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RESEARCH PAPER · Journal of Materials Chemistry A · 2015

A-site deficient perovskite: the parent for in situ exsolution of highly active, regenerable nano-particles as SOFC anodes

Yifei Sun, Jianhui Li, Yimin Zeng, Babak Shalchi Amirkhiz, Meng-Ni Wang, Yashar Behnamian, Jing‐Li Luo

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A-site deficient perovskite: the parent for in situ exsolution of highly active, regenerable nano-particles as SOFC anodesOriginalExsolution of Fe and SrO Nanorods and Nanoparticles from Lanthanum Strontium Ferrite La0.6Sr0.4FeO3−δ Materials by Hydrogen Reduction77Evolution of the electrochemical interface in high-temperature fuel cells and electrolysers769Ni–perovskite interaction and its structural and catalytic consequences in methane steam reforming and methanation reactions76Bifunctional Catalyst of Core–Shell Nanoparticles Socketed on Oxygen-Deficient Layered Perovskite for Soot Combustion: In Situ Observation of Synergistic Dual Active Sites82Impregnation versus exsolution: Using metal catalysts to improve electrocatalytic properties of LSCM-based anodes operating at 600 °C54Synthesis and preliminary study of pure and Zr-doped YMnO3 compounds as Solid Oxide Fuel Cells electrode11Development and performance of anode material based on A-site deficient Sr 2-x Fe 1.4 Ni 0.1 Mo 0.5 O 6-δ perovskites for solid oxide fuel cells52Nanomaterials for Advanced Electrode of Low Temperature Solid Oxide Fuel Cells (SOFCs)32Catalysts and Processes in Solid Oxide Fuel Cells8(La1−xSrx)0.98MnO3 perovskite with A-site deficiencies toward oxygen reduction reaction in aluminum-air batteries129Alternative Ni-Impregnated Mixed Ionic-Electronic Conducting Anode for SOFC Operation at High Fuel Utilization24Controlling cation segregation in perovskite-based electrodes for high electro-catalytic activity and durability376Electrochemical Energy Production Using Fuel Cell Technologies9Hydrogen production from the decomposition of hydrogen iodide over nanosized nickel-oxide-zirconia catalysts prepared by solution-combustion techniques21Characterization of Sr/Ru co-doped ferrite based perovskite as a symmetrical electrode material for solid oxide fuel cells37Nickel‐Iron Alloy Nanoparticle‐Decorated K2NiF4‐Type Oxide as an Efficient and Sulfur‐Tolerant Anode for Solid Oxide Fuel Cells37Nanocatalysis in Solid Oxide Cells0Enhancing Perovskite Electrocatalysis of Solid Oxide Cells Through Controlled Exsolution of Nanoparticles138Exsolution trends and co-segregation aspects of self-grown catalyst nanoparticles in perovskites499Smart tuning of 3D ordered electrocatalysts for enhanced oxygen reduction reaction41Mechanistic Origin of Enhanced CO Catalytic Oxidation over Co3O4/LaCoO3 at Lower Temperature31Niobium Doped Lanthanum Strontium Ferrite as A Redox‐Stable and Sulfur‐Tolerant Anode for Solid Oxide Fuel Cells68Redox cycling induced Ni exsolution in Gd0.1Ce0.8Ni0.1O2 - (Sr0.9La0.1)0.9Ti0.9Ni0.1O3 composite solid oxide fuel cell anodes22Enhanced Li ion conductivity in Ge-doped Li 0.33 La 0.56 TiO 3 perovskite solid electrolytes for all-solid-state Li-ion batteries59The enhanced electrochemical response of Sr(Ti 0.3 Fe 0.7 Ru 0.07 )O 3−δ anodes due to exsolved Ru–Fe nanoparticles59Toward a rational photocatalyst design: a new formation strategy of co-catalyst/semiconductor heterostructures via in situ exsolution50Transition metal oxide-based oxygen reduction reaction electrocatalysts for energy conversion