiometric thermo-sensitivity for a novel borate based red phosphor: NaBaSc(BO 3 ) 2 :Ce 3+ ,Mn 2+58Polypyridyl ligands as a versatile platform for solid-state light-emitting devices125Discovery of New Narrow‐Band Phosphors with the UCr 4 C 4 ‐Related Type Structure by Alkali Cation Effect137Li substituent tuning of LED phosphors with enhanced efficiency, tunable photoluminescence, and improved thermal stability205Energy-Transfer Editing in Lanthanide-Activated Upconversion Nanocrystals: A Toolbox for Emerging Applications162Engineering Tunable Broadband Near‐Infrared Emission in Transparent Rare‐Earth Doped Nanocrystals‐in‐Glass Composites via a Bottom‐Up Strategy68Recent advances in solid-state LED phosphors with thermally stable luminescence325New strategy for designing orangish-red-emitting phosphor via oxygen-vacancy-induced electronic localization348Rare earth ion– and transition metal ion–doped inorganic luminescent nanocrystals: from fundamentals to biodetection98Synthesis, spectroscopic properties and applications of divalent lanthanides apart from Eu2+108Full‐Spectrum Persistent Luminescence Tuning Using All‐Inorganic Perovskite Quantum Dots139Unraveling the Mechanisms of Thermal Quenching of Luminescence in Ce3+-Doped Garnet Phosphors238Relationship of Stokes shift with composition and structure in Ce3+/Eu2+-doped inorganic compounds62Prevailing Strategies to Tune Emission Color of Lanthanide‐Activated Phosphors for WLED Applications278Excitation Wavelength-Dependent Dual-Mode Luminescence Emission for Dynamic Multicolor Anticounterfeiting134Highly Water-Stable Dye@Ln-MOFs for Sensitive and Selective Detection toward Antibiotics in Water218Lanthanide Photonics: Shaping the Nanoworld166Multicolour emission from thermally stable Tb3+/Eu3+ co-doped CaLa4Si3O13 phosphors for single-component w-LEDs application61Non-Rare-Earth Na3AlF6:Cr3+ Phosphors for Far-Red Light-Emitting Diodes125Samarium-Activated La2Hf2O7 Nanoparticles as Multifunctional Phosphors57Tunable lanthanide/transition metal ion‐doped novel phosphors for possible application in w‐LEDs: a review77Insights into the complexity of the excited states of Eu-doped luminescent materials72Evaluating Thermal Quenching Temperature in Eu 3+ -Substituted Oxide Phosphors via Machine Learning81Exploiting bandgap engineering to finely control dual-mode Lu 2 (Ge,Si)O 5 :Pr 3+ luminescence thermometers59Rare-earth-containing perovskite nanomaterials: design, synthesis, properties and applications422Unraveling the impact of different thermal quenching routes on the luminescence efficiency of the Y 3 Al 5 O 12 :Ce 3+ phosphor for white light emitting diodes76UV-Vis-NIR absorption spectra of lanthanide oxides and fluorides96Multiple Substitution Strategies toward Tunable Luminescence in Lu2MgAl4SiO12:Eu2+ Phosphors90Highly Efficient Green‐to‐Yellowish‐Orange Emitting Eu2+‐Doped Pyrophosphate Phosphors with Superior Thermal Quenching Resistance for w‐LEDs99A promising temperature sensing strategy based on highly sensitive Pr3+-doped SrRE2O4 (RE = Sc, Lu and Y) luminescent thermometers72Interstitial Site Engineering for Creating Unusual Red Emission in La3Si6N11:Ce3+57Lanthanide‐Doped Core@Multishell Nanoarchitectures: Multimodal Excitable Upconverting/Downshifting Luminescence and High‐Level Anti‐Counterfeiting188Persistent Emission of Narrowband Ultraviolet-B Light upon Blue-Light Illumination64Site-selective occupation of Eu2+ activators toward full-visible-spectrum emission in well-designed borophosphate phosphors96X‐Ray‐Induced Persistent Luminescence Promotes Ultrasensitive Imaging and Effective Inhibition of Orthotopic Hepatic Tumors81Tri-channel photon emission of lanthanides in lithium-sublattice core-shell nanostructures for multiple anti-counterfeiting67Dual-Channel Luminescent Signal Readout Strategy for Classifying Aprotic/Protic Polar Organic