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RESEARCH PAPER · Progress in Materials Science · 2016

Progress in discovery and structural design of color conversion phosphors for LEDs

Zhiguo Xia, Quanlin Liu

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Progress in discovery and structural design of color conversion phosphors for LEDsOriginalCe 3+ -Doped garnet phosphors: composition modification, luminescence properties and applications1149Broad near-ultraviolet and blue excitation band induced dazzling red emissions in Eu 3+ -activated Gd 2 MoO 6 phosphors for white light-emitting diodes124Design, preparation, and optimized luminescence of a dodec-fluoride phosphor Li 3 Na 3 Al 2 F 12 :Mn 4+ for warm WLED applications101Facile synthesis, morphology and photoluminescence of a novel red fluoride nanophosphor K 2 NaAlF 6 :Mn 4+115Stable narrowband red phosphor K 3 GaF 6 :Mn 4+ derived from hydrous K 2 GaF 5 (H 2 O) and K 2 MnF 677Structure and luminescence behavior of a single-ion activated single-phased Ba 2 Y 3 (SiO 4 ) 3 F:Eu white-light phosphor90Thermally stable K x Cs 1−x AlSi 2 O 6 :Eu 2+ phosphors and their photoluminescence tuning84Tuning of Photoluminescence and Local Structures of Substituted Cations in xSr2Ca(PO4)2–(1 – x)Ca10Li(PO4)7:Eu2+ Phosphors212Influence of Anion/Cation Substitution (Sr2+ → Ba2+, Al3+ → Si4+, N3– → O2–) on Phase Transformation and Luminescence Properties of Ba3Si6O15:Eu2+ Phosphors140Chemistry-Inspired Adaptable Framework Structures368Synthesis and luminescence characteristics of novel red-emitting Ba 2 TiGe 2 O 8 :Mn 4+ phosphor116Temperature and Eu2+-Doping Induced Phase Selection in NaAlSiO4 Polymorphs and the Controlled Yellow/Blue Emission95Novel red-emitting Sr 2 LaSbO 6 :Eu 3+ phosphor with enhanced 5 D 0 → 7 F 4 transition for warm white light-emitting diodes107Probing Eu2+ Luminescence from Different Crystallographic Sites in Ca10M(PO4)7:Eu2+ (M = Li, Na, and K) with β-Ca3(PO4)2-Type Structure145Synthesis of Y3Al5O12:Ce3+ phosphor in the Y2O3–Al metal–CeO2 ternary system108Highly Efficient and Stable Narrow-Band Red Phosphor Cs2SiF6:Mn4+ for High-Power Warm White LED Applications215Critical Review—A Review of the Electronic Structure and Optical Properties of Ions with d3Electron Configuration (V2+, Cr3+, Mn4+, Fe5+) and Main Related Misconceptions109Thermally stable double perovskite CaLaMgSbO6:Eu3+ phosphors as a tunable LED-phosphor material88Non‐Rare‐Earth K2XF7:Mn4+(X = Ta, Nb): A Highly‐Efficient Narrow‐Band Red Phosphor Enabling the Application in Wide‐Color‐Gamut LCD146Silica-Coated Mn-Doped CsPb(Cl/Br)3 Inorganic Perovskite Quantum Dots: Exciton-to-Mn Energy Transfer and Blue-Excitable Solid-State Lighting172Eu3+-doped double perovskite-based phosphor-in-glass color converter for high-power warm w-LEDs91Waterproof Narrow-Band Fluoride Red Phosphor K2TiF6:Mn4+ via Facile Superhydrophobic Surface Modification185Designed synthesis, morphology evolution and enhanced photoluminescence of a highly efficient red dodec-fluoride phosphor, Li 3 Na 3 Ga 2 F 12 :Mn 4+ , for warm WLEDs127A novel double perovskite tellurate Eu3+-doped Sr2MgTeO6 red-emitting phosphor with high thermal stability108Achieving High Quantum Efficiency Narrow-Band β-Sialon:Eu 2+ Phosphors for High-Brightness LCD Backlights by Reducing the Eu 3+ Luminescence Killer356Control of Luminescence by Tuning of Crystal Symmetry and Local Structure in Mn4+‐Activated Narrow Band Fluoride