systems with aqueous electrolytes236Infiltrated Pr2NiO4 as promising bi-electrode for symmetrical solid oxide fuel cells46Exploration of Co-Fe alloy precipitation and electrochemical behavior hysteresis using Lanthanum and Cobalt co-substituted SrFeO3-δ SOFC anode67Performance comparison of Ni Ex-soluted and impregnated La- and Y- doped Sr titanates as anode for solid oxide fuel cell12Single-phase electronic-ionic conducting Sm3+/Pr3+/Nd3+ triple-doped ceria for new generation fuel cell technology23Recent Advances in Novel Nanostructuring Methods of Perovskite Electrocatalysts for Energy‐Related Applications407A Highly Efficient and Robust Perovskite Anode with Iron–Palladium Co‐exsolutions for Intermediate‐Temperature Solid‐Oxide Fuel Cells30Nanometric nickel exsolution in the hexagonal perovskite Ba8Ta6NiO24: Survey of the structural, magnetic and catalytic features12A novel anode for solid oxide fuel cells prepared from phase conversion of La0.3Sr0.7Fe0.7Cr0.3O3-δ perovskite under humid hydrogen25High-Performance La0.5Ba0.5Co1/3Mn1/3Fe1/3O3−δ-BaZr1−zYzO3−δ Cathode Composites via an Exsolution Mechanism for Protonic Ceramic Fuel Cells17Interface engineering: Surface hydrophilic regulation of LaFeO3 towards enhanced visible light photocatalytic hydrogen evolution39Structures, Phase Fields, and Mixed Protonic–Electronic Conductivity of Ba-Deficient, Pr-Substituted BaZr0.7Ce0.2Y0.1O3−δ7Bimetallic nanoparticle decorated perovskite oxide for state-of-the-art trifunctional electrocatalysis106In situ catalyst exsolution on perovskite oxides for the production of CO and synthesis gas in ceramic membrane reactors44Influence of A- and B-Site Modifications of (La 1-x Sr x ) y Cr 0.5-z Mn 0.5-w Ni z+w O 3-δ on Electrochemical Impedance Characteristics of Reversible Solid Oxide Cell9Sulfur Poisoning Recovery on a Solid Oxide Fuel Cell Anode Material through Reversible Segregation of Nickel50Morphology evolution and exsolution mechanism of a partially decomposed anode for intermediate temperature-solid oxide fuel cells29Review of proton- and oxide-ion-conducting perovskite materials for SOFC applications29Nanoengineering of solid oxide electrochemical cell technologies: An outlook30Improving the multicaloric properties of Pb(Fe0.5Nb0.5)O3 by controlling the sintering conditions and doping with manganese14Development of Carbon Tolerant Anodes for Solid Oxide Fuel Cells Fabricated by Solution Precursor Plasma Spraying0Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part A: Synthesis and structure analysis in air12Highly Stable and Efficient Perovskite Ferrite Electrode for Symmetrical Solid Oxide Fuel Cells82Reducing the Barrier Energy of Self‐Reconstruction for Anchored Cobalt Nanoparticles as Highly Active Oxygen Evolution Electrocatalyst115Silver Exsolution-Enhanced Electrical Properties of Lanthanum-Based Perovskites2Approaching Durable Single-Layer Fuel Cells: Promotion of Electroactivity and Charge Separation via Nanoalloy Redox Exsolution91Nickel Exsolution‐Driven Phase Transformation from an n=2 to an n=1 Ruddlesden‐Popper Manganite for Methane Steam Reforming Reaction in SOFC Conditions46Co-infiltration of Nickel and Mixed Conducting Gd0.1Ce0.9O2−δ and La0.6Sr0.3Ni0.15Cr0.85O3−δ Phases in Ni-YSZ Anodes for Improved Stability and Performance11Exsolution and electrochemistry in perovskite solid oxide fuel cell anodes: Role of stoichiometry in Sr(Ti,Fe,Ni)O383Heterointerface engineering for enhancing the electrochemical performance of solid oxide cells319Exsolved