Medium and Naked-Eye Monitoring of Water in Organic Solvents66A novel narrow-band blue-emitting phosphor of Bi3+-activated Sr3Lu2Ge3O12 based on a highly symmetrical crystal structure used for WLEDs and FEDs183Narrow-band emitters in LED backlights for liquid-crystal displays217Rare earth elements (REE) in biology and medicine88Macrocyclic Ligands with an Unprecedented Size-Selectivity Pattern for the Lanthanide Ions94A review on fluorescence intensity ratio thermometer based on rare-earth and transition metal ions doped inorganic luminescent materials440Abnormal Bi3+-Activated NIR Emission in Highly Symmetric XAl12O19 (X = Ba, Sr, Ca) by Selective Sites Occupation106Efficient rare earth cerium(III) complex with nanosecond d−f emission for blue organic light-emitting diodes63Deep-blue organic light-emitting diodes based on a doublet d–f transition cerium(III) complex with 100% exciton utilization efficiency83Enhanced Cyan Emission and Optical Tuning of Ca 3 Ga 4 O 9 :Bi 3+ for High‐Quality Full‐Spectrum White Light‐Emitting Diodes139Energy Transfer in Metal–Organic Frameworks and Its Applications57Structural Engineering of Eu2+-Doped Silicates Phosphors for LED Applications242Anti‐Thermal‐Quenching Bi 3+ Luminescence in a Cyan‐Emitting Ba 2 ZnGe 2 O 7 :Bi Phosphor Based on Zinc Vacancy162Photochromic and fluorescent ink using photoluminescent strontium aluminate pigment and screen printing towards anticounterfeiting documents79Red-tunable LuAG garnet phosphors via Eu 3+ →Mn 4+ energy transfer for optical thermometry sensor application72Nanorods with multidimensional optical information beyond the diffraction limit62Design of a Bismuth-Activated Narrow-Band Cyan Phosphor for Use in White Light Emitting Diodes and Field Emission Displays100Photocatalytic Aerobic Oxidative Ring Expansion of Cyclic Ketones to Macrolactones by Cerium and Cyanoanthracene Catalysis82Doping Lanthanide Ions in Colloidal Semiconductor Nanocrystals for Brighter Photoluminescence241Intense UV long persistent luminescence benefiting from the coexistence of Pr 3+ /Pr 4+ in a praseodymium-doped BaLu 2 Al 2 Ga 2 SiO 12 phosphor57Photon management to reduce energy loss in perovskite solar cells197Recent Advances and Opportunities of Lead-Free Perovskite Nanocrystal for Optoelectronic Application95Improving the thermal stability and luminescent efficiency of (Ba,Sr)3SiO5:Eu2+ phosphors by structure, bandgap engineering and soft chemistry synthesis method98Perovskite Quantum Dots Glasses Based Backlit Displays351Site‐Selective Occupancy of Eu2+ toward High Luminescence Switching Contrast in BaMgSiO4‐Based Photochromic Materials63Eu 2+ Stabilized at Octahedrally Coordinated Ln 3+ Site Enabling Red Emission in Sr 3 LnAl 2 O 7.5 (Ln = Y or Lu) Phosphors61A Review on X-ray Excited Emission Decay Dynamics in Inorganic Scintillator Materials98Exploring Heterostructured Upconversion Nanoparticles: From Rational Engineering to Diverse Applications143Recent Developments in Lanthanide-Doped Alkaline Earth Aluminate Phosphors with Enhanced and Long-Persistent Luminescence68Novel and wide-ranging color tuning photoluminescence properties of Tb3+/Eu3+ doped garnet-type Li3Lu3Te2O12 phosphor: Energy transfer and enhanced thermal stability70Rare earth (RE) doped phosphors and their emerging applications: A review632Advancing Graphitic Carbon Nitride-Based Photocatalysts toward Broadband Solar Energy Harvesting102Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids83MMCT-induced high-bright yellow light-emitting phosphor Bi3+-activated Ba2YGaO5 used for WLED124Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications171Enhancing luminescence intensity and improving thermostability of red phosphors Li3Ba2La3(WO4)8:Eu3+ by co-doping with Sm3+ ions59Multi-responsive deep-ultraviolet emission in praseodymium-doped phosphors for microbial