Phosphors113A green synthetic route to the highly efficient K 2 SiF 6 :Mn 4+ narrow-band red phosphor for warm white light-emitting diodes129A novel Cs 2 NbOF 5 :Mn 4+ oxyfluoride red phosphor for light-emitting diode devices83Controllable optical tuning and improvement in Li + ,Eu 3+ -codoped BaSc 2 O 4 :Bi 3+ based on energy transfer and charge compensation96Efficient rare-earth free red-emitting Ca 2 YSbO 6 :Mn 4+ ,M(M = Li + , Na + , K + , Mg 2+ ) phosphors for white light-emitting diodes117Enhanced luminescence of a Ba 2 GdSbO 6 :Mn 4+ red phosphor via cation doping for warm white light-emitting diodes146Mn 2+ and Mn 4+ red phosphors: synthesis, luminescence and applications in WLEDs. A review706Photoluminescence tuning in a novel Bi 3+ /Mn 4+ co-doped La 2 ATiO 6 :(A = Mg, Zn) double perovskite structure: phase transition and energy transfer78Structural construction and photoluminescence tuning via energy transfer in apatite-type solid-state phosphors81Weak thermal quenching of the luminescence in the Ca 3 Sc 2 Si 3 O 12 :Ce 3+ garnet phosphor87Near UV-pumped yellow-emitting Sr9MgLi(PO4)7:Eu2+ phosphor for white-light LEDs100On the crystal structure and luminescence characteristics of a novel deep red emitting SrLaScO4:Mn4+90Down-Conversion Nitride Materials for Solid State Lighting: Recent Advances and Perspectives794Mining Unexplored Chemistries for Phosphors for High-Color-Quality White-Light-Emitting Diodes136Highly Efficient Blue Emission and Superior Thermal Stability of BaAl 12 O 19 :Eu 2+ Phosphors Based on Highly Symmetric Crystal Structure388Redefinition of Crystal Structure and Bi3+ Yellow Luminescence with Strong Near-Ultraviolet Excitation in La3BWO9:Bi3+ Phosphor for White Light-Emitting Diodes180Luminescence of an Oxonitridoberyllate: A Study of Narrow-Band Cyan-Emitting Sr[Be 6 ON 4 ]:Eu 2+96Glass Ceramic Phosphors: Towards Long‐Lifetime High‐Power White Light‐Emitting‐Diode Applications–A Review356Red-Shifted Emission in Y3MgSiAl3O12:Ce3+ Garnet Phosphor for Blue Light-Pumped White Light-Emitting Diodes112Two-Dimensional-Layered Perovskite ALaTa2O7:Bi3+ (A = K and Na) Phosphors with Versatile Structures and Tunable Photoluminescence115Eu 2+ Site Preferences in the Mixed Cation K 2 BaCa(PO 4 ) 2 and Thermally Stable Luminescence577Tunable Optical Properties and Enhanced Thermal Quenching of Non-Rare-Earth Double-Perovskite (Ba1–xSrx)2YSbO6:Mn4+ Red Phosphors Based on Composition Modulation135Learning from a Mineral Structure toward an Ultra‐Narrow‐Band Blue‐Emitting Silicate Phosphor RbNa3(Li3SiO4)4:Eu2+226Learning from a Mineral Structure toward an Ultra‐Narrow‐Band Blue‐Emitting Silicate Phosphor RbNa3(Li3SiO4)4:Eu2+129Next‐Generation Narrow‐Band Green‐Emitting RbLi(Li 3 SiO 4 ) 2 :Eu 2+ Phosphor for Backlight Display Application532Design and Development of a Bluish-Green Luminescent Material (K2HfSi3O9:Eu2+) with Robust Thermal Stability for White Light-Emitting Diodes106Integrated Surface Modification to Enhance the Luminescence Properties of K2TiF6:Mn4+ Phosphor and Its Application in White-Light-Emitting Diodes102Structural Confinement toward Giant Enhancement of Red Emission in Mn2+‐Based Phosphors165Rb3SiF7:Mn4+ and Rb2CsSiF7:Mn4+ Red-Emitting Phosphors with a Faster Decay Rate90Control of Narrow-Band Emission in Phosphor Materials for Application in Light-Emitting Diodes160A novel rare-earth free red-emitting Li3Mg2SbO6:Mn4+ phosphor-in-glass for warm w-LEDs: Synthesis, structure, and luminescence properties101Persistent luminescence instead of phosphorescence: History, mechanism, and perspective680Structure, Thermal Stability, and Spectroscopic Properties of Triclinic Double Sulfate AgEu(SO4)2 with Isolated SO4 Groups83Effect of alkali metal ions on the spectra of CaZn2(PO4)2: Sm3+ phosphor analyzed by J-O theory81Synthesis and photoluminescence properties of Sm3+ and Dy3+ ions activated double perovskite Sr2MgTeO6 phosphors107Layered Structure Produced Nonconcentration Quenching in a Novel Eu3+-Doped Phosphor185Imaging and therapeutic applications of persistent luminescence nanomaterials313White‐Light‐Emitting Melamine‐Formaldehyde Microspheres through Polymer‐Mediated Aggregation and Encapsulation of Graphene Quantum Dots96An ultra-high yield of spherical K 2 NaScF 6 :Mn 4+ red phosphor and its application in ultra-wide color gamut liquid crystal displays95Coexistence of self-reduction from Mn 4+ to Mn 2+ and elastico-mechanoluminescence in diphase KZn(PO 3 ) 3 :Mn 2+73Full visible light emission in Eu 2+ ,Mn 2+ -doped Ca 9 LiY 0.667 (PO 4 ) 7 phosphors based on multiple crystal lattice substitution and energy transfer for warm white LEDs with high colour-rendering111Mn 2+ -Based narrow-band green-emitting Cs 3 MnBr 5 phosphor and the performance optimization by Zn 2+ alloying141Non-concentration quenching, good thermal stability and high quantum efficiency of K 5 Y(P 2 O 7 ) 2 :Eu 3+ /Tb 3+ phosphors with a novel two-dimensional layer structure78Novel bismuth activated blue-emitting phosphor Ba 2 Y 5 B 5 O 17 :Bi 3+ with strong NUV excitation for WLEDs82Structural design of new Ce 3+ /Eu 2+ -doped or co-doped phosphors with excellent thermal stabilities for WLEDs133Discovery of New Narrow‐Band Phosphors with the UCr 4 C 4 ‐Related Type Structure by Alkali Cation Effect137Synthesis and Luminescence Properties of CsPbX 3 @Uio-67 Composites toward Stable Photoluminescence Convertors99Li substituent tuning of LED phosphors with enhanced efficiency, tunable photoluminescence, and improved thermal stability205Exploration of structural, vibrational and spectroscopic properties of self-activated orthorhombic double molybdate RbEu(MoO4)2 with isolated MoO4 units75Recent advances in solid-state LED phosphors with thermally stable luminescence325Thermally stable double-perovskite Ca3TeO6:Eu3+ red-emitting phosphors with high color purity113Tuning of the Compositions and Multiple Activator Sites toward Single-Phased White Emission in (Ca 9– x Sr x )MgK(PO 4 ) 7 :Eu 2+ Phosphors for Solid-State Lighting115Unraveling the Mechanisms of Thermal Quenching of Luminescence in Ce3+-Doped Garnet Phosphors238Emerging ultra-narrow-band cyan-emitting phosphor for white LEDs with enhanced color rendition515Cr 3+ ‐Doped Broadband NIR Garnet Phosphor with Enhanced Luminescence and its Application in NIR Spectroscopy393Broadband emission of single-phase Ca3Sc2Si3O12:Cr3+/Ln3+ (Ln = Nd, Yb, Ce) phosphors for novel solid-state light sources with visible to near-infrared light output96Sr[Li2Al2O2N2]:Eu2+—A high performance red phosphor to brighten the future340Sr2LiScB4O10:Ce3+/Tb3+: A Green-Emitting Phosphor with High Energy Transfer Efficiency and Stability for LEDs and FEDs107Polyhedron Transformation toward Stable Narrow‐Band Green Phosphors for Wide‐Color‐Gamut Liquid Crystal Display201Enhancing quantum efficiency and tuning photoluminescence properties in far-red-emitting phosphor