Nickel Nanoparticles Acting as Oxygen Storage Reservoirs and Active Sites for Redox CH4 Conversion97Compositional Engineering of a La1-xBaxCoO3-δ-(1-a) BaZr0.9Y0.1O2.95 (a = 0.6, 0.7, 0.8 and x = 0.5, 0.6, 0.7) Nanocomposite Cathodes for Protonic Ceramic Fuel Cells8Studies on structural, morphological, and electrical properties of Ga3+ and Cu2+ co-doped ceria ceramics as solid electrolyte for IT-SOFCs38Vanadium-Doped Strontium Molybdate with Exsolved Ni Nanoparticles as Anode Material for Solid Oxide Fuel Cells38Advanced perovskite anodes for solid oxide fuel cells: A review212Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part B: Conditions of Ni exsolution28Highly Efficient B-Site Exsolution Assisted by Co Doping in Lanthanum Ferrite toward High-Performance Electrocatalysts for Oxygen Evolution and Oxygen Reduction66La0.75Sr0.25Cr0.5Mn0.5O3-δ-Ce0.8Sm0.2O1.9 as composite electrodes in symmetric solid electrolyte cells for electrochemical removal of nitric oxide26Catalytic Steam Reforming of Natural Gas over a New Ni Exsolved Ruddlesden‐Popper Manganite in SOFC Anode Conditions16Advanced oxygen-electrode-supported solid oxide electrochemical cells with Sr(Ti,Fe)O 3−δ -based fuel electrodes for electricity generation and hydrogen production43Exploring Ni(Mn 1/3 Cr 2/3 ) 2 O 4 spinel-based electrodes for solid oxide cells46Highly active and thermally stable single-atom catalysts for high-temperature electrochemical devices68Progress in perovskite anodes for intermediate-temperature solid oxide fuel cells1Understanding of A-site deficiency in layered perovskites: promotion of dual reaction kinetics for water oxidation and oxygen reduction in protonic ceramic electrochemical cells114A-site deficient perovskite with nano-socketed Ni-Fe alloy particles as highly active and durable catalyst for high-temperature CO2 electrolysis65Exsolution of Nickel Nanoparticles from Mixed‐Valence Metal Oxides: A Quantitative Evaluation by Magnetic Measurements9Modifying the Surface Structure of Perovskite-Based Catalysts by Nanoparticle Exsolution50Proton-conducting oxides for energy conversion and storage530Redox-Reversible Electrode Material for Direct Hydrocarbon Solid Oxide Fuel Cells85In situ growth of nanoparticles in A-site deficient ferrite perovskite as an advanced electrode for symmetrical solid oxide fuel cells62Progress and Opportunities for Exsolution in Electrochemistry26In situ embedding of CoFe nanocatalysts into Sr3FeMoO7 matrix as high-performance anode materials for solid oxide fuel cells53Co-generation of electricity and olefin via proton conducting fuel cells using (Pr0.3Sr0.7)0.9Ni0.1Ti0.9O3 catalyst layers66The role of manganese substitution on the redox behavior of La0.6Sr0.4Fe0.8Mn0.2O3-δ28Review on exsolution and its driving forces in perovskites138In Situ Exsolved Metal Nanoparticles: A Smart Approach for Optimization of Catalysts163Ni catalysts for dry methane reforming prepared by A-site exsolution on mesoporous defect spinel magnesium aluminate55Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part C: Electrical and electrochemical behavior8In-situ exsolved FeRu alloy nanoparticles on Ruddlesden-Popper oxides for direct hydrocarbon fuel solid oxide fuel cells41Ni-doped A-site-deficient La0.7Sr0.3Cr0.5Mn0.5O3-δ perovskite as anode of direct carbon solid oxide fuel cells29Nickel exsolution effect on the catalytic behavior of ruddlesden-popper manganites in sofc conditions using colombian natural gas0Construction of Multifunctional Nanoarchitectures