sterilization77Full-visible-spectrum lighting enabled by site-selective occupation in the high efficient and thermal stable (Rb, K)2CaPO4F: Eu2+ solid-solution phosphors58Exploration of Nontoxic Cs3CeBr6 for Violet Light-Emitting Diodes98Water-stable europium(III) and terbium(III)-metal organic frameworks as fluorescent sensors to detect ions, antibiotics and pesticides in aqueous solutions59Recent advances in radiation therapy and photodynamic therapy75A highly efficient narrow-band blue phosphor of Bi3+-activated cubic borate Ba3Lu2B6O15 towards backlight display applications85Rare-Earth Doping in Nanostructured Inorganic Materials1202How to Obtain Anti‐Thermal‐Quenching Inorganic Luminescent Materials for Light‐Emitting Diode Applications252Eu2+ Doping Concentration-Induced Site-Selective Occupation and Photoluminescence Tuning in KSrScSi2O7:Eu2+ Phosphor77Nanochemistry advancing photon conversion in rare-earth nanostructures for theranostics127Realizing Simultaneous X‐Ray Imaging and Dosimetry Using Phosphor‐Based Detectors with High Memory Stability and Convenient Readout Process70Rare‐Earth‐Based Perovskite Cs2AgScCl6:Bi for Strong Full Visible Spectrum Emission90Controlling X-ray-activated persistent luminescence for emerging applications69Low-concentration Ce3+-activated ScCaO(BO3) blue-cyan phosphor with high efficiency toward full-spectrum white LED applications58Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Special Issue: Rare earth luminescent materials167Next generation lanthanide doped nanoscintillators and photon converters118A Hierarchical Structure Perovskite Quantum Dots Film for Laser‐Driven Projection Display121Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure137A novel red-emitting Na5W3O9F5:Eu3+ phosphor with high color purity for blue-based WLEDs61Spectra stable deep-blue light-emitting diodes based on cryolite-like cerium(III) halides with nanosecond d-f emission64Recent development in color tunable phosphors: A review205Ba 3 LuGa 2 O 7.5 :Bi 3+ phosphors with potential application in full-spectrum WLEDs and temperature sensing73Lanthanide molecular cluster-aggregates as the next generation of optical materials69Lead-free hybrid indium perovskites with near-unity PLQY and white light emission using an Sb 3+ doping strategy82Facile Synthesis of Highly Efficient and Thermally Stable BaAl 4 Sb 2 O 12 :Eu 2+ Phosphor in Air72Giant Pressure‐Induced Spectral Shift in Cyan‐Emitting Eu 2+ ‐Activated Sr 8 Si 4 O 12 Cl 8 Microspheres for Ultrasensitive Visual Manometry86Deep‐Red Ca3Al2Ge3O12:Eu3+ Garnet Phosphor with Near‐Unity Internal Quantum Efficiency and High Thermal Stability for Plant Growth Application67Recent progress in lanthanide ions doped inorganic metal halide perovskites69Multimodal luminescence in Pr3+ single-doped Li2CaSiO4 phosphor for optical information storage and anti-counterfeiting applications128Site Occupation Engineering toward Giant Red-Shifted Photoluminescence in (Ba,Sr)2LaGaO5:Eu2+ Phosphors63The Electron Migration Polarization Boosting Electromagnetic Wave Absorption Based on Ce Atoms Modulated yolk@shell Fe x N@NGC141Advancements in rare earth metal-organic frameworks: Harnessing the power of photonics and beyond60Enhancement of Electromagnetic Wave Attenuation through Polarization Loss Induced by Hybridization of Rare‐Earth 4f and Mo‐4d Orbitals in Liquid Plasma93Self‐Calibrated Thermometer and Dynamic Anti‐Counterfeiting Based on YNbO4:Pr3+ Luminescent Material68Suppressed concentration quenching and tunable photoluminescence in Eu2+-activated Rb3Y(PO4)2 phosphors for full-spectrum lighting87Compositional engineering of phase-stable and highly efficient deep-red emitting phosphor for advanced plant lighting systems94Enhanced photocatalytic performance of Ce3+-doped ZnIn2S4 through vacancy engineering for efficient hydrogen evolution and pollutant degradation68