Ca14Ga10Zn6O35:Mn4+ based on chemical unit engineering142Sol-gel processing of Eu3+ doped Li6CaLa2Nb2O12 garnet for efficient and thermally stable red luminescence under near-ultraviolet/blue light excitation75Lanthanide Photonics: Shaping the Nanoworld166Studies on luminescence properties of double perovskite deep red phosphor La2ZnTiO6:Mn4+ for indoor plant growth LED applications91Near UV-pumped yellow-emitting Ca3TeO6:Dy3+ phosphor for white light-emitting diodes74Effects of cationic substitution on the luminescence behavior of Dy3+ doped orthophosphate phosphor87Improved phase stability of the metastable K2GeF6:Mn4+ phosphors with high thermal stability and water-proof property by cation substitution99Engineering of K3YSi2O7To Tune Photoluminescence with Selected Activators and Site Occupancy117Photoluminescence Control of UCr 4 C 4 -Type Phosphors with Superior Luminous Efficiency and High Color Purity via Controlling Site Selection of Eu 2+ Activators112Tunable lanthanide/transition metal ion‐doped novel phosphors for possible application in w‐LEDs: a review77Room temperature synthesis of stable single silica-coated CsPbBr3 quantum dots combining tunable red emission of Ag–In–Zn–S for High-CRI white light-emitting diodes276Divalent europium-doped near-infrared-emitting phosphor for light-emitting diodes660Designing High‐Performance LED Phosphors by Controlling the Phase Stability via a Heterovalent Substitution Strategy76A review on the advancements in phosphor-converted light emitting diodes (pc-LEDs): Phosphor synthesis, device fabrication and characterization731Ultra-high-efficiency near-infrared Ga 2 O 3 :Cr 3+ phosphor and controlling of phytochrome178Multiple Substitution Strategies toward Tunable Luminescence in Lu2MgAl4SiO12:Eu2+ Phosphors90Highly Efficient Green‐to‐Yellowish‐Orange Emitting Eu2+‐Doped Pyrophosphate Phosphors with Superior Thermal Quenching Resistance for w‐LEDs99Phosphor-SiO2 composite films suitable for white laser lighting with excellent color rendering76Lanthanide doping in metal halide perovskite nanocrystals: spectral shifting, quantum cutting and optoelectronic applications260Recent progress on discovery of novel phosphors for solid state lighting88Site Occupation and Luminescence of Novel Orange-Red Ca3M2Ge3O12:Mn2+,Mn4+ (M = Al, Ga) Phosphors106Crosslink‐Enhanced Emission Effect on Luminescence in Polymers: Advances and Perspectives255Enhancing Near-Infrared Photoluminescence Intensity and Spectral Properties in Yb 3+ Codoped LiScP 2 O 7 :Cr 3+345Strategies for Designing Antithermal‐Quenching Red Phosphors216Yellow/Orange-Emitting ABZn 2 Ga 2 O 7 :Bi 3+ (A = Ca, Sr; B = Ba, Sr) Phosphors: Optical Temperature Sensing and White Light-Emitting Diode Applications256Broad-band emission in metal halide perovskites: Mechanism, materials, and applications288Broadband near‐infrared emission enhancement in K 2 Ga 2 Sn 6 O 16 :Cr 3+ phosphor by electron‐lattice coupling regulation87Lanthanide‐Doped Core@Multishell Nanoarchitectures: Multimodal Excitable Upconverting/Downshifting Luminescence and High‐Level Anti‐Counterfeiting188Dual‐Shelled RbLi(Li 3 SiO 4 ) 2 :Eu 2+ @Al 2 O 3 @ODTMS Phosphor as a Stable Green Emitter for High‐Power LED Backlights90Eu3+, Sm3+ Deep‐Red Phosphors as Novel Materials for White Light‐Emitting Diodes and Simultaneous Performance Enhancement of Organic–Inorganic Perovskite Solar Cells84Data-Driven Photoluminescence Tuning in Eu2+-Doped Phosphors76Pressure‐Driven