in One Step on a Composite Fuel Catalyst through In Situ Exsolution of La0.5Sr0.5Fe0.8Ni0.1Nb0.1O3−δ41Efficient Ferrite-Based Perovskite Anode for Solid Oxide Fuel Cells with A-Site and B-Site Co-exsolution27In-situ Ni exsolution from NiTiO3 as potential anode for solid oxide fuel cells14Methane steam reforming in water-deficient conditions on a new Ni-exsolved Ruddlesden-Popper manganite: Coke formation and H2S poisoning24Computational approaches to the exsolution phenomenon in perovskite oxides with a view to design highly durable and active anodes for solid oxide fuel cells13Exsolution manipulated local surface cobalt/iron alloying and dealloying conversion in La0·95Fe0·8Co0·2O3 perovskite for oxygen evolution reaction36Understanding electrochemical switchability of perovskite-type exsolution catalysts89Enhancing the Bifunctional Catalytic Performance of Porous La0.9Mn0.6Ni0.4O3−δNanofibers for Li–O2Batteries through Exsolution of Ni Nanoparticles13In situ and operando characterisation techniques for solid oxide electrochemical cells: recent advances30Understanding the A-site non-stoichiometry in perovskites: promotion of exsolution of metallic nanoparticles and the hydrogen oxidation reaction in solid oxide fuel cells33Organic Photochemistry-Assisted Nanoparticle Segregation on Perovskites14Ni-exsolved La1-xCaxNiO3 perovskites for improving CO2 methanation77Development and performance of A-site rich perovskite-type material for enhanced oxygen evolution reaction in alkaline electrolyte6Ca-doped rare earth perovskite materials for tailored exsolution of metal nanoparticles24High-performance direct carbon dioxide-methane solid oxide fuel cell with a structure-engineered double-layer anode59Metal Exsolution to Enhance the Catalytic Activity of Electrodes in Solid Oxide Fuel Cells55Mechanistic insights into the phase transition and metal ex-solution phenomena of Pr 0.5 Ba 0.5 Mn 0.85 Co 0.15 O 3−δ from simple to layered perovskite under reducing conditions and enhanced catalytic activity55Nanoparticle Ex-solution for Supported Catalysts: Materials Design, Mechanism and Future Perspectives181NdBaFe2–xCoxO5+δ Double Perovskites with Exsolved Co–Fe Alloy Nanoparticles as Highly Efficient and Stable Anodes for Direct Hydrocarbon Solid Oxide Fuel Cells11A -site deficient chromite with in situ Ni exsolution as a fuel electrode for solid oxide cells (SOCs)51Defective Sr 0.9 Mo 0.9 O 3−δ perovskites with exsolved Ni nanoparticles as high-performance composite anodes for solid-oxide fuel cells9Minimized thermal expansion mismatch of cobalt-based perovskite air electrodes for solid oxide cells25Investigation of hetero-phases grown via in-situ exsolution on a Ni-doped (La,Sr)FeO3 cathode and the resultant activity enhancement in CO2 reduction83Progress of Exsolved Metal Nanoparticles on Oxides as High Performance (Electro)Catalysts for the Conversion of Small Molecules120Exsolution of Embedded Nanoparticles in Defect Engineered Perovskite Layers54Nanoparticle exsolution in perovskite oxide and its sustainable electrochemical energy systems43Emergence and Future of Exsolved Materials214Ex-solution kinetics of nickel-ceria–doped strontium titanate perovskites7Performance and Limitations of Nickel‐Doped Chromite Anodes in Electrolyte‐Supported Solid Oxide Fuel Cells16Improving the activity and stability of Ni-based electrodes for solid oxide cells through surface engineering: Recent progress and future perspectives34Perovskite Oxide Catalysts for Advanced Oxidation