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  38. Synthesis, electronic structures, and photoluminescence properties of an efficient and thermally stable red-emitting phosphor Ca 3 ZrSi 2 O 9 :Eu 3+ ,Bi 3+ for deep UV-LEDs

    RSC Advances · 2018-01-01

    Jiyou Zhong, Weiren Zhao, Lunwei Yang, Peng Shi, Zifeng Liao, Menglong Xia, Wenhua Pu, Wei Xiao, Ligen Wang

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  39. Deciphering the Role of Charge Compensator in Optical Properties of SrWO4:Eu3+:A (A = Li+, Na+, K+): Spectroscopic Insight Using Photoluminescence, Positron Annihilation, and X-ray Absorption

    Inorganic Chemistry · 2018-01-02

    Santosh K. Gupta, Kathi Sudarshan, Ashok Kumar Yadav, Ruma Gupta, D. Bhattacharyya, S. N. Jha, Ramakant Mahadeo Kadam

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  40. Biocompatible Chitosan-Functionalized Upconverting Nanocomposites

    ACS Omega · 2018-01-04

    Hau Van Duong, Trang The Lieu Chau, Nhan Thi Thanh Dang, Frankie Vanterpool, Manuel Salmerón‐Sánchez, Erlantz Lizundia, Hoa Thai Tran, Nguyen Viet Long, Thanh‐Dinh Nguyen

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  41. Excitation Position Sensitive Upconversion Emission of Lanthanide Ions Doped β‐NaYF4 Single Microcrystals

    ChemNanoMat · 2018-01-05

    Bing Wang, Jiao Wang, Gaoshan Huang, Shilong Li, Yongfeng Mei

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  42. Optical Properties of Ce-Doped Li4SrCa(SiO4)2: A Combined Experimental and Theoretical Study

    Inorganic Chemistry · 2018-01-05

    Rui Shi, Xiaoxiao Huang, Tiantian Liu, Litian Lin, Chunmeng Liu, Yan Huang, Lirong Zheng, Lixin Ning, H. Liang

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  43. Spectroscopic peculiarities of CsCaI3:Tm2+ single crystals examined through one-photon and excited state excitation spectroscopy

    Journal of Alloys and Compounds · 2018-01-05

    Mirosław Karbowiak, Radosław Lisiecki, Piotr Solarz, Jarosław Komar, Witold Ryba‐Romanowski

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  44. Understanding and Controlling the Emission Brightness and Color of Molecular Cerium Luminophores

    Journal of the American Chemical Society · 2018-01-23

    Yusen Qiao, Dumitru‐Claudiu Sergentu, Haolin Yin, Alexander V. Zabula, Thibault Cheisson, Alex McSkimming, Brian C. Manor, Patrick J. Carroll, Jessica M. Anna, Jochen Autschbach, Eric J. Schelter

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  45. Efficient NIR Emission from Nd, Er, and Tm Complexes with Fluorinated Selenolate Ligands

    Inorganic Chemistry · 2018-01-26

    Wen Wu, Xin Zhang, Anna Y. Kornienko, G.A. Kumar, Dechao Yu, Thomas J. Emge, Richard E. Riman, John G. Brennan

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  46. Energy Transfer in Dye‐Coupled Lanthanide‐Doped Nanoparticles: From Design to Application

    Chemistry - An Asian Journal · 2018-01-30

    Juan Wang, Renren Deng

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  47. Understanding the Interactions between Vibrational Modes and Excited State Relaxation in Y3–xCexAl5O12: Design Principles for Phosphors Based on 5d–4f Transitions

    Chemistry of Materials · 2018-01-30

    Yuan-Chih Lin, Paul Erhart, Marco Bettinelli, Nathan C. George, Stewart F. Parker, Maths Karlsson

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  48. Long-Lived Emissive Probes for Time-Resolved Photoluminescence Bioimaging and Biosensing

    Chemical Reviews · 2018-02-02

    Kenneth Yin Zhang, Qi Yu, Huanjie Wei, Shujuan Liu, Qiang Zhao, Wei Huang

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  49. Bright Photoluminescence of [{(Cp)2Ce(μ‐Cl)}2]: A Valuable Technique for the Determination of the Oxidation State of Cerium

    Chemistry - An Asian Journal · 2018-02-06

    Markus Suta, Nicole Harmgarth, Marcel Kühling, Phil Liebing, Frank Thomas Edelmann, Claudia Wickleder

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  50. Inherently Eu2+/Eu3+ Codoped Sc2O3 Nanoparticles as High‐Performance Nanothermometers

    Advanced Materials · 2018-02-12

    Yue Xiao Pan, Xiaoji Xie, Qianwen Huang, Chao Gao, Yangbo Wang, Lingxiao Wang, Bingxiao Yang, Haiquan Su, Ling Huang, Wei Huang

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