Eu 2+ ‐Doped BaLi 2 Al 2 Si 2 N 6 : A New Color Tunable Narrow‐Band Emission Phosphor for Spectroscopy and Pressure Sensor Applications105Lanthanide spectroscopy in probing structure-property correlation in multi-site photoluminescent phosphors161A novel narrow-band blue-emitting phosphor of Bi3+-activated Sr3Lu2Ge3O12 based on a highly symmetrical crystal structure used for WLEDs and FEDs183Narrow-band emitters in LED backlights for liquid-crystal displays217Design and control of the luminescence in Cr3+-doped NIR phosphors via crystal field engineering105High moisture resistance of an efficient Mn4+-activated red phosphor Cs2NbOF5:Mn4+ for WLEDs106Glass-ceramic phosphors for solid state lighting: A review117Structural Engineering of Eu2+-Doped Silicates Phosphors for LED Applications242Three Birds with One Stone: K 2 SiF 6 :Mn 4+ Single Crystal Phosphors for High‐Power and Laser‐Driven Lighting117Recent progress of zero-dimensional luminescent metal halides873Structure and photoluminescence of Eu 3+ doped Sr 2 InTaO 6 red phosphor with high color purity90Perovskite Quantum Dots Glasses Based Backlit Displays351Learning from Mineral Structures toward New Luminescence Materials for Light-Emitting Diode Applications146A High Efficiency Trivalent Chromium-Doped Near-Infrared-Emitting Phosphor and Its NIR Spectroscopy Application166Glass crystallization making red phosphor for high-power warm white lighting236Unraveling the Luminescence Quenching of Phosphors under High-Power-Density Excitation92Recent prospects on phosphor-converted LEDs for lighting, displays, phototherapy, and indoor farming164Rapid Synthesis of Red‐Emitting Sr2Sc0.5Ga1.5O5:Eu2+ Phosphors and the Tunable Photoluminescence Via Sr/Ba Substitution90Design principles for achieving red emission in Eu2+/Eu3+ doped inorganic solids83Defect Engineering in a Eu2+-Doped β-Al2O3 Structure Blue Phosphor and Its Controllable Zero-Thermal Quenching Luminescence97Efficient and Tunable Luminescence in Ga 2– x In x O 3 :Cr 3+ for Near-Infrared Imaging172Advances in Near-Infrared Luminescent Materials without Cr3+: Crystal Structure Design, Luminescence Properties, and Applications171A Novel Highly Thermal-Stable Red-Emitting Cagdsbwo8:Eu3+ Phosphor with Scheelite Structure for High Cri W-Leds, Security Ink, and Latent Fingerprint74How to Obtain Anti‐Thermal‐Quenching Inorganic Luminescent Materials for Light‐Emitting Diode Applications252Competitive Site Occupation toward Improved Quantum Efficiency of SrLaScO 4 :Eu Red Phosphors for Warm White LEDs103Eu2+ Doping Concentration-Induced Site-Selective Occupation and Photoluminescence Tuning in KSrScSi2O7:Eu2+ Phosphor77Technological Breakthroughs in Chip Fabrication, Transfer, and Color Conversion for High‐Performance Micro‐LED Displays238Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure137Laser Phosphors for Next-Generation Lighting Applications152Recent development in color tunable phosphors: A review205Designing and controlling the Ni 2+ -activated (Zn, Mg)Al 2 O 4 spinel solid-solution for phosphor-converted broadband near-infrared illumination81The role of lanthanide luminescence in advancing technology123Regulating Eu 2+ Multisite Occupation through Structural Disorder toward Broadband Near-Infrared Emission91Efficient and Stable Perovskite White Light‐Emitting Diodes for Backlit Display212A review of recent advances in Ce3+-activated garnet phosphors for blue-chip-pumped pc-WLEDs81