Reactions264Controlling exsolution with a charge-balanced doping approach24Degradation Mechanisms of Metal-Supported Solid Oxide Cells and Countermeasures: A Review67A new in-situ-grown Ni-Sr2WO5−δ cermet to enhance coking tolerance of direct-hydrocarbon solid oxide fuel cells2Recent development of perovskite oxide-based electrocatalysts and their applications in low to intermediate temperature electrochemical devices210Exsolution of Ni Nanoparticles from A-Site-Deficient Layered Double Perovskites for Dry Reforming of Methane and as an Anode Material for a Solid Oxide Fuel Cell61In-situ construction of ceria-metal/titanate heterostructure with controllable architectures for efficient fuel electrochemical conversion41Solid Oxide Fuel Cells: Fabrication and Microstructure1Catalyst-Exsolving Anode-Supported Low-Temperature Solid Oxide Fuel Cell0The modern level of catalysts and technologies for natural gas conversion to syngas6High-performance and durable alcohol-fueled symmetrical solid oxide fuel cell based on ferrite perovskite electrode36Exsolution of nanoparticles on A-site-deficient lanthanum ferrite perovskites: its effect on co-electrolysis of CO 2 and H 2 O49Unveiling the key factor for the phase reconstruction and exsolved metallic particle distribution in perovskites81In Situ Growth of Exsolved Nanoparticles under Varying rWGS Reaction Conditions—A Catalysis and Near Ambient Pressure-XPS Study16Hydrocarbon Compatible SOFC Anode Catalysts and Their Syntheses: A Review29A New Durable Surface Nanoparticles‐Modified Perovskite Cathode for Protonic Ceramic Fuel Cells from Selective Cation Exsolution under Oxidizing Atmosphere248A critical review of the nano-structured electrodes of solid oxide cells40Strain Relaxation in Epitaxial Srti0.5fe0.5o3−𝛿 Thin Films on Laalo3: An X-Ray Reciprocal Space Mapping Study0Modern Level of Catalysts and Technologies for the Conversion of Natural Gas into Syngas12Exsolution in Ni-doped lanthanum strontium titanate: a perovskite-based material for anode application in ammonia-fed Solid Oxide Fuel Cell48The metal/oxide heterointerface delivered by solid-based exsolution strategy: A review53Shape-shifting nanoparticles on a perovskite oxide for highly stable and active heterogeneous catalysis49Recent progress in design and fabrication of SOFC cathodes for efficient catalytic oxygen reduction95Exsolution of phase-separated nanoparticles via trigger effect toward reversible solid oxide cell41In Situ Exsolved NiFe/(NiFe)Ox Core–Shell-Structured Nanocatalysts on Perovskite Anode with Enhanced Coking Resistance16Synergistically Promoting Coking Resistance of a La0.4Sr0.4Ti0.85Ni0.15O3−δ Anode by Ru-Doping-Induced Active Twin Defects and Highly Dispersed Ni Nanoparticles18Strain relaxation in epitaxial SrTi0.5Fe0.5 O 3−δ thin films on LaAlO3: An X-ray reciprocal space mapping study4Improved CO2 electrolysis by a Fe nanoparticle-decorated (Ce, La, Sr)(CrFe)O3-δ perovskite using a combined strategy of lattice defect-building19Exsolved catalyst particles as a plaything of atmosphere and electrochemistry11Recent advances in carbon-resistant anodes for solid oxide fuel cells92Tuning reduction conditions to understand and control Ni exsolution from Sr 0.8 La 0.1 Ca 0.1 Ti 0.94 Ni 0.06 O 3− δ14Enhanced H2 permeation and CO2 tolerance of self-assembled ceramic-metal-ceramic BZCYYb-Ni-CeO2 hybrid membrane for hydrogen separation22Recent Advances in Perovskite Oxides Electrocatalysts: Ordered Perovskites, Cations Segregation and Exsolution17