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  38. Crystal structure and luminescence properties of the blue‐green‐emitting Ba9(Lu, Y)2Si6O24:Ce3+ phosphor

    Luminescence · 2017-01-05

    Huawei Xu, Zhi Zhou, Yongfu Liu, Qunxing Liu, Zhiyuan He, Shen Wang, Linyi Huang, Hongbo Zhu

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  39. Tuning of Photoluminescence and Local Structures of Substituted Cations in xSr2Ca(PO4)2–(1 – x)Ca10Li(PO4)7:Eu2+ Phosphors

    Chemistry of Materials · 2017-01-21

    Mingyue Chen, Zhiguo Xia, Мaxim S. Моlokeev, Ting Wang, Quanlin Liu

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  40. Electrospinning, optical properties and white LED applications of one-dimensional CaAl 12 O 19 :Mn 4+ nanofiber phosphors

    Ceramics International · 2017-01-22

    Ze Liu, Minghua Yuwen, Jiaqing Liu, Caiyan Yu, Tongtong Xuan, Huili Li

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  41. Influence of Anion/Cation Substitution (Sr2+ → Ba2+, Al3+ → Si4+, N3– → O2–) on Phase Transformation and Luminescence Properties of Ba3Si6O15:Eu2+ Phosphors

    Chemistry of Materials · 2017-01-26

    Mengmeng Shang, Sisi Liang, Nianrui Qu, Hongzhou Lian, Jun Lin

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  42. Molten salt synthesis of color-tunable and single-component NaY(1−x−y)(WO4)2:Eu3+x,Tb3+y phosphor for UV LEDs

    Journal of materials research/Pratt's guide to venture capital sources · 2017-02-16

    Fang Lei, Lijing Huang, Ying Shi, Jianjun Xie, Lei Zhang, Weiqin Xiao

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  43. Deep red BaTiF4:Mn4+ phosphor: synthesis, optical properties and application for warm WLED devices

    Journal of Materials Science Materials in Electronics · 2017-02-19

    Guoli Mo, Weiping Wang, Kuanlei Wang, Guohua Wen, Menghan Zhu, Jingxuan Wang

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  44. Insights into the discrepant luminescence for BaSiO3:Eu2+ phosphors prepared by solid‐state reaction and precipitation reaction methods

    Luminescence · 2017-02-21

    Jiao Xu, Yang Zhao, Jingjing Chen, Zhiyong Mao, Yanfang Yang, Dajian Wang

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  45. Luminescence, Energy Transfer and Tunable Color of Ce3+- and Tb3+-Activated Na3Gd(BO3)2 Phosphors

    Journal of Electronic Materials · 2017-02-23

    Xinguo Zhang, Jialiang Pan, Fuwang Mo

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  46. Facile synthesis of yellow-emitting CaAlSiN 3 :Ce 3+ phosphors and the enhancement of red-component by co-doping Eu 2+ ions

    Solid State Communications · 2017-03-01

    Jingjing Chen, Yang Zhao, Guanghao Li, Zhiyong Mao, Dajian Wang, Li‐Jian Bie

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  47. Ce 3+ and Dy 3+ doped Sr 3 B 2 O 6 : Solid state synthesis and tunable luminescence

    Journal of Luminescence · 2017-03-07

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  48. Study on luminescence and thermal stability of blue-emitting Sr 5 (PO 4 ) 3 F: Eu 2+ phosphor for application in InGaN-based LEDs

    Materials Science and Engineering B · 2017-03-26

    Jie Liu, Zhiming Zhang, Zhan‐Chao Wu, Fangfang Wang, Zhenjiang Li

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  49. Synthesis and photoluminescence properties of Eu 2+ activated CaO ceramic powders for near-ultraviolet chip based white light emitting diodes

    Optical Materials · 2017-04-02

    Zhendong Hao, Ying Wang, Liangliang Zhang, Guohui Pan, Xia Zhang, Huajun Wu, Yongshi Luo, Jiahua Zhang

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  50. Preparation, luminescence properties and energy transfer of Ca 9 Y(PO 4 ) 7 : Eu 2+ ‐Tb 3+ phosphors

    Journal of the American Ceramic Society · 2017-04-03

    Miao Tang, Yanting Fan, Zhongxian Qiu, Jilin Zhang, Liping Yu, Chengzhi Li, Shixun Lian, Wenli Zhou

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