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  4. Bifunctional Catalyst of Core–Shell Nanoparticles Socketed on Oxygen-Deficient Layered Perovskite for Soot Combustion: In Situ Observation of Synergistic Dual Active Sites

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  5. Impregnation versus exsolution: Using metal catalysts to improve electrocatalytic properties of LSCM-based anodes operating at 600 °C

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  33. A Highly Efficient and Robust Perovskite Anode with Iron–Palladium Co‐exsolutions for Intermediate‐Temperature Solid‐Oxide Fuel Cells

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  34. Nanometric nickel exsolution in the hexagonal perovskite Ba8Ta6NiO24: Survey of the structural, magnetic and catalytic features

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  35. A novel anode for solid oxide fuel cells prepared from phase conversion of La0.3Sr0.7Fe0.7Cr0.3O3-δ perovskite under humid hydrogen

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  36. High-Performance La0.5Ba0.5Co1/3Mn1/3Fe1/3O3−δ-BaZr1−zYzO3−δ Cathode Composites via an Exsolution Mechanism for Protonic Ceramic Fuel Cells

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  37. Interface engineering: Surface hydrophilic regulation of LaFeO3 towards enhanced visible light photocatalytic hydrogen evolution

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  38. Structures, Phase Fields, and Mixed Protonic–Electronic Conductivity of Ba-Deficient, Pr-Substituted BaZr0.7Ce0.2Y0.1O3−δ

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  39. Bimetallic nanoparticle decorated perovskite oxide for state-of-the-art trifunctional electrocatalysis

    Journal of Materials Chemistry A · 2019-01-01

    Quazi Arif Islam, Rahul Majee, Sayan Bhattacharyya

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  40. In situ catalyst exsolution on perovskite oxides for the production of CO and synthesis gas in ceramic membrane reactors

    Sustainable Energy & Fuels · 2019-01-01

    Georgios Dimitrakopoulos, Ahmed F. Ghoniem, Bilge Yildiz

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  41. Influence of A- and B-Site Modifications of (La 1-x Sr x ) y Cr 0.5-z Mn 0.5-w Ni z+w O 3-δ on Electrochemical Impedance Characteristics of Reversible Solid Oxide Cell

    Journal of The Electrochemical Society · 2019-01-01

    Martin Maide, Päärn Paiste, Priit Möller, Enn Lust, Gunnar Nurk

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  42. Sulfur Poisoning Recovery on a Solid Oxide Fuel Cell Anode Material through Reversible Segregation of Nickel

    Chemistry of Materials · 2019-01-06

    Patrick Steiger, Dariusz Burnat, Hossein Madi, Andreas Mai, Lorenz Holzer, Jan Van herle, Oliver Kröcher, André Heel, Davide Ferri

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  43. Morphology evolution and exsolution mechanism of a partially decomposed anode for intermediate temperature-solid oxide fuel cells

    Electrochimica Acta · 2019-02-27

    Jingwei Li, Bo Wei, Xing Yue, Huan Li, Zhe Lü

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  44. Review of proton- and oxide-ion-conducting perovskite materials for SOFC applications

    Nanomaterials and Energy · 2019-02-28

    Kavitha Karuppiah, Anuradha M. Ashok

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  45. Nanoengineering of solid oxide electrochemical cell technologies: An outlook

    Nano Research · 2019-03-30

    Juliana S. A. Carneiro, Eranda Nikolla

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  46. Improving the multicaloric properties of Pb(Fe0.5Nb0.5)O3 by controlling the sintering conditions and doping with manganese

    Journal of the European Ceramic Society · 2019-05-30

    Uroš Prah, Tadej Rojac, Magdalena Wencka, Mirela Dragomir, Andraž Bradeško, Andreja Benčan, Rachel Sherbondy, Geoff L. Brennecka, Zdravko Kutnjak, Barbara Malič, Hana Uršič

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  47. Development of Carbon Tolerant Anodes for Solid Oxide Fuel Cells Fabricated by Solution Precursor Plasma Spraying

    TSpace (University of Toronto) · 2019-06-01

    Calvin Ng

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  48. Study of (La,Sr)(Ti,Ni)O3-δ materials for symmetrical Solid Oxide Cell electrode - Part A: Synthesis and structure analysis in air

    Ceramics International · 2019-06-04

    Charline Arrivé, Thibaud Delahaye, Olivier Joubert, Gilles Henri Gauthier

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  49. Highly Stable and Efficient Perovskite Ferrite Electrode for Symmetrical Solid Oxide Fuel Cells

    ACS Applied Materials & Interfaces · 2019-06-10

    Weiwei Fan, Zhu Sun, Yu Bai, Kai Ming Wu, Yonghong Cheng

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  50. Reducing the Barrier Energy of Self‐Reconstruction for Anchored Cobalt Nanoparticles as Highly Active Oxygen Evolution Electrocatalyst

    Advanced Materials · 2019-06-13

    Myeongjin Kim, Byeongyong Lee, Hyun Ju, Seung Woo Lee, Jooheon Kim

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